urban air pollution, tropospheric chemistry, and climate change: an integrated modeling study

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Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study Chien Wang MIT

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Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study. Chien Wang MIT. Linking Urban Pollution, Tropospheric Chemistry and Climate Change. - PowerPoint PPT Presentation

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Page 1: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Urban Air Pollution, Tropospheric Chemistry, and Climate Change:

An Integrated Modeling Study

Chien Wang

MIT

Page 2: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Linking Urban Pollution, Tropospheric Chemistry and Climate Change

Impact of urban air pollution on global tropospheric chemistry and climate (e.g., tropospheric O3 and NO

x

budgets, radiative forcing by O3 and aerosols); Impact of future climate change on urban air pollution

and tropospheric chemistry (e.g., effects of clouds, UV, precipitation, H2O, and temperature on reaction rates);

Interaction between urban/tropospheric chemistry and climate under various emissions policies;

Anthropogenic aerosols' impact on human health; Impact of air pollution and climate change on natural

ecosystems

Page 3: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Integrated Modelling Study Climate-chemistry interactions require models with integrated

components of atmosphere, ocean, tropospheric chemistry, emissions (policy and non-policy), and ecosystem;

Integration time: 10 years for tropospheric chemistry studies (primarily due to CH

4 and O

3 simulation as well as aerosol

forcing assessment), 100 years for tropospheric chemistry and climate interaction studies;

Subgrid scale nature of urban and fast tropospheric chemistry as well as lightning production of certain chemical species in current global models with resolution coarser than ~100 km requires adequate parameterizations for relevant processes;

Data base (measurement and emissions);

Computational efficiency (parallel, esp. distributed memory computing)

Page 4: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Atmospheric Chemistry ModelAtmospheric Chemistry Model

25 Chemical species25 Chemical species4 Aerosol groups4 Aerosol groups

Advection, convection, and mixingAdvection, convection, and mixingGaseous and aqueous reactionsGaseous and aqueous reactions

Wet and dry depositionWet and dry depositionClimate ModelClimate Model

MIT 2DLO, MIT 2DLO, NCAR CCM/CSM, MIT AIM/OGCMNCAR CCM/CSM, MIT AIM/OGCM

Circulation and state of atmosphereCirculation and state of atmosphereLand and oceanLand and ocean

Clouds and PrecipitationClouds and PrecipitationRadiationRadiation

Urban Air Pollution Model Urban Air Pollution Model Natural Emission ModelNatural Emission Model

Ocean Carbon ModelOcean Carbon ModelEPPA and Emission PreprocessorEPPA and Emission Preprocessor

Terrestrial Ecosystem ModelTerrestrial Ecosystem Model

NPP, NEP, soil carbon poolNPP, NEP, soil carbon pool

Concentrations Concentrations of chemicalsof chemicals

Winds, T, HWinds, T, H22O,O,

precipitation precipitation and radiative fluxesand radiative fluxes

MIT Interactive Chemistry-Climate Model

Page 5: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Urban Air Pollution Model and Global Chemistry Model

Page 6: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 7: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 8: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Projected Future Increases of Emissions (Emissions/Emissions of 1995; MIT EPPA)

0.5

1

1.5

2

2.5

3

3.5

4

1995 2010 2025 2040 2055 2070 2085 2100Year

Ratios

SO2

BC

OC

Page 9: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 10: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 11: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 12: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

South Pole (102W 87S)

0.00

0.50

1.00

1.50

2.00

2.50

3.00

3.50

Jan Feb Mar Apr May Jun Jul Aug Sep Oct Nov Dec

Month

Su

rfa

ce

BC

in n

g/M

^3

OBS 1989

Model

Barrow (40W 70N)

0.00

20.00

40.00

60.00

80.00

100.00

120.00

140.00

Jan Feb Mar Apr May Jun Jul Aug Sep Oct Nov Dec

Month

Su

rfa

ce

BC

in n

g/M

^3

OBS 1989

Model

Mauna Loa (155.4W 19.3N)

0.00

5.00

10.00

15.00

20.00

25.00

30.00

35.00

40.00

45.00

50.00

1 2 3 4 5 6 7 8 9 10 11 12

Month

Su

rfac

e B

C in

ng

/M^3

OBS 1992

Model

Amsterdam Island (77.3E 37.5S)

0.00

2.00

4.00

6.00

8.00

10.00

12.00

14.00

Jan Feb Mar Apr May Jun Jul Aug Sep Oct Nov Dec

Month

Su

rfac

e B

C in

ng

/M^3

OBS 1991

Model

Page 13: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 14: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 15: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study
Page 16: Urban Air Pollution, Tropospheric Chemistry, and Climate Change: An Integrated Modeling Study

Summary Integrated models are needed for linking urban air pollution,

tropospheric chemistry, and climate; required integration time varies from 10 - 100 years depending on the given topics;

Adequate parameterizations of urban scale air chemistry and other subgrid scale chemical processes in global models are critical to modeling results;

Future black carbon emissions may increase according to the MIT EPPA Model;

Modeled radiative forcing of aerosols is highly uncertain, multiple year integrations with uncertainty analyses are needed for assessment;

Policy and health issues related to urban air pollution and anthropogenic emissions of aerosols need to be explored and inclusion of interaction between tropospheric chemistry and climate change is important.