spin-dependent electronic tunneling at zero magnetic field

4
Spin-dependent electronic tunneling at zero magnetic field A. Voskoboynikov National Chiao Tung University, 1001 Ta Hsueh Road, Hsinchu 30010, Taiwan, Republic of China and Kiev Taras Shevchenko University, 64 Volodymirska Street, 252030 Kiev, Ukraine Shiue Shin Liu and C. P. Lee National Chiao Tung University, 1001 Ta Hsueh Road, Hsinchu 30010, Taiwan, Republic of China ~Received 15 July 1998! The spin-dependent tunneling phenomenon in symmetric and asymmetric semiconductor heterostructures at zero magnetic field is studied theoretically on the base of a single conduction band and spin-dependent boundary conditions approach. It is shown that the spin-orbit splitting in the dispersion relation for the electrons in A III B V semiconductor quantum-tunneling structures can provide a dependence of the tunneling transmission probability on the electron’s spin polarization. The dependence is calculated and discussed for different kinds of tunnel heterostructures. @S0163-1829~98!04548-2# The spin-dependent electron quantum confinement and dynamics in A III - B V semiconductor heterostructures at zero magnetic field call attention during recent years from theoretical 1–4 and experimental 5–10 points of view. In hetero- structures with sharp changes in electronic band parameters at interfaces or with external electric field, the spin-orbit in- teraction provides coupling between spatial motion in plane parallel to the heterointerfaces and the electron’s spin. The spin-orbit splitting of the electron conduction band at zero magnetic field is a consequence of the coupling. That is a well-known phenomenon dealing with the fundamental physical characteristics of the heterostructures. 11–14 Recent theoretical and experimental investigations demonstrated the existence of such effect in asymmetric quantum well struc- tures. Experimentally, the spin-orbit splitting for electrons confined in the heterostructures has been studied by Raman scattering 5–7 and Shubnikov–de Haas oscillation. 8–10 From a practical point of view, the application of the spin-orbit split- ting effect in quantum electronic devices can lead to a new generation of ultrafast spin-dependent electronics. 3 A poten- tial advantage of the devices is that the spin-dependent pro- cesses can be easily controlled by an external voltage. There- fore, a detailed analysis to clarify and to evaluate the effect magnitude is greatly desired. In this paper, we pay attention to another type of the spin-dependent phenomena in the semiconductor hetero- structures—quantum tunneling. Advances in modern epitax- ial growth technologies such as molecular-beam epitaxy and metal-organic chemical-vapor deposition technology provide us an opportunity to construct two-dimensional barrier het- erostructures in which the material parameters can be changed with a wide range and controlled with a consider- able accuracy. We can discuss possible influence of the spin- orbit splitting on the transmission probability for models of the quantum tunneling structures with realistic parameters. The tunneling coupling in double quantum wells 15 and tun- neling transmission processes through barrier between the wells those consider the electron’s in-plane motion 16 are also fields of possible the spin-orbit splitting effect investigation and implementations. We calculate the tunneling transmission probability for heterostructures with space-dependent electron’s effec- tive mass and spin-orbit coupling parameters. The depen- dence leads to the mass and spin-dependent boundary conditions. 3,17,21,18 Since we expect considerable effect with narrow gap A III - B V semiconductors ~where the spin-orbit splitting effect is strong!, it is important to take into account nonparabolicity for the electron’s dispersion relation. 3 In our calculation, we use the well-known approximation for en- ergy and space dependencies of the electronic effective mass. 3,17,21 For the spin-dependent tunneling process we ob- tained a dependence of the transmission probability on in- plane electron’s wave vector. The dependence consists of two parts: the known dependence originated from space- dependent electron’s effective mass, 18 and a new one origi- nated from the electronic wave function’s spin-dependent boundary conditions. 3 Each of them is a result of the band- edge discontinuity at the heterostructure interfaces. It will be demonstrated that the consideration of spin in tunneling pro- cesses can considerably change energy and in-plane wave- vector dependencies of the transmission probability in tunnel structures. The variation of the band-structure parameters for the single barrier tunneling structure to be discussed is shown in Fig. 1. To describe the spin-dependent tunneling in the het- erostructure we use the approximate effective Hamiltonian in the form proposed in Ref. 3. Layers of the structure are perpendicular to z axis, in-plane electron’s wave vector is k @if k is put along an arbitrary x direction, the spin polariza- tion is set along the y axis in the layer plane r 5( x , y ) #. In this paper, we discuss the influence of discontinuity of effec- tive mass and spin-orbit coupling parameters on tunneling processes. The influence from additional external electric field is not discussed here. With the above-mentioned as- sumptions, the total wave function of the electron F s ( z , r ) can be presented as PHYSICAL REVIEW B 15 DECEMBER 1998-I VOLUME 58, NUMBER 23 PRB 58 0163-1829/98/58~23!/15397~4!/$15.00 15 397 ©1998 The American Physical Society

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Page 1: Spin-dependent electronic tunneling at zero magnetic field

PHYSICAL REVIEW B 15 DECEMBER 1998-IVOLUME 58, NUMBER 23

Spin-dependent electronic tunneling at zero magnetic field

A. VoskoboynikovNational Chiao Tung University, 1001 Ta Hsueh Road, Hsinchu 30010, Taiwan, Republic of China

and Kiev Taras Shevchenko University, 64 Volodymirska Street, 252030 Kiev, Ukraine

Shiue Shin Liu and C. P. LeeNational Chiao Tung University, 1001 Ta Hsueh Road, Hsinchu 30010, Taiwan, Republic of China

~Received 15 July 1998!

The spin-dependent tunneling phenomenon in symmetric and asymmetric semiconductor heterostructures atzero magnetic field is studied theoretically on the base of a single conduction band and spin-dependentboundary conditions approach. It is shown that the spin-orbit splitting in the dispersion relation for theelectrons inAIIIBV semiconductor quantum-tunneling structures can provide a dependence of the tunnelingtransmission probability on the electron’s spin polarization. The dependence is calculated and discussed fordifferent kinds of tunnel heterostructures.@S0163-1829~98!04548-2#

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The spin-dependent electron quantum confinementdynamics inAIII -BV semiconductor heterostructures at zemagnetic field call attention during recent years frotheoretical1–4 and experimental5–10 points of view. In hetero-structures with sharp changes in electronic band parameat interfaces or with external electric field, the spin-orbitteraction provides coupling between spatial motion in plaparallel to the heterointerfaces and the electron’s spin.spin-orbit splitting of the electron conduction band at zemagnetic field is a consequence of the coupling. Thatwell-known phenomenon dealing with the fundamenphysical characteristics of the heterostructures.11–14 Recenttheoretical and experimental investigations demonstratedexistence of such effect in asymmetric quantum well strtures. Experimentally, the spin-orbit splitting for electroconfined in the heterostructures has been studied by Rascattering5–7 and Shubnikov–de Haas oscillation.8–10 From apractical point of view, the application of the spin-orbit splting effect in quantum electronic devices can lead to a ngeneration of ultrafast spin-dependent electronics.3 A poten-tial advantage of the devices is that the spin-dependentcesses can be easily controlled by an external voltage. Thfore, a detailed analysis to clarify and to evaluate the effmagnitude is greatly desired.

In this paper, we pay attention to another type of tspin-dependent phenomena in the semiconductor hestructures—quantum tunneling. Advances in modern epiial growth technologies such as molecular-beam epitaxymetal-organic chemical-vapor deposition technology provus an opportunity to construct two-dimensional barrier herostructures in which the material parameters canchanged with a wide range and controlled with a considable accuracy. We can discuss possible influence of the sorbit splitting on the transmission probability for modelsthe quantum tunneling structures with realistic parametThe tunneling coupling in double quantum wells15 and tun-neling transmission processes through barrier between

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wells those consider the electron’s in-plane motion16 are alsofields of possible the spin-orbit splitting effect investigatioand implementations.

We calculate the tunneling transmission probabilfor heterostructures with space-dependent electron’s eftive mass and spin-orbit coupling parameters. The depdence leads to the mass and spin-dependent bounconditions.3,17,21,18Since we expect considerable effect winarrow gapAIII -BV semiconductors~where the spin-orbitsplitting effect is strong!, it is important to take into accounnonparabolicity for the electron’s dispersion relation.3 In ourcalculation, we use the well-known approximation for eergy and space dependencies of the electronic effecmass.3,17,21For the spin-dependent tunneling process wetained a dependence of the transmission probability onplane electron’s wave vector. The dependence consisttwo parts: the known dependence originated from spadependent electron’s effective mass,18 and a new one origi-nated from the electronic wave function’s spin-dependboundary conditions.3 Each of them is a result of the bandedge discontinuity at the heterostructure interfaces. It willdemonstrated that the consideration of spin in tunneling pcesses can considerably change energy and in-plane wvector dependencies of the transmission probability in tunstructures.

The variation of the band-structure parameters forsingle barrier tunneling structure to be discussed is showFig. 1. To describe the spin-dependent tunneling in the herostructure we use the approximate effective Hamiltonianthe form proposed in Ref. 3. Layers of the structureperpendicular toz axis, in-plane electron’s wave vector isk@if k is put along an arbitraryx direction, the spin polariza-tion is set along they axis in the layer planer5(x,y)#. Inthis paper, we discuss the influence of discontinuity of efftive mass and spin-orbit coupling parameters on tunneprocesses. The influence from additional external elecfield is not discussed here. With the above-mentionedsumptions, the total wave function of the electronFs(z,r)can be presented as

15 397 ©1998 The American Physical Society

Page 2: Spin-dependent electronic tunneling at zero magnetic field

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15 398 PRB 58BRIEF REPORTS

Fs~z,r!5C j s~z!exp~ ik•r!,

whereC j s(z) satisfies thez component of the Schro¨dingerequation in thej th region,

H jC j s~z!5EC j s~z!, ~1!

with the effective one-electronic zone Hamiltonian

H j52\2

2mj~E!

d2

dz21

\2k2

2mj~E!1Ejc , ~2!

In Eqs.~1! and~2! mj (E) presents electronic effective main nonparabolic approximation

1

mj~E!5

P2

\2 F 2

E2Ejc1Ejg1

1

E2Ejc1Ejg1D jG , ~3!

E denotes the total electron energy in the conduction baEjc , Ejg , andD j stand correspondingly the conduction-baedge, the main band gap, and the spin-orbit splitting in

FIG. 2. Relative difference between the transmission tunneprobability with accounting of spin in boundary conditions awithout that. The InSb-CdTe-InSb symmetric barrier structurerameters are obtained from Refs. 20 and 21:E2c50.35 eV, E3c

50.0 eV, E1g5E3g50.235 eV,E2g51.59 eV, D15D350.81 eV,D250.8 eV, m1(0)5m3(0)50.0135m0 , m2(0)50.11m0 ~m0 isthe free-electron’s mass!, d520 Å.

FIG. 1. Variation of the semiconductors band parameters inneling heterostructures;z–the normal to the barrier direction.

d,

e

j th region ~E1c50, conventionally in our calculation!. Wesuppose, that the matrix elementP does not depend onz.17

The spin-dependent boundary conditions forC j s(z) atthe interface planez5zj betweenj and j 11 regions havebeen introduced in Ref. 3,

1

mj~E! H d

dzln@C j s~z!#J

z5zj

21

mj 11~E! H d

dzln@C j 11s~z!#J

z5zj

52sk@b j 11~E!2b j~E!#

\2,

C j s~zj !2C j 11s~zj !50, ~4!

where

b j~E!5P2

2 F 1

E2Ejc1Ejg2

1

E2Ejc1Ejg1D jG ~5!

is a position and energy-dependent electronic spin-coupparameter ands561 refers to the spin polarization.

The transmission probabilityTs(E,k) is calculated by thestandard quantum mechanics procedure for a rectangularrier structure with the boundary conditions~4! and is givenby

Ts~Ez ,k!54q2k1k3m2

2

m1m3~ f 121 f 2

2!, ~6!

where

f 1~Ez ,k!5qs31coshS qd

\ D2S q22k1k3

m22

m1m31s21s32D sinhS qd

\ D ,

f 2~Ez ,k!5qS k1

m2

m11k3

m2

m3D coshS qd

\ D2m2S k1

s32

m11k3

s21

m3D sinhS qd

\ D ,

d is the thickness of the barrier, q(Ez ,k)5A2m2(E2c2Ez)1\2(12m2 /m1)k2, kj (Ez ,k)5A2mj (Ez2Ejc)2\2(12mj /m1)k2, and si j (Ez ,k)52skm2(b i2b j ) ~here we discuss the tunneling regime fthe electron, whenq2>0 and k3

2>0!. Ez is longitudinalcomponent of the total energy in the first region

Ez5E2\2k2

2m1~E,k!. ~7!

Using ~2! in Eq. ~7!, we find dependenceE(Ez ,k) and,through that,mj (Ez ,k) ( j 52,3) andb j (Ez ,k) dependen-cies, whenj 51,2,3. We can notice, that the expressions~6!generalizes the approach of Ref. 18 for asymmetric recgular tunneling structures.

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Page 3: Spin-dependent electronic tunneling at zero magnetic field

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PRB 58 15 399BRIEF REPORTS

It is clear from Eq.~6! that for symmetric tunnel barriestructures~when m15m3 , E3c50, k15k3 , s215s32, ands3150! the transmission probability does not depend onelectron’s spin direction, but still is different from the tradtional description for electrons without consideration of telectron spin. At the same time, expression~6! describes thecoupling effect of the wave-vector components.18 We usethis expression to investigate the spin dependence of theneling transmission probability for electrons tunnelithrough different kinds of barrier structures.

For symmetric tunnel barrier structures a relative diffence between results with consideration of spin (Ts) andwithout that (T0) can be evaluated by the following expresion

P0~Ez ,k!5Ts~Ez ,k!2T0~Ez ,k!

T0~Ez ,k!. ~8!

To clarify the difference quantitatively, we show in Fig.P0(Ez ,k) calculated for the structure with parametersInSb-CdTe-InSb.2,19,20The difference is well pronounced folargek-vector magnitude. We show in comparison in Figrelative magnitude of the transmission probabilities callated ~for the same structure as in Fig. 2! with the nonpara-bolic approximation and with the parabolic one. From Figit is clear that using of the parabolic approximation~as it wasdone in Ref. 18! leads to overestimation of the effect’s manitude. It demonstrates again that for narrow gap semicductors with relatively strong spin-orbit interaction it is veimportant to involve the nonparabolic dispersion relationdescribe the spin-dependent phenomena.2 All calculationspresented below~as in Fig. 2 also!, therefore, consider thenonparabolic approximation for all involved semiconducmaterials.

For asymmetric tunnel structures we can expect a difence betweenT1(Ez ,k) andT2(Ez ,k) for the electron withthe sameEz andk. To evaluate the electron spin-polarizatio

FIG. 3. Relative magnitude of the spin-dependent transmistunneling probability for the structure of Fig. 2 within parabolapproximation (Tspar) and with accounting of nonparabolicit(Ts). Ez50.01 eV.

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effect in the tunneling process it is useful to calculate ‘‘cefficient of the polarization efficiency’’~CPE! as follows:

P~Ez ,k!5T1~Ez ,k!2T2~Ez ,k!

T1~Ez ,k!1T2~Ez ,k!. ~9!

It should be notified that, according to the boundary coditions ~2!, CPE demonstrates the well-understood prope

P~Ez ,k!52P~Ez ,2k!.

We calculate the effect’s magnitude for an asymmestructure with sharp discontinuity in the spin-orbit couplinparameters as in InP-AlxIn12xAs-GaxIn12xAs hetero-structure.21 In Fig. 4 a result of the calculations is presenteThe effect is quite significant and probably can be propoto experimental investigation. We can expect also increasof the CPE for tunnel structures with additional asymmeproduced by external electric field.

In short conclusion, we demonstrate in this paper thattunneling transmission probability for single barrier strutures can have recognizable spin dependence with wpronounced magnitude of the dependence for not too lain-plane wave vector of tunneling electrons. The dependeis strong for unstrained heterostructures with sharp disconuity of the band-edge parameters, and can provide in asmetric structures the spin polarization effect in the tunnelprocess. We can expect an opportunity to optimize contions of the effect’s existence especially for resonant tunning systems. The described effect can be a base of devement of spin-dependent fast tunneling electronic devices

This work was supported by the Ministry of EducationR.O.C. under Grant No. B87002, and by the National Sence Council under Contract No. NSC 87-2215-E009-01

FIG. 4. Relative difference between transmission probabilityelectrons with ‘‘spin up’’ and ‘‘spin down’’ for asymmetricInP-Al0.48In0.52As-Ga0.47In0.53As barrier structure. The heterostructure parameters are from Ref. 18:E2c50.252 eV, E3c520.252 eV, E1g51.424 eV, E2g51.508 eV, E3g50.813 eV, D1

50.11 eV, D250.33 eV, D350.361, m1(0)50.077m0 , m2(0)50.075m0 , m3(0)50.041m0 , d520 Å.

n

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v. B

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