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Z)D I m D @BP GRJ D CRD GB? V JL_R[ W�O�? V SRE I X A P GBD M g [ V K)V X D C JLK O�X A P GBD W�� �5@HWBS"j � � 3 a ZUD I�M7? � X M2? V D m D @BP G cJ D C D GB? V JU_ [ W g [ V K)Q ? WHW^� D SH[RP G�hHX A�K @ � %�C � � � 3 m hHK O a � C 8 � q� � 33w,h D J I ? C D W aZ)? A�X W g [ GHV I l @HM7D W6? hBA [ I hHX D I J D+\�? A A D I WBD WHWRJ�M7? W3E�@ B 7 B I�W�F I I B @�[RSHD I.hV@ Q T BPE�B k2C D�A 7 ? j B 7 A a Z)? AX WvSHD I5n�X QRI [ A J I @HQRJ @HI5? SHA [ I hHX D I J D6\v? A A D I)OLX I S�? V A&h�B T k�>�K B >�B I/W�F I I B @7[RSHD I�S� ? @ Q I j Q 9#7 I C D2BE�B k2C D�A 7 ? j B 7 ALh D K D X P GHWBD J a Z)? h�D X�O�D I SHD W"\�? A A D I M7[ V D QRFHV D5SR@HI P G"\�? A A D I A J [ � hHI FBP Q D WRhHX V SR@HWHC�? WSRX D g [ V K A J I @HQRJ @HILC D hH@HWBSHD W � SH? A g [ V K)h�D C X WHW JUK @ � @HX V V D W ag [ V K)Q ? WHW�\v? A A D I�WR@HILhHX A�K @�D X WBD M yRl J J X C @HWHCRA eH@HWHQRJ�m � DUWB? P G g [ V K ? I JLhHX A�K @ � C 8 � q� i c � ��3�wSR@HI P G � SHA [ I eHJ X [ W�hHX WBSHD W a \ l GHI D WBS�SH? AL? hBA [ I hHX D I J D)\�? A A D ILSR@HI P G"^�? CRD I @HWHC�D W J E D I WRJLO�D I SHD WQ ? WHW � V l x JUA X P G�SH? AL? SHA [ I hHX D I J DU\v? A A D ILWR@HIUSR@HI P G�\�l I M7D D X WRO�X I QR@HWHC�D W J E D I WBD W a�� %� � � )�"5�0 ' � )�" � #"'��' � )��� � "'�ZUX D)YUI @HWBSRhB? @BA J D X WBDUSHD I g [ V K A @HhBA J ? WHK)A X WBS7SRX DU[ I CR? WHX A P GBD W&5,D I hHX WBSR@HWHC D W � w x x �=x t$+ wB� ) w zvs �y wRx x �=x t$+ w @HWBS�� s �B{=s {,a�f W�C D I X WHCRD I m [ I M�QR[ M2M2D W ? @BP G � M2X WBD �54 V D � yRl @HI D W �+� V QR[ GB[ V D2@HWBS? WB[ I C ? WHX A P GBD14�D A J ? WBSRJ D X V DUX M g [ V K)_ [ I a4,X AUK @�� � 3(SHD I5n�? A A D&m A X D GBD6k=? h a � a j wUWHX M2M5J6NBD V V @HV [ A D � SRX D6SHD M g [ V K7SRX D3y J I @HQRJ @HI)_ D I V D X G J �D X W a ZU? WBD h D W"SRX D WRJ g D M2X K D V V @HV [ A D)K @HI�5,D I A J D X E @HWHC2@HWBS�^ X C WHX W�K @HI�5,D I hHX WBSR@HWHC7SHD I8y J I @HQRJ @HI a

NBD V V @HV [ A D g D M2X K D V V @HV [ A D ^ X C WHX W3 3 3

\vD X P GHGB[ V K � � c � � � �2c i � � � c i �g ? I J GB[ V K � � c � � � � c � � j � c � �k�? h D V V D5� a j }Bg [ V K K @BA ? M6M7D WBA D J K @HWHC � � � �

� w x x �=x t$+ w X A J,D X W2M2? QRI [ M2[ V D QR@HV ? I D A m ? SHD WHM7[ V D QRFHV a ZUD ILYLI @HWBSRhB? @BA J D X W7_R[ W�N D V V @HV [ A D�X A J�YUV @ cQR[ A D^m �� &�� � "�� w a ZL@HI P G�5,D I QRD J J @HWHC7_ [ W�YLV @HQ [ A D M2[ V D QRFHV D W�D W J A J D GRJ)SRX D A D)GB[RP GHe [ V �RM7D I D2YUD cI FBA J A @HhBA J ? WHK � i �Pm A X D GBD � hHh a � a j w a DUWB? P G d [ V �RM7D I X A ? J X [ WBA C I ? S�W�Q�] WHWBD W�j � �6hHX AL� � � �7YLV @HQ [ cA D M7[ V D QRFHV D5? WBD X WB? WBSHD IUC D I D X GRJUA D X W a ZLX D)n�? QRI [ M2[ V D QRFHV D)SHD I)N D V V @HV [ A DUhHX V SHD Wg\)D J J D W � SRX D)A X P G

j �

� aBg [ V K5? V A�4,I D WHWBA J [ � � a j5T=X C D WBA P GB? E J D W�_ [ W g [ V K

@HWRJ D I � @BA hHX V SR@HWHC�_R[ W"\v? A A D I A J [ �BhHI FBP QRD W"K @"V ? WHC C D A J I D P QRJ D W/4,FHWBSHD V W � SHD W�T=V D M2D WRJ ? I �HhHI X V cV D W � K @BA ? M6M7D WHV ? C D I W a T+J O�?6� �5T+V D M7D W J ? I �HhHI X V V D W�D I C D h�D W�D h D WHE ? V V A,X W m [ V C DL_R[ W7\v? A A D I A J [ � chHI FBP QRD W hHX V SR@HWHC�D X WBD5n�X QRI [ �HhHI X V V D � SHD W"YUI @HWBSRhB? @BA J D X W"SHD I d �B? WHK D WHK D V V O�l WBSHD � �Rj � a

O

H

OH

H

CH2OH

H

H

H

O

O

CH2OH

H

H

H

OH

OH

H

H

OHO

O

CH2OH

H

H

H

OH

OH

H

H

n

OHH OH

OH

O

OH

H

CH2OH

H

H

O

H

Grundstruktur

� hHhHX V SR@HWHC7� a j } y J I @HQRJ @HI E [ I M2D V,NBD V V @HV [ A D

ZUX D�P GBD M2X A P GBD W T=X C D WBA P GB? E J D WqD X WBD A�y J [ � D A�O�D I SHD W SR@HI P GqSRX D � I J�@HWBS � WB[ I SRW @HWHC�A D X WBD IE @HWHQRJ X [ WBD V V D WqYUI @HeHe�D W D WRJ A P GBD X SHD WBS�h�D D X W �H@2x J a m FHI�SRX Dg5,D I hHI D WHWR@HWHC]A X WBS�A X D�_R[ W�h�D A [ W cSHD I D I�4�D SHD @HJ @HWHC � O�D X V�A X D6@HW J D I g X J K D D X WRO�X I QR@HWHC�? V A6D X WHK D V WBD7n�[ V D QRFHV D2? hHC D A eB? V J D WvO�D I SHD Wm m V FBP GRJ X C D w�@HWBS�A [5SHD W&5,D I hHI D WHWR@HWHC A _R[ I C ? WHC7M2? x CRD hHV X P G�h D D X W �H@BA A D W a ZUX DUO�X P GRJ X C A J D W�E @HWHQ cJ X [ WBD V V D W�YUI @HeHe�D W7SHD IUNBD V V @HV [ A DUA X WBS � " &(@HWBS � & � " & m eHI X M2l I D � V Q [ GB[ V D w a 5,[ I�? V V D M SRX DA D GHILI D ? QRJ X _RD W `UgLc YUI @HeHe�D W�V ? A A D W�A X P G"A P GHWBD V V�e �RI [ V X A X D I D W�@HWBS�? WBA P GHV X D x D WBS�[ � X SRX D I D W a) w zvs y wRx x �=x t$+ w X A J,O�X DUN D V V @HV [ A DUD X W d [ V �HA ? P P GB? I X S a NB@BA l J K V X P G7K @�SHD W7? V QR[ GB[ V X A P GBD W"YLI @HeHe D Wh�D A X J K J g D M6X K D V V @HV [ A D�? @BP G]n�D J G �RV c � & � @HWBS � ? I h [ � �RV C I @HeHe D W � #"#" & a+f M/YUD CRD WBA ? J KK @HMqV X WBD ? I D W7NBD V V @HV [ A D M7[ V D QRFHVRO�D X A J+SRX DVy J I @HQRJ @HI=K ? GHV I D X P GBDV\)D J J D WR_ D I K O�D X C @HWHC D W7? @HE a YLI @HWBS chB? @BA J D X WBD6_R[ W g D M2X K D V V @HV [ A D2A X WBS g D � [ A D W�@HWBS d D W J [ A D W a Z)? A5? M GBl @��HCRA J D Wv_ [ I QR[ M2M2D WBSHDn"[ WB[ M2D ILX A J����RV [ A D aRf M(YUD CRD WBA ? J KUK @�SHD I�X W7QRI X A J ? V V X WBD I ` I SRWR@HWHC7? @HE J I D J D WBSHD W"NBD V V @HV [ A DUh D cA X J K JUSRX D)? M7[ I eHGBD�y J I @HQRJ @HIL_R[ W g D M6X K D V V @HV [ A DUQRD X WBD)C I [ x D m D A J X C Q D X J a� s �B{=s { X A J2SHD I ? � � � SHD I7SRX D g [ V K A J I @HQRJ @HI2K @BA ? M6M7D WHGBl V J a�f M�Y)D C D WBA ? J K�K @�NBD V V @HV [ A D�@HWBSg D M2X K D V V @HV [ A D5A X WBS�SRX D5YLI @HWBSHD V D M7D W J D)_ [ W�^ X C WHX W�m d GBD WB[ V eHI [ eB? WBD w�QRD X WBDUK �RQRV X A P GBD W�A [ WBSHD I W? I [ M2? J X A P GBD1y J I @HQRJ @HI D W a ZLX DLK ? GHV I D X P GBD W�I l @HM2V X P GBD Wg5,D I QRD J J @HWHC D W�E FHGHI D W7K @�D X WBD IL? M7[ I eHGBD Wy J I @HQRJ @HI a f M YUD CRD WBA ? J K)K @"SHD W�4�D WHK [ V I X WHC D W"h D X�\L[ GHV D W"A X WBS�SRX D14�D WHK [ V I X WHC D5X W"SHD IU^ X C WHX W cA J I @HQRJ @HI6WHX P G J2@HW J D I D X WB? WBSHD I2_RD I hH@HWBSHD W a ZUX D2OLX P G J X CRA J D W]E @HWHQRJ X [ WBD V V D W�YLI @HeHe D W X M0^ X C WHX WA X WBS�SRX DUeHI X M2l I D W � V Q [ GB[ V D c `Ug @HWBS c �,g � `Ug m A X D GBD � hHh a � a ��w a\�X D7X W ? V V D W ` I CR? WHX A M2D W �HWBSHD J6M7? W]? @BP GvX M g [ V K g D J D I [ ? J [ M2D7OLX D * � [RSHD I� > a ZUX D A DE FHI5SRX D d �B? WHK D6V D h�D WBA O�X P GRJ X C D WvT+V D M7D W J D6C D V ? WHCRD W�? @BA)SHD M 4�[RSHD W"X W�SHD W ` I CR? WHX A M5@BA a 5,[ I? V V D M y J X P QHA J [ ��h D W#] J X C J�SHD I ` I CR? WHX A M5@BA+K @HIV4,X V SR@HWHC5_ [ W7A e D K X �BA P GBD W7T+X O�D X x A J [ ��D W � SHD W7T+W cK �RM7D W a m ? A J�? V V DLhHX [ V [ C X A P GBD W&�UD ? QRJ X [ WBD W � K a 4 aRd �B? WHK D W O�? P GBA J @HM � V ? @HE D W2WR@HI,X W � W O�D A D WHGBD X J_R[ W"T=WHK �RM7D W"? h a^ X C WHX W6OLX I S5X M 4�? @HM K O�X A P GBD W^��X WBSHD+@HWBS6l @2x D I A J D I g [ V K A P GHX P G J8m y eHV X WRJ GB[ V K w�eHI [RSR@HK X D I J a d GBD cW'�RV ? V ? WHX W � D X W�A J X P QHA J [ � GBl V J X C D I5T=X O�D X A A J [ � � C X V J)SH? h D X,? V A�5,[ I V l @HE D I A @HhBA J ? WHK6_R[ W�^ X C WHX W a ZUX DX M d GBD W'�RV ? V ? WHX W�D WRJ GB? V J D WBD W � M2X WB[ C I @HeHe D W � *�& � CRD V ? WHC D W�SH? SR@HI P G"X W"SH? A g [ V K5@HWBS"A X WBSM2X J _ D I ? WRJ O�[ I J V X P G�E FHILSHD Wy J X P QHA J [ � C D GB? V JLX M�4,I D WHWBA J [ ��� � � � a

j i

� aBg [ V K5? V A�4,I D WHWBA J [ � � a j5T=X C D WBA P GB? E J D W�_ [ W g [ V K

CH

CH

OMe

O

CHO

CH2OH

OMe

O

CH2OH

CHO

CH2OH

CH2OH

CH

CH

O

CH

CH

OMe

O

O

CH

CH

OMe

O

CH

CH

CH

HC

OMe

OH

CH

CH

OMe

O

OMe

OH

OH(C6H

10O

5)n

HCOH

CH

OMe

OH

O

CH2OH

OH(C6H

10O

5)n

OMe

CH2OH

� hHhHX V SR@HWHC7� a � }B� @BA A P GHWHX J JU? @BALD X WBD IU^ X C WHX WBA J I @HQRJ @HI

Z)D I+C I [ x D � W J D X V ? W m V FBP GRJ X C D W7X W7SHD I g [ V K A @HhBA J ? WHKUX A J,D X WBD m [ V C DLSHD A+C I [ x D W � W J D X V A,? W2E @HWHQ cJ X [ WBD V V D W2YUI @HeHe�D W5X W6SHD IPy J I @HQRJ @HI a f M YUD CRD WBA ? J K,K @�\L[ GHV D W � SRX D+O�D WHX CRD I=E @HWHQRJ X [ WBD V V DLYLI @HeHe D W? h D I5C I [ xRD6e�[ V � ? I [ M2? J X A P GBD&y J I @HQRJ @HI D Wv? @HE O�D X A D W � SRX D6@HW J D I6k�D M2e D I ? J @HI D X W OLX I QR@HWHC"V ? WHC A ? cM7D IU? @HE hHI D P GBD W � D W J A J D GRJLh�D X M(T+I GHX J K D W�_R[ W g [ V K6D X WBD)C D I X WHCRD)n"D WHC D1\L[ QHA1m A X D GBD)k=? h a � a � w a

j �

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m V FBP GRJ X C D \U[ QHA � A P GBD3 3 3

g [ V K � � c � � j �2c � � � � � � c �\L[ GHV D �6c i � � � c � � � c j �

k=? h�D V V D5� a � } m V FBP G J X CRD)@HWBS&\U[ QHA�h�D X M(T+I GHX J K D W�_R[ W g [ V K)@HWBS&\U[ GHV D

NB@HI � GB? I ? QRJ D I X A X D I @HWHC�E D A J D I^4,I D WHWBA J [ ��D7GHX WBA X P G J V X P G�X GHI D I35,D I hHI D WHWR@HWHC A D X C D WBA P GB? E J D W�@HWBSX GHI D IUD V D M2D WRJ ? I D WvNH@BA ? M6M7D WBA D J K @HWHC7Q [ M6M7D W�E [ V C D WBSHD � WB? V �HA D _ D I E ? GHI D W�K @HI � WRO�D WBSR@HWHC }� f M6M7D SRX ? J ? WB? V �HA D }4�D X5SHD I f M2M2D SRX ? J ? WB? V �HA D�O�D I SHD W SHD I g D X K O�D I J � SHD I � WRJ D X V6? W m V FBP GRJ X C D W A [ OLX DvSHD I\v? A A D I c @HWBS � A P GBD C D GB? V J)SHD A�4,I D WHWBA J [ ��D A�h D A J X M2M5J a

� T+V D M7D W J ? I ? WB? V �HA D }ZUX D�T+V D M7D W J ? I ? WB? V �HA D"C X hHJ � @BA QR@HWHE J7FHh D I�SRX D�M7D WHC D WHM7l x X CRD�NB@BA ? M2M2D WBA D J K @HWHC SHD A4,I D WHWBA J [ � D A=GHX WBA X P GRJ V X P G7A D X WBD I+D V D M2D WRJ ? I D W�YLI @HWBSHA J [ � D8m \L[ GHV D WBA J [ � � \�? A A D I A J [ � � yR? @ cD I A J [ � � y J X P QHA J [ � � yRP GRO�D E D V � � GHV [ I ��a a a w a

k�I [ J K2SHD I b W J D I A P GHX D SHD5X W"SHD IUn"[ I eHGB[ V [ C X D5@HWRJ D I A P GBD X SHD W�A X P G"SRX D g [ V K ? I J D W"W @HIUCRD I X WHC E FHC X CGHX WBA X P G J V X P G"X GHI D IUD V D M2D WRJ ? I D W�NB@BA ? M2M2D WBA D J K @HWHC a

� � � � ��! " � ),+ �*+.),'*' �*'-

4�D X)SHD I^5,D I hHI D WHWR@HWHC �HWBSHD J7K OLX A P GBD W SHD W]hHI D WHW hB? I D W 4�D A J ? WBSRJ D X V D W SHD A&4,I D WHWBA J [ ��D A2@HWBSyR? @BD I A J [ � D X WBD5M2X J)GB[ GBD I6Y)D A P GRO�X WBSRX C Q D X J6? hHV ? @HE D WBSHD2D � [ J GBD I M7D��UD ? QRJ X [ W�A J ? J J a ZL@HI P GvSRX DE I D X O�D I SHD WBSHD7T=WBD I C X D2D WRJ A J D G J2D X W/�U? @BP GHC ? A)GB[ GBD I5T+W J GB? V eHX D a+f WvD X WBD I�y J ? @HhHE D @BD I @HWHC�OLX I QRJSRX D m D A J A J [ �BeHGB? A D�O�X D�D X WBD�FHh D I�SHD W]C D A ? M5J D W m D @BD I I ? @HM�_ D I J D X V J D � @BD V V D�? WU4,I D WHWHC ? A D W� � � � a ZU@HI P G2SRX D d �RI [ V �HA D�SHD A m D A J A J [ � D A=O�D I SHD W �HFBP G J X CRD��LD ? QRJ X [ WBA eHI [RSR@HQRJ D,@HWBS3\L[ QHA eB? I J X Q D VCRD hHX V SHD J aZUX D�5,D I hHI D WHWR@HWHC�_R[ W g [ V K7D I E [ V C J)X Wvk�D X V A P GHI X J J D W a m [ V C D WBSHD35,[ I C l WHC D6V ? @HE D W � hHX A)K @vD X WBD MCRD O�X A A D W"YUI ? S7K D X J V X P G�C D A J ? ��D V J � ? h }j a T+I O�l I M5@HWHC7@HWBS�k I [RP QRWR@HWHC� aLd �RI [ V �HA Di aU`�� X SH? J X [ W

�� �� % � � ���!� ������ ������� � �/� ��� ���� f M(D I A J D WyRP GHI X J J)SHD I�5,D I hHI D WHWR@HWHC7M5@2x�SH? A�4,I D WHWHGB[ V K6? @HE,D X WBD)E FHIUSRX D d �RI [ V �HA DUWB[ J O�D WBSRX CRDk=D M6e�D I ? J @HI+_R[ W2P ? a � � � � hHX A=iR� � � ]D I O�l I M5J+O�D I SHD W a T=h�D WHE ? V V A�M5@2x5SH? A=X M g [ V K,_R[ I GB? WBSHD WBD\v? A A D I+_RD I SH? M6eHE J,O�D I SHD W a D�WB? P G6\v? A A D I C D GB? V J,X M 4,I D WHWBA J [ �7O�X I S2SH? K @6@HWRJ D I A P GHX D SRV X P G7_RX D VT+WBD I C X D)h�D W#] J X C J aT,A�QR[ M2M5JLK @�QRD X WBD IUP GBD M6X A P GBD W�5,D I l WBSHD I @HWHC7X M�4,I D WHWBA J [ � a

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