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THE ANTICANCER MECHANISM OF IBUPROFEN OR INDOMETHACIN IN COLORECTAL CANCER CELLS KHOO BOON YIN UNIVERSITI SAINS MALAYSIA 2007

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Page 1: the anticancer mechanism of ibuprofen or indomethacin in colorectal

THE ANTICANCER MECHANISM OF IBUPROFEN OR INDOMETHACIN IN COLORECTAL CANCER

CELLS

KHOO BOON YIN

UNIVERSITI SAINS MALAYSIA 2007

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Acknowledgements

I would like to extend my thanks and gratitude to my supervisor,

Associate Professor Dr. Soriani Yaacob and co-supervisor, Professor Norazmi

Mohd. Nor for their guidance and support in this project. I am grateful to be

given the opportunity to carry out my research project under their supervision. I

am also grateful for the help and advice given by all the academic and non-

academic staffs of the Department of Microbiology, PPSK, INFORMM and

everyone else who had lend me a hand in my project. It has been a wonderful

experience working with all of you. My sincere thanks to MOSTE for the

National Science Fellowship. Special thanks to Prof. Smith M.-L. (University of

Leeds, UK), Prof. Suzanne Cory (Walter & Eliza Hall Institute of Medical

Research, Australia) and Prof. Shigeaki Kato (University of Tokyo, Japan) in

providing the clones for this study. To my parents and friends, I thank them for

their sound advice and relentless support.

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Abbreviations

Aberrant crypt foli ACF Adenomatous polyposis coli APC Adenosine 5’-triphosphate ATP American Type Culture Collection ATCC Ammonium persulfate APS Apoptosis inducing factor AIF Apoptosis protease activating factor-1 Apaf-1 Arachidonic acid AA Azoxymethane AOM Base pair bp B-cell lymphoma 2 Bcl-2 Bcl-2 associated X protein Bax Bcl-2-associated death promoter homologue Bad Beta-mercaptoethanol β-ME Bovine serum albumin BSA Caspase recruitment domain CARD Chinese hamster ovary cells CHO c-jun N-terminal kinase JNK Colorectal cancer CRC COX-2-negative mice COX-2-/- mice COX-2-positive mice COX-2+/+ miceCyclooxygenase COX Cytokeratin-18 CK-18 Cytotoxic T-lymphocytes CTLs Death domains DD Death effector domain DED Death inducing signaling complex DISC Death receptor 4 and death receptor 5 DR4 and DR5 Diethylpyrocarbonate DEPC Dimethyl sulfoxide DMSO Docosahexanoic acid DHA Dulbecco’s Modified Eagle’s Medium DMEM Effective concentration that causes 50% of drug response EC50Ethidium bromide EtBr Ethylenediamine-tetra acetic acid EDTA Fas-associated death domain FADD Fetal bovine serum FBS European Collection of Cell Cultures ECACC Glycosylphosphatidylinositol GPI Hour h Horseradish peroxidase HRP in situ end labeling ISEL Inhibitors of apoptosis proteins IAPs Insulin-like growth factors I and II IGF I and II Isopropyl-beta-D-thiogalactopyranoside IPTG Kilo Dalton kDa Lactate dehydrogenase LDH

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Ligand binding domain LBD Molecular weight MW N,N,N’N’-Tetra-methylethylenediamine TEMED Necrosis factor-kappa B NF-κB Non-steroidal anti-inflammatory drugs NSAIDs Optical density OD Peroxisome proliferator-activated receptors PPARs Peroxisome proliferators-activated receptor response elements

PPRE

Peroxisome proliferators-activated receptor-alpha PPARα Peroxisome proliferators-activated receptor-delta PPARδ Peroxisome proliferators-activated receptor-gamma PPARγ Phenylbutyrate PB Phenylmethylsulfonyl flouride PMSF Phosphate-buffered saline PBS Phosphoinositol -3-kinase PI3K Poly ADP-ribose polymerase PARP Prostaglandins PGs Receptor-interacting protein RIP Retinoid X receptor RXR RIP-associated ICH-1/CED-3 homologous protein with a DD RAIDD Roselle’s Park Memorial Institute Medium RPMI Serine/threonine kinase Akt Sodium citrate SOC Sodium dodecyl sulphate SDS Standard error of the mean SEM T-cell factor TCF Tdt-mediated dUTP nick end labeling TUNEL Thiazolidinediones TZD TNF receptor-1 TNF-R1 TNFα-related apoptosis-inducing ligand TRAIL TNFalpha TNFα TNF-associated factor 2 TRAF-2 TNFR-associated death domain TRADD Tris borate EDTA TBE Tumor necrosis factor TNF Tumor necrosis factor-alpha TNFα volume/volume v/v weight/volume w/v X-galactosidase X-gal

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List of contents

PageAcknowledgement ii List of contents iii List of Tables vii List of Figures viii Abbreviations x Abstract xii Abstrak

xvi

Chapter 1 Introduction……………………………………………………..... 1 1.1 Introduction of NSAIDs……………………………………………………. 1.2 The non-selective COX inhibitors………………………………………... 1.3 Evaluation of NSAIDs as PPARγ ligands……………………………….. 1.4 The role of PPARγ ligands in cancer……………………………………..1.5 Apoptosis…………………………………………………………………… 1.6 Morphological features of necrosis and apoptosis…………………...... 1.7 The putative mechanisms of PPARγ ligand-induced apoptosis……….

2 5 6 9 11 12 14

1.7.1 Mitochondrial-dependent apoptosis……………………………. 1.7.1.1 Caspases activation in apoptosis…………………... 1.7.2 Death receptor-ligand apoptosis………………........................

15 19 24

1.7.2.1 Signaling by CD95/Fas……………………………...1.7.2.2 Signaling by TNF-R1………………………………...1.7.2.3 Induction of apoptosis by TRAIL…………………...

24 25 29

1.7.3 The survival signaling pathway….……………………………... 31 1.8 Ibuprofen and indomethacin……………………………………………… 1.9 The molecular mechanism of action of NSAIDs…….………………....

33 36

1.9.1 Mutation of APC gene in Wnt signaling pathway……………... 1.9.1.1 Down-regulation of β-catenin by NSAIDs……….……. 1.9.2 The effect of NSAIDs on PPARδ expression….……………....

39 40 41

1.10 Aims of the study…………………………………………………………

41

Chapter 2 Materials and Methods…………………………………………. 46 2.1 Materials……………………………………………………………………..

45

2.1.1 Chemicals and reagents……………………………………….... 2.1.2 Kits and consumables………………………………………….... 2.1.3 Primers and probes used for Real-time PCR…………………. 2.1.4 Antibody used for Western blotting analysis…………...……...

45 47 48 50

2.2 Cell culture…………………………………………………………….......... 53 2.2.1 Human CRC cell lines………………..…………………………..

2.2.2 Preparation of reagents for cell culture work………………….. 2.2.3 Culture procedures and conditions……………………………..

53 53 58

2.2.3.1 Thawing of cells from frozen storage………………2.2.3.2 Sub-culturing of cells……………………………….. 2.2.3.3 Viability test and counting the number of cells……2.2.3.4 Mycoplasma contamination test…………………… 2.2.3.5 Freezing down of cells……………………………....

58 59 60 61 61

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2.3 Cytotoxicity determination…………………………………………………. 62 2.3.1 Determination of the optimal cell concentration……………….

2.3.2 Preparation of NSAID stock solutions…………………………. 2.3.3 Treatment of cells for LDH assay………………………………. 2.3.4 Preparation of LDH assay reaction mixture…………………....2.3.5 Determination of LDH activity…………………………………...

63 65 66 70 70

2.4 Apoptosis detection………………………………………………………... 72 2.4.1 Preparation of buffers and reagents for apoptosis detection...

2.4.2 Treatment of cells for apoptosis detection…………………….. 2.4.3 Detection of apoptosis…………………………………………… 2.4.4 Flow cytometry…………………………………………………....

72 73 73 74

2.5 Western blotting..............………………………………………………….. 76 2.5.1 Preparation of buffers and reagents for protein extraction…...

2.5.2 Treatment of cells for protein preparation……………………... 2.5.3 Extraction of protein……………………………………………… 2.5.4 Protein assay……………………………………………………... 2.5.5 Preparation of buffers and reagents for Western bloting……. 2.5.6 SDS-PAGE……………………………………………………….. 2.5.7 Transfer of proteins onto nitrocellulose membrane…………... 2.5.8 Antibodies and ECL detection.………………………………..

76 78 80 81 82 85 86 86

2.6 Agarose gel electrophoresis………………………………………………. 88 2.6.1 Buffers and reagents for agarose gel electrophoresis………..

2.6.2 Preparation of agarose gel……………………………………… 2.6.3 Agarose gel electrophoresis……………………………………..

88 90 90

2.7 Preparation of total cellular RNA and cDNA samples………………….. 91 2.7.1 Treatment of cells for the preparation of total cellular RNA.....

2.7.2 Extraction of total cellular RNA……………………………….....2.7.3 Measurement of RNA purity and concentration…………….....2.7.4 Synthesis of first-strand cDNA………………………………….. 2.7.5 Confirmation of cDNA synthesis………………………………...

91 91 92 93 93

2.8 Construction of endogenous standards for Real-time PCR………….... 94 2.8.1 Preparation of reagents for cloning……………………………..

2.8.2 Preparation of E. coli competent cells………………………..... 2.8.3 Transformation of competent cells……………………………... 2.8.4 Screening of positive clones by PCR………………………….. 2.8.5 Extraction of plasmid DNA……………………………………….2.8.6 Sequencing……………………………………………................ 2.8.7 Measurement of DNA purity and concentration…………….....2.8.8 Preparation of E. coli glycerol stock…………………………....

94 96 97 101 101 102 103 103

2.9 Real-time PCR…………………………………………………………….... 104 2.9.1 Reagents for Real-time PCR…………………………………….

2.9.2 Real-time PCR set-up………………………………………….... 104 105

2.10 Statistical analysis……………………………………………………….

106

Chapter 3 Cytotoxic effect of ibuprofen or indomethacin in human CRC cell lines………………………..........……………………..

107

3.1 Introduction…………………………………………………………………..3.2 Experimental design……………………………………………………….. 3.3 Results…………………………………………………………………….....

108 113 114

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3.3.1 The COX-2 mRNA expression in CRC cell lines…………….... 3.3.2 The cytotoxic effect of ibuprofen or indomethacin in HCA-7

cells…………………………………………………………………..3.3.3 The cytotoxic effect of ibuprofen or indomethacin in HT-29

cells…………………………………………………………………..3.3.4 The cytotoxic effect of ibuprofen or indomethacin in HCT-116

cells……………………………………………………….......…….. 3.3.5 Determination of the constant EC50 values of ibuprofen or

indomethacin on HCA-7, HT-29 and HCT-116 cells……..…....

114 117 120 122 125

3.4 Discussion…………………………………………………………………...

128

Chapter 4 Cell death induced by ibuprofen or indomethacin in human CRC cell lines…………....……………………………...

131

4.1 Introduction………………………………………………………………… 4.2 Experimental design……………………………………………………… 4.3 Results……………………………………………………………..............

132 135 137

4.3.1 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HCA-7 cells……….......................................

4.3.2 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HT-29 cells…………………………………….

4.3.3 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HCT-116 cells…….......................................

4.3.4 Optimisation of Western blot analysis…………...................... 4.3.5 The expression of pro-caspase-8, -9, -3 and -7 in HCA-7

cells following treatment with ibuprofen or indomethacin……………………………………........................

4.3.6 The expression of pro-caspase-8, -9, -3 and -7 in HT-29 cells following treatment with ibuprofen or indomethacin………………….................................................

4.3.7 The expression of pro-caspase-8, -9, -3 and -7 in HCT-116 cells following treatments with ibuprofen or indomethacin…………………….............................................

137 139 141 143 143 145 147

4.4 Discussion…………………………………………………………………..

149

Chapter 5 Modulation of COX-2, c-myc, β-catenin and TCF-4 mRNA expression by ibuprofen or indomethacin in human CRC cell lines...............................................................................…

154

5.1 Introduction…………………………………………………………………..5.2 Experimental design……………………………………………………….. 5.3 Results……………………………………………………………………….

155 157 158

5.3.1 Confirmation of the specificity of the PCR amplification…….. 5.3.2 Construction of standard curves for COX-2, c-myc, β-catenin

and TCF-4………………………………………………………... 5.3.3 Quality of total cellular RNA extraction……………………...... 5.3.4 Confirmation of cDNA samples………………. 5.3.5 Expression of COX-2, c-myc, β-catenin and TCF-4 mRNA in

HCA-7 cells following treatments with ibuprofen or indomethacin…………………………......................................

158 162 164 164 167

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5.3.6 Expression of COX-2, c-myc, β-catenin and TCF-4 mRNA in HT-29 cells following treatment with ibuprofen or indomethacin…………………………......................................

5.3.7 Expression of COX-2, c-myc, β-catenin and TCF-4 mRNA in HCT-116 cells following treatment with ibuprofen or indomethacin……………………………………………………..

171 174

5.4 Discussion…………………………………………………………………..

177

Chapter 6 Modulation of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA expression by ibuprofen or indomethacin in human CRC cell lines………………………...............................……………..

183

6.1 Introduction…………………………………………………………………..6.2 Experimental Design………………………………………………………..6.3 Results…………………………………………………………………….....

184 186 188

6.3.1 Confirmation of the specificity of PCR amplification of PPARα, PPARδ, PPARγ1 and PPARγ2……………………….

6.3.2 Construction of standard curves of PPARα, PPARδ, PPARγ1 and PPARγ2…………………………………………...

6.3.3 Expression of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA in HCA-7 cells following treatments with ibuprofen or indomethacin…………………………………………………..

6.3.4 Expression of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA in HT-29 cells following treatments with ibuprofen or indomethacin……………………………………………………..

6.3.5 Expression of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA in HCT-116 cells following treatments with ibuprofen or indomethacin………………................................................

188 188 192 197 200

6.4 Discussion…………………………………………………………………...

203

Chapter 7 General Discussion……………………………………………...

209

Reference 217

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List of tables

Page Table 1.1 A list of the main caspases and some of their substrates……… 20 Table 1.2 NSAID classification..…………………………………...………….. 34 Table 2.1 List of general chemicals and reagents…………………………... 47 Table 2.2 List of commercial kits and consumables………………………… 49 Table 2.3 Primer and probe sequences……………………………………… 50 Table 2.4 List of antibodies used for Western blotting analysis……..…….. 52 Table 2.5 Overview of the controls used in LDH assay…………………….. 69 Table 2.6 Composition of RIPA buffer………………………………………... 79 Table 3.1 The general characteristics of HCA-7, HT-29 and HCT-116 cell

lines used in this study……………………………………………... 116

Table 3.2 The EC50 value of ibuprofen and indomethacin determined in HCA-7 cell line……………………………………………………….

119

Table 3.3 The EC50 value of ibuprofen and indomethacin determined in HT-29 cell line………………………………………………………..

123

Table 3.4 The EC50 value of ibuprofen and indomethacin determined in HCT-116 cell line…………………………………………………….

126

Table 4.1 Potential biomarker molecules for apoptosis studies………….... 133 Table 4.2 Summary of the pattern of pro-caspase-8, -9, -3 and -7 protein

expression in HCA-7, HT-29 and HCT-116 cells following treatments with ibuprofen or indomethacin……………………....

150

Table 5.1 Comparison between the sequences of the COX-2, c-myc, β-catenin and TCF-4 cloned PCR products and the corresponding human mRNA sequence access from GeneBank…………………………………………………………….

160

Table 5.2 Summary of the pattern of COX-2, c-myc, β-catenin and TCF-4 mRNA expression in HCA-7, HT-29 and HCT-116 cells following treatments with ibuprofen or indomethacin…...……….

178

Table 6.1 Comparison between the sequences of the PPARα, PPARδ,

PPARγ1 and PPARγ2 cloned PCR products and the corresponding human mRNA sequence access from GeneBank……………………………….. ………………………….

190

Table 6.2 Summary of the pattern of PPARα, PPARδ, PPARγ1 and

PPARγ2 mRNA expression in HCA-7, HT-29 and HCT-116 cells following treatment with ibuprofen or indomethacin…...…..

204

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List of figures

Page Figure 1.1 Classification of NSAIDs based on the relative specificity ratio

of COX-1 to COX-2 in human whole blood assay………………. 4

Figure 1.2 The transcriptional activation by PPARγ…………………………. 8

Figure 1.3 Hallmarks of the apoptotic and necrotic cell death processes…. 13

Figure 1.4 The putative apoptosis mechanism induced by PPARγ ligands.. 16

Figure 1.5 The mitochondrial-dependent apoptosis pathway…..…………... 18 Figure 1.6 Activation of pro-caspases……………………….......................... 21 Figure 1.7 The apoptosis signaling mechanism by Fas death receptor…… 26 Figure 1.8 The tumor necrosis factor receptor-1.....………..………………... 28 Figure 1.9 The signal transduction of survival signaling pathway………….. 32 Figure 1.10 The putative mechanism of action of NSAIDs in human CRC

cells in vitro……………………………………………….…………. 37

Figure 1.11 A summary of the experiment design…………………………….. 44 Figure 2.1 Determination of the optimal cell concentration…………………. 64 Figure 2.2 Determination of LDH activity of indomethacin..………………… 67 Figure 2.3 Determination of LDH activity of ibuprofen………………............ 68 Figure 2.4 Overview procedure of measuring LDH activity………............... 71 Figure 2.5 Apoptosis detection using M30 CytoDEATH assay...…………... 75 Figure 2.6 Maps of plasmid vectors used in this study……………………… 98 Figure 2.7 Maps of plasmid vectors used in this study……………………… 99 Figure 2.8 Maps of plasmid vectors used in this study……………………… 100 Figure 3.1 Principle of LDH assay………………………………………… 110 Figure 3.2 The sigmoid shape of dose response curve……………………... 111 Figure 3.3 Schematic representation of the determination of constant

EC50 value………………………………………………………….. 112

Figure 3.4 The typical epithelial appearance of a confluent monolayer of HCA-7, HT-29 and HCT-116 cells………………………………...

115

Figure 3.5 The cytotoxic effect of ibuprofen or indomethacin in HCA-7 cells…………………………………………………………………..

118

Figure 3.6 The cytotoxic effect of ibuprofen or indomethacin in HT-29 cells……….................................................................................

121

Figure 3.7 The cytotoxic effect of ibuprofen or indomethacin in HCT-116 cells…………………………………………………………………..

124

Figure 3.8 Schematic representation of the determination of constant EC50 values of ibuprofen or indomethacin in HCA-7, HT-29 and HCT-116 cells………………………………………………….

127

Figure 4.1 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HCA-7 cells……...………………………………..

138

Figure 4.2 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HT-29 cells………………………………………..

140

Figure 4.3 The percentage of apoptotic cells induced by ibuprofen or indomethacin in HCT-116 cells.…..............................................

142

Figure 4.4 Western blot analysis of caspase-8, -9, -3, -7 and β-actin expression in HCA-7 cells.……………………………..…………..

144

Figure 4.5 Western blot analysis of caspase-8, -9, -3, -7 and b-actin expression in HT-29 cells.………………………………...………..

146

Figure 4.6 Western blot analysis of caspase-8, -9, -3, -7 and b-actin

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expression in HCT-116 cells.……………………………..……...... 148 Figure 5.1 Gel electrophoresis of PCR products……………………….......... 159 Figure 5.2 Standard curves........................................……………………….. 163 Figure 5.3 Electrophoresis of total RNA samples........……………………… 165

Figure 5.4 The linear regression plot of CT value of β-actin from HCA-7, HT-29 and HCT-116 cDNA samples………………………………

166

Figure 5.5 The modulation of COX-2, c-myc, β-catenin and TCF-4 mRNA expression in HCA-7 cells following treatment with ibuprofen or indomethacin…………………………………………………...........

168

Figure 5.6 The modulation of COX-2, c-myc, β-catenin and TCF-4mRNA expression in HT-29 cells following treatment with ibuprofen or indomethacin……........................................................................

172

Figure 5.7 The modulation of COX-2, c-myc, β-catenin and TCF-4 mRNA expression in HCT-116 cells following treatment with ibuprofen or indomethacin……………….....................................................

175

Figure 6.1 Gel electrophoresis PCR products…………………..……………. 189 Figure 6.2 Standard curves …………………………..………………………... 193

Figure 6.3 The modulation of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA expression in HCA-7 cells following treatment with ibuprofen or indomethacin….......................................................

194

Figure 6.4 The modulation of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA expression in HT-29 cells following treatment with ibuprofen or indomethacin...........................................................

198

Figure 6.5 The modulation of PPARα, PPARδ, PPARγ1 and PPARγ2 mRNA expression in HCT-116 cells following treatment with ibuprofen or indomethacin………………………………………….

201

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The anticancer mechanism of ibuprofen atau indomethacin in

colorectal cancer cells

Abstract

Ibuprofen and indomethacin are among the frequently studied

non-steroidal anti-inflammatory drugs (NSAIDs) for their anticancer

activities. Besides being non-selective cyclooxygenase-2 (COX-2)

inhibitors, both NSAIDs are also direct ligands for peroxisome

proliferators-activated receptor-gamma (PPARγ). However, the precise

mechanism(s) of action whereby both NSAIDs exert their anticancer

effect remain unclear. In this study, we investigated the effects of both

NSAIDs in constitutively COX-2-expressing (HCA-7 and HT29) and non-

constitutively COX-2-expressing (HCT116) cell lines. Our initial aim of the

study was to determine the NSAID growth inhibitory effect as well as the

effective concentration to inhibit 50% of cell growth (EC50) of each NSAID

in each cell line using lactate dehydrogenase (LDH) release assay. The

apoptosis mechanism was then investigated using M30 CytoDEATH

assay prior to flow cytometry analysis. The apoptotic-related proteins

such as caspase-8, -9, -3 and -7 were also investigated using Western

blot analysis, whereas the modulation of mRNA expression of relevant

molecular targets such as COX-2, c-myc, β-catenin, TCF-4 and PPAR

subtypes (α, δ, γ1 and γ2) mRNA was quantified using Real-time PCR

analysis. Our results demonstrated that both NSAIDs produced

remarkable inhibition on the growth of all three cell lines tested. The

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iii

inhibitory effect occurred in a concentration- and time-dependent

manner, with indomethacin (EC50 value >100 µM) being more potent

compared to ibuprofen (EC50 value >1000 µM). Furthermore, the ability

of both NSAIDs in inhibiting the growth of cells is likely not to be

associated with COX-2 expression. The evidence from M30 CytoDEATH

assay suggested that the major mode of cell death caused by both

NSAIDs was caspase-dependent apoptosis. This evidence was further

supported by Western blot analysis which indicated that the induction

occurred via caspase-9-dependent pathway, whereas the Real-time PCR

analysis showed that both NSAIDs appear to modulate gene expression

via a variety of different molecular targets in COX-2-dependent and/or

independent pathway(s) depending on the colorectal cancer (CRC) cell

type. However, alteration of TCF-4 and PPARγ1 mRNA expression are

likely essential for both NSAIDs to induce apoptosis. Thus, Wnt and

PPARγ signaling pathways may be involved in mediating the apoptosis

induced by both NSAIDs in CRC cells. In addition, PPARδ is found to be

another essential molecular target for indomethacin-induced CRC cell

apoptosis. In conclusion, our study may provide additional information

and evidence of the various mechanisms and actions of NSAIDs in

human CRC cells which may be useful in selecting effective apoptotic

drugs against specific CRC types. As we and others have shown, both

NSAIDs have anti-CRC activities and are potential anti-CRC agents.

Further studies on the effect of both NSAIDs on CRC cells remain

important, as they may be developed as chemotherapeutic agents for

human CRC.

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iii

Antikanser mekanisme ibuprofen atau indomethacin dalam sel

kanser kolorektal

Abstrak

Ibuprofen dan indometasin adalah antara drug antiinflamatori

bukan steroid (NSAIDs) yang kerap dikaji untuk aktiviti-aktiviti anti

kansernya. Selain daripada perencat siklooksigenase-2 (COX-2) bukan

pilihan, kedua-dua NSAIDs ini adalah ligan langsung untuk reseptor-

gama pengaktif proliferators peroksimase (PPARγ).

Walaubagaimanapun, tindakan mekanisme atau mekanisme-mekanisme

yang tepat yang mana kedua-dua NSAIDs mengenakan kesan anti

kanser masih lagi tidak jelas. Kajian ini menyiasat kesan garis sel pada

kedua-dua NSAIDs dalam sebahagian ekspresi COX-2 (HCA-7 dan

HT29) dan bukan pada sebahagian ekspresi COX-2. Pada awalnya,

kajian ini dijalankan untuk menentukan kesan perencatan pertumbuhan

NSAIDs dan juga kepekatan (concentration) yang berkesan untuk

merencat 50% daripada sel pertumbuhan (EC50) pada setiap NSAIDs di

setiap garis sel menggunakan dehidrogenase laktat (LDH) yang

mengeluarkan assay. Mekanisme apoptosis kemudiannya disiasat

menggunakan assay M30 CytoDEATH sebelum analisis aliran sitometri

dijalankan. Protein-protein berkaitan apoptotic seperti caspase-8, -9, -3

dan -7 juga telah disiasat menggunakan analisis blot Western, manakala

modulasi ekspresi mRNA untuk molekul sasaran yang berkaitan seperti

COX-2, c-myc, β-catenin, TCF-4 dan subjenis-subjenis PPAR mRNA (α,

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iii

δ, γ1 dan γ2) dikuantitikan menggunakan analisis PCR masa-sebenar

(REAL-time). Keputusan menunjukkan bahawa kedua-dua NSAIDs

menghasilkan perencatan yang luar biasa pada pertumbuhan ketiga-tiga

garis sel. Indometasin (nilai EC50 > 100 µM) adalah lebih kuat jika

dibandingkan dengan ibuprofen (nilai EC50 > 1000 µM). Tambahan pula

kebolehan kedua-dua NSAIDs dalam merencat pertumbuhan sel-sel

mungkin tidak akan dikaitkan dengan ekspresi COX-2. Bukti dari assay

M30 CytoDEATH mengusulkan bahawa mod utama kematian sel adalah

disebabkan kedua-dua NSAIDs adalah apoptosis yang bergantung pada

caspase. Bukti ini seterusnya disokong oleh analisis blot Western yang

menunjukkan bahawa cetusan berlaku melalui laluan yang bergantung

pada caspase-9, manakala analisis PCR masa-sebenar (REAL-time)

menunjukkan bahawa kedua-dua NSAIDs kelihatan memodulat ekspresi

gen melalui pelbagai sasaran molekul yang berbeza dalam laluan atau

laluan-laluan yang bergantung atau tidak bergantung pada COX-2 dan

ini bergantung kepada jenis sel kanser kolorektal (CRC).

Walaubagaimanapun perubahan pada TCF-4 dan ekspresi mRNA

PPARγ adalah agak penting kepada kedua-dua NSAIDs untuk mencetus

apoptosis. Oleh itu laluan-laluan isyarat Wnt dan PPARγ mungkin terlibat

sebagai perantara apoptosis yang dicetus oleh kedua-dua NSAIDs

dalam sel-sel CRC. Sebagai tambahan, PPARδ pula didapati sebagai

satu lagi sasaran molekul yang penting untuk apoptosis sel CRC

cetusan-indometasin. Kesimpulannya, kajian ini mungkin dapat memberi

maklumat tambahan dan bukti pelbagai mekasisme-mekanisme dan

tindakan-tindakan NSAIDs dalam sel CRC manusia, yang mungkin

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iii

berguna untuk memilih drug apoptotic yang berkesan terhadap jenis

CRC yang spesifik. Seperti yang telah kami dan penyelidik-penyelidik

lain telah tunjukkan, kedua-dua NSAIDs mempunyai aktiviti-aktiviti anti-

CRC dan berpotensi sebagai agen anti-CRC. Kajian-kajian lanjut

mengenai kesan kedua-dua NSAIDs pada sel-sel CRC tetap penting

kerana mereka boleh dibangunkan sebagai agen kemoterapeutik untuk

CRC manusia.

Page 20: the anticancer mechanism of ibuprofen or indomethacin in colorectal

Chapter 1

Introduction

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1.1 Introduction of NSAIDs

Non-steroidal anti-inflammatory drugs (NSAIDs) were first

introduced in the 1900s, and have subsequently been widely used to

treat inflammation, mild-to-moderate pain and fever (Vane and Botting,

1998). Although they have been used for more than two decades and

their safety has constantly been reviewed, they have only recently been

proposed as anti-cancer agents (Vane and Botting, 1998). NSAIDs work

mainly by inhibiting cyclooxygenase (COX) and preventing the formation

of prostaglandins (PGs) (Smith and Goh, 1996; Badawi et al., 2000; Han

et al., 2001). There are two isoforms of COX which are known as COX-1

and COX-2 (Sheng et al., 1997; Badawi et al., 2000). COX-1 is

continuously secreted within the stomach and duodenum where it helps

maintain healthy stomach lining, normal kidney function and the clotting

action of blood platelets (Sheng et al., 1997). In contrast, the COX-2

enzyme is primarily found at sites of inflammation (Sheng et al., 1997). It

is induced by inflammatory stimuli such as interleukin-1, and is

suppressed by glucocorticoids (Sheng et al., 1997).

Blocking of COX-2 is effective in relieving pain and inflammation,

whereas inhibiting of COX-1 often produces unacceptable

gastrointestinal side effects such as diarrhea, bloating, heartburn,

stomach upset and ulcers (Vane and Botting, 1998). Various

conventional NSAIDs such as aspirin, diclofenac, ibuprofen,

indomethacin, naprosyn and piroxicam are being used as anti-cancer

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agents (Soh and Weinstein, 2003). These NSAIDs inhibit both COX-1

and COX-2 to differing degrees in terms of the relative specificity ratio

(IC50; Figure 1.1) (Mitchell et al., 1994; Bishop-Bailey et al., 1997;

Bishop-Bailey and Warner, 2003).

The lower ratio value reflects the more potent activity of NSAIDs

against COX-2 inhibition. Thus, SC58125 (celecoxib derivative) and

celecoxib appear to be more selectively involved in COX-2 inhibition

activity than naproxen and flurbiprofen (Figure 1.1). Besides indicating

the selectivity of NSAIDs in COX-2 inhibition, ratio IC50 adequately

explains the variations in the side effects of NSAIDs at their anti-

inflammatory doses (Vane and Botting, 1998). Selective COX-2 inhibitors

such as celecoxib which have higher potency on COX-2 inhibition activity

will have potent anti-inflammatory activity with fewer side effects on the

stomach and kidney (Henry, 2003; Langman, 2003; Wolfe, 2003),

whereas non-selective COX-2 inhibitors such as aspirin, piroxicam,

ibuprofen and indomethacin which have a higher potency against COX-1

than against COX-2 inhibition activity, were found to produce high

gastrointestinal toxicity and cause the most damage to the stomach at

inflammatory doses (Lanza et al., 1989; Rodriguez et al., 1994).

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1.2 The non-selective COX inhibitors

The ability of NSAIDs to decrease the COX-1/COX-2 expression

has allowed consideration of NSAIDs as potential anti-cancer agents for

cancer treatment including human colorectal cancer (CRC) treatment

(Vane and Botting, 1998). COX-2 expression has been shown to be up-

regulated in human CRC when compared with normal adjacent colonic

mucosa (Na and Surh, 2003). Inhibition of the COX-2 expression is

important because over expression of COX-2 provides tumor cells with

growth and survival advantages including resistance to apoptosis, and

increased invasiveness or angiogenesis (Mohammed et al., 1999;

Cianchi et al., 2001; Yamada et al., 2001; Na and Surh, 2003).

Thus, targeting the inhibition of COX-2 is regarded as an affective

and promising strategy for cancer prevention and treatment (Han et al.,

2001; Na and Surh, 2003). Indeed, the expression of COX-2 is

stimulated by growth factors and tumor promoters, and it is often

selectively expressed in tumors cells including CRC cells (Eberhart et al.,

1994; Sano et al., 1995; Han et al., 2001). Thus, the expression of COX-

2 is believe that plays an important role in cancer, and is often correlated

with tumorigenesis. This correlation was supported by the finding that in

two mutated adenomatous polyposis coli (APC) background mice where

the COX-2-/- mice developed fewer intestinal polyps than the COX-2+/+

mice (Oshima et al., 1996; Han et al., 2001).

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Many epidemiologic and clinical studies have revealed that regular

ingestion of NSAIDs such as aspirin, sulindac and indomethacin can

reduce the risk of developing several malignant tumors including CRC

(Giardiello et al., 1995; Giovannucci et al., 1995; Boolbol et al., 1996).

Based on the evidences above, it is logical to choose a selective COX-2

inhibitor that is as effective as non-selective inhibitors and could prevent

PGs formation in inflamed areas without interfering with the activity in

stomach and kidney (Vane and Botting, 1998). However, COX-2 appears

to have multiple functions and has been shown to be important in

ovulation and vasoprotection, and is essential for normal kidney

development (Dahl, 1999). Indeed, both COX-1 and COX-2 are

expressed in inflamed joints, so it is important that mixed COX inhibition

is required for the maximal anti-inflammatory effects (Dahl, 1999).

1.3 Evaluation of NSAIDs as PPARγ ligands

Non-selective COX inhibitors are regarded as effective and

promising anti-cancer agents for cancer prevention or treatment.

However, the fact that NSAIDs retain the anti-proliferative activity in a

variety of cells that do not express COX-2 would argue against the

relevance of COX-2 inhibition as a target for NSAIDs in cancer cells

(Hanif et al., 1996; Zhang et al., 1999; Chapple et al., 2000; Smith et al.,

2000; Han et al., 2001; Hull et al., 2003). Indeed, the concentration of

NSAIDs required to induce cell death was several orders of magnitude

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higher than that required to inhibit the activity of COX (Mitchell et al.,

1993; Han et al., 2001). For example, the IC50 ratio of indomethacin to

inhibit COX-1 and COX-2 in intact cells were reported to be 28 nM and

1.7 µM, respectively (Mitchell et al., 1993), whereas the concentration of

indomethacin used to induce cell death in the same cells was 500 µM

(Zhang et al., 1999). Therefore, the anti-proliferative activity of NSAIDs

would seem to occur via COX-independent mechanisms (Hull et al.,

2003; Soh and Weinstein, 2003).

One possible mechanism was suggested to be via the peroxisome

proliferators-activated receptor-gamma (PPARγ), a ligand-activated

transcription factor pathway (Smith et al., 2000; Hull et al., 2003; Soh and

Weinstein, 2003). According to Lehmann et al. (1997), several NSAIDs

including ibuprofen and indomethacin, can interact directly and

specifically bind with PPARγ ligand binding domain (LBD). Upon ligand

binding, PPARγ becomes activated and heterodimerises with retinoid X

receptor (RXR) (Figure 1.2) (Boitier et al., 2003). The co-repressors will

then dissociate from the complex which leads to an active PPARγ/RXR

complex that binds to the gene regulatory sites on DNA termed PPAR

response elements (PPRE). There is also evidence of the involvement of

co-activator proteins that enhance the activity of the PPARγ/RXR

complex. Binding of the PPARγ/RXR complex to PPRE increases the

transcription of numerous genes including genes involve in

tumorigenesis (Boitier et al., 2003). The ability of NSAIDs to bind to

PPARγ has been previously assessed in a competition-binding assay

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using [3H] BRL49653 and bacterially expressed PPARγ LBD (Lehmann

et al., 1997). Though not all NSAIDs activate PPARγ through direct

interactions with the receptor, the fact that NSAIDs bind and thereby

activate PPARγ activity, subsequently define them as the PPARγ ligands

(Lehmann et al., 1997).

Interestingly, ibuprofen and indomethacin used in this study are

non-selective COX inhibitors and direct PPARγ ligands. Activation of

PPARγ by ibuprofen and indomethacin was the strongest of any of the

NSAIDs that were evaluated in CRC (Nixon et al., 2003). Furthermore,

both NSAIDs may activate more than one PPAR subtypes. For example,

ibuprofen activates PPARdelta (PPARδ) and PPARγ (Kojo et al., 2003),

whereas indomethacin shows agonistic activity for PPARalpha (PPARα)

and PPARγ (Lehmann et al., 1997) or PPARγ alone based on two

different studies (Kojo et al., 2003). As dual ligands have been proven to

be more effective at preventing colorectal carcinogenesis, ibuprofen and

indomethacin are therefore potential anti-cancer agents for human CRC.

1.4 The role of PPARγ ligands in cancer

The mechanisms of anti-cancer effect by the PPARγ ligands have,

however, not been fully elucidated. In general, activation of PPARγ by its

ligand is associated with cancer prevention (Brockman et al., 1998;

Sarraf et al., 1998; Kitamura et al., 1999). The PPARγ ligands have anti-

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proliferative and pro-differentiation effects in slowing the proliferation of

tumor cells including breast (Elstner et al., 1998; Rubin et al., 2000),

colon (Sarraf et al., 1998), prostate (Kubota et al., 1998; Hisatake et al.,

2000; Shappell et al., 2001), gastric (Takahashi et al., 1999) and

pancreatic (Motomura et al., 2000) cancer cells.

In support of the former findings, the thiazolidinediones (TZD)

group of PPARγ ligands has been shown to inhibit proliferation of breast,

prostate and colon cells (Elstner et al., 1998; Kubota et al., 1998; Sarraf

et al., 1998). In contrast, the ligands promote the development of colon

tumors in transgenic mice in which one copy of the gene encoding the

APC is knocked out, predisposing them to colon cancer (Lefebvre et al.,

1998). However, another study demonstrated that treatment of patients

with liposarcomas with a PPARγ ligand results in anti-neoplastic pro-

differentiation which may decrease the proliferative rate of the cancer

cells and slow the progression of the disease (Demetri et al., 1999).

There are also observations that PPARγ ligands induce growth arrest

and the synthesis of differentiation markers in human CRC cells

(Kitamura et al., 1999). Furthermore, PPARγ ligands have been shown to

be potent inhibitors of angiogenesis, a process necessary for solid-tumor

growth and metastasis (Xin et al., 1999). Although much of the evidence

suggests that activation of PPARγ by its ligands could promote the

suppression of tumor growth and inhibit carcinogenesis, the precise

mechanisms involved remain unclear.

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PPARγ ligands have been shown to exert their anti-cancer cell

proliferation through the induction of apoptosis (Yang and Frucht, 2001;

Clay et al., 2002). Although the precise role of PPARγ in cancer cells is

still debatable, accumulating evidence has reported that PPARγ ligands

inhibiting cancer cell growth via apoptosis (Yang and Frucht, 2001; Clay

et al., 2002; Na and Surh, 2003). The apoptosis pathway is currently the

key mechanism by which anti-cancer agents kill tumor cells. The ability of

PPARγ ligands to decrease COX-2 expression and initiate apoptosis has

made them to be considered as potential therapeutic agents for cancer

treatment (Yang and Frucht, 2001; Debatin, 2004). Therefore,

identification of the molecular pathways induced by PPARγ ligands will

be of both basic and clinical importance.

1.5 Apoptosis

Apoptosis, first reported in 1964, is also known as programmed

cell death (Gewies, 2003). It is the physiological process by which

unwanted cells are eliminated during development and other normal

biological processes (Gewies, 2003). Moreover, cytotoxic T-lymphocytes

(CTLs) kill virus-infected cells are also via the induction of apoptosis

(Roberts, 2000). Currently, understanding of the apoptosis plays an

important role in the study of physiological processes, particularly those

involved in cancer research (Roberts, 2000). For example, the mutation

of the p53 gene produces defective proteins that are often found in

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cancer cells which contribute to resistance to apoptosis (Debatin, 2004).

Moreover, immunotherapy of tumors requires target cells with an

apoptosis-sensitive phenotype (Debatin, 2004).

Apoptosis is of major importance in the pathogenesis of several

diseases including cancer, AIDS and neurological disorders such as

Alzheimer’s and Parkinson’s diseases (Roberts, 2000). It is believed that

defects in the apoptotic pathways represent hallmarks of tumorigenesis

(Okada and Mak, 2004). Recent research on new cancer therapies has

therefore focused on devising ways to overcome this resistance and to

trigger apoptosis of cancer cells (Okada and Mak, 2004).

1.6 Morphological features of necrosis and apoptosis

In the cell death process, necrosis occurs when cells are exposed

to a serious physical or chemical insult (Gewies, 2003). The necrotic

mode of cell death, in which cells suffer a major insult, results in a loss of

membrane integrity, swelling and cell rupture (Figure 1.3). During

necrosis, the cellular contents are released uncontrolled into the

environment which results in damage to surrounding cells and a strong

inflammatory response in the corresponding tissue (Gewies, 2003).

In contrast to necrosis, apoptosis is characterised by typical

morphological and biochemical hallmarks including cell shrinkage,

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nuclear DNA fragmentation and membrane blebbing (Debatin, 2004).

The morphological changes such as cell shrinkage and deformation

results in the cells loss of contact with neighboring cells and chromatin

condensation (Figure 1.3). The chromatin is then localised at the nuclear

membrane, the plasma membrane undergoes blebbing and finally the

cell is fragmented into compact membrane-enclosed structures termed

apoptotic bodies. The apoptotic bodies contain cytosol, condensed

chromatin and organelles. They are removed from the tissue by

phagocytosis or secondary necrosis without causing an inflammatory

response.

1.7 The putative mechanisms of PPARγ ligand-induced apoptosis

As described above, treatment with PPARγ ligands has been

widely implicated to reduce the cancer cell growth rate and induce cell

terminal differentiation of a number of human cancers including CRC via

induction of apoptosis (Yang and Frucht, 2001; Boitier et al., 2003).

According to Goke et al. (2000), the induction of apoptosis by PPARγ

ligands is increased by co-stimulation with tumor necrosis factor (TNF)-

related apoptosis-inducing ligand (TRAIL), a member of the TNF family.

Furthermore, inhibition of cell growth observed in human breast cancer

cells treated in vitro with PPARγ ligands is accompanied with a marked

increase in apoptosis and a profound decrease of Bcl-2 gene expression

(Elstner et al., 1998). In addition, troglitazone-induced apoptosis has

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been demonstrated to be associated with caspase-dependent and -

independent mechanisms (Yoshizawa et al., 2002). More importantly,

Yoshida et al. (2003) recently proposed the mechanisms concerning

PPARγ ligand-induced apoptosis would be occurring via a) perturbation

of mitochondrial membrane permeability; b) binding of death receptor to

its ligand; and c) phosphatidylinositol-3-kinase (PI3)-serine/threonine

kinase (Akt)-apoptosis protease activating factor-1 (Apaf-1) system

(down-regulation of survival signaling pathway) (Figure 1.4).

1.7.1 Mitochondrial-dependent apoptosis

PPARγ ligands mainly induce apoptosis via perturbation of inner

mitochondria membrane permeability (Yoshida et al., 2003). This

mitochondrial-dependent apoptosis was termed intrinsic apoptosis where

signals from various stimuli disturb the membrane permeability of the

mitochondria and subsequently release the apoptogenic factor such as

cytochrome c into the cytoplasm (Yoshida et al., 2003). During intrinsic

apoptosis, anti-apoptotic proteins such as B-cell lymphoma 2 (Bcl-2) and

the pro-apoptotic protein such as Bcl-2 associated X protein (Bax) are

induced to oligomerise and migrate from the cytoplasm to the

mitochondria escort by various BH3-Only-Protrein (Debatin, 2004). Once

the protein is inserted into the outer mitochondria membrane, it induces

cytochrome c release by the creation or alteration of the mitochondria

membrane pores (Debatin, 2004).

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In the cytoplasm, cytochrome c combines with Apaf-1 and pro-

caspase-9 to form a complex termed apoptosome, in the presence of

adenosine 5’-triphosphate (ATP) to activate caspase-9 (Figure 1.5)

(Roberts, 2000; Gewies, 2003; Debatin, 2004). Caspase-9 subsequently

activates downstream executor caspases such as caspase-3, -6 and -7

(Roberts, 2000). Activation of caspase-3 and the subsequent degradative

events are probably triggered to initiate the apoptosis (Roberts, 2000;

Yoshida et al., 2003; Debatin, 2004). In most PPARγ ligands induced

apoptosis cases, caspase-3 is the final molecule where activation of

caspase-3 will then causes DNA fragmentation (Yoshida et al., 2003).

However, the mitochondrial pathway must not always associated

with caspase activation (Debatin, 2004). The mechanism varies

depending on the release of apoptogenic factor such as cytochrome c,

Smac/Diablo or apoptosis inducing factor (AIF) (Figure 1.5) (Debatin,

2004). The release of cytochrome c triggers caspase-9 activation through

the formation of cytochrome c/Apaf-1/caspase-9 in the presence of ATP

to form an active apoptosome complex as described above (Roberts,

2000; Gewies, 2003; Debatin, 2004). Thus, the release of cytochrome c

from mitochondria always reflects the mitochondrial→caspase-

9→executor caspase activation→apoptosis (Cai et al., 2002; Debatin,

2004). The Smac/Diablo promotes caspase activation by neutralising the

inhibitory effects of inhibitors of apoptosis proteins (IAPs) and this may

also imply the same caspase activation pathway (Debatin, 2004).

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However, AIF causes DNA condensation or initiate apoptosis without

activating any caspases (Debatin, 2004).

1.7.1.1 Caspase activation in apoptosis

Caspase(s) with the generic name c denotes a cysteine protease

and aspase refers to the aspartate specific cleaving ability of these

enzymes (Gewies, 2003). The individual members are then numbered

according to their chronological order of publication (Robert, 2000).

Caspase activation is recently demonstrated as central importance

(hallmark) in the apoptosis signaling network as well as DNA

fragmentation, which is activated in most cases of apoptotic cell death

(Roberts, 2000; Gewies, 2003; Debatin, 2004). To date, 14 different

members of the caspase have been described in mammals with

caspase-11 and -12 only identified in mouse (Gewies, 2003). In broad

terms, there are two groups of caspases; initiator caspase (such as -2, -

8, -9, and -10) and executor caspase (such as -3, -6 and -7) (Table 1.1)

(Roberts, 2000; Gewies, 2003; Debatin, 2004).

In the cell, caspases are synthesised as inactive zymogens. The

inactive form of initiator caspase (e.g caspase-8) has longer domain than

inactive form of executor caspase (e.g caspase-3) (Figure 1.6 A)

(Gewies, 2003). The inactive form of caspase is so-called pro-caspase

which at the N-terminus carry a pro-domain followed by a large and a

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small subunit. The large and the small subunits are sometimes separated

by a linker peptide. Upon maturation, the pro-caspase is proteolytically

processed between the large and small subunit where the domain is

removed resulting in forming a heterotetramer consisting of two small

and two large subunits. The heterotetramer is an active form of caspase.

The disappearance of pro-caspase bands in Western blot analysis

reflects processing of the zymogen to generate the active form of the

specific caspase (Gewies, 2003; Cheah and Azimahtol, 2004). After the

initiator pro-caspase is cleaved and activated, it subsequently actives the

corresponding downstream executor pro-caspase molecules to become

active caspase which in turn initiating the apoptosis (Figure 1.6 B)

(Gewies, 2003).

The expression level of individual caspase may have an impact on

their overall activity, since deficient expression level may simply impair

caspase activation (Debatin, 2004). For example, MCF-7 breast

carcinoma cells completely lack caspase-3 expression due to a frame

shift mutation within exon 3 of the caspase-3 gene (Janicke et al., 1998).

These cells can be sensitised to treatment with cytotoxic drugs by

transfection of pro-caspase-3. Alternatively, caspase-8 expression was

found to be frequently inactivated by hypermethylation of regulatory

sequences of the caspase-8 gene in a number of different tumor cells

derived from neuroblastoma, malignant brain tumors, Ewing tumors and

small-cell lung carcinoma (Teitz et al., 2000; Fulda et al., 2001).

Importantly, restoration of caspase-8 expression by gene transfer or

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demethylation treatment sensitised resistant tumor cells to death

receptor-induced or drug-induced apoptosis (Fulda et al., 2001). In

contrast, gene knockout experiments targeting caspase-9 and -3 resulted

in mortality as a result of severe defects in brain development (Kuida,

1998). Moreover, caspase-8-deficient embryos died after day 12

(Varfolomeev, 1998). This and the observation indicating that cell lines

derived from such knockout experiments are resistant to distinct

apoptosis stimuli underlines the importance of caspases as pro-apoptotic

mediator (Gewies, 2003). Indeed, it has been recognised that caspases

play an important role in the apoptotic signaling machinery (Earnshaw,

1999).

Given the important role of caspases as the final effectors

molecule of apoptosis, the ability of anti-cancer agents such as PPARγ

ligands to trigger caspase activation appears to be a critical determinant

of sensitivity or resistance to cytotoxic therapies (Debatin, 2004). Indeed,

caspases are useful biomarkers for apoptosis, as outlined below

(Roberts, 2000). As a consequence, determination of caspase activation

in various forms of cell death including PPARγ ligand-induced apoptosis

may be an important factor in cancer chemotherapies (Debatin, 2004).

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1.7.2 Death receptor-ligand apoptosis

The death receptor-ligand system is so called extrinsic apoptosis

because the apoptosis signal is initiated by the death receptor at cell

surface (Goke et al., 2000; Gewies, 2003; Debatin, 2004). The death

receptor belongs to the TNF gene superfamily and generally has several

functions other than initiating apoptosis (Debatin, 2004). The best-

characterised death receptors are CD95 (or Fas), TNF receptor-1 (TNF-

R1) and TRAIL receptor (Goke et al., 2000; Roberts, 2000). The PPARγ

ligand-induced death receptor apoptosis is at all times associated with

the TNF receptor family (Goke et al., 2000).

1.7.2.1 Signaling by CD95/Fas

According to Ashkenazi and Dixit (1998), there are three main

roles of CD95 signaling:

1. mediate killing of cells by T-cells e.g. CTL-mediated killing of virus-

infected cells;

2. mediate deletion of activated T-cells at the end of an immune

response;

3. mediate destruction of inflammatory and immune cells in immune-

privileged sites.