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1 Sandia National Laboratories Albuquerque, New Mexico (505) 844-2384 [email protected] Spectrum 2002 Conference August 4-8, Reno, NV Clifford K. Ho, Bill W. Arnold, John R. Cochran, and Randal Y. Taira * Risk-Based Performance Assessments for Long-Term Cover Systems: Sensitivity and Uncertainty Analyses * Pacific Northwest National Laboratory Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000.

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1

Sandia National LaboratoriesAlbuquerque, New Mexico

(505) [email protected]

Spectrum 2002 ConferenceAugust 4-8, Reno, NV

Clifford K. Ho, Bill W. Arnold, John R. Cochran, and Randal Y. Taira*

Risk-Based Performance Assessments for Long-Term Cover Systems:

Sensitivity and Uncertainty Analyses

*Pacific Northwest National Laboratory

Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000.

2

Overview

• Introduction

• Approach

• Demonstration

• Impact and Summary

3

Introduction

• Engineered covers are needed to assist on-site isolation of subsurface contaminants in landfills, waste tanks, and other disposal sites

• Seven DOE Operations Offices have indicated major needs for long-term cover systems

– Albuquerque, Idaho, Nevada, Ohio, Rocky Flats, Richland, and Savannah River

• DOE 2006 Accelerated Cleanup Plan identifies use of surface barrier systems as a vital remedial option

4

Problem Statement

• Need rigorous method to evaluate long-term performance of covers with quantification of risk and uncertainty

• Need way to identify parameters and processes for performance verification and monitoring

• Need more rigorous methods to compare alternative designs and approaches

– Reduce Costs– Meet regulatory performance metrics and schedules

Develop risk-based performance-assessment approach for selection, design, modeling, and monitoring of long-term covers

5

Overview

• Introduction

• Approach

• Demonstration

• Impact and Summary

6

Approach

Performance Assessment

Engineering Design/Deployment

Performance Monitoring and

Stewardship

Environmental Setting/Site

Characterization

Public and Stakeholder OutreachPublic and Stakeholder Outreach

Regulatory RequirementsRegulatory Requirements

7

Performance Assessment

Process

Scenario 2Scenario 1

Select Select Reject

Scenario 3

Develop and Screen Scenarios

KsatClimate Change Defects

Estimate Parameter Ranges and Uncertainty

ClimateEvapotranspirationSource TermVadose ZoneSaturated ZoneHuman Exposure

Develop Models

PA_process.ai

Perform Calculations00E000E000E000E000E000E000E000E000E000E000E000E0000D63768118>I<FFF8FFF8FFF80038003800380038003800380038003800380038003800380038003800380038003003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380038003800380

Uncertainty AnalysisSensitivity AnalysisAlternative Designs

Risk/Perfor manceCost/ScheduleRegulatory Compliance

Interpret Results

Monitoring Requirements

8

Overview

• Introduction

• Approach

• Demonstration

• Impact and Summary

9

Monticello Disposal Site

• Permanent repository for 2.5 million cubic yards of low-level radioactive mill tailings and contaminated soils

• Sub-humid environment– Average annual temperature ~ 46 F

– Average annual precipitation ~ 15 in

• Repository design consists of– composite cover system

– double-liner system beneath tailings

– leachate collection and removal system and leak-detection system

10

2.6 m

12.5 m Source Term

1.5 cmComposite Liner

Vadose Zone4.6 m

Receptor Well

Confining Layer

Groundwater Flow

Cover

Aquifer

not to scale

Conceptual Model Development

Vertical Percolation/

Evapotranspiration Layer (soil)

Lateral Drainage Layer (sand)

Geomembrane Liner

(60 Mil HDPE)

Barrier Layer(clay)

Uranium Mill Tailings

66”

24”

Vertical Percolation/

Evapotranspiration Layer (soil)

Lateral Drainage Layer (sand)

Geomembrane Liner

(60 Mil HDPE)

Barrier Layer(clay)

Uranium Mill Tailings

Vertical Percolation/

Evapotranspiration Layer (soil)

Lateral Drainage Layer (sand)

Geomembrane Liner

(60 Mil HDPE)

Barrier Layer(clay)

Uranium Mill Tailings

Vertical Percolation/

Evapotranspiration Layer (soil)

Lateral Drainage Layer (sand)

Geomembrane Liner

(60 Mil HDPE)

Barrier Layer(clay)

Uranium Mill Tailings

66”

24”

PrecipitationPrecipitation

Lateral DrainageLateral Drainage

RunoffEvapotranspiration

RunoffEvapotranspiration

InfiltrationInfiltration

Percolation

Radon-Gas Flux

Groundwater Concentration Peak Dose

(HELP, RAECOM codes)Cover

(FRAMES/MEPAS codes)Total System

11

Integrated Performance-Assessment Model• Used FRAMES (PNNL) to integrate models for total-

system performance assessment– Drag-and-drop software platform

– Stochastic (Monte Carlo) analyses

• Source Term

• Vadose Zone

• Saturated Zone

• Human Exposure

http://mepas.pnl.gov:2080/earth/earth.htm

• Radon-Gas Flux (RAECOM)

• Percolation (HELP)

12

Performance-Assessment AnalysesExamples from Monticello Study

• Risk/Uncertainty Analysis

• Sensitivity Analysis

• Alternative Design Comparison

• Meet regulatory performance metrics

• Identify important parameters

• Reduce costs

13

Risk/Uncertainty Analysis• Multiple computer “realizations” are simulated

using stochastic inputs

0

2

4

6

8

10

12

-7 -6 -5 -4 -3 -2

Ksat_1.qpc

Co

un

t

log10

(Ksat

) (cm/s) for Layer 1

Stochastic Inputs(Latin Hypercube Sampling)

Multiple Computer Simulations(HELP, FRAMES)

• Ensemble of realizations yields probability distribution for “performance metric”

Distribution of Results(Present and Future Conditions)

10-6 10-5 10-4 10-3 10-2 10-1 100 1010

20

40

60

80

100present_future_cdf.qpc

Average Annual Percolation through Layer 4 (inches)

Cu

mu

lativ

e P

rob

abili

ty

sing

le d

eter

min

istic

resu

lt

present

future

14

Uncertainty Analysis of Percolation through the Cover

• 95% of all simulated water percolation through cover are less than 10-7 cm/s

• Future conditions yield poorer performance– Increased defects in

liner

– Cooler, wetter climate10-13 10-12 10-11 10-10 10-9 10-8 10-7 10-60

20

40

60

80

100present_future_cdf_cm_per_s.qpc

Percolation Flux through Cover (cm/s)

Cu

mu

lati

ve P

rob

abili

ty

present

future

40 C

FR

Par

t 264

.301

15

Uncertainty Analysis of Peak Dose

• Uncertainties can be quantified

• Can use risk-based evaluation of performance

0.0

0.2

0.4

0.6

0.8

1.0

1.0E-23 1.0E-18 1.0E-13 1.0E-08 1.0E-03 1.0E+02

Peak Cumulative Dose (mrem/yr)

Cu

mu

lati

ve P

rob

abili

ty

present

future

100

mre

m/y

r (D

OE

Ord

er 5

400.

5 II

1.a)

• Single deterministic result cannot quantify uncertainty or risk

16

Sensitivity Analysis

place

ment qu

ality

Ksat-

layer

1

evap

orative

zone

depth

precip

itation

multi

plier

tempe

rature

adjus

tmen

t

maxim

um lea

f-area

index

0

0.1

0.2

0.3

0.4

0.5

Sensitivity Analysis for Percolation through Cover

Present Climate

Future Climate

• Sensitivity analysis can be used to identify parameters and processes most important to performance

• Stepwise linear-regression analysis quantifies relative importance of parameters

∆R2

17

Aquifer

Porosity

Aquifer

Velocity

Distanc

e to w

ell

Aquifer

Radium

Kd

Source

Width

Source

Radium

Kd

Percola

tion Rate

Liner

Hydrau

lic Con

ductiv

ity

Vadose

Zone

Radium

Kd

0

0.2

0.4

0.6

0.8

1

Sensitivity Analysis

∆R2

Sensitivity Analysis for Peak Cumulative Dose

Shallow Aquifer (present climate)

Shallow Aquifer (future climate)

Deep Aquifer (future climate)

18

Alternative Design Comparison• Alternative designs can be compared using a probabilistic

risk-based approach

• “ET” cover design performed adequately for percolation, but it greatly exceeded radon-gas-flux metric

0

0.2

0.4

0.6

0.8

1

0.001 0.01 0.1 1 10 100 1000

Surface Radon-222 Gas Flux (pCi/m2-s)

Cu

mu

lativ

e P

rob

abili

ty Existing Cover Design

Alternative "ET" Cover

40 C

FR

192

.02(

a)

Present Climate

10-13 10-12 10-11 10-10 10-9 10-8 10-7 10-60

20

40

60

80

100ET_cover_comparison.qpc

Percolation Flux through Cover (cm/s)

Cum

ulat

ive

Pro

babi

lity

40 C

FR

Par

t 264

.301

Alternative "ET"Cover

Existing CoverDesign

Present Climate

Cum

ulat

ive

Pro

babi

lity

40 C

FR P

art 2

64.3

01

19

Overview

• Introduction

• Approach

• Demonstration

• Impact and Summary

20

Impact and Summary

• Probabilistic PA approach provides rigorous regulatory-based evaluation of long-term cover systems

– Quantifies risk and uncertainty

• Sensitivity analyses identify processes and parameters most important to performance

– Site characterization– Performance verification and monitoring

• Provides risk-based comparison between alternative approaches and designs

– Reduce costs and meet schedule– Meet regulatory performance metrics

• Software and methods are ready for use– www.sandia.gov/eesector/gs/gh/SAND2001-3032.pdf

21

Backup Slides

22

Monticello Validation

0 20 40 60 80 100

Time (years)

0

200

400

600

Ann

ual P

reci

pita

tion

(mm

)

0.001

0.01

0.1

1

10

100

1000

10000

Ann

ual D

rain

age

Laye

r 2

(mm

)

HELP Simulation Results, Monticello Landfill Cover, Expected-Value Run

2001 Measured Precipitation (278 mm)

2001 Measured Drainage (0.17 mm)

23

Uncertainty Distributions for Input Parameters

• Future Climate Conditions– Precipitation

– Temperature

• Percolation through Cover– Evapotranspiration

– Hydrologic Properties

– Geomembrane Quality

• Transport Parameters– Sorption Coefficient

– Dispersivity

– Distance to Well

• Radon-Gas Flux Parameters– Diffusion Coefficient

– Moisture Content

0

2

4

6

8

10

12

-7 -6 -5 -4 -3 -2

Ksat_1.qpc

Cou

nt

log10

(Ksat

) (cm/s) for Layer 1