the radiative and dynamical impact of aerosols on mixed-phase … · 2017. 3. 31. · impact of...

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The radiative and dynamical impact of aerosols on mixed-phase clouds The radiative and dynamical impact of aerosols on mixed-phase clouds observed during ISDAC and M-PACE observed during ISDAC and M-PACE October Case Study M-PACE: Mixed-Phase Arctic Cloud Experiment 6-11 Oct 2004: At DOE ARM NSA Site: * High Spectral Resolution Lidar * Atmospheric Emitted Radiance Interferometer * Radiosonde launches + Two Instrumented Aircraft with a Compliment of Cloud Physics Probes April Case Study ISDAC: Indirect and Semi-Direct Aerosol Campaign 1-29 Apr 2008: Same measurements at DOE ARM NSA Site + Canadian NRC In-situ Measurements * Aerosol properties * Atmospheric state * Cloud microphysics * Visible and infrared radiation * Flights were coordinated with NASA's B-200 King Air, DC-8, P-3 and NOAA's P-3 M-PACE (10 Oct 2004) vs. ISDAC (8 Apr 2008) Using the regional WRF model with 18/6/1km grids, two-moment microphysics, and effective radius and droplet size varied separately to isolate the indirect effects of aerosols Separating the influence of different boundary conditions from different aerosol concentrations: – M-PACE aerosol and boundary conditions – M-PACE aerosol and ISDAC boundary conditions – ISDAC aerosol and M-PACE boundary conditions – ISDAC aerosol and boundary conditions. Why do mixed-phase clouds with similar structure form in both spring and fall when surface and radiative conditions differ? • To what extent do the different properties of Arctic aerosols in April and October produce differences in the microphysical and macrophysical properties of clouds and the surface energy balance? • How well can cloud parameterizations in mesoscale and cloud models simulate the sensitivity of Arctic clouds and the surface energy budget to the differences in aerosols between April and October? Key Questions Addressed in this Study Amy Solomon, Matt Shupe, Ola Persson (CIRES/University of Colorado and ESRL/NOAA) Hugh Morrison (MMM/NCAR), Jian-Wen Bao (ESRL/NOAA) Experiment Design 1010] 0.1 1 10 !PCASP UHSAS FSSP-300 (Earle et al. 2008) _1000 D (microns) dN/dlogD (cm -3 ) (Morrison et al. 2008) dN/dlogD (cm -3 ) Impact of Varying MPACE/ISDAC BCs (ER=10μm ) ------ AeroS = 72 cm -3 (M-PACE) - - - - AeroS = 1000 cm -3 (ISDAC) Strong surface forcing: Glaciation suppressed by droplet size reduction Weak surface forcing: Glaciation increased by more efficient immersion freezing Model Validation during ISDAC at NSA Site ISDAC M-PACE ISDAC M-PACE Accum Precip (mm) ) W in cloud (m/s) Open Ocean/Sea-Ice to the NE Uniform Sea-ice Aerosol concentrations Atmospheric structure PBL But Similar Surface Temp, PBL Height and Inversion Temp Surface Decoupled from Cloud Top Highly Turbulent PBL Surface conditions Arctic Haze: Aero>1000cm -3 Pristine: Aero<72cm -3 Impact on Microphysics and Radiation (ISDAC BCs) Conclusions ER=4μm ER=10μm SWD (Wm-2) ------ AeroS = 72 cm -3 (M-PACE) -- - - AeroS = 1000 cm -3 (ISDAC) surface based measurements LWP (g m-2) ER=4μm ER=10μm With ISDAC BCS, increasing Aerosol concentration: Microphysical feedbacks: Decreased LWP (and increased SWD) Radiative feedbacks: Decreased SWD (and unchanged LWP) Model capture the IWC that extends up to 3km and descends below 1km after 10Z (but produces too little and the ice-cloud does not persist throughout the day) Model simulates the inversion that develops after 10Z and the mixed-phase cloud 10-24Z Increased aerosol concentration: 1) Reduces droplet size, increasing the reflectivity of the clouds, and thereby reducing the amount of shortwave radiation that reaches the surface--the first indirect aerosol effect 2) Reduces the amount of liquid water that is maintained in the cloud (increasing the downwelling surface shortwave radiation) 3a) Under weak surface forcing conditions, glaciation in increased 3b) Under strong surface forcing conditions, glaciation is supressed (vertical motions are damped?) The net impact of these effects depends on the strength of the surface forcing and the magnitude of the LWP Morrison, H., J.O. Pinto, J.A. Curry, and G.M. McFarquhar, 2008: Sensitivity of modeled arctic mixed-phase stratocumulus to cloud condensation and ice nuclei over regionally-varying surface conditions. J. Geophys. Res. Solomon, A., H. Morrison, O. Persson, M.D. Shupe , and J.-W.Bao, 2009: Investigation of Microphysical Parameterizations of Snow and Ice in Arctic Clouds During M-PACE through Model-Observation Comparisons, MWR, in press.

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Page 1: The radiative and dynamical impact of aerosols on mixed-phase … · 2017. 3. 31. · Impact of Varying MPACE/ISDAC BCs (ER=10µm)----- AeroS = 72 cm-3 (M-PACE) - - - - AeroS = 1000

WRF Model ConfigurationWRF Model Configuration

The radiative and dynamical impact of aerosols on mixed-phase cloudsThe radiative and dynamical impact of aerosols on mixed-phase cloudsobserved during ISDAC and M-PACEobserved during ISDAC and M-PACE

October Case StudyM-PACE: Mixed-Phase ArcticCloud Experiment

6-11 Oct 2004:At DOE ARM NSA Site:* High Spectral ResolutionLidar* Atmospheric EmittedRadiance Interferometer* Radiosonde launches

+ Two Instrumented Aircraftwith a Compliment of CloudPhysics Probes

April Case StudyISDAC: Indirect and Semi-DirectAerosol Campaign1-29 Apr 2008:Same measurements atDOE ARM NSA Site+ Canadian NRC In-situMeasurements* Aerosol properties* Atmospheric state* Cloud microphysics* Visible and infrared radiation* Flights were coordinatedwith NASA's B-200 King Air,DC-8, P-3 and NOAA's P-3

M-PACE (10 Oct 2004) vs. ISDAC (8 Apr 2008)

Using the regional WRF model with 18/6/1km grids, two-moment microphysics, and effective radius and droplet size varied separately to isolate the indirect effects of aerosols

Separating the influence of different boundaryconditions from different aerosol concentrations:– M-PACE aerosol and boundary conditions– M-PACE aerosol and ISDAC boundary conditions– ISDAC aerosol and M-PACE boundary conditions– ISDAC aerosol and boundary conditions.

• Why do mixed-phase clouds with similar structureform in both spring and fall when surface and radiativeconditions differ?

• To what extent do the different properties of Arcticaerosols in April and October produce differences inthe microphysical and macrophysical properties ofclouds and the surface energy balance?

• How well can cloud parameterizations in mesoscaleand cloud models simulate the sensitivity of Arcticclouds and the surface energy budget to thedifferences in aerosols between April and October?

Key Questions Addressed in this Study

Amy Solomon, Matt Shupe, Ola Persson (CIRES/University of Colorado and ESRL/NOAA) Hugh Morrison (MMM/NCAR), Jian-Wen Bao (ESRL/NOAA)

Experiment Design

10-2

10-1

100

101

102

103

104

dN

/dlo

gD

[cm

-3

]

3 4 5 6 7 8 9

0.12 3 4 5 6 7 8 9

12 3 4 5 6 7 8 9

10

D [!m]

PCASP

UHSAS FSSP-300

(Earle et al. 2008)

_1000

D (microns)

dN/d

logD

(cm

-3)

(Morrison et al. 2008)

dN/d

logD

(cm

-3)

Impact of Varying MPACE/ISDAC BCs (ER=10µm )------ AeroS = 72 cm-3 (M-PACE)- - - - AeroS = 1000 cm-3 (ISDAC)

Strong surface forcing:Glaciation suppressed by droplet size reductionWeak surface forcing:Glaciation increased by more efficient immersion freezing

Model Validation during ISDAC at NSA Site

ISDACM-PACE

ISDACM-PACE

Accum Precip (mm)

)

W in cloud (m/s)

Open Ocean/Sea-Ice to the NE Uniform Sea-ice

Aer

osol

con

cent

ratio

nsA

tmos

pher

ic s

truc

ture

PBL

But Similar Surface Temp, PBL Height and Inversion Temp

Surface Decoupled from Cloud TopHighly Turbulent PBL

Surf

ace

cond

ition

s

Arctic Haze: Aero>1000cm-3Pristine: Aero<72cm-3

Impact on Microphysics and Radiation (ISDAC BCs) Conclusions

ER=4µmER=10µm

SWD (Wm-2)

------ AeroS = 72 cm-3 (M-PACE)-- - - AeroS = 1000 cm-3 (ISDAC) surface based measurements

LWP (g m-2)

ER=4µmER=10µm

With ISDAC BCS, increasing Aerosol concentration:Microphysical feedbacks: Decreased LWP (and increased SWD)Radiative feedbacks: Decreased SWD (and unchanged LWP)

Model capture the IWCthat extends up to 3km anddescends below 1km after10Z (but produces too littleand the ice-cloud does notpersist throughout the day)

Model simulates theinversion that develops after10Z and the mixed-phasecloud 10-24Z

Increased aerosol concentration:1) Reduces droplet size, increasing the reflectivity of the clouds, and thereby

reducing the amount of shortwave radiation that reaches the surface--thefirst indirect aerosol effect

2) Reduces the amount of liquid water that is maintained in the cloud(increasing the downwelling surface shortwave radiation)

3a) Under weak surface forcing conditions, glaciation in increased3b) Under strong surface forcing conditions, glaciation is supressed (vertical

motions are damped?)

The net impact of these effects depends on the strength of the surface forcingand the magnitude of the LWP

Morrison, H., J.O. Pinto, J.A. Curry, and G.M. McFarquhar, 2008: Sensitivity of modeled arctic mixed-phase stratocumulus to cloudcondensation and ice nuclei over regionally-varying surface conditions. J. Geophys. Res.

Solomon, A., H. Morrison, O. Persson, M.D. Shupe, and J.-W.Bao, 2009: Investigation of Microphysical Parameterizations of Snow andIce in Arctic Clouds During M-PACE through Model-Observation Comparisons, MWR, in press.