skinath: a computer program for solving the reactor point

68
a

Upload: others

Post on 14-Feb-2022

3 views

Category:

Documents


0 download

TRANSCRIPT

a

..... __ ___ .. __ .......... __

~ .......... ___ . _ ......... __ .. _,_ .

_ ....... ....... _ _x_ .....-.....

ORNE/CSDbTM-21 0

S K I N A T H - A Computer Program f o r Solv ing t h e Reactor Po in t

K i n e t i c s Equat ions wi th Simple Thermal-Hydraulic Feedback

H. L. Dodds, Jr. Nuclear Engineering Department

The Unive r s i ty of Tennessee Knoxville, Tennessee 37916

and

R. M. Westfall COMPUTER SERVICES

a t Oak Ridge Na t iona l Labora tory

Post Office Box x Oak Ridge, Tennessee

Date P u b l i s h e d - S e p t e m b e r 1984

Martin Marietta Energy Systems, Inc. o p e r a t i n g the

Oak Ridge Na t iona l Labora tory Oak Ridge Gaseous D i f f u s i o n P l a n t

O a k Ridge Y-12 P l a n t Paducah Gaseous Di f fus ion P l a n t

under Con t rac t No. BE-AC05-840R21400 f a r t h e

DEPARTMENT OF ENERGY

T a B L E OF CONTENTS

.&%.e

ACKNOWLEDGMENT. . . . . . . . . . . . . . . . . . . . . . v

A B S T R A C T . . . e . e . V i i

1 . I N T R O D U C T I O N . . . . . . . . . . . . . . . . . . . . . . . . 1

2. T H E O R Y . . a . . * 1

3 . RESULTS AND CONCLUSIONS . . . . . . . . . . . , . e . . . . 3

4 . RECOMMENDATIONS FOR FUTURE WORK . . . . . . . . . . , . . . 7

REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . 8

APPENDIX A . . . . . . , . . . . . . . . . . . . * . * . 9

APPENDIX € 3 . . . . . . . . . . . . . . . . . . . . . a . . 15

iii

ACKNOWLEDGMENT

This work was supported by the Oak Ridge Gaseous Diffusion Plant a s p a r t of a m u l t i s f t e s tudy on t h e p l a u s i b i l i t y and consequences of low- power c r i t i c a l i t y e v e n t s . The authors e x p r e s s t h e i r a p p r e c i a t i o n to D. J. Hamby for t h e preparat ion of the manuscript .

V

ABSTRACT

A FORTRAN computer program named SKINATH has been developed for s o l v i n g the r e a c t o r p o i n t k i n e t i c s equa t ions with s i m p l e thermal- h y d r a u l i c feedback. The program u t i l i z e s t h e o r d i n a r y d i f f e r e n t i a l equa t ion s o l v e r , LSODE, developed by Hindmarsh a t the Lawrence Livermore Nat iona l Laborat,ory. Based on comparisons w i t h bo th a n a l y t i c a l and o t h e r numerical s o l u t i o n techniques , the program g i v e s a c c u r a t e r e s u l t s w i th impress ive ly s h o r t r u n times.

v i i

1 . I N T R O D U C T I O N

SKXNATH aimpic t i c s and Xhermal-&ydraulics, is a FORTRAN computer program developed f o r t h e IBM 3033 (double p r e c i s i o n ) f o r s o l v i n g t h e reactor p o i n t k i n e t i c s e q u a t i o n s ' coupled wi th a s imple thermal-hydraulic feedback model. SKINATW c o n s i s t s of a main r o u t i n e which e s s e n t i a l l y sets up the i n p u t for c a l l S n g LSODE, a n o r d i n a r y d i f f e r e n t i a l equa t ion s o l v e r developed by Hindmarsh3 a t t h e Lawrence Livermore Nat iona l Laboratory, and one s u b r o u t i n e which i s r e q u i r e d by LSODE. The e n t i r e program c o n s i s t s o f about one hundred FORTRAN s t a t emen t s , exc lud ing LSODE, and u s u a l l y e x e c u t e s i n less than two CPU seconds (IBM 3033) for most problems of i n t e r e s t .

S e c t i o n 2 of t h i s document p r e s e n t s a brief d i s c u s s i a n o f the equa t ions which are so lved and P few comments about t h e methodology employed i n LSODE.

I n S e c t i o n 3 r r e s u l t s ob ta ined wi th S K I N A T H are compared wi th r e s u l t s ob ta ined a n a l y t i c a l l y and with other numerical r e s u l t s .

A listing of t h e program is presented i n Appendix A which inc ludes the i n p u t for a sample problem. The ou tpu t f o r t h i s sample problem is presented i n Appendix B.

2. THEORY

SKINATW s o l v e s the fo l lowing equa t ions :

1 . 2 5 - - dT I E P ( t ) - AHD.75 [ T ( t ) - Tc] /T(t)*25) dt C - - t P

dCi B i W - - - d t A - hiCi(t), i = 1, ....., M ( 3 )

Equation (1) r e p r e s e n t s a n energy ba lance f o r a r e a c t o r I n t he shape of a long h o r i z o n t a l c y l i n d e r which is cooled e x t e r n a l l y by an idea l gas v i a n a t u r a l convection.2 T is the reactor tempera ture , Cr, i s t h e heat c a p a c i t y of t h e r e a c t o r , H and D are t h e r e a c t o r height and diameter, r e s p e c t i v e l y , Tc is the c o o l a n t tempera ture (which is cons tan t w i t h r e s p e c t to time, t ) , and A is a c o n s t a n t determined by

2

where K i s t he c o o l a n t thermal conduc t iv i ty (J/m-sec-cc), i s t h e coo lan t is the coolant v i s c o s i t y (~g/m-sec) , and eP is the C O O I ~ ~ L ~ p o ~ c i r ^ i c heat. (J/Kg-"C). The va lue af A (17.52) l i s t e d in t h e sample problem I n Appendix A i s for air a t s tandard temperatuse and pressure . The E i n Equat ion ( 1 ) i s t h e f r a c t i o n of t he energy from f i s s i o n depos i t ed as heat i n the! system.

pc 2 d e n s i t y (Kg/m3), g is t h e g r a v i t a t i o n a l c ~ n s t a n t (mlsec. ),

Equat ions ( 2 ) and (3) are t h e s t anda rd p o i n t k i n e t i c s equa t ions where P i s the neut ron d e n s i t y (neutrons/cm3), which is p ropor t iona l t o the reactor power, p is t h e system r e a c t i v i t y ( d o l l a r s ) , A i s t he system generatj-on t i m e : (seconds) and Xi, C i , B i ii1-e t h e decay cons tan t ( s e c o n ~ s ) , precur so r concen t r a t ion ( n u c ~ - e i / c m ~ 1, and delayed neut ron fraction, r e s p e c t i v e l y , for pi-ecursor group i. The number of delayed

p recu r so r groups is M and B Pi. S i s an ex t raneous neutron

SQU~TB neutrons/cm3) OP known magnitude.

M

i=l

The system r e a c t i v i t y , p, c o n s i s t s o f an e x t e r n a l d r i v i n g functioPi which may be ei ther a s t e p , linear r m p , or a q u a d r a t i c i n time p l u s a l i n e a r feedback component as shown below:

where t is i n S ~ C Q ~ ~ S and the r e a c t i v i t y feedback c a e f f i c i e n t , R'HOCOF, has UnitS Of dollars De?." " c .

Most oi' t h e a p p l i c a t i o n s cons idered t h u s fa r have used s i x (M = 5 ) delayed neutron p recu r so r groups 90 that eight equa t ions are being solved by LSODE. The energy balance equa t ion i s t h e first equation fa l lowed by t h e neut ron ba lance equation and t hen t h e s i x precursor ba lance equations.

LSODE s o l v e s i n i t i a l va lue problems for e i t h e r stiff or r im-s t i f f s y s t e m of first o rde r ordinary d i f f e r e n t i a l equat ions, either l i n e a r or non-linear. I n t e g r a t i o n time s t e p sizes m e selected au tomat i ca l ly by LSODh". accord ing t o t o l e r a n c e parameters s p e c i f i e d by the user which con- t.rsl the accuracy of the r e s u l t s . M O D E r e q u i r e s the Jacobian matrix i n some form which may be e i the r user supp l i ed via an a d d i t i o n a l u 3 e ~ w r i t t e n sub rou t ine OF LSQDE w i l l compute i t i n t e r n a l l y us ing d i f f e r e n c e

3

q u o t i e n t s . SKIMATH also assumes tha t t he i n i t i a l c o n d i t i o n o f t h e r e a c t o r is s t e a d y state delayed cs i t ical w i t h no thermal-hydraulic feedback, I n o t h e r words, the feedback i s not i n equ i l ib r ium w i t h t h e n e u t r o n i c s a t time zero. The u s e r s p e c i f i e s t he i n i t i a l neut ron d e n s i t y ( o r power), t he coo lan t tempera ture (which is set equa l t o t h e i n i t i a l r e a c t o r tempera tuse) , the e d i t times (i.e., when r e s u l t s are desired), and v a l u e s f o r the o t b e r c o n s t a n t s appear ing i n Eqs. ( 1 ) 4 4 ) which model t h e system o f i n t e r e s t ,

3 . RESULTS AND CONCLUSIONS

Eva lua t ion of SKINATH has been accomplished by comparing r e s u l t s ob ta ined w i t h S K I N A T H w i t h a n a l y t i c a l r e s u l t s and wi th o t h e r numerical r e s u l t s .

The first problem cons idered i n t h e e v a l u a t i o n is a problem tha t can be so lved a n a l y t i c a l l y . S p e c i f i c a l l y . a s t e p change i n r e a c t i v i t y (7 c e n t s ) w i t h 0ne delayed neu t ron group (M = 1, h l = 0.1, B 1 = 0.0065) and no thermal -hydraul ic feedbaok (RHOCOF = 0.0). The i n i t i a l r e l a t i v e power is 1 .O and A = 5.OE-05 see.

1

The numerical e v a l u a t i o n o f the a n a l y t i c a l s o l u t i o n f o r t h i s problem is shown i n Table I along with SKINATH r e s u l t s and also r e s u l t s ob ta ined v i a a f o u r t h o r d e r Runge-Kutta p r ~ c e d u r e . ~ The Runge-Kutta s o l u t i o n employed 0.01 sec time s t e p s and r e q u i r e d approximately 8 CPU seconds on t h e IBM 3033 for the 15 minute t r a n s i e n t . The S K I N A T H s o l u t i o n r e q u i r e d on ly 0.12 CPU seconds f o r 15 minutes of t r a n s i e n t time. Thus, i t is concluded t h a t SKINATH produces a c c u r a t e r e s u l t s w i t h ve ry s h o r t r u n times for s imple k i n e t i c s problems wi th no thermal- hydrau l i c feedback.

The nex t problem cons idered i n t h e e v a l u a t i o n of SKINATH is a step change i n r e a c t i v i t y ( 4 . 3 c e n t s ) wi th s i x delayed neut ron groups and thermal-hydraulic feedback p r e s e n t (kWQCOF = -0.306 c e n t s pe r degree Ce lc ius ) . The i n i t i a l r e l a t i v e power and t h e i n i t i a l r e a c t o r tem- p e r a t u r e are 0.01 watts and f o r t h i s sample problem are i s presented i n Appendix B. so lved i n Reference 2 which t h e power, (2) i gnores t h e and ( 3 ) u s e s E u l e r ' s method

20 *C, r e s p e c t i v e l y . Other inpu t parameters presented i n Appendix A. The problem ou tpu t

T h i s problem was o r i g i n a l l y de f ined and ( 1 ) assumes a pure exponen t i a l behavior f o r prompt neut ron c o n t r i b u t i o n t o r e a c t i v i t y , f o r the time i n t e g r a t i o n , A f o u r t h o r d e r

Runge-Kutta procedure was also used to o b t a i n a t h i r d s o l u t i o n t h i s problem ( w i t h A t = 0.01 sec). P l o t s of the power v e r s u s time obta ined by each of these three s o l u t i o n approaches are presented i n F igu re 1 . Corresponding tempera ture p l o t s are presented i n F igu re 2. Addi t iona l S K I N A T H r e s u l t s f o r t h i s problem ou t t o a f i n a l time of 1000 minutes are presented i n Appendix B.

of

4

0 .o 1 .o 2 " 0 3 00 4 .o 5 .e 6 .Q 7 .0 8 .O 9 .Q 10 .0 11.0 12.0 13.0 14.8 15.0

100 .o 50 .a

1 .o 1.688 2.651 4.162 6.536 10.26 16.11 25.30 39 -73 62.39 37.96 153.8 241.5 379 -3 595.5 935 1 675.1 E+7 424 .OE+17

1 .o 1.688 2.651 4.163 6 .is36 10.26 16,12 25 -31 39 074 62.39 97 0 97

153.8 241.6 379.3 595.6 935 -2 675.5E*7 424.4E917

1 .o 1.687 2 -649 4.154 6.510 10.21 1s .02 25,111 39.47 67.91 99 02 152.2 238 97 374.6

922 0 9 i OI

* Results not computed.

5

0 R N C- D W Q 8 3C - 16676

RUNG.€-KUTTA

0 20 40 60 80 100 120 140 TIME (mln)

Figure 1. P o w e r V e r s u s T i m e f o r P r o b l e m No. 2

-I- 0 20 46 o 100 120 14

F i g u r e 2 . Temperature Versus Tiine € o r Problem N o . 2

7

Note t h a t t h e SKINATW r e s u l t s are similar t o t h e r e s u l t s of Reference 2 whish employed sevwal s i m p l i f y i n g assumptions. The Runge- Kut ta and SKINATH r e s u l t s are also q u i t e similar. More impor t an t ly , t he Runge-Kutta r e q u i r e d 6 minutes o f CPU time on t h e IBM 3033 for a t r a n s i e n t time Qf 130 minutes; whereas, SKIMATH r e q u i r e d on ly 1.8 seconds of CPU time for a t r a n s i e n t time of 1000 minutes. The Reference 2 r e s u l t s were obta ined us ing a d i f f e r e n t computer.

c a l c u l a t i o n

Based on these r e s u l t s and o t h e r comparisons t h a t were performed bu t are no t presented i n this document, w e conclude t h a t SKINATH is an a c c u r a t e and e f f i c i e n t program for s o l v i n g p o i n t k i n e t i c s problems wi th s imple thermal-hydraulic feedback.

4 . RECOMBNDATIOMS FOR FUTURE WORK

The c u r r e n t v e r s i o n of S K I N A T H employs t h e LSODE o p t i o n t o c a l c u l a t e the Jacobian i n t e r n a l l y by d i f f e r e n c e q u o t i e n t s . An improvement i n accuracy and/or computing e f f i c i e n c y might be realized i f the Jacobian is c a l c u l a t e d by t h e u s e r as recommended i n the LSODE documentation. The improvement may be s i g n i f i c a n t p a r t i c u l a r l y f o r stiff problems.

The thermal-hydraulic model i n SKINATH i s r e a l l y q u i t e crude. Many improvements could be made depending on the system being modeled. One improvement t h a t could be made is to i n c o r p o r a t e an energy ba lance f o r the coolant . Cur ren t ly , t h e coo lan t is modeled as an i so the rma l heat sink which is u n r e a l i s t i c for most a p p l i c a t i o n s .

As i n d i c a t e d earlier i n t h i s document, e q u i l i b r i u m between the n e u t r o n i c s and thermal -hydraul ics a t time zero does no t ex is t i n t h e c u r r e n t v e r s i o n o f SKINATH. Such e q u i l i b r i u m is desirable, a l though no t necessary , f o r most practical problems of i n t e r e s t and should be implemented i n a la ter v e r s i o n of SKINATH.

F i n a l l y , comparing SKINATH r e s u l t s w i th t he r e s u l t s of s e v e r a l t r a n s i e n t exper iments should be performed i n order t o better e v a l u a t e both the models employed i n SKINATH and its s o l u t i o n methodology.

a

REFERENCES

1. A. F. Henry, Nuclear-&eactor A n ! , NIT Press, Cambridge, Chapter 7, P. 308 (19755).

2. C, E. Newlon e t a l . , wAn assess ent of the Minimum Criticality Accident of Concern," N d: R Technical Associates , H ti R 82-2, Oak Ridge, Tenn. (1982).

3 . A, C. Hindmarsh, "LSODE and LSODI - Two New I n i t i a l . Value Ordinary Differential Equation Solvers," ACN-Signum Newsletter, Vsl. 15, No. 4 (1980).

4 . R. L. Burden e t a l . , Numericah , Prindle, Weber and Schmidt, Boston, p. 244 (1978).

APPENDIX A

Program Listing and Sample Problem Input

10

L

IL

L.

lA

l.

2.

t- b- c

t- Cb

- - c- f- )..

I- t- +

4

a

U

4

44

a

a

4

ea

u

a

.XU

a 4 a

4

- I

Y

Y

YY

Y

Y

Y

YY

YY

YY

Y

Y

ir a

0 7

iii U

li

II: JJ

a' Y

n

z w >

J

- c

1

In U

L-

I

- W

z Y

I- -. - U a W

J

a I

m 1

> L

4

n

I

c

4

Y

m

I- x W

c

2

X

Id

Jl z

r

L

2

-I U

UU

JU

UL

'UU

UU

UU

Ub

UU

UU

UU

LJ

UL

UU

U

JL

3 ... 7

1

2

-0

U

U

v

a

I

h

J

ui

> I

J

C T H ~ R ~ A C T I V I T Y F ~ E ~ R A C K CO~FFICIENT I S NEXT. R h O C J F = -. 003 O h 3 + 0 *UT SOURCF = O m OD+ 0

03550533 J0000540 0 00 0 0 55 0 no000~60 J 5000570 o 93 on 580 nor) o o w J o nooo 60 0

0noooh3n oon 3065 3

n 00 0 0 67 o o o o o o m 3 3n03ohw1 O O O O O T ~ o

0000n74 0

O O O O O T ~ O

OOOO0610 0 300@6? 3

00000b43

3JJOOhb 3

0 0 00 0 70 3

30030720 00 0 0 3 7 3 0

0500075J

300J0713 0 J00070J 00000793 a m a o e o o 0000051 00000 32 3 0

O O O i i 0 8 J O 000 3384 0 000 90850

00000973 0003J?99 03000890 00003000 O c ) O O 0 9 1 0 03003')20 000009JO 000 00 Q4 0 O O O J J Y 5 3 000 0 d 96 3 00000970 00000980 00000993 00031000 0000 I01 0

03001030 30001 940

00001060 00001 370

000 0 1090 ODOOl LOO

ooono 363

00001020

ooon i 05 3

oaooioao

C c C C

T H t H H A L - - H Y D l + A U L I C I N P U T

EPSIL =1.00+0

TC = 20.940 A = 17.52,)+0 H = O . Z 3 U + O

4Hd75 A t H * D * * . 7 5 0 4 0 o = o . ~ m + o

C P = 1 ~ 0 0 . 0 + 0 * 3 . 1 4 1 5 9 2 h 5 0 4 0 * 0 * 0 / 4 . ~ + 0 * ~ * 1 0 0 ~ . 0 t 0 Y(1) = TC

C

C C C C c

G F N E R A L I N P U T

4 F J = 9 I T O L = 1 ? T O L = 1.0-05

I T A S K = 1 I S T A T F = 1 10PT = 1 LRW = 200 L I W = 200 UF = 2 2 I C U U N T = 1 T = O.D+O

O T = 60.0+0 TflUT = OT F O R M A T ( I H J . 'L I ST

T S T P P =60009.0*0 WR I T € I 6 . 4 4 ) F G R M A T I I H J . ' T H E F ' I L L C * I N G TWO L I S T 3 ECHO T H E I N P U T ' ) W l + I T E ( 6 . 4 5 L E P S I L . A H D 7 ~ ~ T C ~ C P ~ ~ ~ O E X . ~ H ~ C G F ~ ~ ~ ~ A . ~ ~ T A . G E N . ~ T

F O R M A T ( l H O . * L f S T l ' r 6 S 1 7 . 4 1 WR I TE I h r 4 6 )NEQ V

A T r L = 0.n4n

T H t T I M E S T F P S I L E ( S ' C C N D 3 ) FUfi C D I T I N G C)JTPUT I S Y E X T .

2 * .6Gl7.4 I THE FINAL T I M C I S E C O Y O S ) F C P THE T R A N 5 I E N T I S NEXT.

XI SOURCE

T TOUT 9 I TOL e e T O L ATCL I T 4 S K I S 7 A 1 E. I CPT. Xbl WORK .C RW I WONK .LI W J€ X .MF

C

46 C

ISN 0052 ISN 105-

I S N 0055 ISN 0054

IS^ c n 5 e ISIV o n 5 7

4 4

4 5

C C c C C

HkLLC THERE

I S N 005P SSN 0 0 5 9

I S N 0060 1SN I ) O h l

42

47

12

07000000000

00000000000

00000000000

OOOOOOOO~OO

~

X.

- n I

II

W

+- t

a

VI a CC

+z

V

IW

NF,

vc

ailc

W

O~

L*

IO

LT

~~

WV

C~

NP

I

GC CSSa

cc

cc

cc

"c

cu

~u

u

00

0000 ocoooooooococ

co 0900 ococoococcc"o

13

c 0

N

N

400000000000000

Nm

8tm*"m

eO-N

maln

S

mm

Rm

mq

nO

dd

dd

+b

d

oooooooeooooo~o

000000000000000

OOOOOOooOOoooOO

OOOOOOOOOOOOOPO

44-...-,4---*..----

n

U

\

0

.-, l L

J-

c

w

IU

-3

-

c

-a

E?

!

*I

-

ur

n

0.

u

z

-a

!Y

*

.

a

I-

0

*Y

i

t-

4

-.* -

I- L

-

m 0

-w

I

NO

a

IT

5;

;

or

-

0

W

ZJ

u

3-

ha

I?P

UlD

y)P

-aJI(E

O

0000000-

00000000

00

0r)0

0D

0

14

APPENDIX €3

Sample Problem Output

1G

I n

00

3cI

oo

oo

oo

oo

~o

no

oo

~e

oo

~~

oo

o~

0

P

N

... ........................ 0

00

05

a0

00

60

00

00

00

00

0O

ao

a

N

rr

c

m

01

1N

50

0

m 0 I

VI

0

m-

b

-

N-

.

e

00

n 10

-

00

I

on

n

o

-r

m

2g

.. a

o

r(

0

I 0

00

O

d

.N

0

-

N*

c- 3 9

0

-N

w-

9: b

u

V

w ln

t- m

J

C

0

wa

3

.

t-

-

W

Z

'. G

J

d

cli - U.

t

win

I

-

am

r

3

c

N

0

NN

0

0

II

Fl

6-

0

00

I

ll

D

n

a

00

0

00

0

NO

0

win-

... 0

3

0

0

0 . d

0

0

d

d

IC c

oo

ow

o

Q a I 0

01

OI

m

.-. 0

I 0

0 . "

I- ln

..

m 0

I a 0 0

c

N

0

n

0

I 0 0

U

10 c 0 . 4

t- ln

,-, JJ

J

o0

00

00

00

05

00

00

00

w0

00

o0

0

....................... G

OO

OO

OO

OO

OO

O0

O~

O~

0O

OO

~~

oo

ao

oo

oo

~o

~o

oo

oo

oo

oo

oo

8

....................... 0

OO

0O

OO

QO

OO

0O

OO

OO

OO

OO

O0

d

oo

oa

o~

oo

00

oo

oo

oo

oo

o~

0o

o

00

0@

00

0~

00

00

00

00

00

00

0~

0

.......................

0

0

6 0

I 0 0

U

0 ,. . 0 (\I

t- m

J

... J

J 0

0

0 . 0 N

t- m

J

h.

00

00

..

GO

00

..

NN

t-

I-

v

rm

c

-

JJ

J 0

0

0

0 . N

!- bl

J

-

0

0

c * c N

t- m

d I

Jd

00

00

..

00

00

..

NN

!-e

ln

v,

-I

JJ

J 0

0

0 . 0 N

lr m

J I

JJ

0

0

0 . 0 N

+" m

"I H

JJ

J 0

0

0

0 . N

c

m

-I 3

8

0 . 0

0 . N

P

v) -

-1

J

h rl

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

C

0

0

c 0

C

0

c c

0

0

0

0

0

0

0

0

G

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

c *O

0 -0

G *C

0 *@

@ -0

0 *O

c -0 C -0

c =o e '0

0-0

0.C

0-0

0-0

0.0

0.0

0.0

0.0

0.0

0.0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

G

G

0

0

G

G

c 0.0

0-0

0.0

0.0

0'0

0.0

0.0

0.0

0-0

0.0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0. Q

0.0

0.0

0.0

0.0

0.0

0.0

0.0

0.0

0.C

0

0

0

0

0

0

0

0

0

0

c 0

c 0

0

0

0

0

0

0

0

0

0

002

0 *O

0 *O

0.0

0 '0

0 *O

0 *O

0.0

0 -0

0.0

0.0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

0

G

0

C

0

0.0

6.0

0.0

COO

0.0

0-0

6.0

0.0

0-0

0.0

0.0

2 *SI1

2 IS11

z IS17

2 IS11

a If11

z IS11

E IS11

2 1511

a 1517

2 IS11

2 IS11

2 IS11

a IS17

2 &SI3

2 IS11

2 AS11

2 IS11

2 IS11

2 IS11

2 is11

2 IS11

2 IS11

2 IS11

L IS11

2 IS17

2 IS11

2 IS11

2 IS11

z IS17

2 IS11

2 1511

z 1517

2 isr-i

z &SI1

0

0 0 c 3

n

0 0 c.

0

00

00

00

00

00

0

N

00

00

00

60

00

T IHE(MKN1 --------- l.00U

2.000

3.000

4.000

5.000

6 . 000 7.000

P.000

4.000

10.00

I 1 .OO

12.00

13.00

14.00

L5100

16.00

17.00

l R . 0 0

19.00

20.00

21000

P2.00

23.00

24.00

25.00

26.00

0 e 4 3 ODD-Q 1

0.4 2 0 3 D-0 A

0.4 3000-0 1

0.4 3 005-0 1

0.43000-01

0 a 43000-0 f

0.4 3000- 0 1

0.43000-0 1

C.43000-0 1

0 4 2 99 0- 0 1

0*42' i90-0 1

0.02990- 3 I

0 4 2990- 0 1

0 04 2FBD-0 1

n. 4 2980-0 t

0 4 2480- 0 1

0 42970-0 1

0 4 2 %50- 0 1

0 42450-6 I

0 4 2 940-0 1

0.42930-01

0.4291 D-0 1

0 . 4 2 5 e ~ - o i

0.4285O-0 I

0.4282D-0 1

0 42 77D-0 1

20.00

20.00

20.00

20.00

2 0 . 0 0

20.00

20.00

20.00

20.00

20.00

20.00

20.00

20.00

20.00

20.0 1

20 .01

20.01

20.01

20.02

20.02

20.02

20.03

20.04

20.0s

20.06

20.07

0.1391 0-0 1

0.17440-01

0*21RC)D-O1

0.2 724 0-0 a 0 34020-0 1

0 424 80-01

0 53 050-0 1

0.66250-01

0.82730-01

0.1033

0.1290

0.1611

0.2012

0.2512

0.3136

0.3916

0.4890

0.6105

0.7522

0.9515

1.188

1.482

1.850

2.308

Z.BR0

39591

4.0 18

4.357

5.997

7.459

9.302

l l r 6 1

14.50

14.10

22.61

28 .23

35.25

44 .02

54.97

58-54

85.71

107.0

133.6

166.8

208.3

260.1

324.7

405.3

505 8

631 -2

787 6

982 5

11.49

14 - 4 5

18.09

22.61

28 24

35 27

44.05

55.01

68 69

85.78

107.1

133.9

167.0

208.6

26004

325 2

406 0

501.0

63209

790.2

986.4

1231

1537.

1917.

2392.

2984.

2.074

3 . 860

4.827

hrQ31

7.533

F.407

a 1.75

14 *6?

16-32

22-88

28.57

2 5 - 6 7

44.55

55 62

e9.46

l36.72

108.3

135.2

168.6

210.7

263.0

220 a 3

409.7

511.2

637.8

795.5

2.345

2.941

3.677

4.594

5.738

7.166

3.944

11.16

13.96

lam43

21.76

27 .17

33.93

4 2 37

52.9 1

bb.06

82 .41

103.0

128.6

160.5

200.e

250.1

3 1 2 . 1

339.4

485.8

605.0

0.1824

0.2287

0.2853

0.3572

0.446 1

9.5572

0.4959

O.FlhZI9

1 * 085

L .345

I . 6 Y P

2 . 1 1 2

2.639

3 2"14

4.114

5.135

6.41 3

0.037

9 996

12.4R

15.58

1 Y * * 4

24 -26

3i).??

3 7 . 7 7

47.10

0.24923-01

0.3 1240-0 f

0. CI ? 0 6 J - O I

3.4580?1-0 L

O.fi095J-01

0 .7~120- -01

0.93 060-0 1

0.LL37

0.1482

0 .1451

0.211 2

0.2357

0.3604

0.4201 I-r

0.5620 v)

0 . 7 3 1 7

O . R ? b l

1.394

1.366

1.705

1 . 1 2 8

2.656

3.315

4.136

5 .160

8.435

T h WE ( Y I N ) --- - -__ - -

27.00

28.00

29.00

20.00

31.00

32.00

33.00

3 4 00

35.00

36.00

37 00

38.00

39.00

40.00

41.00

42.00

43.00

44.00

4 5 . w

46.00

47.00

48.00

9 9 - 0 0

SO.c?O

SL.00

52.00

53.00

0 .4 2 72 D - 0 1

0.42650-01

0.425613- 31

0.42451)-01

0.423 1 D - 0 1

0 4 2 150-0 1

0.41940-01

0.4LL6,RD-01

0 4 1 360-0 I

0.40960-01

0 4047D-0 1

0.39870-01

0 39 140-0 1

0.35250-01

0.37170-01

0.3587D-0%

0 3 4 32C-0 I

0 3 24AD- 0 1

0 30340-0 1

0.27RbD-01

0 2 5 350-0 i

0.23F3D-01

(3. I R43D-08

0.14hBD-01

0 1 0 720-0 1

0 66093-0 2

0.24379-02

20.09

20.12

20.14

20.ie

20.22

20.28

20.35

20.43

20.54

20.67

20.83

21.02

21.26

2 1 - 5 5

21.91

22 .33

22.84

23.44

24.14

24.95

25.97

26.93

28.03

29.25

30.55

31.89

33.26

4.478

5.580

6.951

9.654

10.76

13.38

16.61

20.563

25.46

31.43

38.69

41.47

58.00

70.51

85-20

102.2

121.6

143.2

166.6

191 .3

216.5

240.5

263 - 2

782.2

295.6

305.5

308.4

1225.

1525.

1904.

2372.

2952.

3672.

456 3.

5664.

7019.

5683.

O i l O 7 2 D J 5

0.13190 05

O . I S l R . 3 35

0.1’3760 05

0.24020 05

0.29020 05

0.34820 05

0.41410 05

0.4876C 05

0.56779 05

0.65240 05

0.73880 05

0 . 8 2 3 3 ~ 55

0.90180 05

0.96980 0 5

0.10230 06

3 . 1 0 5 9 D 06

3721

4638.

5 7 7 9 .

7 1 97.

9955.

0 . 1 1 1 3 D 05

0.13830 05

0.17150 05

0 . 2 1 2 4 D 0 5

0.26250 05

0.32353 0 5

0.39760 05

0.49689 05

0.59330 05

0.71900 35

0.86510 0 5

3.10340 06

0.12240 06

0.14330 06

0.16550 06

0.18880 Ob

0.21190 06

0.23379 06

4.25310 06

0.268RD 0 6

0 . 2 7 9 5 0 06

991 .8

1236.

1540.

1917.

2385.

2965.

2681.

4563.

5647.

6973.

8587.

0.10541) 05

0.12890 05

5.15680 05

0.18960 05

0.22780 05

0.27150 05

0.31993 05

0.37300 05

0.42933 05

0.48673 35

0.54290 05

0.59490 05

0.639h0 05

0.67431) 0 5

0.69670 05

755.4

941.5

1 1 73.

1460.

1816.

2257.

2 8 0 3 .

3473 .

4248.

5306.

65 4 3 .

H016.

9797.

0.11910 05

0.14403 05

0.17280 05

0 . 2 0 5 Y D 05

3.24233 05

3.29220 05

3.32449 35

5.36730 05

3.40900 05

0.44740 05

0.4ti02D 55

0.5053C, 3 5

0.521 ID 35

0.28550 0 6 0.70450 05 0.S26TD 5 5

58.73

73.19

91.17

113.5

141.2

L 75.5

217.8

2 70.0

374.0

412.3

507.6

622.9

700.4

925.2

I 1 18.

1341.

1596.

1673.

2 188.

2513.

213.31.

3164.

3459.

3734.

3900.

4 O i R .

4058 .

t3.023

9.199

12.46

15.51

19-29

23. $7

27.75

36.38

45.63

56.32

49.34

9 5 - 0 7

103.9

125 .4

152.7

13.3.2

217.9

256 6

2 9 R . 7

343.0

3hY. 1

4 3 1 . 8

1 7 1 . Y

595.0

531.9

545. J

5531.4

13 0

T I b ' E ( Y I N ) --------- 54 e 3 0

55.03

56.03

57.09

5.9.00

59.00

60.00

f i t .00

62.00

e3.00

6 4 00

65.00

6 0 00

67.00

68.00

f9.00

70.00

71.00

7P -0 0

73.00

74 00

75.00

76.00

77.00

78.00

79.00

eo. 00

P E A C T . ( $1 -------___ - 0 . 1 7 1 30-02

-0.5760D-02

-0.90320-32

-0 .1327D-0 1

-0.16640-01

-0 19700-0 1

-0.22440-0 1

-0 t 2 4 e7 D- 0 1

-0.2 7000- 0 1

-0 2 8940- 0 1

-0 B 3O43D-0 1

-0.31 730-01

-0.32430-91

-0 33 739- 0 I

-0.34460-01

- 0 3 5040- 0 1 -0 35490- 01

-0.3581 0-01

-0.36040-01

-0 3 6 1 90-0 1

-0.34260-01

-0.3426D-01

-0.36220-01

-0.36120-01

-0 35 990- 0 1

-0.35820-01

-0 ' 35630-0 1

34 -6 1

35.917

37.20

38.39

39.49

40.49

41.39

4 2 - 1 6

42.88

43.49

43.99

44.42

44.7e

45.08

45.3i

4 5 - 5 0

45.65

45.76

45.83

45r8R

45.90

45.90

4 9 - 8 9

45.06

45.81

45-76

45.70

305.5

296.9

283.8

266.4

247.5

226.6

205.2

1R4.0

163.7

i44.6

126.9

110.9

96.55

133.77

f 2 . $ 3

42 60

53.99

46.50

4 a. 03

34.44

29-43

25**9

21.94

i8.m

16.27

14.02

12.09

------I--_

0.10750 06

0.10720 06

0.134YD 06

0.10100 06

0.95680 05

0,09380 0 5

0.82430 05

0.75160 35

0.67840 05

O s 6 0 6 9 C 05

0.53890 05

0.47550 05

0.41730 05

0.36450 05

0,31720 05

0.21520 05

0.23020 OS

0.20570 05

0 .17740 05

0 . 1 5 2 9 0 0 5

0 .13170 05

0.11330 0 5

9752 e

8393.

7225.

6222.

536 2

P R E C U R S O R

0.28580 06

0.2aom 06

0.21080 06

0.25700 Ob

0.24020 06

0.22150 O b

0 + 2 0 1 9 D Ob

0.18210 O b

0.16270 06

0.14430 06

0.12720 04

0.11150 O h

0.97260 05

0.8454D 0 5

0.73280 05

O o h 3 3 6 D 05

0.54640 0 5

0.47140 0 5

0.40600 0 5

0.34940 0 5

0.300613 05

0 * 2 5 0 6 0 05

0 - 2 2 2 5 0 05

0.1915D 05

0.16490 05

0.1421D 05

0.12250 05

0 . 7 0 0 7 0

0.68300

0 .os430

0 .fill593

0 a573 20

0.525AO

0 -4760D

0.4232'O

0.38140

0 -3372Q

0.29630

0.2591D

0 -22570

0.1959D

0 * 1 6 9 6 0

0 14650

0.12640

0 e 1 0 8 9 0

9371.

8033.

6937.

5968.

51350

4421.

? R O T .

3281 . 2030.

C D b C ENTH A T I ON S --------_-I

O S 0.52210 35

05 O . 5 O A L D 95

05 004360D 05

05 0.4~750 a5 05 0.424'0 35

05 0.3Bt390 05

05 0.35240 05

05 0.3fh2U 05

05 O.LJ13D 0 5

0 5 0.24HCD 05

05 0.21B43 05

05 0.k90GO 05

05 3 . 1 6 6 2 D 05

05 0.14420 05

05 0.124RD 05

05 0.107'RU '35

05 '9295.

0 5 80J9.

E893.

5931

5107.

4389.

3777.

3252.

2 R O L

24 14.

2052.

T IYE { MF h > _ _ _I A 1 .oo 82.03

83-09

H4.00

e5.00

R6.00

87.00

A R . 0 0

R9.@(1

FO -00

5 1 .00

52.01

S3.03

$4.00

45.00

F6.00

$7.00

58.09

49.00

100.3

101.0

102.9

103.0

104.0

105.0

106.0

107.0

R E A C T . IS 1 --------I--

-0.354 f D- 01

-0.35I70-01

-0.34910-01

-0.34640-01

-0.34360-01

- C 34 060-0 I

-0.33760-01

-0 33450-01

-0.3314D-0 1

-0.3232D-OI

-0.3249U-OL

-0.3216D-01

-0 .3 1 R 3 D - 0 1

-0 .31500-01

-0.31 170-01

-0.30940-01

-0.30500-01

-0.30 170-01

-0.29830-(91

-0.2940D-01

-0.29160-01

-0 2863 0- 0 P

-0.28490-01

-0.2 8 160-0 I

-0.27930-01

-0.2750D-01

-0.27170-31

' TEMP<CELCi US) PCWERl W ) -___I______ -I____ -

45.62 L 0.44

45.55 9.022

4 5 - 4 6 7 804

45.37 6.758

U5.2Y 5.858

45.1 B 5 . 0 8 3

45.09 4.416

44.99 3.842

44.88 3.346

44.78 2.917

44.67 2.547

44.56 2.226

44.46 1.949

44.35 1 707

44.24 1.498

44.13 1.316

44.02 1.158

43-91 I .029

43.80 0 8996

43.69 0.7945

43.59 0.7025

43.47 0.4220

43.35 0.5515

43.26 0.4896

43. LI 5 0.4352

43-09 0.3873

42.93 0.3452

PRECURSLiR C3NCENTRATIONS

4623.

3990.

3446

2979.

2579.

2233.

1937.

168 1

1461.

1272.

I 1 0 8 .

966 5

Ag4-2

733.2

646 4

566 8

497.5

437.3

384 9

339.2

299.3

264.5

234 - 0

207.3

183.9

163.3

145.2

3 .10570 35

9130.

7893.

6030.

5917.

5131.

4455.

3872.

3370

24 36

2562.

2237.

1957.

1714.

1502-

1319.

I 1 59.

1021.

899.4

793.7

701.3

620.5

549.7

487.6

433. I

385.2

343.0

2443.

2 1 1 1 .

1826-

1580.

1370.

1188.

1032.

e 9 7 . B

781.7

BR1.5

594.8

519.9

454.9

398.6

349.7

307.1

270.1

237-9

209.5

185.2

163.5

145.0

128.5

114. I

101.4

ci0.20

80.37

1798.

1553.

1343.

1 1 63.

1008.

t374.3

740. I

6 6 1 . 1

57s . 7

501.9

43P.?

383. C'

335.2

293.7

257.7

226.4

LS9. I

175.4

154.7

136.6

620.3

106.9

94.90

84.15

7 4 - 8 0

66.57

59.32

137.7

P 19.0

102 .9

R J . 1 0

77.24

67.02

5 8 . 2 3

50.65

44.11

3R.4h

33.54

29.35

2 5 - 6 9

22.51

19.?5

17.35

15.26

13.45

L l.ri6

10.47

[J. 250

ti.199

7.769

5 .453

5.736

5.115

4 .549

1 R. 7 5

16.20

14.01

1 2 . 1 3

10.52

4.127

7.329

6.397

6.506

5.237

4.572

3.997

3.498

3.565

2.690

7.363

2.07cJ

1.531

1.615

1 .424

1.153

1.117

O " V 9 3 C i

0.6789

0 . 7 R 1 2

0 .h953

0.61 94

23

0

d 7

d

3

r- N 9

'0

0.

r- Q

? in 0

4 a . 1.4 e m r. N

m

m . I

- cv m

(r N

O . N

t

N

Q

-. 0

I 0 N

U) 9

N

0

I C

0 . 2

s

Ln Cjr ,* 9

9

a e rd . 3

X

r- r,

4

m . - m ul CO

N

4

0

N

CL

m 0

N

N

G . m

N

U . - 0 I 0

h

32 in N

0

I 0

e

d

r- 9

m N 0

ln 0

-4 . rd

* J

r- N

. * P. P

l

? ?- a "I

9

N

9

9

c

Q a

d

0 0

U

.- ru -7 ..I

0

I 0

0

L" Q

P

I . 0 I c

.f . 4

0

in M

4

0

h

d

4

"

0

m. U - d

..I . 0 N

m m a

a

P

* v1

M

r)

r)

0

I n N

* 0

- - 9

Ir) 3

.- 0

m

*I . I

0

N 10

4

m F- r.

n . co

e

N n d

0

I 0 d

9

m ts a

h

9'. .d

B

.. 0 n 0

t- N

Kb 0

I

n 0

.- N

4

N

9

d

d

0

h

0

r- P-

c

an e . 0

4

R

h

M . - v

) 0

pc 0

. 9

d

N

5:

d

0 I

s

m

m

'c

I:

0

Q D

* C

0 . 3

d

* 3c

h: 4 e e

r(

R

RI

d

in U

@

2 L

0

4

0

I 3

(\i h

0

c 0

Lc N

0.

F

0

a: r- r- e

. p? d

0 . c

M c * d CP - . m I

3

I TI Q

r, M

\

C

.+ N

d

n 0 . 1

9 0 . h N

d

U)

P I

h

(u

0

d . ..I

9 . 'fl

-e

0

0

... o

oa

00

0

Il

l

4

0

I 3

ITi 6 9

0

? FJ

2 4 0

h

d

d

0

c

In n . * 4

0

4

m ln c

2 - 0 I 0 U

l I-. m 0

O e 0

#

.4 0

I 0 Ln c

(r . 0 l 0

.d

2 - 0

I c 6 *, N b

'

0

In d e

m

n

r- 0 0

u- . d

9

r- W . cr d cc N . 0

P.

-. 3

.. 0 I 0

(r

cr N 0

"

VI m 0

V

d

0

5 I

0

U

o\ c

0

I

0

&

m

4

4

13 I C d d 3

* 0 . N C N

"i

0

F. U

N

Q e

9

m r- U) . 2 . * N

r. Q

Q

m r. 0

I 0

9

r. d N

0

0

N

0

U . - a A N

o? m

.. 0

I 0

* m .-

-* 0

I 9

io

c m 0

r-

0

a

c

N

3

0

N

Y)

PI

c

m

iD

* Q

M

Q

N . P- OI

m

m 8

* 0

I 0 0

I

e

N

Q

I

0

0

8

-4 0

I

d

N

m

a

c

0

I

c

0 . I?

d

0

I d d

N

Y

0

c

r4

I.

OJ

0

m

C 0

n

. m Q

d)

.-I . U ? e .* 9

0 4

c

6.

.

0

I 0

c 0

(D

0

I) [3

0

m . *

(

0

l e

U,

P. a

c

0

I

c

m

2

,- 0

I

c 0

n

”!

0

c 0

N

ru 0

*, c cc N

Q

c

9: F

)

m

N

a

... c(

m

(0

9 . * 0

I a 9 I. 9

0

M

. d

I. % n

0

1

6

m

c

n

*

0

I c

cr . 2

... 0 I 0

6

h

N

13

r(

m

#

0

N

0

c

10 0

pu . 0. 0

a

m

0

... J1 * f . 9

- 0 I a

In v)

n

r. . 0 a 10

P

r)

. e.l

0

I n

.- CI

c

d

0

I 3

0 . f

... 3

I

m

d

N

0

m

- 4

d

c c

...“ 0

In

m

N

a . 0

s4

- . rr

r? 0

. 2 N

0

N

a 8

c”

0

I 0

U

U

m I

0

10 8

0

m

d

0

I m

Ill rD

n

.A

0

I

0

N

Q

* - 0 I

3

I-. * N

N

0

J

Q 0

0

9

Q

+

N

9

0‘ ‘0

N

m 4

. N

e

0

04 ” d . ”m

0

l a

N

In N

sl

0

c

m 8

0

PI

’4

0

I a[\ N

9

n

+ . 0 I

c

m

* e

&

3

I

3

N

T

r

3

c)

-4

e

m c . 13 0

4

h . d

e

10 R

)

N . (c

4

a)

U

N

6)

m

? c 0

I n

* 0

d

d

0

0

4

m PI

I

0

I 0

0

d

U) “

0

I

0

ID

Q c

e

0

I 3 0

c -. .-4 0

rl: In N

d

0

m

I? Q

1

N 0

ru ru . CCI 0

N

m 6

r- r.

m

rd

0

I 0

0

N

cn 0

0

(\r C

(r C

)

. - 0 I a 2 cn ..I . 0 I 0

c

d

,-4

.-. 0 I h

0 9

c

- -* a

Q

h

4 c

0

0

m

cn e

m

UJ 0

N . 0,

0

m

- a

h

0

0

N

0

I d Ip

N 0

m 0

II 0

a! ri

c 0

l a

(u

v. Q

d

. 0 I

0

W

d . 4

4

0

I 7 n 0

r

* O

h‘ 0 e

c

0

4

* d P

Q

m v . li m

I. 0

oc’

cl m N

m . N

0

I a 0

I. m

91

0 . * m

m

F)

* 0

I c? r. Q

Q

e

0

I

0

0‘ 0

. -.

*

C I 3

0

.f e

.-“ 0

:

0

- 0

.c B

rr: . 4 M

m

4

. -4

9

c

Lo

c . N

m 0

I? . N

O

I 0

m In m

h

0

m r- (D

rl

4

0

I 4

a- il 0

* 0

I

C

0

2

4

0

I c\ v2 4

0

..s * 0 4

0

I 3

9

h 9

h

0

4

m 0 3

0 . In Q 0

-4

N 0

? lP #

Q

N

N . cu 0

I 9

N

Q

In

0

n

h‘

PI

a? m

. e

0

I a

f. 0

I?

I

0

I

0

tn m .

rz 3

I r N

m

m 0

0

0

I

s In N

c

0

N

m

0’

0

a

d

c

N

.-3 e

D

N

v)

m

-4

I

N

N

a I

D

9 0

In

cn 0

Q

N . W

b

l

0

0

I n

6: R

I

- *

0

I

0

9

M . r

(

N

0

I P

Q

* ;7 c. 0 . 4

0

I s 0

10 0 0

c3

P

N

3

a?

0

N 0

N . .m m 0

n

0 . 0

0

0

N

N 0

I Q

0

N

VI

0

*

111 P

. m

PI

r(

0

I 0 m

0

N

4

0

I

0

c

m . .-I

N 0

I c

P

0

OI R

0 . ..“, 0 I c m

Q

m

4- 0

0

9

I.

0 . 4

N 0 . 4

0

In N

e . P

OI d . e

N

0

I a * e 4

0

0

d

6

b

It)

* 0

1 0

0

c

4

0

I

0

0

0

e

N

\3 I 0 N

c

IP h

0

.* 0

l 0

0

ul In

cn 0 . Q

N

N

c 0 . 0

h

(r

0

m

N

e

0

e . 0

e

16 . d

N

6

I a a N

N

Q

0

N a . c

m

d

0

I a

d a

+

- 0

I

0

d

Q

I

YEACT.(S)

162.3

ib3.0

164.0

165.3

166.0

167.0

1 6 9 . 9

169.9

173.*?

1 7 1 . 2

172.3

173.0

174.')

175.0

176.0

177.0

1rc1.0

179.3

190.0

181.0

1P2.0

183.9

1R4.J

185 .0

ia6.o

1 8 7 . 3

189.0

- 0 . 1 1 2 9 D - 0 1

-0 I 1040-0 1

-0 . iq73n-01

-0.10540-01

-0 I O 3 O D - O 1

-0.10053-0 1

-0.98120-02

-0 95 730-02

-0.93300-02

-0.90910-02

-0.9353D-02

-0 '361 70-0 2

-0.9 3 5 10- 3 2

-0 8 1470-02

-0 79 I 4 D- 0 2

-0.76'2D-02

-0.7P52C-02

-0 722-70-32

- 0 .5 9 44 0- 0 2

-0 -67679-02

-0.65420-02

-0 e 6 3 170-0 2

-0.60$40-02

-0.Ta710-3?

-0 56500-02

-0 e54 300-02

-0 5 2 1 t 0-0 2

37.74

37.b6

3 7 . S P

37.50

3 7 . 4 2

'7.34

37-26

37.1 r?

37. I O

37.02

36.95

36.37

36179

36.71

36.64

36-56

36.49

36.4 1

36.34

36.26

36.14:

36.12

36.04

35.97

35.90

75.83

35-16

0.40140-02

0.38220-02

0.36440-02

0.34770-02

0.33220-02

0.31 77 0-02

0.304 10-02

0.291 40-02

0.27960-02

0.26650-02

0.258IO-O7

0.2464D-02

0.23930-0?

0.2 3 07 D - O P

3.2 22 7 3- 0 z 0 2 1 520-02

0.2 08 10- 02

0 201 50-02

0.19530-02

0.18950-0i!

0.18400-02

0.17890-02

0.1740D-02

0.1695r)-02

0.16539-02

O.lb130-02

0 e I576D-02

1.529

1.454

1.354

1.319

10258

1.201

1.i4H

t.09R

1 e 0 5 2

1.009

0.9685

0.9306

0 1 R 9 5 1

OeR619

0.8308

0.8316

0.7742

0.7085

0 - 7 2 4 4

0.70 I R

0 . 6 ~ 0 6

0 a 6 6 O b

0.6419

0 - 6 2 4 4

0 - 6 0 7 9

0.15924

015779

3.643

3.657

3.494

3.323

3. 1 7 3

3.032

2.901

2.779

2 0 6 6 4

2.557

2.456

2.362

2.274

2.192

2.115

2.042

1 974

1.910

1 650

1.794

1.741

1.692

1.645

1.602

1.561

1 . 522

1.486

0 m'3254

O.SRl1

0 a8398

0.0013

0 e7654

0.7318

0 r7005

0 - 6 7 1 1

0 . 6 4 3 8

0.htR1

0 -5941

0 ~ 5 7 1 6

0 -5.506

0 -5308

0.5123

0 . 4 9 4 9

0.4781

0.4639

0.4490

0 .4355

0 -4229

0.4110

0 -3999

0.3894

0 a3796

0.3704

0.3618

0.6673

0.6545

0.6239

0.5 '353

0 .So87

0 5438

0.5206

0.4rRH

o.ccrd'~

0.4595

0.4417

0 e4250

0 .a994

0.3948

5.3713

3 3667

0.3561

0.3447

0-3341

0.3241

0.3147

3.3053

3 . 2 9 7 6

3,289'3

O . 2 R ? 6

o .2 75.8

0 2694

lPS.0

190.0

191.3

192.9

193.5

194.0

195.0

1 9 C . O

197.0

199.0

199.0

200.0

201.0

202.3

203.0

204.0

205.0

206.0

207.Q

204.0

209 .0

710.0

211.0

212.0

213.0

2 1 4 . 0

215.0

-0.49%30-02

-0.4777c-02

-0.456lD-02

- 0 4 3470-0 2

-0. U 1330-02

-0 392 10- 02

- 0 .3 7 10 c- 3 2

- 0 . 3 5 O O l - l - 0 2

-G.3291C-0?

-0 30FI3D-02

-0.2876D-02

- 0.26 700- 0 2

-0 2465P-02

-0 .?262D--02

-0.2osqc-02

-0 18579-02

-0 .16570-02

- C . I457D-02

-0.125YD-02

-0 1061 0-02

-0.86490-03

- 0 h h9 3 D - 3 3

-0.47470-03

-0.281?D-03

- 0 fl @ B 90-0 4

0.10291)-03

0.29343-03

35.6P

35.51

35.54

-75.47

35.40

35.33

35 26

35.20

35.13

35-96

34 99

24-92

34.66

34.79

34.73

34.t.b

34.59

34-53

34.46

34.40

34.33

34.27

34.21

3 4 . 1 4

34.08

34.02

33.96

0.15410-02

0.15083-02

0.14770-02

0 14490-02

0.14220-02

0.13970-02

0.13740-02

0.13520-32

0.i332D-02

0.13140-02

0.12970-02

0.12820-02

0.1267O-02

0.1255D--3?

0.12430-02

0.12330-07

0.1223O-O?

0.12150-02

0. L2090-Or?

0.12030-02

0. I 1 9 R D - 0 7

0. f 4 950-02

0.11920-02

0 . 1 I 9 3 3-02

0. : 1900-02 O d 1 9 1 D - 0 2

0.1 B 930-02

0.5643

0.55 I 6

3.5397

9.5285

0.5181

0.5093

0.4993

0.4908

0.4829

0.4757

0.4639

0.4627

0 .4!=.?0

0.4513

0.4471

0 . 4 4 2 8

0.4390

0.4356

0.4326

0.4300

0 .4278

5 e 4 2 6 1

0 04247

0.4236

0.4230

0.4227

0 .4229

I . 452

1.421

1.391

i 3 6 3

1.338

1 . 3 1 3

1.291

1.270

1.251

1.233

1.216

1.201

L.1R7

1.175

1.153

1.153

1.144

1 . 1 3 6

1 . 1 2 9

1.123

1 . 8 1 8

1.114

1 . 1 1 1

1 . 1 1 0

1.109

1.109

1.1110

0.3537

0 e346 1

0 e339 1

0 e3329

0 -3263

0 -3205

0.3151

0 03102

0 - 3056

0.3013

0 -2974

0 2938

0 -2905

3 -24375

0.2848

0 -2824

0 -2803

0 02784

0 - 2 7 6 8

a .2754

0 -2743

0.2?35

0 ~ 2 7 2 Q

0 - 2 7 2 5

0 -2724

0 a2725

0 02724

0 2634

0.2578

0.2525

0.2476

0 24Jd

0.2383

5 . 2 2 4 8

0 . 2 3 1 i

5.2271

3.224h

0.221h

0.2190

15 e 2 266

3 . 2 1 4 3

0.2124

0.2106

0.2090

3 -2075

0.2064

0.2055

0.2047

0 2 04 3

c) - 2 0 3 6

0.2334

0.2033

3.2034

0 -7037

0.2 02 3:)- ir 1

0. SF85D- '31

0. 19440-51

0.19073-51

0.19713-51.

0.113390- 0 1

0. 1 8 O t l D - 0 1

0. ; 78011- 1 1

3.3 7543- 0 1

0. 1 7 2 O U - 0 ) I

3.17Or'J-01

0. 16.373- 0 1

3.16tA3- 0 L

3.16513-01

0. i6364)-0 t

'3. 16220-01

0. lhlOD-0t

3.15990- 0 1

0. 1590 ) - 0 1

0 . i 5833- 0 1

0 . 157711-01.

0.157213-06

I]. 15c>9L>-ol

3 . 15670-01

(3. 15660- 0 1

0. 15673- 3 1

5. 15093- 01

3 . ?7643-02

0.27053-02

0.2t.503-07

0.75Y4C-02

0 . 2 5 5 1 J - C Z

0.25 063-02

0.24 b 5 ? - 0 2

0 - 7 4 2 6.J- C. 2

0 . L 3 3 : J-32

0.23583-02

0.2 3 2 7 3 - 0 2

0.22993-02

3.27 743-07

0.2251 1-22

0.21303-02 h)

0.221 ! 7 - @ 2

0.21 953-27

0.21e13-02

0.2165 F-02

0.215eJ-32

0.7 P 50 3-02

0.21 43c)-02

0.21 390-02

0.21 3 t ; ) - i 2

0.2 1 3 69- 0 2

0.2 I37i)-07

o.zi93')-02

T I Y E i M I N )

2 l b . O

217.0

218.0

2 1 9 . 0

220.0

221.0

222.D

223.0

224.0

225.0

220.3

227.0

225.0

229.0

235.1)

231 0 0

232.0

233 0

234.0

235.0

236.0

237.0

238.0

23Y .o 240.0

241 a 0

242.0

0 - 4 S 3 0 D - 0 3

0.67 i r D-o 3 0.95;940-03

0 * 10460-0 2

0.12 320-0 2

0 1 4 170-37

0.1601 D-0 2

0.17840-02

0.1')660-02

0 2 1470-0 2

0 2 3370-3 2

0 - 2 5 C h D - 3 2

0 26 340-0 2

0 .?8620-02

0.70 :sc I -52

0.32 140-3 2

0 . 3 3 Y Y D - 0 2

0 35630-0 2

0 3 7360- 0 2

0.3 4 080-0 7

0.4079D-02

0.42500-02

0.44190-02

0.45360-02

0.475630-02

0 e4923D-02

0.5 0890- 0 2

33.69

33.53

33.77

33.71

33.65

93.54,

33.53

33.47

33.41

33.35

33.29

'3.23

33.1 P

33.12

33-06

33.00

72.94

32.89

72.83

32.78

72.72

32.66

32.61

32.55

22.50

32.44

32.39

0.1 1 960-02

0.11990-02

0.1204O-02

0.12100-02

0.121 70-02

0.1225D-02

0 1234 D-02

0.12450-02

0 12560-02

0- 12690-'3?

0.1282D-02

Oei298D-02

0.13140-02

0 133 10-02

Q * 135 30-02

0.13710-02

0.13920-07

0.14160-02

0.1441D-02

0.1467D-01

0.1495D-02

0.1525D-G2

0.15570-02

0.1590D-02

0.16260-02

0.16640-02

0.1704D-02

-----I - 0.4233

0.4242

0.4254

0.4270

0.4290

0.4313

0.4341

0.4372

9 -4407

0 a 4 4 4 8

C -44'30

0.4537

0.4509

0.4645

0147a6

0.4772

9.4843

0.4918

0.4999

0.50Rb

0.5178

0.5275

0 a 5 3 S O

0.5490

0.5607

0.5731

0 05863

PRECURSOR CSkCENTHA T I ON5

1.112

1.115

1.119

1.124

1.130

1.137

1.145

1.154

1.164

1.175

1.167

1.201

1.215

t . 2 3 1

1.248

1.266

1 286

1.304

1.329

1.353

1.378

1.405

1.433

1.464

1.496

1.530

1 e566

0.2735

0 -2743

0 -2754

0.2767

0 -2763

0.280 1

0.2821

0,2844

0 e 2 0 7 0

0.2899

0 e 2 9 3 0

0.29154

0.3001

0.3040

0 -3083

0 e 3 1 2 9

0.3179

0.3231

0 -3268

0.3348

0.341 1

0 -3479

0.3551

0.3627

0 -3708

0 c.3794

0 -3884

0.2041

0.2348

S a 2 0 5 6

3.2066

0 . 2 J i . R

0.2091

0.2107

3 si! 124

0 . 2 1 4 4

0. % I h 5

3.2 $89

0.2210

0.2242

3 .2272

0 2304

0.2339

0 2376

0.2415

0 2457

0.2SO2

0.2550

0.2601

Or2655

0 .;I71 2

0.2743

0 2837

0.2905

28

-I

NN

0

10

0

bl

mm

C

I

IO

0

-I

N 0

I 0 r. (P

ru n 0 . 3

I 0

c

* P"

0

- U

m

W

0

Q

2 Q. 0 h

Q

9 . 4 9

0

r

? 0

N 0

I c

m

m

m

M

0

V)

N

N

W

h' 0

I 0

N

a

U

Ui

0

0

tn U

N

N

u I

"- cc e

'3

C

-4 ,-

Q I

3

N

ln

u- t\ . 0 P 0

pi

rl

0 . N

N

B

4 0 0

oc c e 4

In 4

10 :

C

ry 0

I 0

Q 6

d

0

.. N

N

CI m

&N

0

0

I1

M

f.

e

o

r-0.

my

,

00

on

..

00

.. or-

uv

N

lU

C?

0

I a

c

m M m

c

e

0

I 0

-2 RJ 9

N

0

U 0

U

Fl

0 . 0

* m Q

0 . r? 9

. * (I) N

m O

? N

0

I

10 (I) 0

n

e

0

r. 0

N

rn . N 0

I Q

't 10 0

0

0

0

a? * N . N

V

I 2

r. Q

10 I*

0

0

I ij

p:

0

h

nr 0

d 0

In

19

0 . m

0

9

Q

0 . * 9) a

.a

B

N

0

c 0

N

0

I 0

In II) 0

N

0

N 0

N

m . N 0

I n

m N

N 9

0

0

,3 B

N

r.1 0

I 0

(I) 01 c m C

..

4

3

I

li-l

a: n. 0

c

I.

0

Q

F7

0

4

Q

N

rn d. 0 s

U

I3 . d

0

rr) N

r. 0

N

0

1

lr n

d

I

N

0 . \c

9 @

m N 0

I (1

Q

(I. m

rg

0

0

0

G

N

. c. 0

I

h

J m 0

c

.d

c

0

I n

h

h

a)

"i

r-J

(II

N

c.

3

4

h

U

0

0

0

0

N . m

Q

0 c 0

N 0

I

B a

(\I

0

a

.- - OI

r)

e

N

0

I n

r- U

M 0

u

0

c

Ln IL

N

0

I n

N

9

C

U * 0 - 3

I

p" a' b I 0

n

- Q

a2 m

0 . N

F1

UI

0

r(

. m 9 0

nl . Q

r- d c

R I

nl 0

I 0

m

In N

N

0

'0 9)

ri

N

0

I 0

c

0

0

n

N

m

llI

ru 0

I r)

0

ro V

B

n

+ 3

I

3

b. n 7 . 9 n

ai m

hl * c)

- Q

9 0

0 . 4 c

N

N

(I) d

* 0

0 . h' 0

I 0

c

m

e

(u

0

e

IC . d W

N

0

I a Q

F.

w

r . 0 0

0

In

1u .

N

0

I Q

Q

0

e .I

a

-I 0

I A

'97 z m

0

0

03 rn .s 0

Q

0

m

v: e N

0

m

N

9

P)

h

m, 0 &I 0 I 0

* c m N

0 . c? 4 c m

N

0

I 0

'3- 0

fl h

0

0

0

m

1u

N 0

I n

... \

/

m

h

e . 0

M

0

I n

ln 0

M

r- 0

srl 0

IC1 Q

n . b 9

0 0 * 0

In m

Q

N . @

m

0

0; 0 nl 0

I

ip,

9 9

N

0

n

.-a 9

r)

.4

(u 0

l a

W

S

Q

h

0

0

h

M

(U

ru 0

I

m m

m

Ln

0

m I

4

3

I 3

9. m

3

- * ro 9

0

m 0 . a 9

h

10 a 0

0

c.

N

4

.I) 0 0

4

N 0

I 0

B c

(I) N

0 . \c

Q

d

m

N 0

I 0

0 P

h

0

- . 0 * 0 a cu

R1 0

I 5

c

6: c

in

0 . .D

3

I 0

r) N

CU P

3

rb h

Q

m

. a Q 0

m

c 0 . a,

N

P

N

e m 0

*

N

0

I 0

4

N

m

c31

4

fl

d

ri

N 0

I 0

N

e

N

Q

3 . 0

n: W 1u

ru 0

I 23 N

0

m IC

0

I

0

l a

,?-I c" m

d

0

N

9.

0

T 0

(I) 0

, In

h

. 0 m d 0

ic)

9

N

.- . 4

N

0

I a d

Fl m

0

+

A

m . "4 F

l

N 0

I 0

c rJ

-4

ai

0

0

m

W

(\I

PJ 3

I ci t.

m

e: 0

0

,d

0

I D

)c.

m

e 0

m

m

N 0. m

0 . OI 0

01 I. 0

4) 9

.. m

N

h

r(

. 4 &

0 I 0

r. c B

rn o

10 N

I

m

N

0

I 0 0

B

M

a,

0

0

a

u2 <v

N

3

I c

LT V

0

IJ

n

I,

4

3

I '3

m

n

c

d

0

N

c 0

- n

m m N

2 0 IF b 0

rn

I", N . 4 N

O

I

N

N

10 W

0

n . +

N

ri d

N

5

I C

d

IC

u2 9)

0 . 0

u- W N

cu 0 I

i? h

h

c c

h

d

3

I

in 9

0

e

C

n

ip,

m

B

9

O

IC

(0

v, 9

0 . m

m

* i?

0

h

N

4

N

0

I 0

10 h

h

Q

0 . c * 4

rl

N

0

I 0

m

m a

?1

0 . c

c

0

N

.

N

0

I 7

M

D 0

r- 0

0

I

0

m

U' 0

n

- - -4

1c ro O

. h

In Q

tD

e . M

m In

ri

e

N

? d

N

0

l a 6

m

P

m 0

N

.-i

r)

N 0

I 0

N

c P m 0

c

+ Q

w

N

0

I r: In I- m

r. 0

e c I n

h

n

&

P

0 . U 0

0

I. 0

@

* n rr 0 . 4

* i- m

0

rc rl hl

4

a l

a

(\I 4

4

d

0 . r. a . M

p1

N

0

l D

a? N

m 0

... 3

K*

Q

N

N

0

I

Q 0

h

r. 0

n

M

0

I n

X

9

0

0

n

r. "1

h

0

m

m (I)

O

2 e

h 0

(I) . rr)

c

* Q

.*

N 0

I 0

ro P

N

Q

0 . N 0

Td

PI

N 0

I 0

pi

r. N

6

0

C

3 0

N

T I M E ( M I N ) ---------

270.0

271.0

272.0

273.0

2 7 4 . 0

275.0

276.3

277.0

273.0

279.0

283.0

201.0

2R2.0

203.n

264.0

265.2

286.0

2R7.0

if3800

289.0

290.J

291.0

292.9

293 .o 294.0

595.3

296.3

0.94 170- 02

0.95hlD-02

0.9 7040-0 2

0.98460-02

0 . 9 9 P ? D - 0 2

0.13 130-0 I

0.10?70-0 1

3.10419-01

0.10550-01

0.1064D-01

0.1 oe20-0 1

O e 1 0 5 6 D - 0 1

0.1 1 o9n-o 1

Oal1>3D-Ol

0 1 1 360-0 1

0 .11550-01

0 .11630-O 1

0.1 1769-0 1

0.11400-01

0 .12030-0 I

0.12160-01

0.12290--01

0.12420-0 I

0.12550-01

0.12470-31

0 I 2 5 O D - 0 1

0 12930-0 I

30.97

70.93

30.88

30.83

30.79

30.74

30.70

30.65

30.61

30.56

30.52

30.47

20.43

30.38

30.34

30.29

30.25

30.2 I

30.16

30.12

30.0@

30.04

29.99

2 9 - 9 5

29.91

29.87

29.03

0.44900-02

0.46970-02

0.49170-02

0 5 15 1 Q-02

0.53 990- 02

0.5664i)-02

01 59450-OZ

0.62450-02

0.6§64D-O2

0.69040-32

00 72660-02

0.76530-02

0. a 0650-0 2 0.85050-02

0.e975D-02

0.94780-02

0.10010-01

0.10590-01

0 1 1 20D- 0 1

0.1 lA5D-01

0.1257D-01

0.1332D-0 1

0.14130-01

0 . 1 5 O O D - 0 1

0 e 1 5930-0 11

0.16930-01

O.lAO00-01

1*555

1.573

1.645

1.722

1.303

1.890

1.982

2.080

2.184

2.295

2.414

2.540

2.675

2.e19

2.972

3.136

3.31 1

3.498

3.697

3.91 1

4.140

4.355

4,648

4.930

5.231

5.555

5 . 9 0 3

4.082

4.269

4.467

4.678

4.902

5.140

5.393

5.663

5.950

6.256

6.582

60929

7.700

7.696

R. 119

8.570

9.053

9.568

10.12

10.71

11 e34

12.02

12.75

1 3 0 5 2

llb.46

15.25

1 4 - 2 2

1.021

1.068

1.117

1.170

1 - 2 2 7

I 287

1.351

1.418

1.491

1.568

1.850

1.738

1.831

1.931

20037

2.151

2.273

2.403

2 542

2.891

2.851

2.021

3.205

1.401

3.819

3.838

4.081

0 .7543

0.3001

0. d375

0.8773

3.9196

0 . 9 5 9 C

1.012

1.063

I . I l H

1.17f

1.237

1.303

1.373

1 e 4 4 8

1 528

1.614

1 705

1. t403

1.107

2.015

2.139

2.267

2.435

2.552

2.711

2.361

2.063

0.5F053-Si

9. c 1779--31

0. h6iJbO-3 1

0. c 7 7 3 0 - a i

0.7 1 O O U - c I 1

0.7447a- 0 L

0. TEI 7b-0 i

3.9211J-i11

0.9e303- 0 1

0.997783- 0 1

0. s5530- 01

0.1 OOf1

3.1300

0.1113

0.1183

0.1245

0.1317

0.1392

0. 1473

0.1550

0. 1452

0. I751

0 0 1857

3.1271

0.2294

0.2225

0.2366

5 i W E < M 3 ~ 1 - - - - ___ - -

207.0

295.15

299.0

330.0

30 1 .O

307.0

303 .0

204.0

305.0

106.0

207.0

3 0 3 . 7

'09.9

310.0

3 % 1.0

?L2.0

511.5

314.0

315.0

' I C .o ?I7.0

318.0

319.0

320.3

321.3

322.0

373.0

0.13059-011

0.13180-01

0. I330D-0 1

0.13430-0 b

0. i 3550-01

0. t 3670-0 1

0.13800-0 I

0.1 'S2D-0 II

0.1404D-01

0 . i a 1 0 n - 0 1

0.1428U-os

0.1440C-O\

0.1452C-01

0 1464D-0 X

0.14 750-0 1

0.14970-03

3.84490-01

0.15 100-0 1

0.15220-0 1

0.1533D-3 I

0. L E44D-5 I

0 I556D-0 i

0. L 5670-0 L

O.%57HD-OI

0.159VD-01

0.16COD-01

0.!5i19-01

29.74

29.75

29.70

29.66

29.62

29.58

29.54

29.50

29.46

29.42

2 9 - 3 9

29.35

29.31

29.27

29.23

29.1F

29.15

29.12

29.08

29.04

29.91

28.97

2 8 - 9 3

28.90

2 8 . 8 6

28.02

28.79

0.19150-01

0.2 O39D-01

a. 2 1 720-01

0.23?60-01

0.24700-01

0 2 6 3 6 0-0 1

0 281 60-0 1

0.30090-0 1

0.32170-01

0.34920-0 1

0.3485 0-0 1

0.3947D-01

0.42300-0 1

0.45369-01

0.486AD-OL

0.52260-0 1

0.541 50-0 1

0.60350-01

3 6 4 9 1 D-0 1

0.69850-01

0.752 LO-09

a. 81 023-0 1

o. 87343-01

0.9420 0-0 1

0.1017

0. i o 9 8

0.1186

t " ; E C U H S O R C O N C E N T ? A T I J N S ~ ~~

6.276

6.677

7.108

7.571

8.070

8.607

9.185

9.eoa 10.43

's1.20

11.95

12.83

13.74

14.72

65.79

16.94

18.18

19.53

20.99

22.57

24.29

26.25

28. P 7

30.36

32.74

35.32

38 . i4

17.25

18.36

19.55

20.d4

22.22

23.71

25.31

27.04

2B.YO

30.91

33.38

35.42

77.95

40.69

93.65

46.R5

50.31

54 - 3 6

58.13

42.53

67.31

72.49

78.12

$4.23

90 e 8 7

98.09

1.35.9

4,342

4.622

4.924

5.249

5.598

5.974

E.380

t.917

7 285

7.797

E . 346

E.F39

S.580

10.27

11.02

1 1 .R3

12.71

13.66

19 - 6 9

15.01

17.02

16.33

19.76

21.31

29.00

24.83

26.02

3.254

3.475

3.697

7.741

9.203

4.483

4.731

5.11')

5.473

5.856

6.26F;

L.714

7.136

7.717

Q . 2 R O

tl.840

5.550

13.26

1 P - 0 4

a 1 .sn 12.79

13.TR

14.85

26.02

1 7 - 2 9

18.46

20.16

0.251 r j

0.2681

e. 7856

3 . 7044

0.3247

0.3466

0. 3701

3.3055

0. 42713

0.4c24

0.4843

0.51 jY

0 . >.Sf, LJ

0.5563

u. f 3 9 8

0. € 8 7 3

0. 7380

0. 7Y32

0.1531

0 . 3 1 f l l

0.48.45

1.065

1 . L 4 P

1 * 233

1.356

1 .a43

1.558

~~~

0.31355-01

0.36570- c 1

0 .399 t l - c l I

3.41533-1;3.

0.443 0 0 - 0 1

0.47783-01

0.5O503-0 1

3.53969-3 1

c ) . 5 7 7 0 > - 0

0.6 1733-0 i

o.f>c cia>-3 B

0.707Ci)-01

0. 7581JI)-O 1

O.r j l 351>-01

0.97299-01

0.93 723-0 1

0.1 0 0 7

3.1332

0 . 1 1 6 4

0.1253

0 . 1 349

0 . i 453

S. 11566

O.lbW5

3.1923

0.1968

9.2126

w 0

T IHE( H I hi) -- -_--_-- 224 -9

325.0

326.0

327.3

323.0

229.0

230 .0

2 3 1 . 3

332.0

333 n

234.0

T35.0

736.')

737.0

338.0

339.0

340.0

34 I .C)

347.0

343.9

'144.0

'45.0

346.3

747.0

348.0

749.0

350.0

0.16220-0\

0.1 C33D-0 1

0.lh44D-01

0.15540-01

0.16690-01

0.lb7hD-'31

0.16a60-01

3.lh57P-31

0.17070-01

0.17 17n-0 I

0.17Z70-0 1

0.17370-0 1

0.17470-01

0.1757C-01

0.1767D-0 1

0.17779-01

0.17870-0 1

0.17Fh0-01

0 1 8 060-0 1

0.18150-01

0 . 1 9 2 4 0 - 0 1

0.18 330-0 1

0.1 P420-0 1

0 .18510-01

0.18600-0 1

G.186R0-01

0 0 1 8 76 0-0 1

29.75

28.72

28.ee

2 8 . 6 5

23.61

28.SR

28.54

28.51

28.47

29.44

29.4 1

28.37

28.34

28.31

28.2P

23-25

2d.21

28.1 e

25.14

2 8 . 1 2

2 8 . 0 9

28.06

28.03

2 8 - 0 0

27.99

27.95

27.92

0.1282

0. I 3 8 6

0.1500

0.1624

0.1759

0.1907

0.2068

0.2243

0 2435

0 2645

0.2874

0 .3125

0.3399

0.3695,

0.4029

0.4387

0.4782

0.5214

0.5669

0 .6209

0.6780

0.7407

0. R096

0 885%

0.4684

1 . O b 0

1 . 1 6 0

41.19

44.52

49.15

52.09

56-39

61.09

66.19

71.77

77.83

84.51

91.78

99.72

108.4

1 1 7 . 9

126.3

139.7

152.1

165.8

180 e 8

197 2

215.2

235.0

256.7

280 5

306 7

335.5

367 1

114.5

123.8

133.9

144.9

157.0

170.1

184.4

200.0

217.0

235.6

256.0

278.2

5 0 2 . 6

329 2

359.4

390 e 3

425.3

&6 3 - 6

505.6

5 5 1 -8

602.4

657.9

719.9

7e5*9

559.5

940.5

r o r g .

28.99

31.35

33.92

'6.72

39.78

43.1 1

4 6 - 7 4

5 0 -7 1

55-04

f9 .78

e4.95

73.61

76.00

f53.58

G l r O U

94.12

108.0

117.8

128.5

140.2

153.1

167.3

182.8

IYY.9

2 1 8 . 6

239.3

2 b l . 9

21.7'4

23.57

25.50

2 7 . 6 1

29.91

32141

35.15

3'3.1'3

41 *481

44.96

48.85

53.1 I

5 7 . 7 7

e . a 7 bH* 4 5

74.57

n i .27

e 6 2

46 .h7

105.c.

115.2

125.9

137.6

15iI-4

164.5

180.1

197.1

I .€hS

I . 822

1.971

2 . 1 3 4

2.312

?*50',

2 . 7 1 7

2.443

3.233

3 4 7 6

3.777

1 . 1 0 6

4 . 4 6 7

4 . B b l

5.2+3

5 74r>

6.294

h 952

7 . 4 f 5

R . 1 5 3

d . S 0 3

3.733

13.64

1 1 . 6 3

12.72

13.93

1 c.25

5.7293

0.2486

3.26QLj

0.2912

0.3155

0.3419

0137178

0.4J2.3

3.9367

0.4743

0.5154

0. 5bcr.3

0. S J 35

J e - 3 3 3

tr,7:22

3.7567

0.4575

0.9 35 9

1.020

1 . 1 1 3

1.216

1.328

1 . 4 5 2

1.5d7

1 . 7 3 6

1 .+OD

2. OR' I

251 .o

-752.9

553.9

-154.0

‘55.0

’56.0

257.0

25e.n

: s Y .3

260.0

361 .U

363.0

ze3.0

-764.0

365.0

3 6 6 . 0

767 .o

3 6 R . 0

‘69.0

370.0

37: .0

‘72.0

-773.0

3 7 4 . 0

375.0

376 .0

377 .o

0 . l ”q4D-0 1

0. ie92c-o i

O.lq00D-01

0.19073-0 i

0.I915C-01

0.1921u-01

0 . I 92~30-0 1

0.19340-0 L

0 . 1 9 4 0 D - 0 1

0.19460-0 1

0.195iO-OP

0 .19560-01

0 .19600-0 i

0.1Y640-01

0.19670-01

0.19690-01

0 P 4 ? I D - 0 1

0 .19720-0 1

0 19720-0 1

0 1971 0-0 i

0.1969D-3 1

0.14663-5 I

3 .19628-0 L

0.19560-01

0 19490-0 1

0 . 1 9 4 1 3 - 0 1

i r . 1 9 3 i D - O B

27 .89

27 .87

27.84

21.82

27.80

27 .77

27 .75

27 .73

23.71

27.64

27 .68

27 .66

27 .65

2 7 . 6 4

27 .63

27.h2

27-61.

2 7 . 6 1

2 7 . h t

27.61

27.6?

2 7 . 6 3

27 .64

27 .66

27 .68

27 .71

27-74

1 e 271

1.393

L - 5 2 7

1 m674

I .a36

%.015

7.212

? .429

2.668

2.93?

3.222

3.542

3 .895

4.283

4.71 I

5.282

4.701

6 .273

6.901

7.592

9.352

9.1~36

l O . 1 0

I1.PO

12.20

1 3 - 4 0

14 .72

4 0 1 . 9

4 4 0 2

4 q 2 . 3

5 2 3 7

57’5.7

635 9

697.7

755.9

a41 .o

923.7

IOL5.

1 1 1 5 .

12?4.

1 3 4 8 .

t4R2.

1630.

1793.

8973.

2 1 7 0 .

2 3 R R .

2627.

2RSi9.

3178.

3495.

384 2.

4222 .

4638.

1127 .

1235.

1354,.

9 4 8 4 .

1628 .

1786 .

1960.

2152.

7363.

2596 .

2 8 5 3

3 1 36.

3448 .

3791.

4170.

4587 .

5046.

5551.

6 1 0 7 .

h719 .

7392.

8 1 3 0 .

R 9 4 1 .

9833

0.1081~ 05

3.11873 0 5

3 .13040 0 5

2 8 0 . 9

314.3

244.6

377 .8

414.4

454 .8

499.2

548.1

632. t

6 6 1 . 5

727.0

799.2

e78.7

565.3

IO€3.

1169.

1286.

14 IS.

1557.

1713.

l a m . 20 72

2279.

2535.

2753.

2025.

3321.

215.9

236.6

255.4

284.4

312.0

342.4

375. t3

412.7

0511.3

49n.0

547.4

6 0 1 . 7

661 .0

721.6

900.3

860.3

>et?.5

I 3 6 6

1 1 72.

i2FO.

i 4 1 9 .

1 500.

1716.

18d6 .

1 0 7 3 .

2277 .

2500.

i 6.70

i 8 - 3 0

20.06

22.0@

24 .13

7f>.YR

3 9 - 0 7

31 - 9 2

3 5 . 0 6

30 .52

42 .34

4c>.34

S l . 1 6

5b.2t3

r , l . Y O

c,cl.OY

74.91

n2.42

Y >.OY

Y ‘ > . 7 h

iOY.7

220.7

132 .7

145. Ci

%&>9.3

i76.1

193.4

2.279

7 . 4 9 7

2 .737

3 .002

3.7 93

3 . 6 1 3

3 . 9 6 7

4 . 3 5 6

4.735

5.257

5 . 7 7 8

1 . 3 5 1

6 . 9 8 4

7 . 5 6 0

R . 4 4 7

9.2 SI?

1 3 . 2 2

11.25

12-37

13.62

14. $8

16.47

1 3 . 1 1

I >. 3 L

21.48

2*. 04

2b. 3 9

33

ln

?

(D

nr N

N

nr . d

. m Q

r- (L . d * ro

ri

Ul 0

0, m U 0

e

0 ..

ma

00.

ON

m

Pl

e.

O

m

0.P-

Dm

V

I v

an

0

0

00

O

N

ln

t-

an

\.I-

.. e

o ln

rn

lnln

0

00

0

..

e.

N

SN

N

-*mt.

9l

cm

cT

)

km

o~

.

b-

PW

D

oc

-

.... N

NN

N

bc

mm

co

OO

OD

.... -

Nq

*

ma

ma

10

ri m

P

I

U

v! . r)

. N

4

.4

JI e Q

01 h

0

M 0

0

a

c

Q

oi . I> . 9 .O

v) 0

oc 0 0

P) . m N

u? cu . d

0

I C rc v IC

h '0

_.

-I

... 0

00

In

J 0

II, . . 9 N

Y, 9

e *

m 0 4)

US 0

0

Q

N

B

m 0

0 0

0

OI N

(u

4

0

m

(?

Q

m . M % a2 N

d

0

I rc: in u

a c

0

0

m

IT . m

a 3

J 0 N

4

t- .. v. ... 0

0

Qb

r-

mm

T

...... t

n-

rn

m-

~

n0

v)

Ul

mY

,

0

0 0 0 0

0

1n to

u7 ln

ln 0

30

60

00

00

00

00

VI

IP

00

V)

M

00

00

00

Du

oo

oo

S

Ln

ON

Cr

Uh

m0

-h

-

4-

NN

N

00

00

00

am

am

ln

m

...... mm

ln

m

DO

00

00

00

oo

ou

N

OC

UP

.

ON

Fl

PI

Q

In

Qt

-

NN

NN

00

00

.... * 0

0

.. . iir P

3

-. in 0

c) 0

N

Q

... . 0 VI 0

0

00 m ai 4 0

n

0

0

v, 0

\D h

h

0 0

0 0

rl (c

0 :

(h

-4 rl a!

OD

C

n(r: .. $

5

.. n

in

N

U

d-

44

ln

v)

0

3

d.

cv

ma?

4P

ao

..#1

*.

0

0

ln

v)

0

0

ln

m

dC

an

22

e

.

00

0v

)

00

03

mt-

mo

a

0

hr

n

00

am

0

0

00

m

w

.,@

PO

N

N

.. 0

0

..

t-33

hl

m

VI

9

6r

n

..

- 0 I 0 m

'I! m .. . 0

c

0

1 0 0

U: 0 4 . 0

N o I 0

N

P 0

@

0 .

(L

0

I e a

n

4

r . 0

N 0

I 0

t- 0

4

0

..I .

-i

t

-l

7 I PIE ( Y I N d ---------

405.0

406.0

457.3

408.0

409.0

410 .0

411.0

4 12.0

413.0

414.0

415.0

416.3

417.0

418.0

419.0

420.0

429.0

422.3

423.0

424.0

425.0

426.0

427.0

425.5

429.0

430.0

433.0

2 E A C F . i 0 1 ------I-_-

9.30450-02

0 19750-02

0.90214-03

-0.l6hhU-03

-0.12250-92

-3.22680-02

-0.3288D-02

- 0 . 4 2 n m - 0 2

-0.52459-02

- 0 -6 1720-02

-0.7361 0-02

-0.79070-07

-0.87090-02

-0.94650-02

-0.10l7D-0 1

- 0 . $0840-31

-0.11450-01

-0.12020-01

-0.12540-08

-0. I301 0-0 1

-0.13440-31

-D.P3R3D-03

-0.14180-01

-0 .1449D-01

-0.14760-01

-0 . \4F90-01

-0.LSIBD-OI

lEMPlCEkCb US)

33.06

33.41

33.76

34.1 1

34.4.:

34 .79

35.13

35.45

35.77

2 6 - 0 7

36.36

76.64

3 6 . Q O

37.65

27.3e

37.54

37.79

37.98

38.25

38.30

39.45

38.57

3 8 - 6 9

38.79

38.87

38.95

39.02

PCWERC Y a - -_-_ --_ 85.07

~ ~ 1 . 8 4

H9. I 6

69.05

e e . 5 0

87.55

86.25

84.49

82.47

80.16

77.61

7 4 - 0 7

7 1 . 9 7

58.95

65.86

62.73

59.59

56.48

53.41

50 .40

47.48

44.65

41.94

39.33

36.85

34.49

32.26

0.30530 05

0.3099D 05

0.31310 05

0 .31430 05

0.31490 05

0.31353 05

0 .31070 0 5

0 .30640 J 5

0 .30390 0 5

0.294213 0 5

9.2R64D 05

0 .27180 05

3.26840 05

0.25849 05

0.24800 05

0.2372G 05

0.22630 05

0.21520 05

0.20420 05

O . l c 1 3 3 D 05

0 . 1 8 2 7 0 05

O.IY22D 05

0.16210 05

0 .15240 0 5

0.1431D 0 5

0 . 1 3 4 1 D 05

0 . :2560 0 5

P R E C l l R S b F l ---- ------------- -

0.81390 as a.2oa20

0.8232D 05 0.20310

0.92850 0 5 0.20403

0.82960 05 0.20390

0.82680 0 5 0.20280

0.81990 05 0.20070

0.80940 05 0.1978D

0 .79530 0 5 0 . 1 9 4 0 D

0 .77810 05 0.18940

0.75R13 05 O . t B 4 3 D

0.73560 05 0.17am

0.71100 05 0.19230

5.684BD 0 5 0*165?i,

0.65730 0 5 Q * 1 5 8 $ 0

0.62890 05 5 .15150

0.60000 0 5 0 .14460

0.57090 0 5 0 .13740

0.54170 0 5 0.13030

0.5L29D 05 9.12330

0.4R46D 0 5 0.11640

0 .45700 0 5 0 . 1 0 9 6 D

0.43023 05 0.103PU

3 .43438 05 F660.

0.3795D 05 S O 8 9 .

0.35580 0 5 P517-

0.33320 0 5 7973.

0 .31183 0 5 7457.

CONCEMTRATIJNS

O S 0.15033 05

05 0.15160 0 5

0 5 0.1522D 0 5

05 0.15219 05

05 0.15120 05

05 0.14963 05

05 0 .14733 05

35 0 . 1 4 4 5 3 05

0 5 0.14153 0 5

0 5 9.13713 05

0 5 0.132ao ot, 05 0.1281D 05

05 0.12320 0 5

a s o . i i ~ o a 0s

05 0.1 129i) 05

05 0.10740 0 5

95 0 . B 0 2 t O 0 5

0 5 9673.

05 9145.

0 5 8635.

05 8135.

0 5 7651.

7 1 86.

5 7 4 1 .

6 3 1 6 .

5922.

5529.

.---- I 1 59.

]I 169.

I 1 73.

I172 .

1165.

1152.

$ 1 3 4 .

t 112.

1 OCJb.

B 0 5 5 .

?. 022 .

YP5.6

9 4 7.5

Y 07.8

867.2

826.0

794.7

743.7

7133.3

553.7

625.3

%

552.3

5 i a . o

485 .4

454.3

424.4

159.0

159.4

160.0

a59. e

l E 8 . 8

157.1

154 .7

1 5 i - 6

1 4 8 . 0

L 4 3 . R

i J 3 . 3

134. 3

129.1

123.7

1 I s.2

112.6

136.7

i o 4 .4 95-84

03.45

R 5 . 2 0

8'3. I4

75.26

70.59

6 6 . 1 4

61.90

57 .90

T I WE( Y IN)

432.0

433.0

434.0

435.0

436.0

437.3

435.5

4 3 9 . 0

440.0

441.0

442.0

443.0

4 4 4 . 9

445 e 0

446 0

447.0

448.0

449.0

450.0

451.0

452.9

453.0

454.0

455.0

456.0

457.3

458.0

-0 15360-0 1

-0. 15500-01

-0 .15510-01

-0 - 1 5 70 0-0 1

-0 1 57bD-0 1

-0 15300-0 1

-0.15R20-0 1

-0. I532D-91

-0 I 5 500- 0 1

-0 1 5 7 h D - D l

-0 .1571D-01

-0.15640-01

-0 0 15‘560-0 1

-0.15470-01

-0 15360-0 1

-0 I525D-0 1

-0 1 5 1 3 0-0 I

-0.150oc-31

- 0 14860-0 1

-0.14710-01

-0 1455D- 0 1

-0.14390-0 t

-0.14230-01

-0 .14060-01

-0.i3a~0-01

-0 13700-01

-0.1352C-01

39.07

39.12

39.15

39.1 B

39.20

39 *2 2

39.22

y79.22

39.21

39.20

39.1 5

3 9 - 1 6

3 9 . 1 4

39.1 1

39.07

39.04

39.00

38.95

38.91

3 8 . R h

38-81

38.76

35-70

38.65

38r59

3e.53

38.47

30.15

28. kb

26.29

24.54

22.90

21.36

19- 93

1 R e 5 9

L 7.3s

16.19

15.11

14.11

13.18

12.31

11.51

10.76

10.07

9.431

0.835

8.282

7.769

7.292

6.850

6.439

6.057

5.703

5.373

0 . 1 1 7 5 G 05 0.29150 0 5

0.10990 05 0 . 2 7 2 4 D 05

0.10270 05 0.25441) 0 5

9591.

4954.

9357.

7795.

7276

671 6

6334.

591 l r

5517 .

515 1

481 0

4494

4200.

3927.

3674.

3439.

322 1

3019.

2831

2656.

2495.

2344.

220 4

2075.

0.23740 05

0.22150 0 5

9.20680 0 5

0.19290 05

O . l B O O D 0 5

0.16790 05

0 . t5670 05

0.14620 0 5

3.13650 05

0.1275D 05

0 . 1 1 9 1 0 05

’ 3 e 1 1 ! 3 D Q 5

O o l O b O D 0 5

9733.

9 1 10.

8531

7994.

7496.

7034.

6609.

6206.

5 R 35

5491.

5171.

E4 7 0 .

651 I

607Y

5674.

5 2 9 5 .

4940e

4609.

4300 e

4 0 1 1 .

3743.

’494.

3262.

2 0 4 7 -

5846.

2661.

2488.

232.3.

2180.

2042.

1919.

1795.

l oas .

1582.

1 4 8 ? *

1399.

13170

1241.

51 68

4627.

4507.

4 2 0 7 .

-5925.

3662.

3416.

3187,

2974.

277’5.

2590.

2418.

2259.

2111.

1973.

L845.

1726.

1616.

1514.

1419.

1331 - 1 2 C O .

1 1 74.

11 03.

10.38

977.0

920.5

3 37.1

370.9

340.3

323.?

3’) l .b

2dl . ‘b

2 t2 .5

2U4.4

??&. 5

2 t 3 . 2

1GQ.3

1 e5. Y

173.b

I b2.2

1 5 1 . 6

1 4 1 . 4

132 .7

124.2

1 1 6 . 4

1 3 9 . I

102.?

96.04

93.21

84-30

79.7 7

75. 1 0

70.76

54.11

59.54

47.19

44.34

4L. 09

S c i . 3 4

3 s . 7 7

3J.37

31.14

29.05

27.12

25.32

23.65

22. L 0

213.66

19-32

LS.08

16.93

15.56

14.36

13.34

13.09

12 .29

11 .56

17.67

10.23

9.042

w Ln

m n

z IU z

... l- r c a

U

z 0

U

a. 0

m

3

U

w U

a

Y 0 0

J.

N

e 9

il:

0.

t. a Lu

Q

?- - n

d

h

m Q

d

M

6,

.e U

..I W

U

n I W

c

w

.., d m m

0

a

Ln

if i

b

N 9

0

v rg

d

4 0

d e

. e) 01 n

4

N

Q

m

r.

c

oc h

* m

m

B) r, . c 0

I 0

d

*I d

d

0

0

0

Q

P

d

0

d

a 3

d

P

in . 0 . m

c

h . N 4

2 . 0 d 0 d . a rri c I

4 ul a . W

N

m

m

c 0

I 0

k? w N

d

W I

c

4

c

P

N

9

tT 9

in n

0

rc 01

d

M

c

N

N

m W . 0

h

9

m . d 0 Q

4

* N

pc

m . v. 0 . a, r>

L

0

I 0

!r P

N

d

0

1

0

4

Q

U

m 0 in

r)

N

IC

r- e

0

0

N D

o\

M

m

W

d c 0

m

0) a

m - 0

N

4 m

N

0

n

r?

-4

0 I 4

M

N

P

”-. 0

l

0

u)

0

U

u- 0 0

0

m ?“

4

0

..4 m

M

0

uj

P

4

. Q

c 0

N

. m 5

I

*

a

m

N

a! h

m

..d c7 l a !n

m

d

0

I

O

e 9

U

n s

N

m

FI 9

J? . r

0

P 0

>

a @

p. W

. 4 N

u? N

. m

N

4 6

01 Q

0.

N . n

h

P. r?

i @ W

L

- . 0 I

c

D 9

Q *

IC c 10 d

9

in

CI

h

h

9

m a

0

IC

In n . 0. m 4

N

0

m d

0 . - M a e4

in in

h

rn

.. c I .3 c

a

0

&

0

I

C

N

r- u

D

vi c1

e ‘c W

n

0

Lo a . 4

* c 9 Ill

Q

N

p1 N

cc N

N

I7

0

r? Q

N . ru

4 t. m

I

0

I a

r

c

0 c . 0 I

0

r? c

* 3

P

r.

* h’

0. “J

5

0

m

r)

10

N

Ut . ” m

N

N

... 0.

0

B

a! . 0

N

N

N

..j P1

IC

ri . .-a 0

1 0

2 0 I 0

I

0

in r- U

I

N

r

m m 0

a’

cv 51

d c

(7

U

0

0.

Q . * sl

m 0 N

a,

m 0

m 0. N

* * ru

c N

c

F)

N 0

l 0

rn * a2 O

0

I . 0

Q e

Q

0

9

ro n

9

z 0

w Y

b

Q

m

m

(P

Q

Q . LD

Q

b

e

0

01 9

c-

0

d 0

N . c;.

N

h

ri

N

0

l

in III ul JI

0

I

a 0

h

P

0

9

u7 0-

h,

c .- - w rd

tn . c

ru

.*

0

P

PI

0. N

‘f: In . 4

0

9

rn 0

9 . W

r-

u2 ri

N 0

I 9

m

rn 0

I

n

d

C

m Q

d

v, 9

c

IL

N e

0

N

”7 0 9

N . ’D

ul 0

PI

. P) c * -4

m 0

c

v,

4

0

ln . 4

N

r- a . P1

N

n l

is 0

d

4’

0

I

4

0

U a

0 .

T 1 M E ( M I N ) --------- 486.0

4 0 7 . 0

488.0

404 0

490 0

491.3

492.0

493.0

434 .o 495 0

436.0

497.0

49e. 0

493.0

SCG. 0

501.0

502.0

503.0

504.0

595.0

505 5

E O i . 0

508.0

509 0

510.0

5 1 1 . 0

512.0

- 0 e 7 7 26D-0 2

-0.75150-02

-0 7 3 050-02

-0.7OSSD-J7

- 0 a 5 R56D-02

- C 6 h 77 0-02

-0-64690-02

-0.62610-02

-0 .6054D-02

-0 -58480-02

-0.56420-02

-0.54370-02

-0.52?3D-02

-0.502VD-02

-0 s 4 32f.W 3 I

- 0 . 4 6 2 4 0 - 0 2

-0 e44220-02

-0 *42220-02

-0 . 4 02 20- 0 2

-0 3 3230-02

-0 .36233-O2

-0.3427D-OZ

-0.3231D-02

-0.30350-02

-0.28400-02

-0.26460-02

-0 -2453D-02

36.58

2 6 - 5 1

36.44

36.37

36.30

2 6 - 2 3

36.1 7

36.10

3 6 . 0 3

35 e 96

35.90

35.83

35.76

35.70

35.63

35.56

3 5 . 5 0

25.43

35.37

35.30

35-24

35.1 7

35.1 I

35.04

34.98

34.92

34.85

?. -446

1 e 3 9 8

1.353

1.311

1.271

1.234

1.190

1.165

1.134

1.105

1.077

1 051

1 e526

1.003

0.9819

0.9617

0.9427

0.9250

0.9084

0 . 8 9 2 4

0.8784

0, a54 9

0,8524

o,mo8 0.8301

0.8203

0.81 12

538.7

520 -2

5 0 2 0 8

486 . 5 471 * 1

456 6

443 .#

430.1

418. I

406 7

396 0

386.0

376.5

357.7

359.3

351 .s 344 1

333.2

330.7

324 7

319.0

313.d

308.8

304.3

300 . 0

29b. 1

292 5

13720

1326.

1283.

1242.

1204.

1168.

1134.

1102.

1072.

1043.

1017.

931 .a 9h9.2

946.1

975.3

905.6

887.5

970.4

054.3

839.3

825.3

312.3

800.1

708.9

178.4

76e.a

7 6 0 . 0

232.6

321.5

311.2

z01.4

292.2

2 8 3 . 5

275 .4

2 6 7 . 7

260.5

252.7

247 .3

241 .3

235.7

2 3 0 . 4

225.4

220.7

216.4

212.3

208.4

204.8

201.5

198.4

195.5

192.8

190.3

166.0

185.9

2 4 7 . 4

239.2

2 3 1 . 5

2 2 4 . 2

2 1 7 . 4

2 1 1 . 0

20s. 0

199.3

193. v

1 f l Y . O

Ids. 1

1713.7

175.5

171.6

167.9

164.4

161.2

150.1

155.3

152.6

1 5 0 . 1

1 4 7 . 8

145.7

193 .7

141.9

140 .2

138.6

19.03

1 8 . 4 1

1 7 - 3 1

1 7 . 2 6

16.73

16.24

1 5 . 7 7

15.34

l4IY.4

1 4 . 5 4

14.17

L 3.33

1 3 - 5 1

1 3 - 2 1

12 - 9 2

1 P . h f i

12.41

12.17

11.96

lt.75

11.56

11.3%

11.22

1 l . W

l0.42

10.79

10.68

7.594

2.509

2 . 4 2 8

2.352

3 .281

2,213

2.15n

2.031

2.335

1.982

1.932

1 486

1 342

1.801

1.762

L 726

1 . 6 9 1

1 . t r S O

1 .e30

1.602

1.576

1.552

t D 5 2 9

I .50Y

1.489

1.472

1.455

w al

T I M E Y K N 3 R E A C T . t B B

513.0

514.0

515.0

5 1 4 . 0

517.0

5 1 e . o

519.0

520.0

52 1 .n 522.0

523.0

524 - 0

-25.0

526.0

527.3

529.3

529.0

530.3

531.0

532.0

533.0

534.0

535.0

536.0

537.0

E3a.o

539.0

-0 .2 26 10-02

-0 20699-02

-0- 18790-02

-0.16890-02

-0 1 5 00 D- 0 2

-0.13 130-0 2

-0.1 1260-02

-0 '3 3 46 0- 0 3

-0.754SD-03

-0.5702~-33

-0.3nE9D-03

-0.2045C-0 3

-Om? 3 0'30-04

0.15750-03

0.3371 D-03

0.51570-33

0.69750-03

0 . 9 7 020-03

0.10450-02

0.12210-02

0 . 1 3 C j S D - 0 2

3.156RD-02

0.17400-02

0 1 F L 10-C2

0.20A10-02

0.2250D-O2

0 -24 180- 5 2

IEHP(CEFCI US) PcmERt w j __-_- --____- -

34.19 0.8030

34.73 0 7956

34.6 7 0 7808

34.60 0.7829

34.54 0.7776

34.48 01 7730

34.42 0.7691

34.36 0.7659

34.30 0.7433

34.24 0.761 4

34.1 e 0.7601

34.12 0.7595

34.06 0.7595

34.00 0.7601

33.94 0.7613

0 7632 33.88

3 3 . P 3 0.7657

33.77 0.76BR

33.71 0.7726

33.65 0 . 7 7 7 0

33.60 0.7821

33.54 0.7875

33.4e 0 7942

33.43 0.8013

33.37 0.8091

33.32 0 . 8 0 7 6

33.26 0.8268

299.2

286 2

293 4

280.9

278.7

276 9

275.1

273 .A

272 . 4 271 a 4

270.6

270.1

269 H

269. a

269.8

27'3.2

270.8

271.6

272 4

273 9

275.4

277 1

279 0

281.2

283 7

296.3

289.3

751.9

744.6

739.0

732.0

726.7

722. I

718.2

716.8

712.1

713.0

708.5

707.5

707.2

707.5

708.3

709 .?

711.7

714.3

717.5

7 2 1 . 3

725.7

730.7

736.3

742.5

749.4

757 0

755.2

184.0

it32.3

180.7

179.3

17Y.9

177.0

174.3

175.4

i74.M

174.3

174.0

a73.n

173.9

173.9

174.2

174.6

175.1

175.9

176.7

177.6

178.8

180. I

181.5

LB3. I

184.9

186.8

188.9

137.2

135. (>

134.W

133.7

i32.8

132.0

131.4

130.8

130.4

130.3

129. t3

129.7

127- 7

12Y.H

130.3

190.3

130.7

139.3

1 5 1 . 9

132.6

133.5

134.5

135.6

1 3 b . t j

138.?

1 3 Y . 5

L41 1

P H E C U R S S R CONCENTRhV IONS .- ---- - - - - -- 10.57

L 0.47

10.3'3

10.30

i 0.23

10.17

1 0 . 1 2

1 U.0Y

10.04

10.02

10.00

i . 9 9 3

9 . 9 9 3

I0.0Ll

10.02

15.04

10.07

i o . 1 2

19.17

10.22

1 0 . 3 Y

1 0 . 3 4

1 J.45

19.54

13.64

10.76

L 0.88

. - ------ 1.441

8.427

1.415

1.405

1.395

1.387

I. 3Hcl

1.374

1 . 3 6 4

1 . 3 6 6

1.364

1.363

1 . 3 6 3

1 164

1.36t

1.36'1

1.374

1.377

L. 3 8 6

1 . 3 9 4

9.403

1.413

1 . 4 2 5

3 . 0 3 7

1 . 4 5 1

1.4b7

1.483

W OD

T I YE( H I N 3 --- -- - ---

540 e 0

5 4 1 . 0

5 4 7 . 0

543.1)

544 -0

545.0

546. u c47.r)

548.0

549.0

550.0

5 5 1 -0

552.0

553.0

554.0

555.0

556.0

< 5 7 . 0

558.0

559. n

560.3

561.0

Fh2.0

563.0

5 6 4 0 0

5 6 5 . 0

566.0

0.25850-02

0.27510-02

0.29160-02

0 30.3 1 D- 0 2

0 e32440--02

0 e 34 C 6 0 - O 2

0 . 3 5 5 7 0 - 0 2

0.37270-02

0 -3884D-02

0 . 4 0 4 4 0 - 0 2

0.4 2 0 1 D-0 2

C e 4 35 70- 02

o .4si in-02

0.4 Ch5iD-02

0 4 P 17D-02

0.44690-02

0 5 I I 9 D-'2 2

0 . 5 2 6 A D - 3 2

'I 54 160-0 2

0 55630-02

0.57090-32

0 .St353D-02

0 59970-0 2

0.6 1 390-0 2

0.62790-02

C. 6 4 190-0 2

0.65570-02

23.2 1

33.15

33.10

33.05

32.99

-72.94

3 2 - 0 9

32.83

37.78

32.73

32.6.F

32.63

32.5F!

32.53

d i . 4 P

92.43

32.3P

Z2.31

32.28

32.23

32. I9

32.14

32.09

37-05

32.00

31 094

3 1 . 9 1

0.8365

0.8476

0.8592

0.8716

0 . 8 R 4 d

0.8989

0.9139

0 9299

0 9469

0.9649

0.9839

1.004

I . 02s

1.044

I . 372

1 097

1 . 1 2 3

1.151

i . i a i

1.212

1.244

1.279

1.315

1.354

1 394

f 0436

1.481

292.5

295.9

299 8 7

303 7

308 0

312.6

317.5

322.7

328.3

334 - 2

340.5

3 4 7 . 1

354 1

361.6

369 s 4

377.7

386.5

3 9 5 . 7

405.5

415.8

426 6

43n. I

450.1

462. a 4 1 6 . 2

490 3

505 .1

774.1

763. t3

794.1

905.3

817.2

829.9

e43.4

e57.8

873.1

599.3

906.5

924.7

944-0

964.3

9615.8

1039.

10330

1059.

1084.

1 113.

1 1 4 2 .

1173.

1 2 3 5 .

1241.

1277.

1316.

1356.

191.1

193.6

196. 2

199.0

202.0

205.2

208.6

2 1 2 . 2

216 .1

220.2

224.5

229.1

233.9

239.0

2 4 4 . 4

250.1

256 .1

252 .5

269.2

27h.i'

283.0

291.5

299.7

2oe.4

Z 1 7 . 6

127.7

237.3

142. a 14a.6

1 4 b . O

1 4 3 . 7

151.0

153.4

155.9

1 S B . h

161.5

1F.196

167.8

171.3

174.4

178.7

182.8

187.1

1 L I . f i

196.3

201.3

206. f

212.2

219.1

224.3

230.0

237.6

244.9

252.5

11.01

1 1 . 1 5

1 1 -30

t 1 . 4 7

1 1 eb'4

\ l e 6 3

: 2 . 0 2

12.23

1 2 . 4 6

12.6'3

LL.94

1 3 . 2 1

1 3 . 4 3

1 3 . 7 6

1 4 . 1 0

14.43

14 .78

L 5.14

15.53

15.94

t 6 - 3 7

I bod?

17.30

1 7 . 9 0

1 s.3 3

l b a 9 . I

19.41

1 . 4 0 1

1.520

1.541

1 5h3

1 .587

1.'113

1 . 6 3 Y

1 . h B Y

f . J '3 ';

1 . 7 3 1

1. 765

1."01

1 . 8 3 9

1 380

1 . 9 2 2

I.*:>?

2.315

2 . 0 6 5

2 , 1 1 3

2 .174

7.73?

2.294

2.358

2.42Y

2.509

2.57h

2.657

567.d

568.0

569.0

570.0

571.0

5 7 7 . d

573.0

574.0

575.0

576 0

577.0

578.0

579.0

580.0

5 R 1 .o 5R?. 0

587.0

584.0

5AS.0

585.0

587.0

5 6 M . O

CS4.0

E.90.0

591.0

C9T.0

593.0

0.6hS4+02

0 6 8 290-0 2

0 -6963D-02

0 . 7 0 5 C D - O i i

0.72273-02

0 73560-02

0.74840-02

0.76lln-02

0 7 7 3 6 0 - 0 2

0 . 7 e s 9 r ~ 0 2

0.79SiD-02

0.9101c-02

0.e2190-02

0. e335Q-02

0.844VD-122

0. U S 6 10-3 2

o. e671w-32 0. P77SD-92

0.8885D-02

0.8489D-02

0. 0 Q 3 D - 0 2

0.9 iR9D-02

0.9294n-02

0. Q 3783-02

0 44 6RD-0 2

0.95560-02

3 9641 9-02

3P - 8 5

31.82

31.78

31.73

71 -69

3 1 - 6 5

2 1 - 6 1

31.57

31 -52

71.48

? I -44

31.41

31.37

31.33

J I .20

31.25

31.22

31.18

31.15

31.11

9 1 . 0 8

31.35

31.02

30.99

30.96

:0.93

30.90

1.528

1.578

1.630

1 .dB5

1.793

1.504

1 869

t .937

2.008

2.084

2 0 163

2 . 2 4 7

2.335

2.429

2.527

2.631

2.740

2 856

2.977

3. I05

3.242

3.385

3.536

3.696

3.864

4.042

4.230

P R E C W H S 3 R C O h C E N T R A T 1 O N 5

520 7

537.2

554.5

572.8

592 -0

612.3

633.6

656.1

679 - 9

704.9

731 .z

?59 .o 788.3

ai9.2

R 5 1 e7

aab. 1

922.3

960.5

100 1.

L043.

1088.

1136.

1196.

1239.

1294.

1353.

1415.

1399.

11944.

1491.

1541.

1594.

8643.

1707.

1769.

1834.

1902.

1974.

2050.

2130.

221Q.

2303.

2397.

2496

2600.

2711.

2827.

2 9 5 0 .

3079.

3 2 1 6 .

3360.

3513.

3674

3844.

148.0

259.3

271.2

383.7

396.9

410.7

425.4

440.8

457.0

474.2

492.2

511.2

531.3

552.5

c 7 4 . e 598.3

623.2

€49.4

e77 . I

706.3

737.1

769.6

903.9

E40. t

F 7 R . O

518.8

S 6 1 . 4

260.5

269.0

277.9

287.2

297.1

307.5

318.5

3 3i). i

342.7

355. I

368.6

382.7

337.4

4 1 3 . 0

430.6

443.2

466.9

486.5

507.7

529.2

552. 4

576.7

b32.4

b2r.b

659.3

688.f.

720. b

20.10

20.75

23 - 4 4

2 L . i b

22.93

2 3.73

24-54

23.*7

Z ' . . d I

27.40

2*.45

2-7.55

33.71

31.14

33.23

34.54

30.93

37.55

3 J . 1 5

4 1.94

42.63

4 4 - 5 1

26.53

4E.60

53-81

53.15

5 5.02

2.74 I

2.G.30

2.924

3.023

7.127

3.236 /. 3 5 3 .i . 4 7 4

7 . t> J 3

3.777

3.dUi)

4.033

4.139

4.536

4.532

+.?It.

4-91 5

5.122

5.340

5.573

5.814

h. 1371

h. 44 3

6.625

6.039

7 . 2 3 0

7.597

T I M E ( H IN)

594.0

595.0

596.0

597.0

598.0

599.0

l300.0

cot10

€02.0

CO3.0

604.0

€05.0

606.0

607.0

608.0

609.0

t 1 0 . 0

e 1 1.0

e12.0

613.0

f 1 4 . 0

615.0

616.0

617.0

e i e . 0

t19 .0

620.0

R E A C T . ( S J --l__l__

0 9 723D-02

0 9 8 0 1 0-0 2

0 98760-0 2

0 9 9479-0 2

0 . 1 0 0 1 0 - 0 1

0. 10080-0 1

0 tO 140-0 I

0.10190-01

0 1 O24D-0 I

0 f 0290- 0 I

0 . t 0339-0 I

0.1037C-01

0.1040n-01

0.10420-01

0. \0400- -n~

0.10460-01

0 * 10460-0 1

0.10460-01

0.1046D-Q I

0 10440-0 1

0.10420-01

0 1039D-0 1

O e 1 0 3 S O - 0 1

0.1031D-01

0.1025D-01

0.1019D-01

0.10 1 I D - 0 1

T E M P f C E L C I US) ----I---

75 .87

30.85

30182

30.80

30.78

30.76

' C . 7 4

30.72

3 0 . 7 0

30*69

3o.ae 30.66

30.55

30.65

JcJ.Oa

30.63

30.63

30.63

30.63

30.64

30.65

30.66

30.87

30.60

30.70

30.72

30.75

POWER( U t

4.429

4.630

4.859

5.092

5.339

5.598

5.873

6.162

6.467

6. 789

7.128

7.486

7r862

6.259

3.676

9.115

9.577

10.06

10.57

11.18

1 1 066

12.25

12-86

13.50

14.17

14.67

15.60

---I---

148 1 . 1550.

1623.

1700.

1752.

1868.

1959.

2054.

2155.

2262.

237 4.

2493.

2618.

274 9

28-98.

3033.

3187.

3348.

3518.

3695.

388 2

4078.

4283.

4497.

47.21

4956.

5200.

PRECURSOR .--------------------

4023. 1006.

4212. 1054.

4412. 1104.

4623. 1157.

4046. 1213.

5061. 1272.

5329. 1334.

5591. 1400.

5867 1459.

6158. 1542.

6 4 5 5 . 1619.

6789- 1700r

71 30. 1786.

7459. 1876.

7867. 1971.

6265 . 2070.

8693. 2175.

9123. 2205.

9584 2 4 0 1 .

0 .10070 0 5

0.10580 0 5

O . l l l f 0 05

0.1161D O S

0.12250 0 5

0 . L 2 R 6 0 05

0.13491) 05

0.14150 05

2522.

2650.

2783.

2922.

3068-

2220.

2379.

3544.

CONCENTRATIONS ------_-__-I_

754.3

790 0

B27r6

867.3

909.3

Y53.5

1000.

$ 0 4 9 .

1 1 0 1 .

11 56.

1214.

1275.

1339.

1406.

1478.

1552 rn

1631

1713 .

LeCJO.

1891

1986.

2086.

2191.

7300.

2414.

2533.

2656.

.-----I- 54.27

b3.98

63.34,

bas96

76-20

73.61

71.22

31.02

tlc.04

R Y . 2 7

95.73

99.43

133.4

1 Od. 6

114.1

114.8

125.9

132.3

1'19.0

1 4 6 . 0

i53.4

1 5 1 . 1

169. &

17T.5

186.4

195.5

205.1

7.94 3

1.318

3.715

9.133

9.575

IO. 04

10.53

21.35

11.60

12. L R

12.76

13.43

14. t 5

1 4 . ai 15.5fi

1 6 . .35

1 7 - 1 5

1R. 05

I S , 96

19.92

20.32

21 97

23.07

23.22

25.42

Z S . h ?

27.97

0

z 0

t

a

ff

M

t

z W

W

0

V

x 0

m CL 3

U

W

ff

L

a

I?

rl i? hi

0

In N

.-I

la m

r- N

2 I.) h

ln 0 a

Q

a2 Q

.4 * 0 * B

a

d

VI

LT N

. 0

a

VI

a 0

0

10 a

a . 0 Q

t- n d

d

F

"4 . d

c

a 0

1'1 . N

c? I c m 15 CJ F

0

0

N

N

Q

0

'9 e 0. I- 0

d

v, 0

o

0

n

9

Q . 0 . II C rn P

P 0

I- .. d

W

0

pii

N

O I

Q

r- N

nJ (2

0

0

m N

'v

CP 10

2 ..

c

I- d

N

0

0

N

m . 0 r- N s

m 0

a

(c

0 P

- e 0 . c (c

N

9

I?.

p.

m . .." W

CF

0

PJ . N

0

I Q 0

r- CF

0

M

C

d

N

\o

in jo

\c m 4

0

r. nr . 0 0 n m

0

IC

rc a VI

0

0

W 9

m

- . i3 . In r- b! 9

Q

VI 0

h . c

(r

0

m

N 0

I 13 N

Q

4

0

0

0

D

N

9 .

9

m . m P 0

M

M 0

a m m 0

N

0 . . 0 V

I b

- 0

d

N

N

. F

0 * I*

m

N

0

I n

U

h'

0

0

&

0

e

N

w

LT r) . n7

m UJ -4

a

0

n

I- N

N

0

.-I

. . rl

0

b)

(a

d

Is:

f? N

r, d

. .-A r

l

N 0

l o! .Y v m

0

a

0

(2

N

u? .

om

--

o

mr

-0

O

..

Ih

id

8

84

4

....

....

rn

VI

VI

aa

a

00

00

00

...... O

OO

QO

n

...... N

NN

NN

N

ri P

I F)

F)

m

m

NN

NN

hl

N

00

00

00

I

II

II

I

............ O

OO

OO

OO

OO

O0

O

.

T I M E ( Y f N ) --------- P 4 R . 0

649.0

650.3

65 1 .o 652.0

c53.0

654.0

655.0

656.1

657.0

659.0

659.9

k F 3 . 3

661.0

6 6 2 . 3

6.63.0

664.0

665.0

666.5

667.0

6 6 q . U

669.0

F75.0

671.0

672.3

F.73.0

674.0

0.32 030-02

0.28 0 6 9-02

0 2 3990-02

0 . 1 S R t j D - 0 2

0 1 5 7 4 0 - 0 2

0 I 1 590-0 2

0.74‘30-03

0.32cilD-03

-0. e37.30-04

-0.4 S 360-03

-0.99S3D-03

-0.13 0 70-0 2

-0 1 6549-02

-0 2 0 8 10-02

-0.?4600-0?

-0.28303-02

-0.31400-92

-0.35390-02

- 0.38 78D- 0 2 -0.42040-02

-0.45190-02

-0 e4820D-02

- 0 5 109D-0 2

-0 .SlgH4D-62

- 0 - 56 45 D- 0 2

-0.58930-02

-0.61270-02

33.00

33.14

33.27

33.40

23.54

33.67

33.81

23.94

34.08

?4*21

34.35

34.4 e 34.61

34.73

34. H15

34.9E

35.09

35.2 I

35.32

35.43

35.53

35.63

35.72

35.81

35.90

35.98

36.05

40.72

41.24

41 -69

42.07

42.37

42.59

42.72

42.78

42.76

42.65

42.47

42.21

41.87

41.47

41.00

40.47

39.87

39.23

38.54

37.81

37.03

36.23

35.39

34.54

33.66

32 7 0

31.88

PRECURSOR C O N C E Y T R A T I O N S

O.lQI4C 0 5

0.L4360 05

0.14550 05

0.14720 O S

0 . 1 4 R 6 D 0 5

0.1Q990 05

0.15060 05

0.15120 05

0.15150 05

0.15150 05

0.15120 05

0.15070 05

0.14993 0 5

0.14880 05

0.14740 05

0.14591: 05

0.14410 05

0014200 05

0.13930 05

0.13750 05

0.13490 05

0.13220 35

0.12940 05

0112659 05

0.123513 05

0.12050 05

0.11730 05

0.37610 0 5

0.35130 05

J.3859D 05

0136980 05

0 . 3 9 3 0 D 05

0.39540 05

0.39710 05

0.39800 05

0133821) 05

0.39760 05

0.39630 0 5

0.39430 05

0.3916D 0 5

0 . 3 e ~ 2 0 05

0.3841(9 0s

0.3’1950 05

0.37430 0 5

0.36860 05

0.36240 0 5

0.35570 O S

0.34870 35

0.3414D 55

0.33389 os 0.32590 OS

0.31790 0 5

0.30971) 0 5

0.30140 OS

S2L7.

4420.

4526.

4614 .

5685.

9738.

5773.

4799.

4735.

9164.

F725.

9668.

4594.

4504.

$395.

4274.

9145.

F000.

8843.

e6?7.

E‘501.

e31a.

e l 2 B .

7933.

7733.

7531

7326.

6947.

7039.

7 1 16.

71 81

72 32

7270

7295.

7335.

1302.

7 2 ccq.

7254.

7 2 1 0 .

71 54

7 0 8 5 .

7 c - {U%J6.

6 9 1 5 .

6815.

6706.

6589.

6463.

E3.31.

6 1 9 4 .

6052.

5906.

5757.

5605

5452.

535.5

542.5

549.5

453.5

5 5 7 . 4

560.3

5t-3.1

9 b 2 . Y

5f.2.6

5 f 1.2

558.8

5 55.4

551. J

545.7

537.5

532.5

524.8

510.3

507.2

497.6

4r57.4

4 76.8

465.9

454.6

443.1

431.4

41S.6

73.04

73.98

74.79

75.4 1

79.00

76.40

76.65

7h. 75

75. 7 0

7.5.52

76.19

75. 72

75.12

74.40

73.54

72.50

7 1 - 5 4

70.39

09.15

57.~3

b 6 r Q 5

65.50

63.51

t . l . 9 7

60.40

5a.6t

57.20

6- w

T I & ' € < Y l h r 1 -- ----I _ I

6 7 5 -0

676.0

677 .0

67r3.0

679.0

C60 -0

6 8 1 . 3

682.9

6 8 3 . 3

684 .'I

685.0

686.0

eu7.9

698.0

699.0

6590.0

691.3

692 .3

693.0

094.0

695.0

696.0

t97.0

698.0

599.0

700.0

701.0

- 0 -63470-02

-0.65530-02

-0 6 7450-02

-C.59743-02

-3.7Or390-02

-0 7 2 4 10-02

-0.7379D-02

-0.75C5D-02

-0 -76 150-02

-0.77200-02

-0.7604D-G2

-3.7EH70-02

-0.7953D-02

-0 9CCJD-02

-0 r?O=40-02

-0 . e O S O D - 0 2

-0 8 1 15D-02

-0. p 131 0-02

-0 8 1380-02

-0 .@%36D-02

-0.a1270-02

- 0 8 1 0 9 0- 0 2

-0.80840-02

-0. P O 5 10-02

- 0 .RO 120-32

-0 78660-02

-0 7 9 13D-0 2

26-11 3

36.19

36.26

36.3 I

36.37

36.42

36.46

76.50

35.54

36.5fl

26.60

26.63

36.6s

35.67

3he6P

36.70

36.70

36-73

36.71

36.71

36.71

36.70

36.69

3 6 . 6 P

36 -6 7

36-66

3 6 - 6 a

3 c. 98

30- 07

29. I 7

28.27

27.38

26.50

25.64

24.763

23.95

23.13

22.33

21-56

20.80

20.07

19.35

16.66

I8.00

P 7.35

16.73

16.13

15.55

15.00

14.46

13.95

13.46

12.99

12.54

0 d l 4 2 D 05 0.29300 0 5

O.lllO0 05 0.284613 05

0.107aD J 5 0.27629 05

0.10460 0 5 0.26780 05

0.10140 05 0.75950 05

9826.

9514.

9206.

890 2.

A 6 0 4

931 3.

9 0 2 H .

77s0.

7479.

7216.

5960

67 13.

647 3.

624 2.

6019.

590 3.

5596

5 3 9 6

520 4

5019.

4842.

9672.

0.25120 05

0.24310 05

0.23510 05

0.22730 0 5

3.21960 05

0.21200 0 5

0.20470 05

0.1975LJ 05

0.1906D 05

0.1838D 55

0.17730 35

0 - 1 7 1 0 0 35

0.16490 0 5

0.15899 05

0.15330 0 5

0.1478D 05

0.14250 05

0.13743 O S

0.13258 05

0 .12780 05

0.\2330 0 5

0.11900 05

7 1 1 9 .

C912.

6706

c 5 0 0 .

C296.

6094.

5596.

57 00 . 5509.

E32P.

5 1 38.

4959.

4785.

4 6 1 1 .

4453.

4294.

4141.

2992.

3849.

3711.

7579.

3451.

3320.

'210.

3097.

2988.

2884.

5258.

5134.

4989.

4836.

4684.

4534.

4386.

4240

4097.

3959.

3821

x a a .

3559.

3433.

3311.

3153.

3075.

2469.

2663.

2700.

2661

2566.

2475.

2397.

2303.

2222.

2145.

4'37.7

355.Y

384.9

372.2

360.5

348.9

33-r.5

326.3

315.3

304.5

294.0

213.5

273.9

264.2

254. F1

245.7

236.9

228.4

220.2

212.4

204.9

L s7.4

100.4

183.7

177.2

3 71.0

165.0

55.58

5 3 . 56

52.34

5 0 . 7 3

4Y. I 3

47.55

45.00

44.47

4?. Y7

4 1 . 5 1

40. O C

34. b P

37.32

2 6 . 0 1

34.73

33.44

32.29

31.14

3 J. 02

2 8 . 04

77.91

26. Y1

25.95

25.03

24. '5

23.30

22.4s

T I Y E ( M 1 N ) _-- -----_

702.0

703.0

704 .0

705.0

705.0

707.0

704.0

70910

710.0

71 1.0

712.0

713.0

714.0

715.0

78690

717.0

719.0

719.0

720.0

721 00

722.0

723.0

72400

725.0

726.0

727.0

928.0

- 0 . 7 YSSD- 02

-0.774 10-0 2

-0.772 10-0 Z

-0.76470-02

-0 75670-02

-0 .74930-02

-0.?3450-02

-0 .7393D-32

-0.7206D-02

- 0 . 7 1060-02

-0 7 0 030-0 2

- 0.6d SF: 0-0 2

- C 6 7960- 0 2 -0.657.30-02

-0 -65599-32

-0.644i)D-02

- 0.6 3 I 9 D - 0 2

- C . 6 1 5 6 0 - 0 2

-0.6072D-02

-0.59450-02

-0.5816D-02

-0.5656D-02

-0.55flO-02

- 0 . 5 4 200-0 2

-0 a 4 2 860-0 2

-0.51500-02

-0.50 120-02

36.62

36.60

36.5e

36.55

36.53

30.50

26.47

3 5 - 4 4

36.4 I

36.37

36.34

36.31

36.27

26.2 3

3‘5.23

36-16

36.1 2

36=OF!

36-04

36.00

35.95

35.91

35.87

35.82

35.78

25-74

3Ej.69

12.10

11-69

11.29

10.91

10.54

10.20

9.864

9.546

9.292

8.952

8.675

8.411

Q.159

7.91 tl

?.6R3

7,469

7.260

7.060

6.870

6 0 6 R Y

6.516

6.352

6.195

6.046

5.F03

5.768

5.639

450 9

4352.

4233-

4059

3922.

3791.

3665.

354 5 . 3430 a

332 1 e

32 16.

31 16.

3020.

2929.

2642 .

P759.

2690

2604.

2532.

2464 .

239 8.

2336.

2276.

2220 0

7166.

21 14.

2065.

0.1149D 0 5

0.11090 05

0 .10710 05

0.10351) 05

0.1000D 0 5

9672.

9354.

9051

876 I

8484.

8219.

7987 *

7726.

749s.

7276.

7066.

6867.

6676.

6494.

6321.

6156.

5998.

5848.

5 7 0 6 -

5569.

544 0 0

5317.

2 784

2688.

2597,

2509.

2425.

2345.

2 268

2195.

2125.

5 0 5 8 .

1995.

1934.9

1675.

1820.

t f b 7 .

1716.

1668.

1622.

1579.

1537.

1497.

1459.

1423.

1388.

1356.

1324.

i 295.

2071.

1999.

1931.

1366.

1004.

1744.

1687.

1633.

1581.

1531

14.34.

1439.

1396.

1354.

1315.

1277-

1242

1207

1175.

1 1 4 4 .

I 1 14.

1096.

1059.

1034.

1009.

486.2

964.2

159.3

153. A

149.6

143.6

130.9

134.2

124.9

12’5.7

121.7

1 1 7 . 8

1 1 4 . 7

1 1 0 . 7

197.4

104.2

191.2

418.31

95.56

92.94

30.43

93-05

05.77

8 3 . 6 1

8 1 a 5 4

7G.58

77.70

75.’32

74.22

21.71

70. 57

29.26

1 9 . 5 7

1 8 - 9 2

1 7 - 3 0

17 .70

17. a3

¶ b. 58

I F , . C 6

15.57

1 4 . 0 9

14.64

14.2 1

13.79

13.40

13.03

12.67

12.33

12 .00

1 1 - 4 4

1 1 e 4 i )

11.12

10.55

t o . 5 9

13.35

10.12

T I V E ? M K k . I ) ---------

729.0

730.0

731.0

732.0

733.0

734.0

735. 0

736.0

737.0

738.0

739.0

740 0

741.3

742 .o

743.0

744.0

745.0

746.0

747.0

74e.o

749.0

750 0

7 5 1 . 0

752.0

753.0

754.0

755.0

-0 -48740-02

-0.47350-02

-0 -45F5D-92

-0.44540-02

-0 4 3 120-02

-0 -4 1700-02

-0.40270-02

-0.3RR4Q-02

-0.37490-02

-0 35 96 0-0 2

-0.3451 0-02

-0.33070-02

-0.31620-02

-0 30 L 70-02

- 0.28720-0 2 -0 2 7270-02

-0.25920-02

-0 -24370-02

-0.22420-02

-0.21470-02

-0.2002D-02

-0 18580-02

-a. 17140-02

-0. L5700-02

-0 14273-02

-0.IZRYD-02

-0. IB410-02

35.65

35.60

35.55

35.51

35.46

35.42

35.37

35.32

35.27

15.23

55.113

25 .13

35.09

35.04

34.99

34.94

34.90

34.85

34.80

34.75

34.71

34.66

t 4 . t I

34.57

34.52

34.4 7

34.43

5.51 7

5.400

5.259

5.184

5.004

4.990

4.900

4.814

4.734

4 658

4.586

4.51$

4.453

4.393

4.336

4.283

4.2’34

4.187

4.144

4. I04

4.067

4.033

4.002

5.974

3.948

3 - 9 2 5

3.905

2019.

1974.

1932.

1892.

1854.

1 9 1 8 .

1764.

1751.

1720.

169 1

1663.

i 6 3 7 .

1612.

1589.

1567.

1547.

1527.

1509.

1492.

1477.

1462.

1448.

1436.

1425.

1414.

1435.

1396.

5199.

5088.

4902

4591.

4785.

4694

4608.

4526.

4449.

4376.

4307.

4241.

4179.

4121.

4067.

4015.

3967.

3923.

398%.

3842.

3806.

3773.

3742.

37 14.

36 89

3663

3 6 9 J .

1267.

1240.

12 14.

1190.

1167.

t 145.

1124.

1105.

1086

L 0 6 8 .

1052.

1036.

1021 . 3 0 0 7 .

S 9 4 . 2

S R I .Y

S70.4

959.7

s49.7

940.4

53 1.9

S24.0

916.8

510.2

904.3

E99.0

e94.3

943.7

923.2

904.3

386.2

869. I

852.9

537.5

822.9

809. i

796. i

283.7

772.1

76i.1

750.7

741.0

731.9

723.4

715.4

708.0

701.2

694.8

6R9.0

683.7

678.8

674.4

670.5

667.0

72.69

7i.oe

69.42

6t2.23

h6.92

65-67

64.49

bJ.36

62.30

61.30

60.35

5‘1.45

5 8 - 6 1

5 7 . 8 1

57.37

56.37

55.71

55.10

54.53

54 -0 I

53.52

53.07

52.64

5 2 - 2 9

5 1-95

5 1 .h5

5 I .39

9.498

9.685

c).490

9.302

9.122

8.952

P. 791

8.638

8.493

R. 357

13.277

5.105

7.Q90

7 . 9 6 2

7. ?eo 7.585

7.596

7.512

7.435

7.363

7.297

7.236

7.180

7.129

7. $83

7.042

7.006

T I F E f M IN) REACT. IS 1

756.0

757.0

75R.O

759.0

760.0

761.0

762.0

763 e 0

764.3

765 -0

766.9

767,O

768.0

769-0

770 0

771 e 0

772.0

773.0

774.0

775.3

776.0

777.0

778 0

779.0

780a0

781 e 0

782 0

-0.49 4.30-03

-0.E577D-03

-0.71660-03

-0 576 I 0-0 3

-0.4362G-03

-0.29700-03

-0.1 5040-03

-0.20930-04

0.1 lbBD-03

0.25320-03

o . 3 a w m o j

0.523RD-0 3

0 6 5 7 R D - 0 3

0.79100-03

0 9 2 3 2 D- 0 3

0.10550-02

0 . 1 1 R5D-02

0 .1314D-02

0 .14430-02

0.15?00-02

0.16560-02

0.1 82 10-0 2

0 19459-02

0.250AD-02

0.21900-02

0.2 3 100-0 2

0.24300-02

34.38

34.33

34.29

-74.24

34.19

34.15

34.1 0

34.06

34001

33.97

33.93

,73.R@

33.84

33.79

33.75

33.71

33-67

33.62

33.58

33.54

33.50

33.46

33.42

33.3e

33.34

33.30

33.26

3.888

3. e73

3.860

3.850

3.843

3.838

3.R35

3.835

3.838

3 .a42

3.849

3.859

3.871

3.855

3 902

3.921

3.943

3.967

3.994

4.023

4.055

4.089

4.126

4.166

4.209

0.254

4.302

PRECURSOR CONCENTHATIaNS

1389.

1382.

1377.

1372.

1368.

1365.

1363.

1362.

1362.

1362.

1364.

t 3 6 6 .

1369.

1373.

1 3 7 R +

1363.

1390.

1397.

1405.

141 5 .

1425.

1436.

1448.

1460.

t474.

1439

1505.

3629.

3614.

360 1

3590

3582.

3576.

3573.

3571.

3572.

3575.

3581.

3599.

3598.

36110

3625.

3642.

3660

36-52.

3705.

3731

3759.

3790-

3823.

3859.

3897.

39 38 0

3981

e90.2

ee6.7

883.7

E 9 1.4

€79.6

E70-4

e77.7

e??. 6 0 7 8 . I

679.1

E R 0 . 6

E82.7

esC. 3

888.5

e 0 2 : 3

e96.6

4.01.5

$06.9

512.9

F19.5

F2b.7

934.5

442.9

S51 .9

961.6

5 7 1 . 8

982 II 8

664.0

661.4

659.3

657.6

656.3

655.4

65’5.0

654.9

€55.3

h56.1

651.3

654.9

660.5

6 6 3 . 3

bh6* 9

t69.4

673.1

577.2

581.7

665.7

692.1

698.0

704.3

7 1 1 e 0

719.3

726- 0

734.2

51.16

53.96

50.79

53.06

50.57

50.50

50.47

53.46

50rU9

50.5b

53.55

50.77

50.93

51.17

51133

5 1-59

51cRS

52-19

52.54

52.93

53.35

53.90

54.23

5 4 . 8 1

55.37

55.96

56.60

5.975

6.946

4.925

E . 9 0 R

6.894

6.685

6.881

b l n a i

C.385

6.593

6.1306

5.”)23

4.944

e. 979

7.035 & U

7.035

7.074

7.117

7,165

7.31 7

7.274

7.33€

7.402

7.4 74

7.550

7.431

7.718

48

01 0

30

h

h

ni

h

0

3

N

Q

e

d

U

01 v . m

N

0

4

c

N

5

Q 0

0.

e

m

@

c

5 . "4 . Y

In

e . h 0 0

M

. 9 b 0

U . 0. m M

,- I- O

U

U

W

n

IT

PI

N

0

l

U

'% u

ru 0

a 0

U

h .

0

0 3

,n

P) e

m 0

'I:

4

Q

IC

0

N

0

4

. m N

U

r(l

. m

In z ul a ut

4

B . m

rl

N

0

I a Q. b

N

0

r I

0

u7 k

e I

h

* 3

'0

Ipi

u1

m u7

.", . N

c

h

m

R 0

4

* m

d:

e .. Q

r- M

e

0

N

In

d . e c

n

m

N 0

I n

m

v pc hi

0

0

u? m IC

P- e c

m Q

4

!Y c

*)

\o 0

T

0. c

0

d

d a

m d . m

d 9

4

u)

(u

h

ut . 0

'3

m

m . ni

0

I

in

h

Ir:

0

n

n . 0

0

OD h

Q

3

.c 'T,

m

c

I

3

m T

VJ I

9 0 0

c

. r(

n

U

Q . 0. 9

d

.4 Q 0

h

U

ug

0. N r)

N

0 I c r?

PT m

m C

C

0 . E

m

0. 5:

cc.

- CJ

10 c h-

k

Q

w

N

m

d

d

ur r- m e N

N

5 h

In

m Q . 0

oc N

ri

N

0

1 PI U

M

m 0

n

0

N

K

d

d

0

D

ru R

9

n

Iu

0

.E m H

In

-4 I

. N

M 9

4 . 0

n

P- d

N

U

Q

Ln . 9

rc

N

m . N

0

I

9

e 9

n

n . 0 0

m . K

m N

c

0

0

m . k 4

ffi

* N

G-

P- Fl

N

..E rD 01 0' d

C

h

m

d

0

N

B

v) . .T b

N

C)

N

0

l a

K 0 d 0

0

c E

$7 in

0

r*

T

4

. r- e

d

0 0

c

0. r: "1

P

m 0 ut . p. N

0

N

m 9 9

v) . .. 9 N

PI

. N

0

I n e 0

c B

0

0

&

0

a-!

M

r- 0

r(

4

d

Q .. N

N

0

.-I

b 0

2 a

M

'a 4

. D G 0

N

N

01 5

In

0

Ln

N

m

N 0

t a ;f; d d 0

@

N

0 4

.

53 G"

0

0

'0

3 9

d

Q 0

.d

v? Q

P

c

. m

m 9 In

N

4

d

N

0

N

a

d

5: n

N

R

N 0

I a

c?

u7 r

CJ

0

m

Q

w

ry N

I

9

N

rb 0- . c Q

0

r(

e a

N

U c

m

VI r- M

. IC

m

N

6

e

10 N

9

R1 n

N

m . N 0

I a

0

Ln 9

Q

0

0

a 0

m

r- e3

+

- m 3

f

m

0

01 3

- 9

s . N

U

CE m

e d 0

N

N

m

0. m

c . .-4 m * N

m

N

0

I 0

Q

hi e

0

0

C

cn 0

(u

0 0

Rl

.... e

8 . L 3i

,A

d * c . P

N

? ... 0 9

4

U 0

P,

N

m 9

9

as . '0

0

N

m . N

0

d 0'

(r u? d

0

0

r- 0 W

X

N

N

d

N

0

0

b

?- 9 r*

.-*

4

Q

2 . m

Q

N

8 . d)

Ui n

N

0

c

a

m . m

B

N

r)

N

0

1 0

0

m

Q

* 0

0

a 0

QJ .

A

rrl hl

n

Q

m 0

Q . 0

nr U (r . . m

.j

0 . 0

* N

d

0'

0.

2 m 02 v,

U . c 0

m m

(L 0

t a m 0

i?

0

C

Ir.

e a

r. P?

2

d

'u

d)

Lo 4

G

'3

P . io . N

I? ..I

r"

e Ln 01 N

M

. P- m

2 Q

4

P-

m . d

? N

m N

0

I D

4

m

a 0

4

0

0 0

W

v)

z a

-4

+" 4

x c Z

w V

z 3

I)

5

G

v)

2

W

w

n! a -

1

*I

N

N

m .

T I C E ( Y 1 N ) --- -- -- --

P1J.J

E l 1.3

e12.0

e l 3.0 P 1 4 . 0

e i5 . s

816.0

e17.3

818.0

P19.0

P23r 3

e21.3

F22.0

823.0

P 2 U . D

e25.0

fJ26.0

e27.3

62.3.0

e29.3

P30.0

e3t.o

P32.0

e33.0

834.0

P35.0

836.0

0.5J840-02

0 - 5 1 47 0- 0 2

0.520AD-0 2

0.52650- 0 2

0.5320L7-0 2

0.52710-02

0 s 5 4 l9D-0 ?

0.54640-02

0.55060- 0 2

0.5 5450- 0 2

0.55L?JD-02

0 5 C, 1 1 3-3 2

0 . S h 7 Q P - 0 2

0.5663D-02

0 50 E3D-02

0.509YD-02

0.57110-32

0.57 1 9D-0 2

0 r5723D-02

0 -5 7 230-0 2

0.57 180-0 2

0.5709D-3 2

0.56950-02

0 .Sh 77 P O 2

0.56530-02

0.562SD-02

0 -55920-92

32.39

3 2 - 7 7

22.35

52.33

32.31

22.30

32.28

32.27

32.25

32.24

'2.23

32.22

32.21

32.20

32.20

32.1q

32.19

32.1 e 32.18

32.1 e

32.1 8

32.19

32.1q

32*20

32.20

32.21

32.22

7.173

7.347

7.527

7.714

7.908

9.108

9.31 5

9.530

9. f 5 L

3.980

3.217

4 .4b l

9.713

9.972

14.24

10.52

10.80

11.09

t 1-39

11.70

1 2 - 0 1

12.34

12.67

13.01

13.36

L3.71

14.07

P H E C U R S O R CONCENTRATIONS

2468.

2526.

2584

2651

2716.

278 1).

2854

2927.

3002.

30AO.

316 1

324 4

3329

3410.

352 9

360 3.

3700.

3799 . 390 2

400 7.

4 1 1 6 .

4zz7 .

4 3 4 0 . 445 7.

4577.

4699.

4823.

6594.

6753.

691 7.

70 88

7265.

7448.

763?.

7833.

BO 36.

F?245.

8462.

8685.

8916.

9154,

9399.

9 6 5 1

9 9 1 1 .

3.1010D 05

0.10450 0 5

5.10740 '35

0.11030 05

0.11320 0 5

0.11633 0 5

0.11940 O S

0.12260 0 5

0.1259D 05

0.1292D 05

t636 .

1675.

17 16.

175.7.

1803.

1848.

1896.

1944.

1995.

2047.

2 1 0 1 .

2156.

2214.

2273.

2334.

2347.

2451.

2528.

2596.

2666.

2738.

2812.

2389.

2'365.

3044.

3125.

7207.

1223.

1253.

1284.

1316.

1348.

1383.

141f3.

1454

14c12.

1531.

1572.

Ib13.

1656.

1700.

1746.

1793.

1841.

1891.

1942.

1945.

2048.

2 : 04.

2 1 0 0 .

2213.

2277.

2338.

23 3 9 .

94.35

96.64

c 3 9 . 3 1

131.5

134.0

1 3 6 . 6

1 O G . 9

112.2

1 1 5 . 1

t t R . 1

t d l . 2

124.4

1 1 7 . 7

L 3 1 . 2

1 3 4 . 7

138.3

142.0

t 4 5 . 9

143.8

153. Q

156.0

542.3

I hhr 6

L 71.1

1 r s . 7

L 83.3

L 8 5 . 1

12.d7

l ? . i P

13.53

13.H4

1 4 . I R

14.54

14.92

15.3d

t5 . T O

3 6 3 . 1 1

16 .53

I f , . 47

17.42

t 7. %%

1n137 4-

\ d. 86

1 '3 .37

19.84

25.43

79.98

21 .55

22. L 3

2 2 . 7 2

21.33

2 3 . 4 0

24.59

25.24

u4

T I C E ( M I h r 1 --------- P 3 7 . 0

836.0

e 3 9 . 0

e40.0

8 4 1 . 3

F42.0

843.0

e44.0

845.0

€346.0

P47.3

€548.9

“9.0

850.0

(351.0

P52.0

t3571.0

P54.0

855.0

e5t5.0

P 5 7 . 0

e 5 f l . o

e 5 9 . o

260 .o r?61.0

267.0

863.0

O 55549- 02

0.5528D-02

0.5463D-02

0.54 1 OD-0 2

9 -53570-02

0.52”RO-O2

0 .5% 1 9 D - 3 2

O.Ci45D-02

0.50650-02

0 4 9 R O 0-0 2

9.489YD-02

0.4793O-OZ

0.465213-02

0.45860-02

0 44 74 0-0 2

0 4 3 5 70- 0 2

0 42350-02

0 . 4 I O R O - 0 2

0 3 9 750-02

0.383RD-02

0.76470-02

0.355017-02

3.34000-02

0.3 2450- 0 2

0.3 0869-02

0.2 9230-0 2

n . 2 756~1- 02

32.24

32.25

32.27

32.28

22.30

32.32

32.35

32.37

32.40

32.42

32.45

2 2 - 6 9

32.52

32.55

32.59

32.63

32.67

32.71

32.75

32.80

32.84

32.89

32.94

32.Y4

’3.04

33. k 0

33.15

14.44

114.81

15.20

15.5R

15.9B

15-37

1 6 - 7 6

17.18

17.59

19.00

L8.41

1 a. 8 3

19.24

19.66

20.07

20.49

29.88

21.25

7 i r 6 a

22.06

22 4 4

22.82

23.1R

23.52

23.86

2 4 . 1 4

24.49

495 1.

508 1.

5 2 k 3 -

534 7.

5484.

562 2

5763.

590 5

6048.

6193.

633 5

6454.

663 1

6777.

6 9 2 4

7070

7215.

7359 0

7502.

764 2

7780.

7 9 1 6 .

8048.

8177.

a302.

8423.

8539.

0 . t 3 2 6 0 0 5

011360D 05

0.1396D 0 5

0.14310 35

0.146RD 05

0.15040 05

0.t592U 35

0.15790 05

5.16170 05

0.1655D 05

0.16946) 0 5

0.17320 0 5

0.17710 0 5

0.1809D 0 5

O.IR48D 05

0 . 1 R 8 6 0 o s

0.1924D 05

0.19610 35

0.19980 0 5

0.20350 0 5

0.20710 0 5

0.21060 0 5

0 .21400 0 5

0.2’1730 0 5

0.22050 0 5

0.22350 0 5

0 0 2 2 6 5 0 05

329l

2377.

2464.

?552.

‘642

3733.

1825.

7917.

4011.

4 105.

4 199.

42’34.

4389.

4404.

4579.

4672.

4764.

4356.

4947.

5936.

5123.

5208.

5291.

537’1.

5449.

5523.

5594.

2462.

2526

2591.

2657.

2?24.

2792.

2.961.

2930

30d0.

3079.

3 9 4 1 .

321:.

3282.

3353.

3423

3493.

3562.

3630.

369d.

3 7 6 4 .

382ci

3893.

3954.

4 0 9 4 .

4072.

4 1 2 7 .

41~0.

1 dY. ‘9

190. -2

139.7

2 15. i)

2 1 3 . 1

215.4

2 2 0 . b

226.0

2 3 1 . 4

P36.B

242.2

2+7.7

’53. I

258.5

264.0

269.3

2 74.7

790.0

285.1

200. -3

255 . .+ :so. 1

3 0 4 . Y

309.5

323.c)

318.2

322.2

25.90

20.57

27.26

37. ‘15

29.66

29.3 7

39.04

30.32

31.55

32.29

73. 0 3

3.3. 7 7

14-52

35.26

27.4 b

39. t 8

38. t3H

3.9.5e

a0.26

Q 0 . 93

4 1 . 5 7

42.25

42. R O

43.3e

43. ’j4

T I Y E ( Y I N 1 - -- €64.0

e65.0

er5fi. 0

867.0

F6R.O

P69.0

875.0

e7 1 .o B7?.0

R73.0

e74.0

875.0

e76.0

E77.0

P78.O

R7'i.O

880.3

ea1.o

887.3

883.3

P 8 4 . 3

885.0

PR6.0

887.0

688.0

P8Q.O

e90. s

0.25970-02

0 24 140-02

0 22380-02

0.2059D-02

O.le7RD-02

0.16S5D-02

0.15 110-02

0 13240-02

O.ll38D-02

0.94570-a3

0 7 6 1 3D-03

0.5727U-03

0.35420-03

0 I S63D-0 3

0.9 1260-05

-3 a 17590-0 3

-0.36 140-53

-0.54620-03

-C* 72500-03

-0 90340-03

-0.107r)D-02

-01 1252G-02

-0.14"O-02

-0 a 159ao-02

-0.i7~10-02

-3 19090-02

-0 a20640-02

33.21

33.26

33.32

33.38

33.44

73.50

33.56

23-62

33.68

33.74

33.130

33.87

33.93

23.9.4

34.05

14.1 1

34. I 7

34.23

34.29

39.35

34.40

34.46

34.52

34.57

34.62

34.68

1'4.73

24 79

25.06

25.32

25.56

75.78

25.99

26.16

26.32

26.45

2 6 - 5 7

26.65

26.72

26.77

26.79

26.79

26.77

26.72

?6.*5

26.56

26.45

26.31

26- 16

25.99

25.80

25-59

?5.37

25.13

PRECURSOR C O N C E b i T R A T I O N S

8649.

5755.

8855.

8946,

90.35.

91 15.

91a9.

9255

9313.

9364,

9407.

944 1.

9469 .

9487.

9497.

4500

9 4 9 4

94'30

9459.

9 4 2 9 -

9392.

9348.

9296.

9230.

9L73.

9102.

9 0 2 4 -

0.22930 05

0.23200 0 5

0 0 2 3 4 4 0 05

0.23680 35

0.27R9D 05

0.24090 0 5

0 - 2 4 2 7 D 0 5

0.24429 0 5

0.24560 0 5

3.246RD 05

0.24770 05

0.24850 05

0.24900 05

0.2493D 05

0.24950 05

0.24930 05

0.24900 05

0.24850 55

0.247eo o s 0.24688 O S

0.24570 05

3.24440 05

0.2429D 05

0 ~ 2 4 1 2 0 35

0.23940 05

0.23740 05

0.23520 0 5

5662.

5 725.

5765 .

5 4 4 1 .

5892.

5938.

59830-

6017.

6049.

6 0 7 5 .

E097.

6L 13.

0124.

6 1 30.

8131.

0126.

6 1 1 6 .

c131.

6081.

C056.

6026-

5992.

5954.

5 3 1 1 .

5864

5513.

5759.

4230

4277.

4321.

4362

4400.

4435.

4465.

4493 I)

4516.

4536.

4551.

4563.

4571 e

45 75.

4575,

4571 *

4503.

4552

45%.

4517.

44 95.

4459.

4440.

44 38.

4 3 7 2 -

4334.

4293.

326.1

329.7

333.1

3 36.3

339.2

141.8

344.2

3.16.2

343.0

3 4 9 . 5

350- 7

5 5 1 . 6

352.2

352.5

7 5 2 - 5

3 52.3

351.6

350.7

349.5

448.0

3464.3

344.3

342.U

354.5

53e. n

3 3 3 . 6

3 30.7

44.46

44.56

45.42

45. Y 5

46-25

4:>.51

41,. 43

47.2 1

47.45

47.46

47.93

47-94

4%. 5 2

431 5 6 cn

48. O h w 4%. 0 2

47.35

47.81

4 7.65

47.45

617.21

U b . 9 4

6615.3

45.25

45.92

45.51

45.08

R E A C T . < % )

P91.0

e92.0

e93.0

1394.0

e95.3

e96.0

E97.0

P O f l . 0

899.0

soo.0 401.0

502.0

so2.o

504.0

405.P

506.1)

F07.0

408.0

S09.7

Sl0.0

SI1 .o

FLT.3

213.0

4 14.0

C15.0

416.3

417.1

-5.2214D-02

-0.23600-02

-0.7507f3-02

-0.263eo-07

-0.2770D--32

-0.2 ~ 9 7 0 - 0 2

-0.30 I e O - 32

-9.3 1-45e-02

-0.32460-07

-0 - 3 3 5 2 D - 0 2

-0.34520-02

-0 ?54?3-02

- 0 . 3 c 3 7 0 - 0 2

-0.3 721 0-02

-0.3749r)-02

-0.3 4 73D- 0 2

-0 3941 P O ?

-0 - 4 0 C 3 D - 0 2

-0.406 10-0 2

-0.41130-02

-0.41600-02

-0.42020-32

-0.4238D-02

-0 ~92700-02

-0 9 2S7D-0 2

-0.43199-02

-0.43373-02

34.78

3 4 . a ~

34.R7

34.4, I

3 4 . 9 6

3s.o 0

35.04

3 5 . 0 P

35.1 I

35.15

35.18

35.2 i

35.24

7 5 . 7 7

-75.29

25.32

35.34

35.36

35.38

35.40

35.4 1

35.4 2

35.44

35.45

35.46

35.46

35.47

2 4 . ~ 7

2 4 . 6 1

24 .33

?4.03

23.73

2 3 - 4 2

23.10

22.77

?2.43

22.09

21.75

p i . 4 0

21.05

20.70

20.34

1 Q. 99

19.63

19-28

1 8 - 9 3

1 e.58

18.23

i 7 . m

17.54

17.21

1 6 - 5 7

16.55

14.22

8942.

0853.

8760.

866 2.

8560.

R455.

934 5.

8233.

81 17.

9000.

7580

7758.

7635.

7 5 1 1

7386.

726 d.

713s.

7009.

6384.

6759.

6634.

6511.

6309.

626 7

6148.

6029.

5913.

0.23290 o s 3.23050 0 5

0.22790 0 5

0.22530 0 5

0.22250 0 5

0.21960 3 5

0.216TD 05

0.21370 0 5

0.21060 0 5

0.20750 0 5

0.20430 0 5

0.20100 05

0.19789 0 5

0.19450 05

0 . 1 9 1 2 0 0 5

o . i n 7 ~ 0 5

0.18460 05

0.19130 0 5

0.17803 05

0.17470 0 5

0.17150 05

0.14830 05

O.LQSI0 0 5

0.16190 0 5

0 . 1 5 8 8 D 05

0 -15570 0 5

0 . 1 5 2 7 D 0 5

5 7 3 1 .

5640.

5576

5 5 1 0 .

5-44 1.

5370.

525.7.

5222.

5 145.

5068.

4 9 8 9 .

4909.

4 9 2 9 .

4748.

4667.

4526.

4504.

4423.

lt343.

4 2 6 2 .

41 83.

9104.

4026.

3949.

2R?3.

'796.

3724.

4250

4205.

4157.

4107.

4055.

4002.

3947.

3891.

38 34.

3776.

3717.

3655.

35S8.

3537.

3 4 77.

3414.

3356

3795.

3235.

3 1 75.

31 16.

3057.

2999

2941.

2R85.

2829

7774.

327.3

3 2 3 . h

370.1

3 1 C . J

712.3

3Q3.2

394.0

2q9.7

2 J 5 . 3

270.5

286.2

2t31.7

217.0

372.4

267.7

? b3.0

25fl.4

253.7

24'2. 1

244.5

? 3 9 . Q

2 35.4

233 .9

276.5

2 2 2 . 1

217.8

213 .5

I-__--- --- a 4 . 6 3

44. I5

4 % . h Y

4 3 . 1 2

42.58

42.07

41.44

43. (35

40.25

31.64

3 Y . 02

3 21 . 4 fJ

37.77

3 7 . 1 3

36.50

35.86

35.22

34.54

3 3 . 9 4

3 3 . 3 3

3 2 . 7 0

JZ. o q 3 i .4R

30.87

3 0 . 2 . e

2G.69

7Y. 1 1

53

L? Z

5

Y c

d

ir c

z W

U

z 0

V

Q

v)

U 3

U

W

a a

a

d

m

E

N

d

3

C

N

0

nl h

N

c1

Lo 9

m

Lo 0

0

b

O

U - . 0 m

01 b

in

-I

Z

I

W

CI

N 0

I O 0

M

m

Q

0

I . al (P

h

N

P)

0

0

ni

ul

Q

9

N . 0 a: M

PI

M 0

0

m

u)

d 1

. 0 . Lo m

9

m 0 0

in . 4

ar 4

e M

pr)

N 0

I 0 J) m

m

* 0

I n

rj\

0

Lo

in

V)

ul

MM

ml

ni

n

OC

OO

OO

OC

O

bb

0Q

Q.

M h

d

mm

mo

c1

0m

op

?

n)

ml

lF

)N

NR

IN

-

-r

le

+m

-t

-~

-

......... 0

00

00

00

00

on

oo

on

o_

c~

n

RN

N

00

0

Il

l

oc

lo

h

m

ri m

m

$%

.. e

bb

0

00

I

ll

*e

. N 0

I 0 0

N

m

* 0

I . N

cu

0

0

II

O

h

c(

c

r)

N

Qd

00

I

1

no

.. ry 0

I 0. .4 N

Q

0

I

n .

h

d

rJ

N

4

N

\o

... . nr .- ..(

iL . Lo m Q

N

ln 0 0

N

2 CI

. 0 0

@

0

* 4

M

m

N

4

d

d

Lo . VI

N 0

I aD 4

4

0

n d

0

..

# m

6P

9

T)

d

N

c 0

,n +

UI

"j 0

N

. N

m b

N

M 0

0

N

m

a 4

. 0 . m

m R

Q

CI

0

4

r.

6

m rl, m N O I UI

ro 0 d

0

I

a . 0

m

m

0"

UJ Q.

0

o!

rn r)

in 4

. c@ LY 3 e

m

m R M 0

n 0 0

-I

4 * 0

m M

N

e 3 9 . m -. P- m . in IT

N 0

I n O

N

O

6. 0

I 0

d

m

v

0

4

n

N

. -. b7 e

rl sr e

-4 . in m

UJ N

M 0

a 0

m 0

..I e 0

. 9 h d c

a, d . r

*

VI m

Lo rn

N

0

I 0 m

h

P

m 0

I c

U! Po w

4

N

0

N

n UJ

U

d

a N

0

-4 e

CD in IU

a

M 0

2 ro 0

0

L . . N 0 4

* Q

N . * r?

M

rI

? N 0

l

0

N

P

m

0

I

a 0

0

17 v . o* c I

0'

rt

4 3

VI * cc - . m 4

M

tu

M

0

0

01 # 0

4 . 0 6

N

0

U

m 0 * - -. N

m

Lo . ri

N

0

I 0

a

m rs 0

I

n . 0

h

VI (P

. in in

.T. ... 4

rl 3 d

. rv c m -.(

0 0

u)

<u

m 0

0

4

N 0

.*

0

. o\ In 0.

p1

0

T 0

d

0

'1 w- R

N

0

I 0 3

m

m 0

I

e

3

h

Pl

I? . N

N

". e

0 * - .t

.d . ")

m

I

IC 0

Q

N

in 0

h 0

0

a - . 0

..(

CI. m

rr)

I

b

0

w

N

m

m . N

O I 0

ur h

F1

0

I

4

0

0,

m

w

in N

a

..I N

U

r)

. ..I * p*

Q

b

r( P @

m m

N

. t? h

U) (r . 0

0

c

r)

d

N . 0 d

N

N

Lo m

N

0

l rl u in P

)

0

1 a 0

N

d

CF ... 13

m

- ... * ,m n .=4 2 IC

4

. N O

m

N

e r- (u

d

@ . 0 4

9

R

e

0

0

4

CI. * M

m 4

N

0

I D 9 6

* rl 0

I 0

m

d

L" . r) c c

.. P

" 0 r)

d

. 0. oc Q

4

. 9 iD N

N 0

0

N

(r

m e N

m

M

m

N

m

m

0.

h

d

* Lo m

N

0

I 0

r- c\i

* m 0

I

0

4 d

* VL

54

cir 9

n

-4

d N

m OI . M

c

N

1

. d

0

r. .-4 e N

c

01 Q

(F

Q

9

N

9

9

d

r- N

B

U m . N

0

l a e

m c

- . 0 I

0 . M

c 0

9N

P

Or

-

In in

P- B

0

>I

a

rl .

.A

d

m

r- 8 c

9

r. 0

I

. 0 m 0

m

0

4

@

r-l 0

N

9

c . N

Q. VI ru 0

I 0 0

m

rD

N

0

I

0

B

VI w

. 0

U

4

e

N

4

4

9

In

4 2 01 4

d

9

@

h

rn IC

0

m

0

N

m

U

0

[o

* PJ

N 0

I 0 c

m

N

0

I

r(

0

Lo M

lr . d

+

I

-4

0.

c . 4

d

rn rl

Q c

. m

e r

(

. p- 0

m

r- . P- r? 0

m In N

Q

m

3

a: U

m . N 0

I n

9

W

Q

P4

0

I 0

9

VI w

mP

>

r-

d

N

BY;

Md

wm

.. -

4

-lr

mr.

CI

c

p7

,

..

.. O

'N

@a,

NN

-4

*

.* W

(cc

N2

-

c

.I

0

0

no

0

0

be

.. *

*

om

e

a

NN

r-

m

eo

In

0

.. r

-r

.

Q'

VI $

4

*i

t

PI

IC,

NN

0

0

11

0

Nr

)

rn

N

I(

*

.. 0

0

II

00

.. 0

8

Qr

.

0' LP

a0

Q

N

.. m

0

d

N

.D

.4

..a . m 0 m d v)

N 0

N

. m

m

N

m

r(

2 0 m

m

m U

c

0.

* ri

01 0

l 0 O

N

u. rrl

0

I

c . N F U'

d

0

4

m

* .. 4

. .. cp * c . 0

0

0

IU

3

r- m

0

m

m ..I d N e

U

UI

? 'Y ci

N 0

I 0

'4

rl r- N

0

I (3

m m

LP .

Q

9

4

CF 0

hl

4

0

t- VI -4

e e 0

tu ".I . -4 N 9

m

it N

P

) PI

01 rl:

0

.1 . m 0

m

r1

(L 0

I 0

e

w 0

9- 0

I c? 0

0

U' .

.ct .I

t- CII 13 . 4

. ,9 Q

.- . 0 0

4

. Q 0

m

r.

N

3 0

m rl m m

o? e

m Q

m

nl 0

I

0

u

d

N

0

l n

0

P- IP U

' . d

F. In

W 0

d

01 0

f 0

o 0

.e a ;c) N

F. h

5- 0

OI

N

0 e

N

lr - ll Q . r)

N 0

I 0

m ". m

N

0

0

m

M

w .

.. 17

0

.I

m

N

r*

I?

9

Q

d

N

m

N

tu . m

m

Q

..4 . c N

M

m

..

N

0

I n

IC

NN

NN

0

00

0

m

m

r? 0

I

.... Q

OO

O

Il

l1

-I

Z

I

00

0c

TIVE(MIN) YEACT. ( 0 I

572.0

S73.0

574.0

975.0

57&.0

577.0

S78.9

479.0

F 8 O .O

461.3

582.3

583.0

584 .o 585.0

586.3

SR7.0

408.0

S R 9 . 0

$90.0

s91.0

592.3

993.0

994.0

595.0

S96.0

997.0

598.3

-0.1047D-02

-0.95510-03

-0.86310-03

-0.77120-03

-0.6754 0-03

-0.5 @ 77D- 03

-0.49630-03

-0.40520-03

-0.3 1430-03

- 0 2 2380-0 3

-0.13370-03

-0.43990-04

0 4 5240-04

0.13400-03

0.22225-03

0.30580-03

0.3568 0-0 3

0 ~ 4 8 3 1 D - 0 3

0.56880-03

0.65370-03

0.73790-03

0.82 120-03

0 9 (I 370-0 3

0 98540-03

0.10660-02

0 P 1460-02

0.12250-0 2

74.39

34.36

34.33

34.30

24 e 2 7

34.24

34.21

34.18

3 4 - 1 6

34.13

34.1 0

24 07

34.04

34.01

33.9e

33.95

33.92

33.89

13.87

33.84

3 3 . 8 1

33.7e

33.76

33.73

33.70

33.68

33.65

7.431

7.399

7.3ro

7.344

1.322

7.302

7.286

7.273

7.263

7.256

7.252

7.251

7.252

7.257

7 .245

7,275

7.289

7.305

7.325

7.347

7.372

7.401

7.432

7.466

7.503

7.543

7.585

2655.

2642.

25.30.

2620

2510.

260 2

25514

2588

2503.

2579.

2576.

2575.

2574

2574.

2575.

2578.

2581.

2586

259 1

%59 R I

2505.

261 4.

262 3

2634.

2646.

7659

267 2

6937.

6906.

6877.

6852.

6829.

6810.

6793.

6779.

6768.

6760.

6755 .

6752.

6752.

6755.

5?6 I >, 6769,

6780.

6794.

6811.

6830.

6852.

6B77.

6904.

6934.

6967.

7003.

7041.

1702.

1694.

1687.

1681 . 1676.

1672.

1648.

1665.

1662.

1661.

1659-

1659 .

1659.

1660.

1662.

1664.

1667.

1671.

ie75.

1680.

1666.

1652.

1699.

1707.

1716.

1725.

1734.

1269.

12G4

1259.

1254.

1250.

1247.

1244

1242.

1240.

12.39.

1238.

12.38.

1239.

1239.

1 2 4 0 .

1242.

1245.

I247

1251.

1254.

1 2 s .

1263.

!269.

1275.

1 2 c r I .

1288.

1295.

37.78

97.36

96.93

96 -64

96.034

9 h . O Y

95.87

92.717

95.51

95.47

95.42

93.40

45.42

$5.49

95.59

95.73

c15.99

96-12

90.33

96.67

97.00

17.37

97.73

Y U . 2 . 3

9 8 - 7 1

99.24

99.~30

13.33

1 3 - 2 7

13.22

1 3 . 1 a

13.14

1 3 . 1 0

t 3 . 0 7

t 3.05

13.03

1 5 . 3 2

1 3 . 0 1

13.01

13. J 1

13.02

33.03

13-05

13.158

1 3 . 1 1

13 .14

1 3 . 1 8

13.23

13.28

1 3 - 3 3

13.39

13.46

13.53

13.61

56

3r

D

01

.

-1

z

i

-1

:

"I,

0

n 0

+ VI I

N

0

U

I

a

-

57

ORNL/@SD/TM-210

INTERNAL DISTRIBUTION

1. R. C. Baker, PAD 2. D. E. Bartine 3. H. P. Carter/G. E. W h i t e s i d e d

C S L ib ra ry 4. Y. Chen, K-25 5. J. G. Cleveland, Y-12 6. D. H. Cook, K-25

7-11. H. L. Dodds, Jr. 12. H. R. Dyer, K-25 13. J. Dykstra , Jr., K-25 14. M, E. Easter 15. E. P. E l l i o t t 16. W. W. Engle 17. G. I?. Flanagan 18. D. W. Frye 19. P. W. Gaffney, Y-12 20. U r i Gat, Y-12 21. W. R. Gol l ihe r , 8-25 22. G. L. Grametbauer, K-25 23. S. R , Greene, Y-12 24. C. M. Hopper 25. J. C. Ingram, K-25 26. J. 0. Johnson 27. W. C. Jordan

28. W. T. King 29. A. J. Eegeay, K-25 30. J. T. Plihalczo 31. E. M. Oblow 32, R. 3. Renka 33. E. 0. Sternberg , K-25 34. R. G, Taylor , Y-12 35. J. T- Thomas 36. J. L. Thompson 37. R. D. Timerman 38. F. M. Tinch, K-25 39. €3. E. Vaughn, K-25 40. D. R. Vondy 41. C, W. Walter, PAD

42-46. R. M. Westfall 47* B. A. Worley

48-49. Cen t ra l Research Library 50. Y-12 Document Reference

Sec t ion 51-52. Laboratory Records

53. Laboratory Records - RC 54. ORNL Pa ten t Sec t ion 55. K-25 Plant Library

EXTERNAL DISTRIBUTION

56. J. M. Rogers, Div. 8324, Sandia Labora tor ies , Livermore, CA 94550 57. Div is ion of Engineering, Mathematics and Geosciences, DOE,

Washington, DC 20545 58. Office of Ass i s t an t Manager f o r Energy Research and Development,

DOE-ORO, Oak Ridge, TN 37830 59. R. H. Odegaarden, Transpor ta t ion Branch, Of f i ce of Nuclear Material

S a f e t y and Safeguards, Nuclear Wegulatory Commission, Washington, DC 20555

60. Michael V, Gregory, Savannah River Laboratory, Aiken, SC 29801 61, R. B. Perez, Univers i ty of Tennessee, Knoxville, TN 37916 62. Larry Miller, Univers i ty of Tennessee, Nuclear Engineering Dept.,

Knoxville, TN 37916

58

EXTERNAL DISTRIBUTION (CONT’D)

63. R. W. Tayloe, Goodyear Atomic Corp., P. 0. Box 628, Piketon, OW 45661 64, K. D, L e w i s , G o o d y e ~ Atomic Corp., B. 0. Box 628, P ike ton , OH 45661 65. J. G e m , Gaodyear Atonic Cokp., P. 0, Box 628, Piketon, OW, 1-65661 66, M. L. M i l l i a m s . Louis iana State Un ive r s i ty , Nuclear Science Center ,

67. E. M. Katz, Univers i ty of Tennessee, Knoxville, TN 37936 68. T. W, K e r l i n ? Univers i ty of Tennessee, Knoxville, TN 37916 69. A. F. Henry, Massachusetts I n s t i t u t e o f Technology, Nuclear Engineering

‘70. A. C. Hindmarsh, Lawrence Livermake Nat ional Laboratory, P. 0, Box 808,

71. W. R. Rhyne, H&R Technical Associates , Inc., 977 Oak Ridge Turnpike,

72. Ed F u l l e r , Technology f o r Energy Corporation, One Energy Center,

73. J. C. Robinson, Technology f o r Energy Corporation, One Energy Center ,

74. R. E. Pevey, Savannah River Laboratory, Aiken, SC 29801

Baton Rouge, LA 70803

Dep t, e , Cambridge, MA

Livermore, C A 94550

Oak Ridge, TN 3 7 8 3

P e l l i s s i p p i Parkway, Knoxville, TN 37922

P e l l i s s i p p i Parkway, Knoxville, TM 37922

75-101, Technical Information Center, Oak Ridge, TN 39831