soil gas radon concentration and permeability at “valle

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Soil Gas Radon Concentration and Permeability Soil Gas Radon Concentration and Permeability at “Valle della at “Valle della Caffarella” Test Site (Roma, Italy). Caffarella” Test Site (Roma, Italy). Evaluation of Gas Sampling Techniques and Radon Measurements Evaluation of Gas Sampling Techniques and Radon Measurements Using Different Approaches Using Different Approaches Italian team Mauro Castelluccio, Massimo Moroni, Paola Tuccimei Czech team Matej Neznal, Martin Neznal 10 th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPING September 22 nd – 25 th , 2010 - Prague, Czech Republic

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Soil Gas Radon Concentration and PermeabilitySoil Gas Radon Concentration and Permeability

at “Valle dellaat “Valle della Caffarella” Test Site (Roma, Italy). Caffarella” Test Site (Roma, Italy).

Evaluation of Gas Sampling Techniques and Radon MeasurementsEvaluation of Gas Sampling Techniques and Radon Measurements

Using Different ApproachesUsing Different Approaches

Italian teamMauro Castelluccio, Massimo Moroni, Paola Tuccimei

Czech teamMatej Neznal, Martin Neznal

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

1 2

3

4

5

Tevere river

GRA ring road

0 1 2 km

ROMA

N Aniene river

Almone river

Roma (Italy)

Simplified geological map

1 1 PlioPlio--PleistocenePleistocene marine marine tototransitionaltransitional depositsdeposits

2 2 SabatiniSabatini districtdistrict volcanites volcanites

3 Colli Albani 3 Colli Albani districtdistrict ignimbritesignimbrites

4 Colli Albani 4 Colli Albani districtdistrict lavaslavas

5 5 AlluvialAlluvial sedimentssediments ofof Tevere Tevere River and River and itsits tributariestributaries

Valle della Caffarella Test Site

12

3

45

Seasonal Change of Soil Radon Concentration

30 cm 80 cm Rain (mm)

Winter 07 Winter 08 Winter 09

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPING September 22nd – 25th, 2010 - Prague, Czech Republic

PREVIOUS WORK AT VALLE DELLA CAFFARELLA TEST SITE (1)

Monitoring at Permanent Station 1, on Colli Albani ignimbrites

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPING September 22nd – 25th, 2010 - Prague, Czech Republic

SOIL RADON MAPPING

PREVIOUS WORK AT VALLE DELLA CAFFARELLA TEST SITE (2)

PERMANENT STATION 1

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPING September 22nd – 25th, 2010 - Prague, Czech Republic

Soil Radon – Winter Soil Radon - Summer

PREVIOUS WORK AT VALLE DELLA CAFFARELLA TEST SITE (3)

SOIL RADON MAPPING – 80 cm depth

1 2 3 4

Sampling stations Sampling stations December 2009 and June 2010December 2009 and June 2010

Permanent Station

Mobile Station

Inner profile(RAD 7)Outer profile(Radon v.o.s.)

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

THIS WORK

Sampling depths:

Shallow: (~ 30 cm)

Deeper: (~ 80 cm)

Italian Team � Durrridge approachDurridge Probe and alpha counting (RAD 7)

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Roma, 11 e 12 giugno 2010Il radon: un rischio geologico 8

• ID 7 mm

• OD 11 mm

• Point maximum diameter 13 mm

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Italian Team � Durrridge approachDurridge Probe with fixed point

Roma, 11 e 12 giugno 2010Il radon: un rischio geologico 9

Special care to tamp down the soil around the probe

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Main concern : leakage of fresh air down to the sampling point

Roma, 11 e 12 giugno 2010Il radon: un rischio geologico 10

www.radon-vos.cz

www.radon-vos.cz

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Check Team � Radon v.o.s. approach Radon v.o.s. Probe and Lucas cell + Ionization Chamber

• ID 8 mm

• OD 12 mm

• Point maximum diameter 12 mm

“LOST” TIP

www.radon-vos.cz

SOIL GAS PERMEABILITY MEASUREMENTS

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

)**()*(

tpFVk ∆= µ

(Neznal & Neznal, 2005)

V: air volume in the rubber suck µ: air dynamic viscosity at 10°C F: Shape factor of the probe ∆p: pressure difference between the surface and the s ampling depth t: opening time of the cell

The principle consists of air withdrawal by means of negative pressure driven by a rubber sack, with one or two weights.

Air is pumped out from the soil under constant pressure through the probe with a constant surface of contact between the probe head and the soil.

The gas permeability (k in m2) is calculated using the known air flow through the probe.

SOIL GAS PERMEABILITY USING THE RADON-JOK PERMEAMETE R

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

•Winter campaign

• Total of 60 soil radon measurements including replicates for Lucas Cells and Ionization Chambers

• Soil Radon and Thoron measurements using RAD7

• 21 soil gas permeability determinations

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Results of the Winter campaign

Deeper depth (~ 80 cm):

� The three methods (alpha counting, Lucas Cell and Ionization Chamber) gave comparable results � Durridge approach up to 15 % lower

�Low permeability � averagely in the range of 10-13 - 10-14 m2

Shallow depth (~ 30 cm):

� Durridge approach gave results 60 % sistematically lower than Radon v.o.s.

� Higher permeability � 2.5 · 10-12 m2

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

100 – 200 kBq / m3

30 – 180 kBq / m3

Roma, 11 e 12 giugno 2010Il radon: un rischio geologico 15

Enhancedeffect at

shallow depth

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Discussion

Durridge approach gave lower soil radon concentrati ons because of leakage of

fresh air down to the sampling point

DURRIDGE RADON V.O.S.

Atmospheric air

Soil gas radon from shallower

depth

HOLLOW SPACE

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

Summer campaign

� Replication of winter measurements� Increased care to seal the probe hole� Testing a mixed approach at station C:

Radon v.o.s. probe + RAD7 continuous monitor

Results of the Summer campaign

� Lower values of soil radon and higher permeability compared to winter

Deeper depth (80 cm):

� The three methods (alpha counting, Lucas Cell and Ionization Chamber) gave comparable results �Durridge approach just 5 % lower

Shallow depth (30 cm):

� Reduced differences between the two approaches

� The mixed approach gave comparable results with Radon v.o.s. approach

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic

40 – 160 kBq / m3

20 – 50 kBq / m3

Conclusions

•Gas sampling techniques affect soil radon concentration results more than analytical methods

• Fresh air leakage down the sampling hole is is due to the combined effect of the probe tip relative size and the poor sealing of the sampling hole.

• Summer soil radon concentration are lower because of enhanced radon release to the atmosphere when soil is drier, warmer and more permeable.

•Soil gas permeability is a crucial parameter to interpret spatial soil radon variability and seasonal changes

10th INTERNATIONAL WORKSHOP on the GEOLOGICAL ASPECTS OF RADON RISK MAPPINGSeptember 22nd – 25th, 2010 - Prague, Czech Republic