“review of electron linac based neutron sources for nuclear data study"

29
“Review of electron linac based neutron sources for nuclear data study" Mitsuru Uesaka (Nuclear Professional School, University of Tokyo), ○ Walter Wuensch (CERN) February 6, 2014 CLIC Workshop 2014@CERN, Switzerland

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February 6, 2014 CLIC Workshop 2014 @CERN , Switzerland. “Review of electron linac based neutron sources for nuclear data study". Mitsuru Uesaka (Nuclear Professional School, University of Tokyo), ○ Walter Wuensch (CERN ). CONTENTS. - PowerPoint PPT Presentation

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Page 1: “Review of  electron  linac  based neutron sources for nuclear data study"

“Review of electron linac based neutron sources for nuclear data study"

Mitsuru Uesaka (Nuclear Professional School, University of Tokyo), ○ Walter Wuensch (CERN)

February 6, 2014CLIC Workshop 2014@CERN, Switzerland

Page 2: “Review of  electron  linac  based neutron sources for nuclear data study"

CONTENTS

1. Necessity of more precise nuclear data for melt fuel analysis in Fukushima and design of ADS

2. S-band electron linac neutron system in Belgium, USA and Japan

3. L-band electron linac neutron system in Japan

4. Proposal of new X-band linac system

Page 3: “Review of  electron  linac  based neutron sources for nuclear data study"

Debris in TMI-2 have been analyzed by INEL (USA).EC and Canada also analyzed debris supplied by USA.JAERI (JAEA) also analyzed debris obtained at 1991.

3

Research Background and Purpose

Quantity of nuclear materials in melted cores which are generated in nuclear accident like Fukushima is measured by non-destructive and high accuracy methods

Non-destructive measurement method of nuclear fuels in melted core hasn’t been developed yet.

J. M. Broughton, et al., “A Scenario of the Three Mile Island Unit 2 accident”, Nucl. Technol. 87, 35 (1989). H. Uetsuka, et al., “Gamma Spectrometry of TMI-2 Debris” (written in Japanese), JAERI-Research 95-084.

Hideo Harada (JAEA)

Page 4: “Review of  electron  linac  based neutron sources for nuclear data study"

Conceptual Diagram of NRD Facility

4

• By NRTA, 3-7 kg of small sized MF will be measured within 20 min. (The 3-7 kg: a MF area of 300-700 cm2 and a thickness of 10 g/cm2). • By NRCA, 30 g of MF including 109 Bq (mainly 137Cs) will be

measured within 1 hour for each beam line.

Neutron detector

Sample for NRTA

Gamma detector

Beam dump

n ~ 1012 n/sec

Sample for NRCA

Accelerator for pulsed neutron

generation

Hideo Harada (JAEA)

Page 5: “Review of  electron  linac  based neutron sources for nuclear data study"

TOF Measurement by Small Pulse Neutron Source

5

A Rough Sketch of Prototype Neutron Resonance Densitometer

Flight path = 5 m for NRTA

Hideo Harada (JAEA)

Page 6: “Review of  electron  linac  based neutron sources for nuclear data study"

Typical NRTA Data of Nuclear Materials

Neutron Energy / eV

Tran

smis

sion

1 2 4 6 8 10 20 40

240 P

u24

1 Am

243 A

m

242 P

u

239 P

u23

8 U238 U

131 X

e

152 S

m23

5 U

145 N

d24

1 Pu

236 U

133 C

s23

8 U

235 U

239 P

u

235 U

Behrens et al., Nucl. Techn. 67 (1984) 162

6

Hideo Harada (JAEA)

Page 7: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 8: “Review of  electron  linac  based neutron sources for nuclear data study"

Precision of nuclear data

Page 9: “Review of  electron  linac  based neutron sources for nuclear data study"

FacilityReference

Beamenergy

Beam powern Intensity

Beam pulse widthPulse per sec

Flux

IRMM, GELINAND2007, p.563

Electron100 MeV

6 kW 1 ns800 Hz @ 12 m

ORNL, ORELAND2007, p.441

Electron180 MeV

5 kW1013 n/s

8 ns525 Hz @ 40 m

Kyoto, e LinacND2007, p.591

Electron30 MeV

1 kW 100 ns100 Hz @ 10 m

CERN, n-TOFND2007, p.537

Proton20 GeV

9 kW1015 n/s

6 ns0.4 Hz

4×105 n/cm2/s@ 185 m

LANL, LujanND2007, p.415

Proton0.8 GeV

80 kW 135 ns20 Hz @ 20 m

J-PARC, MLF(Expected)

Proton3 GeV

1 MW ~ 1017 n/s~ 100 ns

25 Hz~ 109 n/cm2/s

@ 22 m

Neutron TOF facility for nuclear data measurements

9

Page 10: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 11: “Review of  electron  linac  based neutron sources for nuclear data study"

CONTENTS

1. Necessity of more precise nuclear data for melt fuel analysis in Fukushima and design of ADS

2. S-band electron linac neutron system in Belgium, USA and Japan

3. L-band electron linac neutron system in Japan

4. Proposal of new X-band linac system

Page 12: “Review of  electron  linac  based neutron sources for nuclear data study"

EC – JRC – IRMMInstitute for Reference Materials & Measurements

Page 13: “Review of  electron  linac  based neutron sources for nuclear data study"

Pulsed white neutron source (10 meV < En < 20 MeV)

Neutron energy : time – of – flight (TOF)

Multi-user facility: 10 flight paths (10 m - 400 m)

Measurement stations with special equipment to perform:

• Total cross section measurements• Partial cross section measurements

TOF - Facility GELINA

FLIGHT PATHS SOUTH

FLIGHT PATHS NORD

ELECTRON LINAC

TARGET HALL

Mondelaers and Schillebeeckx, Notizario 11 (2006) 19

Page 14: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 15: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 16: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 17: “Review of  electron  linac  based neutron sources for nuclear data study"

Hokkaido University 45 MeV electron linac

1717

6.12m3.5m

3.5m

Neutron room

1m

6.4m 1.96m

21.1m

Target roomTarget room + LINAC =42.5 m

Electron energy ~45MeV (gun current   ~50mA )~30 MeV ( gun current~210 m A )

Electron current Average ( example, 60μA   pulse width 3μs)

Pulse rate 10 ~ 100p.p.s(variable 、 single pulse )

45 MeV LINAC

Page 18: “Review of  electron  linac  based neutron sources for nuclear data study"

Performance of Hokkaido University 45 MeV electron linac

18

•S-band electron linear accelerator•Maximum energy:45 MeV•Maximum current: 140μA•Repetition: single 10pps~200pps•Pulse width: 10ns ~3μs

•The electron beam is transported to the target room.•RIGHT: Pulsed cold neutron source•CENTER: Pulsed thermal neutron source, electron beam irradiation•LEFT: Fast neutron experiments

Page 19: “Review of  electron  linac  based neutron sources for nuclear data study"

Typical Neutron and Photon Source

19

Cold neutron

Intensity of neutronsBelow 25.3meV 1.0×103 (1/cm2/s)@L=6m 4.8×10^9(1/s)@Neutron Source

• 2mm thick lead radiator• Electron Beam Energy = 25 MeV• Pulse Width = 0.2 μs• Rep.rate = 50 pps• Electron beam current = 2 μAIntensity 20~30MeV ~1012 (1/s)

Bremsstrahlung photon

PHITSSimulation

By Prof. Kiyanagi, and Prof. Kino’s presentation

exp

Page 20: “Review of  electron  linac  based neutron sources for nuclear data study"

CONTENTS

1. Necessity of more precise nuclear data for melt fuel analysis in Fukushima and design of ADS

2. S-band electron linac neutron system in Belgium, USA and Japan

3. L-band electron linac neutron system in Japan

4. Proposal of new X-band linac system

Page 21: “Review of  electron  linac  based neutron sources for nuclear data study"

・ Specification of injectorelectric gun : YU-156(EIMAC)incident voltage : 100kV DC, incident current : Max 10A・ Specification of RF driveroutput : 3kW, frequency : 1300.8 MHz・ Energy of electron for neutron generation : ~ 30 MeV・ Peak current : ~ 5A (short pulse) 2 ~ 100ns width ~ 0.5A(long pulse) 0.1 ~ 4 ms width・ Frequency : 1 ~ 300 Hz (short pulse)

1 ~ 100Hz (long pulse)・ Neutron target : Ta with H2O moderator・ Power on target : Maximum 6 kW (200mA, 30MeV)・ Electron beam diameter on target : 1 cm・ Neutron production : ~ 8×1012 n/s @6kW

Present status of KURRI-L-band LinacResearch Reactor Institute, Kyoto UniversityJun-ichi Hori

Page 22: “Review of  electron  linac  based neutron sources for nuclear data study"

Injector and accelerator tubes

Ta target and water moderator (Type-1)

Target roomWater moderator in Al case

Ta target

Ta target and water moderator (Type-2)

Page 23: “Review of  electron  linac  based neutron sources for nuclear data study"

2. Flight path

Target room

Ta target

Flight tube : 2 linesFlight path : 10.0, 12.7, 24.2 m

Measurement room at 10m

Measurement room at 24m

Measurement room at 12.7m

Control room

Cooling tower

Lead spectrometer

Experimental room

Page 24: “Review of  electron  linac  based neutron sources for nuclear data study"
Page 25: “Review of  electron  linac  based neutron sources for nuclear data study"

CONTENTS

1. Necessity of more precise nuclear data for melt fuel analysis in Fukushima and design of ADS

2. S-band electron linac neutron system in Belgium, USA and Japan

3. L-band electron linac neutron system in Japan

4. Proposal of new X-band linac system

Page 26: “Review of  electron  linac  based neutron sources for nuclear data study"

TOF (Time-Of-Flight) system for nuclear data measurement

電子ビーム

レーザー

X 線

電子ビーム

レーザー

X 線

Ce:LiCAF

Laser

X-ray

Page 27: “Review of  electron  linac  based neutron sources for nuclear data study"

電子ビーム

レーザー

X線

電子ビーム

レーザー

X線

Existing X-band 30 MeV electron linac will be moved for neutron source

70 cm accelerator tube

5 m TOF planning area

More than 10 m TOFplanning area

More than 40 m TOFplanning area

Klystron and power source are set around the reactor

20 keV electorn gun + 5 MeV buncher+30 MeV structure+ Neutron target

Peak Beam current: 250mA (Beam energy: 30MeV ・ Pulse width: 1μsec)Beam Power: 0.375kW (50pps)( S-band 30MeV 1kW(Hokkaido ⇒

Univ.) )

30 MeV X-band Linac

Page 28: “Review of  electron  linac  based neutron sources for nuclear data study"

S-band vs X-band- Electron Energy: Both are available- Charge per microbunch: X is ~1/10- Bunches for RF pulse: X is 3~4 times- Charge and Peak Current per RF pulse and

Average Current/Power: S is higher by ~2. However, X-band 6 MW 400Hz Klystron is under development so that the current/power becomes closer.- Size: X is smaller.- Price is linear to Beam Power, maybe.

Page 29: “Review of  electron  linac  based neutron sources for nuclear data study"

Summary

• Several L/S-band electron linac neutron sources are operating for nuclear data study in the world.

• Precision of nuclear data must be improved for Fukushima accident analysis and design of new nuclear system such as ADS.

• New X-band electron linac neutron source is proposed and under construction at University of Tokyo.

• Almost all L/S-band systems are older than 40 years and it is the time of renewing.

• Due to compactness of X-band system, it can be installed in existing shielding facilities. Even its intensity is expected to be upgraded by new X-band high rep rate klystron.

Thank you for your attention.