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1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and mode locking Homogeneous vs. inhomogeneous gain media Spatial modes

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Page 1: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

1

The Generation of UltrashortLaser Pulses II

The phase condition

Trains of pulses – the Shah function

Laser modes and mode locking

Homogeneous vs. inhomogeneous gain media

Spatial modes

Page 2: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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There are 3 conditions for steady-state laser operation.

Amplitude conditionthresholdslope efficiency

Phase conditionaxial modeshomogeneous vs. inhomogeneous gain media

Transverse modesHermite Gaussiansthe “donut” mode

x y

|E(x,y)|2

Page 3: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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1/exp)()(

cLiEangleEangle

rtbefore

after qL

c

rtq

2(q = an integer)

An integer number of wavelengths must fit in the cavity.

Steady-state condition #2:

Phase is invariant after each round trip

length Lm

collection of 4-level systems

Round-trip length Lrt

Phase condition

Technically, this should be: rt m air m sapphireL L n L n

Page 4: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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“axial” or “longitudinal” cavity modes

Mode spacing: = c/Lrt

0

laser gain profile

qL

c

rtq

2

(q = an integer)

Longitudinal modes

fits

does not fit

But how does this translate to the case of short pulses?

Page 5: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Femtosecond lasers emit trains of identical pulses.

where I(t) represents a single pulse intensity vs. time and T is the time between pulses.

Every time the laser pulse hits the output mirror, some of it emerges.

The output of a typical ultrafast laser is a train of identical very short pulses:

R = 100% R < 100%

Output mirror

Back mirror

Laser medium

t-3T -2T 0 T 2T 3T-T

Intensity vs. time

I(t) I(t-2T)

Page 6: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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The Shah Function

The Shah function, III(t), is an infinitely long train of equally spaced delta-functions.

III( ) ( )m

t t m

t-7 -6 -5 -4 -3 -2 -1 0 1 2 3 4 5 6 7

… …

The symbol III is pronounced shah after the Cyrillic character , which is said to have been modeled on the Hebrew letter (shin) which, in turn, may derive from the Egyptian , a hieroglyph depicting papyrus plants along the Nile.

Page 7: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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If = 2n, where n is an integer, the sum diverges; otherwise, cancellation occurs and the sum vanishes.

{III( )} III(t Y

) exp( )m

t m i t dt

III(t)

So:

exp( )m

i m

) exp( )m

t m i t dt

t-7 -6 -5 -4 -3 -2 -1 0 1 2 3 4 5 6 7

… …

F{III(t)}

2-7 -6 -5 -4 -3 -2 -1 0 1 2 3 4 5 6 7

… …

{III( )}t Y

The Fourier Transform of the Shah Function

Page 8: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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The Shah Function and a Pulse Train t

-3T -2T 0 T 2T 3T-T

E(t)

t-3T -2T 0 T 2T 3T-T

E(t)

t-3T -2T 0 T 2T 3T-T

E(t)f(t) f(t-2T)f(t) f(t-2T)

where f(t) is the shape of each pulse and T is the time between pulses.

III( /( () ))t TE t f t But E(t) can also can be written:

(( ))m

f t mE t T

An infinite train of identical pulses can be written:

( )m

f t mT

To do the integral, set: t’/T = m or t’ = mT

( ) (III( / ) ( / ) )m

t T t T mf t f t t dt

Proof:

convolution

Page 9: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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An infinite train of identical pulses can be written:

The Fourier Transform of an Infinite Train of Pulses

E(t) = III(t/T) * f(t) t-3T -2T 0 T 2T 3T-T

E(t)

t-3T -2T 0 T 2T 3T-T

E(t)

t-3T -2T 0 T 2T 3T-T

E(t)f(t) f(t-2T)f(t) f(t-2T)

II ) () / 2( I(E T F

The spacing between frequencies (modes) is then T or T.

The Convolution Theorem says that the Fourier Transform of a convolution is the product of the Fourier Transforms. So:

-4 -2 0 2 4

F() ( )E

Page 10: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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The Fourier Transform of a Finite Pulse TrainA finite train of identical pulses can be written:

[III(( ) ( () )/ ) ]t T g tE t f t

where g(t) is a finite-width envelope over the pulse train.

g(t)

t-3T -2T 0 T 2T 3T-T

E(t)f(t)

[III( / 2 ) ( )( ) ]( )TE FG

F()

-6/T -4/T

0 /T /T /T-2/T

( )E

Use the fact that the Fourier transform of a product is a convolution…

G()

Page 11: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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A laser’s frequencies are often called longitudinal modes.

They’re separated by 1/T = c/2L, where L is the length of the laser.

Which modes lase depends on the gain and loss profiles.

Frequency

Inte

nsity

Here, additional narrowband filtering has yielded a single mode.

Actual Laser Modes

Page 12: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Mode-locked vs. non-mode-locked light

Mode-locked pulse train:

A train of short pulses

( ) ( 2 / )m

F m T

Non-mode-locked pulse train:

exp( )( ) ( ) ( 2 / )mm

iE F m T

Random phase for each mode

A mess…( ) () /exp( 2 )mm

F m Ti

( ) ( III( / 2 )E F T

Page 13: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Generating short pulses = Mode-lockingLocking vs. not locking the phases of the laser modes (frequencies)

Random phases

Light bulb

Intensity vs. time

Ultrashortpulse!

Locked phases

Time

Time

Intensity vs. time

Page 14: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Q: How many different modes can oscillate simultaneously in a 1.5 meter Ti:sapphire laser?

A: Gain bandwidth = 200 nm = (c/2) ~ 1014 Hzbandwidth/mode = 106 modes

That seems like a lot. Can this really happen?

Therefore = c/Lrt 100 MHz

200 nmbandwidth!

Wavelength (nm)

Ti:sapphire: how many modes lock?

Ti: sapphire crystal

pump

Typical cavity layout: length of path from M1 to M4 = 1.5 m

Page 15: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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independent of

We have seen that the gain is given by:

200

1/121)(

satII

Ng

02where

q

laser gain

profileq+1q1

losses Q: Suppose the gain is increased further. Can it be increased so that the mode at q+1 oscillates in steady state?

A: In an ideal laser, NO!At q, Gain = Loss!

Homogeneous gain media

Suppose the gain is increased to a point where it equals the loss at a particular frequency, qwhich is one of the cavity mode frequencies.

Page 16: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Suppose that the collection of 4-level systems do not all share the same 0

Consider a collection of sites, with fractional number between 0 and 0 + d0:

000 )()( dNgdN

)(; 000 gd h

The modified susceptibility is:

homogeneous “packet”inhomogeneous

line

“packets” are mutually independent -they can saturate independently!

Inhomogeneous gain media

Page 17: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Lorentianhomogeneous line shape

Gaussian inhomogeneous distribution of width

200)2ln(4

00 ;

ed h

No closed-form solution

For strong inhomogeneous broadening ( ):

" = Gaussian, with width = (NOT )': no simple form, but it resembles h'

Examples:Nd:YAG - weak inhomogeneityNd:glass - strong inhomogeneityTi:sapphire - absurdly strong inhomogeneity

Inhomogeneous broadening

Page 18: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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Q: Suppose the gain is increased above threshold in an inhomogeneously broadened laser. Can it be increased so that the mode at q+1 oscillates cw?

A: Yes! Each homogeneous packet saturates independently

“spectral hole burning”

multiple oscillating cavity modes

a priori, these modes need not have any particular phase

relationship to one another

q

laser gain profile

q+1q1

losses

q q+2 q+3

Hole burning

Page 19: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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There are 3 conditions for steady-state laser operation.

Amplitude conditionthresholdslope efficiency

Phase conditionaxial modeshomogeneous vs. inhomogeneous gain media

Transverse modesHermite Gaussiansthe “donut” mode

x y

|E(x,y)|2

Page 20: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

20propagation kernel

Steady-state condition #3:

Transverse profile reproduces on each round trip

How would we determine these modes?

"transverse modes": those which reproduce themselves on each round trip, except for overall amplitude and phase factors

An eigenvalue problem:

nm nm 0 0 nm 0 0 0 0E x, y K x, y; x , y E x , y dx dy

Condition on the transverse profile

Page 21: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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, nm n mE x y u x u y

Solutions are the product of two functions, one for each transverse dimension:

"TEM" = transverse electric and magnetic

"nm" = number of nodes along two principal axes

Notation:

2

2

2 exp

n n

x xu x Hw w

where the un’s are Hermite Gaussians:

w = beam waist parameter

Transverse modes

Page 22: The Generation of Ultrashort Laser Pulses II - brown.edu · 1 The Generation of Ultrashort Laser Pulses II The phase condition Trains of pulses – the Shah function Laser modes and

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TEM00 TEM01 TEM02 TEM13

http://www.physics.adelaide.edu.au/optics/

x y

|E(x,y)|2

12 mode

x y

|E(x,y)|2

A superposition of the 10 and 01 modes: the “donut mode”

Transverse modes - examples