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Scintillation in Liquid Noble Gases Alexander Neumeier 1 Martin Hofmann 1 , Thomas Dandl 2 , Thomas Heindl 2 , Jochen Wieser 3 , Andreas Ulrich 2 1 Physik-Department E15 2 Physik-Department E12 Technische Universit¨ at M¨ unchen 3 Excitech GmbH Schortens, Germany 29.11.2013

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Page 1: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Scintillation in Liquid Noble Gases

Alexander Neumeier1

Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,Andreas Ulrich2

1Physik-Department E152Physik-Department E12

Technische Universitat Munchen3 Excitech GmbH Schortens, Germany

29.11.2013

Page 2: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

1 Noble gases - An Overview

2 The Scintillation Process in Liquid Argon

3 Detector Concepts

4 Liquid Noble Gas Experiments

5 Summary and Conclusions

Page 3: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Motivations in Particle Physics

Liquefied noble gases well suited detector medium for rare eventsearch

Efficient scintillation medium with high light yields”Easily” scalableChemical purification up to a high level of purity

Good background suppression needed

⇒ Particle discrimination on an event-by-event basis

⇒ Detailed investigation of scintillation propertieswavelength- and time-resolved

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 3 / 18

Page 4: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Motivations in Particle Physics

Liquefied noble gases well suited detector medium for rare eventsearch

Efficient scintillation medium with high light yields”Easily” scalableChemical purification up to a high level of purity

Good background suppression needed

⇒ Particle discrimination on an event-by-event basis

⇒ Detailed investigation of scintillation propertieswavelength- and time-resolved

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 3 / 18

Page 5: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Scintillation of Noble Gases (e−-beam induced)

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 4 / 18

Page 6: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

VUV Scintillation Efficiencies (e−-beam)

Morozov et al. J. Appl. Phys. 103, 103301 (2008)

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 5 / 18

Page 7: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Possible Candidates for Detectors

Helium and Neon1

Boiling temperature far below LN2 → cooling rather expensiveScintillation light dominantly emitted at λ <90 nm → no transparentwindow materials

ArgonSuitable candidateLow priceNatural atmospheric argon: 1Bq

kg of 39Ar (β-decay, T 12=269a,

Q=565keV)

KryptonIn principle suitable candidateBut non-negligible traces of 85Kr (β-decay, T 1

2=10.75a, Q=687keV)

XenonSuitable candidateHigh A → High σ for coherent WIMP scatteringHigh price due to low natural abundance

1LNe considered as an option in the MiniCLEAN experimentAlexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 6 / 18

Page 8: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Possible Candidates for Detectors

Helium and Neon1

Boiling temperature far below LN2 → cooling rather expensiveScintillation light dominantly emitted at λ <90 nm → no transparentwindow materials

ArgonSuitable candidateLow priceNatural atmospheric argon: 1Bq

kg of 39Ar (β-decay, T 12=269a,

Q=565keV)

KryptonIn principle suitable candidateBut non-negligible traces of 85Kr (β-decay, T 1

2=10.75a, Q=687keV)

XenonSuitable candidateHigh A → High σ for coherent WIMP scatteringHigh price due to low natural abundance

1LNe considered as an option in the MiniCLEAN experimentAlexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 6 / 18

Page 9: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Possible Candidates for Detectors

Helium and Neon1

Boiling temperature far below LN2 → cooling rather expensiveScintillation light dominantly emitted at λ <90 nm → no transparentwindow materials

ArgonSuitable candidateLow priceNatural atmospheric argon: 1Bq

kg of 39Ar (β-decay, T 12=269a,

Q=565keV)

KryptonIn principle suitable candidateBut non-negligible traces of 85Kr (β-decay, T 1

2=10.75a, Q=687keV)

XenonSuitable candidateHigh A → High σ for coherent WIMP scatteringHigh price due to low natural abundance

1LNe considered as an option in the MiniCLEAN experimentAlexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 6 / 18

Page 10: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Possible Candidates for Detectors

Helium and Neon1

Boiling temperature far below LN2 → cooling rather expensiveScintillation light dominantly emitted at λ <90 nm → no transparentwindow materials

ArgonSuitable candidateLow priceNatural atmospheric argon: 1Bq

kg of 39Ar (β-decay, T 12=269a,

Q=565keV)

KryptonIn principle suitable candidateBut non-negligible traces of 85Kr (β-decay, T 1

2=10.75a, Q=687keV)

XenonSuitable candidateHigh A → High σ for coherent WIMP scatteringHigh price due to low natural abundance

1LNe considered as an option in the MiniCLEAN experimentAlexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 6 / 18

Page 11: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

The Excimer Potential

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 7 / 18

Page 12: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

The Emission Spectrum of Liquid Argon

Hofmann et al. Eur. Phys. C (2013) 73:2618Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 8 / 18

Page 13: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Gas Kinetic Processes

Incident particle χ

? ? ?multiple ionisation

Ar + χ→Ar x+ + x · e− + χ′

excitation

Ar + χ→ Ar∗∗ + χ′ionisation

Ar + χ→Ar+ + e− + χ′

?ionic excimer

Ar+ + Ar → Ar+2

?-losses

recombination

Ar+2 + e− → Ar∗∗ + Ar

?de-excitation

Ar∗∗ → Ar∗

?� -excimer

Ar∗ + Ar → Ar∗2

resonance linesAr∗ ↔ Ar + γ

?third continuum

?first cont. / second cont. / LTP Ar∗2 → 2Ar + γ

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 9 / 18

Page 14: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Time Structure of the Second Continuum Emission

Hofmann et al. Eur. Phys. C (2013) 73:2618

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 10 / 18

Page 15: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Fitted Time Constants (Second Continuum Peak Emission)

projectile τs [ns] τt [ns] IsIt

Ref.

32S 6.47 ± 0.09 1224.0 ± 17.9 2.19 ± 0.07 (1)

p+ 3.20 ± 0.02 1355.8 ± 5.8 0.28 ± 0.01 (1)

e− <6.2 1300 ± 60 0.51 ± 0.05 (2)

IsIt

=

∫∞0 As ·exp{− t

τs}dt∫∞

0 At ·exp{− tτt}dt

(1) Hofmann et al. Eur. Phys. C (2013) 73:2618(2) Heindl et al. EPL, 91 (2010) 62002

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 11 / 18

Page 16: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Single Phase Detectors

Figure: arXiv:1206.2169v1 (2012)

Simple sphercial geometry:

→ Good self shielding→ Good optical coveragepossible

Particle identification:

Only time information→ Big difference between τsand τt necessary

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 12 / 18

Page 17: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Single Phase Detectors

Figure: arXiv:1206.2169v1 (2012)

Simple sphercial geometry:

→ Good self shielding→ Good optical coveragepossible

Particle identification:

Only time information→ Big difference between τsand τt necessary

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 12 / 18

Page 18: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Double Phase Detectors, (TPCs)

Figure: arXiv:1206.2169v1(2012)

Simultaneous measurement ofscintillation and ionization

3D vertex reconstruction →z-resolution: <1 mm, xy-resolution∼3 mm (XENON100)

Powerful background rejection:

FiducializationMulti scatter-identificationChargeLight → Particle identification

Pulse shape discrimination (LArdetectors)

Optical coverage and light yield smallercompared to single phase → increasedthreshold

Technical challenges of highvoltage system

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 13 / 18

Page 19: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Double Phase Detectors, (TPCs)

Figure: arXiv:1206.2169v1(2012)

Simultaneous measurement ofscintillation and ionization

3D vertex reconstruction →z-resolution: <1 mm, xy-resolution∼3 mm (XENON100)

Powerful background rejection:

FiducializationMulti scatter-identificationChargeLight → Particle identification

Pulse shape discrimination (LArdetectors)

Optical coverage and light yield smallercompared to single phase → increasedthreshold

Technical challenges of highvoltage system

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 13 / 18

Page 20: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Double Phase Detectors, (TPCs)

Figure: arXiv:1206.2169v1(2012)

Simultaneous measurement ofscintillation and ionization

3D vertex reconstruction →z-resolution: <1 mm, xy-resolution∼3 mm (XENON100)

Powerful background rejection:

FiducializationMulti scatter-identificationChargeLight → Particle identification

Pulse shape discrimination (LArdetectors)

Optical coverage and light yield smallercompared to single phase → increasedthreshold

Technical challenges of highvoltage system

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 13 / 18

Page 21: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Double Phase Detectors, (TPCs)

Figure: arXiv:1206.2169v1(2012)

Simultaneous measurement ofscintillation and ionization

3D vertex reconstruction →z-resolution: <1 mm, xy-resolution∼3 mm (XENON100)

Powerful background rejection:

FiducializationMulti scatter-identificationChargeLight → Particle identification

Pulse shape discrimination (LArdetectors)

Optical coverage and light yield smallercompared to single phase → increasedthreshold

Technical challenges of highvoltage system

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 13 / 18

Page 22: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Double Phase Detectors, (TPCs)

Figure: arXiv:1206.2169v1(2012)

Simultaneous measurement ofscintillation and ionization

3D vertex reconstruction →z-resolution: <1 mm, xy-resolution∼3 mm (XENON100)

Powerful background rejection:

FiducializationMulti scatter-identificationChargeLight → Particle identification

Pulse shape discrimination (LArdetectors)

Optical coverage and light yield smallercompared to single phase → increasedthreshold

Technical challenges of highvoltage system

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 13 / 18

Page 23: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Liquid Argon DM Experiments

Exp. Type Mass [kg] Veto Status Site

DarkSide TPC 50Water +B-doped LS

Comm.LNGS(Italy)

ArDM TPC 850Passive PEn-shield

Comm.Canfranc(Spain)

DEAP Single36001000

WaterCherenkov

Comm.SNOLab(Canada)

MiniCLEAN Single500150

WaterCherenkov

Comm.SNOLab(Canada)

DARWIN TPCtonscale

WaterCherenkov

R&D tba

MAX(Ar/Xe)

TPCtonscale

WaterCherenkov

R&DHomestake(USA)

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 14 / 18

Page 24: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Liquid Xenon DM Experiments

Exp. Type Mass [kg] Veto Status Site

ZEPLIN-III TPC125.1

Plasticscintillator

EndBoulby(UK)

XENON100 TPC16162

Passiveshield

ActiveLNGS(Italy)

XENON1T TPCtonscale

WaterCherenkov

R&DLNGS(Italy)

XMASS Single835100

WaterCherenkov

Re-Comm.

Kamioka(Japan)

LUX TPC370100

WaterCherenkov

ActiveHomestake(USA)

LZ TPCtonscale

tba R&D tba

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 15 / 18

Page 25: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Current WIMP cross-section Limits - Liquid noble Gases

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 16 / 18

Page 26: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

The current Situation

http://luxdarkmatter.org/talks/20131030 LUX First Results.pdfAlexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 17 / 18

Page 27: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18

Page 28: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18

Page 29: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18

Page 30: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18

Page 31: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18

Page 32: Scintillation in Liquid Noble Gases - TUM · 2013-11-27 · Scintillation in Liquid Noble Gases Alexander Neumeier1 Martin Hofmann1, Thomas Dandl2, Thomas Heindl2, Jochen Wieser3,

Summary and Conclusions

Liquid noble gases → High density targets with high scintillationefficiency

Particle dependent scintillation of liquid argon investigated in ourgroup → switch over to ArXe mixtures, IR emission and pure xenon

Basically two detector concepts:

Single phase → Pulse shapeDual phase TPC → Charge

Light ratio

Bigger target volumes planned for the future → VUV lightattenuation measurements(A. Neumeier et al. Eur. Phys. C (2012) 72:2190)

Many of the DM experiments are based onLAr(upcoming)/LXe(established)

Most stringent limit at the moment in the WIMP parameter space →LUX

Alexander Neumeier (E15) JAPS-Scintillation in Liquid Noble Gases 29.11.2013 18 / 18