synchronization and clustering in a quantum dot laser evgeny viktorov paul mandel université libre...
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Synchronization and clustering in a quantum dot laser
Evgeny Viktorov
Paul MandelUniversité Libre de Bruxelles
Yann TanguyJohn Houlihan
Guillaume Huyet
National University of Ireland, Cork, Ireland
Andrei VladimirovWeierstrass Institute, Berlin, Germany
Outline• Self-assembled quantum dot lasers: some properties of a different laser
• Multimode lasing: clustering
• Correlation measurements: antiphase dynamics- from disordered to « regular » switching
• Modeling: physical background
• Modeling: (non)degenerate Hopf, normal forms
Quantum dots: nanocrystalline gain medium
- nanoscale islands -form spontaneously during the epitaxial growth process on a semiconductor substrate -atomlike properties - "artificial atoms" -discrete energy spectrum- 1011 dots per cm2
Applications:
lasersoptical amplifiers information storage quantum computingquantum cryptography
A summary of laser performance:
• Low threshold current < 30 A/cm2 (Huang 2000; Park 2000)
• Modulation characteristics: 10 Gb/s (Hatori 2004, Kuntz 2005)
• CW operation up to 80°C
• Small factor < 1 or as low as 0.7 (Martinez, 2005) ??
Prospects:
Lowest threshold current
High temperature operation
Tunability
High quality beam
Low sensitivity to feedback
Reliable lasing without filamentation and parasitic instabilities for ultrahigh-speed applications
« dream » laser
Seminal picture
Quantum dot laser is an ensemble of independent nanolasers ???
Multimode lasing
We know:
Quantum dots have different shapes and sizes:
- strong inhomogeneous broadening and
- multimode lasing
- up to 50 modes
We measure/calculate:
modal oscillation frequencies
-modal timetraces
-modal correlations
-Hilbert phases
wavelength, nm
1235 1240 1245 1250
Pow
er (
a.u)
Multimode Spectrum: equally separated optical frequencies
We measure with:
- a high bandwidth (4 GHz) detector.
-an electronic spectrum analyzer
-a low bandwidth amplified InGaAs detector (50 MHz, Thorlabs PDA255).
Important limitation:
Only TWO modes can be measured simultaneously
Control parameter (pumping current)
leads to increasing :
• number of lasing modes• asymmetry in the gain profile • -factor - a global measure of the phase-amplitude coupling.
Experimental timetraces
Antiphase fluctuations :
• strongly chaotic• 40 % of the amplitude• low frequency range : up to 50 MHz
50 MHz << 5GHz (relaxation oscillation frequency – timescale of field-matter interaction):
Mode-to-Mode coupling???
Experimental timetraces
Observations:
• total output remains nearly constant
• antiphase fluctuations : perfect antisynchronization, correlation???
• "Chaos must shimmer through the veil of order“, Novalis
Experimental power spectra:-different modes can have different averaged frequencies of fluctuations
- clustering in averaged frequencies
-the spread of frequencies narrows with increasing current from 11 MHz to 3 MHz.
Experimental Hilbert phases:
We define:
two modes belong to the same cluster if the difference between two Hilbert phases is bounded
Detection noise influence
two detectors, the same mode, phase difference.
Equally separated clusters?
Correlation dimension vs clustering
We measure the correlation dimension of the modal signals.
-the modes from the central region of the spectrum have lower values of the correlation dimension, ≈2.8, and the modes at the edges have higher values, ≈3.3.
-the trend is similar (?) to the distribution of frequencies across the spectrum suggesting that the modes from different clusters can (?) exhibit different levels of complexity.
-we link the difference to the stochastic processes which govern the appearance of new lasing modes at the edges of optical spectrum (stronger influence of noise).
Cross-correlation measurements:
Results: • this time changes randomly for low currents when the spread of the frequencies is large• becomes linear for the higher current when the frequency spread of the fluctuations among the
modes was smaller• linear dependence indicates the propagation of perturbations through the spectrum
“from blue to red” - oscillations are equally phase-shifted
We measure:
-normalized cross-correlation function of all modes with respect to a reference mode.
-a maximum value of 1 is expected when the two modes are identical in amplitude and phase and, therefore, perfectly correlated.
-the time corresponding to maximum correlations between the modes as a function of modal frequency difference between the two recorded modes
Cross-correlation measurements: from disorder to regularity
Main Results
• clustering in averaged frequencies
• the spread of frequencies narrows
• oscillations can be equally phase-shifted
• Switching « from blue to red »
• MODE-TO-MODE COUPLING
Quantum Well Laser: experiment
• nearly constant total output
• similar frequency range
• periodic modal switching « from blue to red»
• originate from the Hopf bifurcation (statistical analysis)
Experiments:
Institut Non-lineaire de Nice, France, 2004
Quantum Well Laser: more advanced modeling
I 1,Itotal
I 2I 3
time(ns)
0 200 400 600 800 1000
I 4• Simplified equations,
four-wave mixing and global coupling:
dEm
dt 1
21 i Gm 1Em
k,p
pm EkEpEk p m ,
dFm
dt P Fm 1
k
N
mk |Ek |2.
#
#
• dominant mechanism – four-wave mixing • large a-factor (asymmetry in phase-
amplitude coupling) defines the unique sequence of switching from »blue to red»
• Hopf? Heteroclinic?
Two types of semiconductor lasers
Quantum Well Laser
-factor 4-5
• homogemeous material
• strong carrier diffusion
Quantum Dot Laser
-factor <1, increasing with the current
• inhomogemeous material
• small carrier diffusion
• total output remains nearly constant
• antiphase fluctuations
• low frequency range
• periodic, 100 % of the amplitude
• the same frequency of oscillations for all modes
• total output remains nearly constant
• antiphase fluctuations
• low frequency range
• chaotic, 40 % of the amplitude
• different frequences of oscillations, clustering
Physical model
• Equations:
The modal gains
and the cross-coupling coefficient
typically depend on four-wave-mixing processes and inhomogeneous broadening,
but physical mechanisms are complex and not fully understood yet
dE j
dt 1
21 i G j nk,Ek;k 1 N 1E j
dnj
dt P1 nj nj
k
N
gjkn,E; 1 N |Ek |2
#
#
G j nk,Ek;k 1 N
gjk n,E; 1 N
Challenge Quantum dot laser is an ensemble of independent nanolasers ??? carrier capture and recombination in individual quantum dots are random
processes so each quantum dot couples to its own excited carrier
• Conclusion: UNCORRELATED OUTPUT FROM THE DIFFERNET QUANTUM DOTS
We assume:• Modes are globally coupled• Hopf bifurcation• Inhomogeneous broadening (different shapes/sizes) results in different frequencies of oscillations
Two main effects to describe:
-frequency clustering
-antiphase state
Degenerate Hopf• Equations:
First “good” approximation: frequency dependent parameters are equal
Degenerate Hopf, normal form equations:
dE j
dt 1
21 i G j nk,Ek;k 1 N 1E j
dnj
dt P1 nj nj
k
N
gjkn,E; 1 N |Ek |2
#
#
tzj i zj azj k 1
N
|zk |2 bzj
k 1
N
zk2 czj|zj |
2 cN
k 1
N
zk |zk |2 O5
G j nk,Ek;k 1 N fnj, |Ek |2
gjk n,E; 1 N g and gkk n,E; 1 N 1
#
#
Hopf: nondegeneracy
- the modes have different average oscillation frequencies.
- we relate this non-degeneracy to the high degree of inhomogeneous broadening.
weak perturbation of the linear part
Phase approximation: Kuramoto, Hansel
Global linear coupling do not exhibit phase clustering behavior right after Hopf bifurcation (Okuda,1993)
Nonlinear coupling: frequency clustering? antiphase state?
tzj i jzj azj k 1
N
|zk |2 bzj
k 1
N
zk2 czj |zj |
2 cN
k 1
N
zk |zk |2 O5
Normal forms, N=5
5000 10000 15000 20000 25000 30000
50
100
150
200
29920 29930 29940 29950 29960
0.3
0.4
0.5
0.6
0.7
5000 10000 15000 20000 25000 30000
0.45
0.5
0.55
0.6
0.65
0.7
Normal forms, N=5: clustering
2000 4000 6000 8000 100000.35
0.45
0.5
0.55
0.6
0.652000 4000 6000 8000 10000
-2000
-1500
-1000
-500
9920 9940 9960 9980 10000
-2060
-2040
-2020
-2000
9920 9940 9960 9980 10000
-2005
-2000
-1995
-1990
9992 9994 9996 9998 10000
0.2
0.3
0.4
0.5
0.6
9992 9994 9996 9998 10000
0.45
0.5
0.55
0.6
0.65
conclusion
Modal oscillations in quantum dot laser result from the global coupling and exhibit clustering and antiphase state.
Thank you!