retrieval of mixing height and dust concentration with lidar

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Boundary-Layer Meteorol (2007) 124:117128 D O I 1 0 . 1 0 0 7 / s 1 0 5 4 6 - 0 0 6 - 9 1 0 3 - 3 O R I G I N A L P A P E R Retrieval of mixing height and dust concentration with lidar ceilometer Christoph Münkel · Noora Eresmaa · Janne Räsänen · Ari Karppinen Received: 1 December 2005 / A ccepted: 1 2 J une 2006 / P ublished online: 5 A ugust 2006 ' S p r i n g e r S c i e n c e + B u s i n e s s Me d i a B . V . 2 0 0 6 Abstract T h e V aisala ceilometers CT25K and C L31 a re eye-safe single lens lidar sys- t e m s r e p o r t i n g a t t e n u a t e d b a c k s c a t t e r p r o l e s ; t h e y o f t e n o p e r a t e 2 4 h a d a y i n f u l l y a u t o m a t e d , h a n d s - o f f o p e r a t i o n m o d e . T h e s e p r o l e s c a n b e u s e d f o r m o r e t h a n j u s t c l o u d - b a s e h e i g h t d e t e r m i n a t i o n . I n d r y w e a t h e r s i t u a t i o n s , t h e r e i s a f a i r l y g o o d c o r r e - l a t i o n b e t w e e n t h e c e i l o m e t e r n e a r - r a n g e b a c k s c a t t e r a n d i n s i t u P M 1 0 c o n c e n t r a t i o n r e a d i n g s . T h e c o m p a r i s o n o f m i x i n g h e i g h t v a l u e s b a s e d o n s o u n d i n g s a n d o n c e i l - o m e t e r b a c k s c a t t e r i n g p r o l e s i n d i c a t e s t h a t c e i l o m e t e r s a r e s u i t a b l e i n s t r u m e n t s f o r d e t e r m i n i n g t h e c o n v e c t i v e m i x i n g h e i g h t . I t s e n h a n c e d o p t i c s a n d e l e c t r o n i c s e n a b l e s t h e C L 3 1 c e i l o m e t e r t o d e t e c t n e b o u n d a r y - l a y e r s t r u c t u r e s w h o s e c o u n t e r p a r t s a r e s e e n i n t e m p e r a t u r e p r o l e s . Keywords A e r o s o l · Ceilometer · L i d a r · M i x i n g h e i g h t 1 Introduction L i d a r (l i g h t d e t e c t i o n a n d r a n g i n g ) i s a n a c t i v e r a n g e - r e s o l v i n g o p t i c a l r e m o t e m e a - s u r e m e n t t e c h n i q u e . C o m m e r c i a l l i d a r c e i l o m e t e r s h a v e t o d a t e b e e n m a i n l y i n s t a l l e d at airelds and meteorological s tations to report c loud layers , vertical v isibility , and c l o u d c o v e r ( W e i t k a m p 2 0 0 5 , p p 1 7 5 1 8 1 ) . A d d i t i o n a l l y , t h e i r r e g u l a r b o u n d a r y - l a y e r s c a n s c a n b e e x a m i n e d f o r t h e r e t r i e v a l o f p a r a m e t e r s s u c h a s e x t i n c t i o n c o e f c i e n t proles , v isibility mixing h eight, and dust c oncentration. Being c onstructed t o operate C . M ü n k e l ( B ) V a isala GmbH, Schnackenburgallee 41d, 22525 Hamburg , Germany e - m a i l : c h r i s t o p h . m u e n k e l @ v a i s a l a . c o m N . E r e s m a a · A . K a r p p i n e n F i n n i s h M e t e o r o l o g i c a l I n s t i t u t e , H e l s i n k i , F i n l a n d J . R s n e n V a i s a l a O y j , V a n t a a , F i n l a n d

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Page 1: Retrieval of mixing height and dust concentration with lidar

Boundary-Layer Meteorol (2007) 124:117–128DOI 10.1007/s10546-006-9103-3

ORIGINAL PAPER

Retrieval of mixing height and dust concentrationwith lidar ceilometer

Christoph Münkel · Noora Eresmaa ·Janne Räsänen · Ari Karppinen

Received: 1 December 2005 / Accepted: 12 June 2006 / Published online: 5 August 2006© Springer Science+Business Media B.V. 2006

Abstract The Vaisala ceilometers CT25K and CL31 are eye-safe single lens lidar sys-tems reporting attenuated backscatter pro�les; they often operate 24 h a day in fullyautomated, hands-off operation mode. These pro�les can be used for more than justcloud-base height determination. In dry weather situations, there is a fairly good corre-lation between the ceilometer near-range backscatter and in situ PM10 concentrationreadings. The comparison of mixing height values based on soundings and on ceil-ometer backscattering pro�les indicates that ceilometers are suitable instruments fordetermining the convective mixing height. Its enhanced optics and electronics enablesthe CL31 ceilometer to detect �ne boundary-layer structures whose counterparts areseen in temperature pro�les.

Keywords Aerosol · Ceilometer · Lidar · Mixing height

1 Introduction

Lidar (“light detection and ranging”) is an active range-resolving optical remote mea-surement technique. Commercial lidar ceilometers have to date been mainly installedat air�elds and meteorological stations to report cloud layers, vertical visibility, andcloud cover (Weitkamp 2005, pp 175–181). Additionally, their regular boundary-layerscans can be examined for the retrieval of parameters such as extinction coef�cientpro�les, visibility mixing height, and dust concentration. Being constructed to operate

C. Münkel (B)Vaisala GmbH, Schnackenburgallee 41d, 22525 Hamburg, Germanye-mail: [email protected]

N. Eresmaa · A. KarppinenFinnish Meteorological Institute, Helsinki, Finland

J. RäsänenVaisala Oyj, Vantaa, Finland

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118 Boundary-Layer Meteorol (2007) 124:117–128

permanently and unattended for several years in all kinds of meteorological environ-ment quali�es these eye-safe instruments also for air quality surveillance purposes.

2 Ceilometer basics and technical properties

2.1 Simpli�ed lidar equation

The optical power received by a ceilometer from distancex is

P(x,λ) = c2x2 P0AηO(x)�t

︸ ︷︷ ︸

instrument speci�c

× β(x,λ)τ2(x,λ)︸ ︷︷ ︸

attenuated backscatter

, (1)

where c is the speed of light,�t is the (laser) pulse duration, P0 is the average laserpower during the pulse, A is the area of the receiver optics andη is its ef�ciency.O(x) is the range-dependent overlap integral between the transmitted beam and the�eld-of-view of the receiver (complete overlap at O(x) = 1). β(x, λ) is the backscattercoef�cient, τ(x, λ) is the transmittance of the atmosphere between the lidar and thescattering volume,λ is the wavelength of the emitted laser pulse, andx is the distancebetween lidar and scattering volume.

After solving for all the instrument speci�c factors, constants and squared distance,the attenuated backscatter coef�cient can be retrieved. This quantity is the productof the volume backscatter coef�cient β at rangex and the square of the transmittanceof the atmosphere between the lidar and the scattering volumeτ2.

During all cases with range valuesx above 30 m discussed in this paper, the mete-orological optical range at ground level exceeded 10,000 m, leading toτ2 values thatare greater than 0.83. This is reasonably close to 1 to take the attenuated backscat-ter coef�cient as a measure for β. If we further assume that the scatterer propertiesremain unchanged through the sample volume, the backscatter values would alsocorrelate with the range-resolved aerosol concentration. Correspondingly, having thescatterer properties at a certain height constant with time would enable seeing tem-poral variations in aerosol concentration in a selected volume.

2.2 Optical ceilometer designs

The instrument involved in the measuring campaigns treated in Sect. 3 and Sect. 4.2.1is the Vaisala ceilometer CT25K, which is a single lens lidar system equipped withpulsed near-infrared diode lasers. To obtain suf�cient signal-to-noise ratios, the returnsignal of 65,000 laser pulses is integrated for each range gate. A beam splitter givesfull overlap of the transmitter and receiver �eld-of-view already at an altitude of 0 m.Direct re�ections at the lens surfaces give a high signal at the receiver. To preventreceiver saturation by this strong cross-talk signal between transmitter and receiver,compensation electronics are used with an optical �bre feeding the negative amountof the transmitter signal to the receiver. Figure 1 contains a schematic arrangementof the CT25K optical concept.

The latest Vaisala ceilometer CL31 (Fig. 2) uses a novel single lens design, whosemain innovation is in the way the common lens is used for transmitting and receivinglight. The centre of the lens is used for collimating the outgoing laser beam, whereasthe outer part of the lens is used for focusing the backscattered light onto the receiver.

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Boundary-Layer Meteorol (2007) 124:117–128 119

Fig. 1 Optical concept of thesingle lens lidar ceilometerCT25K

Fig. 2 Ceilometer CL31,overall height = 1190 mm

The division between transmitting and receiving areas is provided by an inclinedmirror with a hole in the centre as shown in Fig. 3. This arrangement signi�cantlyreduces the optical cross-talk between transmitter and receiver. The need for sep-arate compensation mechanisms is avoided leading to a simpler and more reliableinstrument design. The new single lens design is also robust against changes in themechanical alignment of the optical parts. Measurement examples obtained with theCL31 ceilometer are presented in Sects. 4.2.2 and 4.2.3.

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120 Boundary-Layer Meteorol (2007) 124:117–128

Fig. 3 Enhanced single lensoptical concept of the lidarceilometer CL31

Table 1 Technical properties of the ceilometers CT25K and CL31

CT25K CL31

Measurement range (m) 0− 7500 0− 7500Resolution (m) 15 10Laser system InGaAs MOCVD laser diode InGaAs MOCVD laser diodeWavelength (nm) 905 905Pulse properties 100 ns, 1.6µJ/pulse 110 ns, 1.2µJ/pulseMean pulse repetition rate (Hz) 4369 8192

2.3 Ceilometer technical properties

Table 1 lists the main technical properties of the two lidar ceilometers used for thisstudy. Eye-safety considerations do not allow larger single pulse energy values; thisdisadvantage is overcome by using high pulse repetition rates increasing the signal-to-noise ratio.

3 Aerosol concentration measurements

One task within the VALIUM measuring campaign carried out at the site of the LowerSaxony State Agency for Ecology (NLÖ) in Hanover, Germany, was the comparison ofceilometer near-range backscatter data with PM10 and PM2.5 concentration reportedhalf-hourly by point sampling sensors. Figure 4 shows the measurement set-up, wherethe PM10 and PM2.5 inlet probes were situated 20 m above the ceilometer level.

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Boundary-Layer Meteorol (2007) 124:117–128 121

Fig. 4 Measurement set-upfor ceilometer aerosolconcentration measurements,PM10 and PM2.5 inlet probeslevel is 20 m above theceilometer

For comparison with in situ dust concentration, CT25K ceilometer attenuated back-scatter from the two lowest range gates covering the elevation interval from 0 to 30 mhas been averaged over a period of 30 min. Wet haze, fog, and precipitation situationswere excluded from the data analysis by using only those 30-min intervals with relativehumidity values below 62% and no precipitation detected. The latter information wasprovided by an optical yes/no precipitation monitor. 75.5% of all datasets gatheredduring the period between 1 March 2002 and 23 April 2003 were thus eliminated. Theremaining 5736 “dry” datasets show a fairly good correlation (R = 0.8351) betweenthe PM10 in situ concentration values and the average attenuated ceilometer back-scatterβ30 (Fig. 5). Raising the 62% relative humidity limit decreases the correlationquality ( R = 0.8138 for a 74% limit, R = 0.7730 for a 86% limit); a smaller limit bringsno signi�cant quality increase. Assuming a linear relationship between β30 and PM10concentration values, a correlation analysis gives a simple equation for the estimationof PM10 concentration ρPM10 with a ceilometer. The resulting linear �t coef�cientsare m = 2.023× 107 µg m−2 sr and b = −1.6304µg m−3,

ρPM10 = mβ30 + b. (2)

Figure 6 shows the comparison of PM10 concentration derived from ceilometer datawith in situ values for a fair weather period. The in situ measured PM2.5 concentrations

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122 Boundary-Layer Meteorol (2007) 124:117–128

0 1 2 3 4 5 6 70

20

40

60

80

100

120

140

Attenuated ceilometer backscatter in 10–6 m –1 sr –1

PM

10 c

once

ntra

tion

in µ

g m

–3

Line of regression: f(x) = –1.6304 + 2.023⋅107 * xCorrelation coefficient: 0.8351

Fig. 5 Ceilometer attenuated backscatter versus in situ measured PM10 concentration, 5736 dryweather datasets, NLÖ Hanover, 1 March 2002—23 April 2003

06 07 08 09 10 110

10

20

30

40

50

60

70

80

Day in April 2002

Con

cent

ratio

n ρ P

M10

, ρ P

M2.

5 in µ

g m

–3 ρPM10

from in situ sensor

ρPM10

from ceilometer

ρPM2.5

from in situ sensor

Fig. 6 PM10 and PM2.5 concentrations reported from in situ sensors and ceilometer, NLÖ Hanover,April 2002

are also plotted. In some instances these exceed the PM10 values; this is not reason-able because PM10 concentration includes all particles with sizes ranging from 0µmto 10µm and should therefore not be smaller than the concentration of all particlesbelow 2.5µm. This �nding illustrates that the 30-min averaging interval for in situ PMassessment is a challenge for PM measurements in general.

4 Mixing height retrieval

4.1 Methods

As it was stated in Sect. 2, we can expect the lidar backscatter pro�les to track theaerosol concentrations in a reasonably transparent atmosphere. The aerosol concen-trations, in turn, can be expected to reveal details about the vertical structure of theatmospheric boundary layer, such as mixing height.

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Boundary-Layer Meteorol (2007) 124:117–128 123

Generally, a number of methods for retrieving mixing layer height from lidar back-scatter pro�les have been presented (Menut et al. 1999; Steyn et al. 1999; Cohn andAngevine 2000; Davis et al. 2000).

The known methods are mostly based on two assumptions about the atmosphericdistribution of scattering aerosols. Firstly, the mixed layer is expected to have a some-what constant concentration that is higher than in the layers above. Consequently, thedifference between the mixed layer and the air above is assumed to be seen as a shiftfrom a relatively strong backscatter inside the mixed layer to a lower backscatter levelabove it (Steyn et al. 1999). The methods used in this study are the so-called gradientmethod and the idealised backscatter method introduced by Steyn et al. (1999).

It must be emphasized, however, that not in all cases do lidar backscatter methodsprovide a good measure of the mixing height. During late afternoon when the plan-etary boundary layer is collapsing, the aerosol concentrations remain high and showthe maximum depth of the daytime mixed layer. The aerosol concentration trace innocturnal surface inversions is often too weak and dominated by high residual layers,as is the morning growth of the mixed layer. Examples will be discussed in Sect. 4.2.

4.1.1 Idealised backscatter method

The method relies on the assumptions mentioned above. The technique is based on�tting an idealised backscatter pro�le B(z) to the measured attenuated backscatterpro�le β(z) (see Fig. 7b). Fitting parameters include mean mixed layer backscatterBm, mean backscatter immediately above the mixed layerBu as well as mixing heightitself and a measures proportional to the entrainment zone thickness (Steyn et al.1999),

B(z) = Bm + Bu

2−

(

Bm − Bu

2

)

erf(

z − MHs

)

. (3)

The �tting procedure results in a mixing height estimate and a value characterisingthe entrainment zone.

4.1.2 Gradient method

The gradient method selects the maximum of the negative gradient (−dβ/dx) of thebackscatter coef�cient to be the top of the mixed layer. To reduce sensitivity to noiseand temporary details in atmospheric structure, vertical and temporal averaging maybe applied before or after differentiation. Also, there are options of using eitherabsolute maximum or local maxima for boundary-layer characterisation.

4.2 Measurements and results

4.2.1 One year campaign in Vantaa, Finland

The data used in this section were obtained on the premises of Vaisala Oyj, Vantaa(suburban Helsinki), Finland between 16 December 2001 and 10 November 2002 witha CT25K ceilometer. In convective situations, mixing height (MH) is estimated fromradiosoundings using the Holzworth method—this follows the dry adiabatic startingat the surface up to its intersection with the temperature pro�le. In stable situationsthe Richardson number method (Joffre et al. 2001) is used, with a critical value of 1.

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124 Boundary-Layer Meteorol (2007) 124:117–128

CT25K Backscatter and Mixing Height on 2002–05–29

Local Time (h)

Hei

ght (

m)

2 4 6 8 10 12 14 16 18 20 220

200

400

600

800

1000

1200

1400

1600

1800

2000CT25K Mixing HeightSounding Mixing Height

0 200 400 6000

200

400

600

800

1000

1200

1400

1600

1800

2000

Backscatter (a.u.)

Hei

ght (

m)

Ceilometer Backscatter at 0845

12 14 16 18 200

200

400

600

800

1000

1200

1400

1600

1800

2000Sounding at 0845

Potential T (°C)

Hei

ght (

m)

CeilometerIdealised Backscatter

a

b

Fig. 7 Ceilometer and radiosounding data from Vaisala test �eld in Vantaa, suburban Helsinki,Finland on 29 May 2002. The backscatter image(a) includes the mixing height retrieved with theidealised backscatter method and mixing height computed from the radiosounding data. A snapshotat 0845(b) con�rms the match between ceilometer and sounding in more detail

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Boundary-Layer Meteorol (2007) 124:117–128 125

The MH is determined from the ceilometer attenuated backscatter pro�le using theidealised backscatter method. In the �tting half-hourly averaged pro�les have beenused. A 24-h period of ceilometer observations is displayed in Fig. 7a. The methodlocates the boundary-layer top consistently on the clear spring day in question. Thecalculated mixing height is apparently reported to the residual layer height until about0330 because trends in backscatter decrease with height are rather weak. After that, astable layer with mixing height around 200 m is reported. Unfortunately, there are noradiosonde soundings available from the night to con�rm if ceilometer data correctlyreport the conditions.

After sunrise, a convective boundary layer develops, eventually reaching about1,300 m. There were four radiosoundings made on this day (see Fig. 7a) and they showvery good agreement with the ceilometer mixing height. The increased backscatter at11:30 local time may be connected to the start of the sea breeze from the directionof downtown Helsinki. It is readily seen how turbulence becomes stronger and theMH grows after the sun rises. The mixing height values after 23:00 local time showthe residual layer.

A comparison between the mixing heights measured by the ceilometer and ra-diosoundings during the one year measuring campaign is shown in Fig. 8. A total of71 convective and 38 stable clear sky cases were analysed. In convective situations15 observations, and in stable situations a single observation, were rejected becauseof low backscattering signal near the surface (observations marked with a circle inFig. 8), involving both the measured backscatter and the �tted Bm values from Eq. (3).A regression line is �tted to the remaining observations (stars in Fig. 8). The regres-sion lines and correlation between MHs determined by ceilometer and soundings arelisted in Table 2; the error margins in Table 2 correspond to 95% con�dence level ofthe regression coef�cients.

0 200 400 600 8000

100

200

300

400

500

600

700

800

Mix

ing

heig

ht b

ased

on

ceilo

met

er (

m)

Mixing height based on sounding (m)

Stable situations

0 500 1000 1500 2000 25000

500

1000

1500

2000

2500

Mix

ing

heig

ht b

ased

on

ceilo

met

er (

m)

Mixing height based on sounding (m)

Convective situations

Accepted case (N=56)Rejected case (N=15)Regression line

Accepted case (N=37)Rejected case (N=1)Regression line

Fig. 8 Correlation between ceilometer and radiosounding MH

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126 Boundary-Layer Meteorol (2007) 124:117–128

Table 2 Correlation and regression between MHs determined by ceilometer and soundings

Correlationbetween ceilometerand sounding

Regression(x = MHby ceilometery = MH bysounding)

Number ofacceptedcases

Number ofrejected cases

Convectivesituations

0.9 x = (0.8 ±0.1)y + (47±89)

56 15

Stablesituations

0.8 x = (0.62±0.15)y + (124± 32)

37 1

Fig. 9 Sliding average (150 m, 15 min) CL31 ceilometer attenuated backscatter pro�les recordedin Vantaa, Finland on 04 April 2005 together with mixing heights determined by ceilometers andsoundings. Residual layers are visible up to a height of 1,800 m

4.2.2 Inter ceilometer comparison for one day

Figure 9 shows a diurnal boundary-layer cycle on a nearly cloudless day, and con-tains attenuated backscatter pro�les measured with the CL31 ceilometer and mixingheights calculated with the idealised backscatter method for both the CT25K andCL31, together with available radiosounding MHs for that day. Additionally, a gradi-ent method that selects the absolute maximum of the negative gradient as the mixingheight has been applied to the CL31 data. In most cases, this method shows a tendencyto smaller mixing height values, with a decreased probability of reporting the heightof the residual layer.

4.2.3 Boundary-layer structures and temperature inversions

The improved measurement performance of the CL31 ceilometer sharpens the viewon structures in aerosol density. This can be studied using measurements made in arural (Fig. 10) and an industrial environment (Fig. 11). Temperature inversion heightsfrom radiosoundings are also plotted in Fig. 10. They are very close to local minimaof the gradient of the attenuated backscatter pro�le. Strati�cation expected from thetemperature pro�les seem to accurately correspond to aerosol structures revealed in

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Boundary-Layer Meteorol (2007) 124:117–128 127

Fig. 10 Attenuated backscatter sliding average (50 m, 90 s) density plot recorded in Vantaa, Finlandon 15 October 2004. For additional reference, potential temperature pro�les from the soundings at0728 and 1040 local time are shown

Fig. 11 Attenuated backscatter sliding average (50 m, 90 s) density plot recorded in Hamburg,Germany on 01 February 2005

backscatter pro�les. The scattering aerosols are tracers of the prevailing atmosphericcondition, and therefore produce a readable signature.

The upper edge of the boundary layer is very clearly visible in Fig. 11, and nofurther calculation is necessary to retrieve the mixing height.

When the gradient method is used in a way that selects the absolute maximum ofthe negative gradient of the attenuated backscatter coef�cient as the mixing height,the highest local maxima from Fig. 10 are picked as the mixing height, except for thetime interval from 0725 to 0850, when the �rst maximum at 50 m is chosen.

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128 Boundary-Layer Meteorol (2007) 124:117–128

5 Summary and conclusions

Ceilometers are affordable, reliable, and essentially maintenance free tools for mixingheight assessment and boundary-layer scans in clear sky cases.

A promising algorithm for dust particle concentration measurements with ceilo-meters has been developed, though further studies incorporating the new ceilometerCL31 are required for its re�nement and �nalisation, and for testing its ability toobtain vertical concentration pro�les. Special attention has to be paid to the correctidenti�cation of weather situations that rule out the applicability of this approach. Ameasuring campaign close to a meteorological mast should be performed to investi-gate the in�uence of the relative humidity pro�le.

Ceilometers show promising performance and take a step towards automated mix-ing height measurement. The results indicate that applying the idealised backscattermethod to ceilometer data works for both stable and unstable conditions. The gra-dient method extracts signi�cant information from the pro�les. A matter for furtherstudies would be, e.g., comparing the methods against a reference such as frequentradiosoundings, SODAR, windpro�ler, or RASS measurements.

References

Cohn SA, Angevine WM (2000) Boundary-layer height and entrainment zone thickness measured bylidars and wind-pro�ling radars. J Appl Meteorol 39:1233–1247

Davis KJ, Gamage N, Hagelberg CR, Kiemle C, Lenschow DH, Sullivan PP (2000) An objectivemethod for deriving atmospheric structure from airborne lidar observations. J Atmos OceanicTech 17:1455–1468

Joffre SM, Kangas M, Heikinheimo M, Kitaigorodskii SA (2001) Variability of the stable and unstableBoundary-layer height and its scales over a Boreal Forest. Boundary-Layer Meteorol 99:429–450

Menut L, Flamant C, Pelon J, Flamant PH (1999) Urban Boundary-layer height determination fromlidar measurements over the Paris Area. Appl Optics 38:945–954

Steyn DG, Baldi M, Hoff RM (1999) The detection of mixed layer depth and entrainment zonethickness from lidar backscatter pro�les. J Atmos Oceanic Tech 16:953–959

Weitkamp C (Ed.) (2005) Lidar: range-resolved optical remote sensing of the atmosphere, Springer,New York, 460 pp