thin viscous films: i. coating flows inside a rotating ... · • at slow rotation rates, a thin...

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Thin-film free-surface flows Jacqueline Ashmore DAMTP, University of Cambridge, UK APS DFD meeting, November 21st 2004 Copyright Jacqueline Ashmore, 2004

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Page 1: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Thin-film free-surface flows

Jacqueline AshmoreDAMTP, University of Cambridge, UK

APS DFD meeting, November 21st 2004

Copyright Jacqueline Ashmore, 2004

Page 2: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Fundamentals of coating flows:interaction of viscous stresses

& capillary stresses (due to curvature gradients)

solidsurface

low Reynolds # Newtonian coating flows characterized by capillary number:

viscosity surface tensioncharacteristic velocity

viscous stresscapillary stress

free surface

capillary pressure gradient

viscous stress

U

Copyright Jacqueline Ashmore, 2004

Page 3: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

The Landau-Levich-Derjaguin scalingLandau & Levich (1942), Derjaguin (1943)

flat film

liquid

static meniscus: gravity balances surface tension

dynamic meniscus: viscous force balances surface tension

asymptotic matching of the surface curvature in the two regions:

ρ,η

σ

(meniscus curvature)

U

l

provided

(low capillary number limit)

Copyright Jacqueline Ashmore, 2004

Page 4: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Rimming flows:coating the inside of a rotating cylinder

with Anette Hosoi (MIT) & Howard A Stone (Harvard University)

Ω

R θ

free surface

cylinder

filling fraction

density

viscosity

surface tension

R

equation for is usual coating flow equation, but this problem has two unusual features:1) solutions must be periodic2) conservation of mass imposes integral BC

Copyright Jacqueline Ashmore, 2004

Page 5: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

A rich variety of behavior …

“sharks’ teeth” with pure fluid(Thoroddsen & Mahadevan, 1997)

banding of a suspension(Tirumkudulu, Mileo & Acrivos, 2000)

Copyright Jacqueline Ashmore, 2004

Page 6: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Literature review(not comprehensive)

• films outside a rotating cylinder: Moffatt (1977)

• analyses in the absence of surface tension:e.g. O’Brien & Gath (1988), Johnson (1988), Wilson & Williams (1997)

• surface tension included in numerical studies:e.g. Hosoi & Mahadevan (1999), Tirumkudulu & Acrivos (2001)

• an unpublished study including analytical work:Benjamin et al. (analytical, numerical and experimental)

no previous detailed analytical study of surface tension effectsno previous detailed analytical study of surface tension effects

Copyright Jacqueline Ashmore, 2004

Page 7: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Focus of our study: surface tension effects• two-dimensional (axially uniform) steady states• consider significance of surface tension in “slow rotation” limit• compare theoretical predictions & numerical results

surface tension is a singular perturbationsurface tension is a singular perturbation

Ω

σAssumptions

• lubrication approximation

• negligible inertia R

filling fraction A

ρ,η

Copyright Jacqueline Ashmore, 2004

Page 8: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

constant flux, to be determined

viscous gravitysurface tension

“higher order” gravity

nonlinear third-order differential equation

nonlinear third-order differential equation

determines film thicknessNondimensional flux equation:

boundary condition

curvature

3 nondimensional parameters when inertia is neglected:

gravitygravitysurface tensionviscous

filling fraction (note )

Copyright Jacqueline Ashmore, 2004

Page 9: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Dependence of solutions onin absence of higher-order gravity & surface tension no solutions for

bottom of cylinder direction of rotation

λ=12

35

1020

50

θ

h(θ)

λ

points denote value of flux from numerical simulations in low

capillary # limit; B=100, A=0.1

3 qualitatively different regimes:(“shocks”); (pool & thin film)

(uniform coating);

π 2π

Copyright Jacqueline Ashmore, 2004

Page 10: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

approximately uniform coating

“shocks” develop

high capillary # limit: surface tension not important

(Tirumkudulu & Acrivos, 2001)

pool in bottom with thin film coating sides and toplow capillary # limit:

surface tension generates films with

LLD scaling

Overview of solutions

Copyright Jacqueline Ashmore, 2004

Page 11: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Film thickness when

theoretical prediction:

B=100, A=0.2

scaling of pool determined from static considerations

log

q

log λ

0.119−2(log λ)/3

2/3

log(

q λ) λ=10000, A=0.2

log B

−0.214+(log B)/6

Copyright Jacqueline Ashmore, 2004

Page 12: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

Coating the inside of a rotating cylinder: conclusions

• inclusion of surface tension facilitates an analytical description of a steady 2-D solution at very slow rotation rates

• at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder

• thickness of the film in low capillary # limit calculated by asymptotic matching

• dimensional film thickness:

Copyright Jacqueline Ashmore, 2004

Page 13: Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder • thickness of

With special thanks to …

Advisor: Howard A. Stone (Harvard)Co-advisor: Gareth H. McKinley (MIT)Eric R. Dufresne (Yale)Michael P. Brenner (Harvard)Anette (Peko) Hosoi (MIT)

Copyright Jacqueline Ashmore, 2004