an assessment of cmaq with teom measurements over the eastern us

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An Assessment of CMAQ with TEOM Measurements over the Eastern US. Michael Ku, Chris Hogrefe, Kevin Civerolo, and Gopal Sistla. PM Model Performance Workshop, February 10-11, 2004, RTP, NC. Model Simulations. MM5 – 108/36/12 km two-way nesting. SMOKE – 1996 CSA emission inventory. - PowerPoint PPT Presentation

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An Assessment of CMAQ with TEOM Measurements over the

Eastern US

Michael Ku, Chris Hogrefe, Kevin Civerolo, and Gopal Sistla

PM Model Performance Workshop, February 10-11, 2004, RTP, NC

Model Simulations

• MM5 – 108/36/12 km two-way nesting.

• SMOKE – 1996 CSA emission inventory.

• CMAQ – 12 km domain only; both CB-IV and RADM2; IC/BC used background values.

• Simulation Period – July 2 – August 1, 1999

TEOM Measurements

21 sites include SLAMS, USDOE, NEOPS, and SEARCH.

TEOM MeasurementsOrganization # of Sites ID used in analysis

Iowa (SLAMS) 6 1 - 6

New Jersey (SLAMS) 5 7 - 11

New York (SLAMS) 1 12

North Carolina (SLAMS) 1 13

South Carolina (SLAMS) 2 14 - 15

USDOE (PA) 2 16 - 17

SEARCH (AL & GA) 3 18 - 20

NEOPS (PA) 1 21

Total 21

20 40 60 80 100 120 140 160

20

40

60

80

100

120

140

Modeling Domain and TEOM Sites

Model Evaluation

• Examine the Model Error

• Examine the Model skill

-- Compare the spatial structures

-- Compare the temporal patterns

Statistics: Hourly Data

Parameter TEOM Observed

CMAQ

CB-IV

CMAQ

RADM2

Mean 22.28 29.99 28.05

S.D. 14.29 25.37 23.89

R 0.46 0.46

Mean Bias 7.8 5.78

RMSE 23.76 22.26

Comparison at each site

-20

-10

0

10

20

30

40

50

1 3 5 7 9 11 13 15 17 19 21

Site CB-IV RADM2

0

10

20

30

40

50

60

1 3 5 7 9 11 13 15 17 19 21

Site CB-IV RADM2

-0.2

0.0

0.2

0.4

0.6

0.8

1.0

1 3 5 7 9 11 13 15 17 19 21

Site CB-IV RADM2

Statistics: Daily Averaged Data

Parameter TEOM

observed

CMAQ

CB-IV

CMAQ

RADM2

Mean 22.23 29.99 28.05

S.D. 11.59 22.60 21.24

R 0.57 0.57

Mean Bias 7.80 5.75

RMSE 19.98 18.38

CMAQ (CB-IV) predicts slightly higher daily averaged values

than CMAQ (RADM2).

0 20 40 60 80 100 1200

20

40

60

80

100

120Daily Averaged Data

CB-IV

RA

DM

2

0 20 40 60 80 100 1200

20

40

60

80

100

120

TEOM

CM

AQ

(C

B-I

V)

CMAQ (CB-IV) underpredicted low-end and overpredicted high end of the daily averaged values.

0 20 40 60 80 100 1200

20

40

60

80

100

120

TEOM

CM

AQ

(R

AD

M2

)

CMAQ (RADM2) underpredicted low-end and overpredicted high end of the daily averaged values.

Compare Spatial Structures

-Calculate Cross-correlation coefficients of TEOM measurements and CMAQ outputs at the TEOM sites. The calculations yield a 21x21 symmetric matrix of correlation coefficients which represent the correlation of the sites with each other.

-If CMAQ produces similar correlation coefficients matrix with TEOM, the CMAQ is able to capture the TEOM measured spatial structures.

-0.2

-0.1

0

0.1

0.2

0.3

0.4

0.5

0.6

0.7

0.8

1 3 5 7 9 11 13 15 17 19 21

2

4

6

8

10

12

14

16

18

20

site

site

TEOM

0

0

0

0

0

0

0.2

0.2

0.2

0.2

0.20.2

0.2

0.2

0.2

0.2

0.20.2

0.20.2

0.2

0.2

0.2

0.4

0.4

0.4 0.4

0.4

0.4

0.4

0.6

0.6

0.6

0.6

0.6

0.8 0.8

0.8

0.8

0.6

0.6

-0.2 -0.2

-0.2

-0.2

0.4

0.4

0.40.4

0.4

0.4

-0.2

-0.2

-0.2-0.2

0.4

0.4

0.6

0.8

0.8

0.6

0.4

0.4

-0.2

-0.2

0

0

0.4

0.4

0.6

0.6

0.8

0

0

0.8

0.6

0.8

0.8

0.80.8

0.6

0.6

0.80

0 -0.2

-0.1

0

0.1

0.2

0.3

0.4

0.5

0.6

0.7

0.8

1 3 5 7 9 11 13 15 17 19 21

2

4

6

8

10

12

14

16

18

20

site

site

CB-IV0

0

00

0

00

0.2

0.2

0.2

0.2

0.2

0.20.2

0.2

0.2

0.2 0.2

0.20.2

0.4

0.4

0.4

0.4

0.4

0.4

0.4

0.4

0.4

0.6

0.6

0.6

0.6

0.6

0.6

0.80.8

0.80.8

0.8

0.8

0.8

0.4

0.4

0.4

0.4

0.4

0.40.4 0.6

0.6

-0.2

-0.2

-0.2-0.2

0.60

0

0

00.

4

0.4 0.4

0000

-0.2

0

0

0

0

0.8

0.6

0.6

0.8

-0.2

-0.2

-0.2

0.6

0.6

0.6

0.8

0.8

0.8-0.2

The similarity of the two contour plots indicates that CMAQ (CB-IV) is able to capture the spatial pattern of the TEOM measured data

Compare Temporal Patterns

• Hourly time series

• Synoptic components

• Diurnal variation

Hourly time series: Examples of good comparison

2 6 10 14 18 22 26 300

50

100

150

ug

/m3

TEOM CB-IVRADM2

2 6 10 14 18 22 26 300

50

100

150

ug

/m3

2 6 10 14 18 22 26 300

50

100

150

Day

ug

/m3

R = .62

R = .61

site: 7

site: 10

R = .78 site: 16

Hourly time series: Examples of poor comparison

2 6 10 14 18 22 26 300

20

40

60

80

ug

/m3

TEOM CB-IVRADM2

2 6 10 14 18 22 26 300

20

40

60

80

100

ug

/m3

2 6 10 14 18 22 26 300

50

100

150

Day

ug

/m3

R = -.05 site: 2

R = .3 site: 13

R = .2 site: 19

Examine the Synoptic Components

• KZ filter is used to extract the Synoptic Components from TEOM measurements and CMAQ predicted data.

• Compare the Synoptic Components for data averaged over three regions: Iowa, Northeast, and SEARCH.

Iowa Region

2 6 10 14 18 22 26 300

5

10

15

20

25

30

35

Day

ug

/m3

TEOMCMAQ

Northeast Region

2 6 10 14 18 22 26 300

10

20

30

40

50

60

70

80

Day

ug

/m3

TEOMCMAQ

SEARCH

2 6 10 14 18 22 26 300

10

20

30

40

50

60

Day

ug

/m3

TEOMCMAQ

0 3 6 9 12 15 18 2120

30

40

50Diurnal variation

ug

/m3

0 3 6 9 12 15 18 2120

30

40

50

ug

/m3

TEOM CB-IVRADM2

0 3 6 9 12 15 18 2120

30

40

50

Hour

ug

/m3

site = 7

site = 10

site = 16

Diurnal variation: Examples of good hourly time series comparison.

0 3 6 9 12 15 18 210

10

20

30Diurnal variation

ug

/m3

TEOM CB-IVRADM2

0 3 6 9 12 15 18 2120

30

40

ug

/m3

0 3 6 9 12 15 18 210

20

40

60

Hour

ug

/m3

site = 2

site = 13

site = 19

Diurnal variation: Examples of poor hourly time series comparison.

SUMMARY• CMAQ overpredicted TEOM measurements at high end

and underpredicted at low end.• CMAQ captured the spatial pattern of the TEOM

measurements.• TEOM measurements and CMAQ predictions show no

typical diurnal variation. • CMAQ performed well in capturing the average synoptic

temporal pattern in the northeast region, but failed to capture the temporal pattern in the other two regions.

• Analysis should be expanded to include PM speciation data.

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