progress towards laser cooling strontium atoms on the intercombination transition
DESCRIPTION
Progress towards laser cooling strontium atoms on the intercombination transition. Danielle Boddy Durham University – Atomic & Molecular Physics group. The team. Progress towards laser cooling strontium atoms on the intercombination transition - May 2011. Motivation: Rydberg physics. - PowerPoint PPT PresentationTRANSCRIPT
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Progress towards laser cooling strontium atoms on the
intercombination transition
Danielle BoddyDurham University – Atomic & Molecular Physics group
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The team
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
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Motivation: Rydberg physics Ionization
threshold
Ener
gy
States of high principal quantum number n.
Exaggerated size and lifetimes.
Can be prepared through laser excitation.
Greatly enhanced inter-atomic interactions.
Strong, tunable, long-range dipole-dipole
interactions among the atoms.
Applications include quantum computation. M. Saffman et. al., Rev. Mod. Phys. 82, 2313 (2010)
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
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Motivation: Dipole blockade
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Y Miroshnychenko et al., Nat. Phys. 5, 115-118 (2009)E Urban et al., Nat. Phys. 5, 110-114 (2009)
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Sr88 is an alkaline earth metal with no hyperfinestructure.
Two valence electrons permits two electron excitation.
Motivation: An introduction to strontium
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Ground state
Rydberg state
Doubly excited state
Two-electron excitation of an interacting cold Rydberg gas J. Millen, G. Lochead and M. P. A. Jones Phys. Rev. Lett. 105, 213004 (2010)
Spectroscopy of strontium Rydberg states using electromagnetically induced transparency S. Mauger, J. Millen and M. P. A. Jones J. Phys. B: At. Mol. Opt Phys. 40, F319 (2007)
At present, we’re investigating the spatial excited state distribution.
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Motivation: Dipole blockade regime
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
rB
T ~ 5 mKDensity ~ 1 x 109 cm-3
T ~ 400 nKDensity ~ 1 x 1012 cm-3
No blockade
How do we enter the dipole blockade regime?
Blockaded
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Motivation: Laser cooling of strontium
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
1P1
3P0
3P1
3P2
1S0
λ = 689 nmΓ = 2π x 7.5 kHz2nd stage cooling
λ = 461 nmΓ = 2π x 32
MHz1st stage cooling
1S0 → 3P1 intercombination transition → TD ≈ 180 nK.
Photon recoil limits TD → Tmin ≈ 460 nK.
Introduce two stages of cooling:
First cool on the (5s2) 1S0 → (5s5p) 1P1.
Second cool on the narrow-line (5s2) 1S0 → (5s5p) 3P1 .
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Outline
Simple laser stabilization set-up
Laser system
Pound-Drever-Hall (PDH)
Locking to an atomic transition
Fluorescence
Electron shelving
Summary
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
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Simple laser stabilization set-up
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Laser system
Fabry-Perot
cavity
Atomic signal
Red MOT
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Simple laser stabilization set-up
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Laser system
Fabry-Perot
cavity
Atomic signal
Red MOT
Laser system
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Laser system
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Compared old and new designs.
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Laser system
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
time
frequency
OLD
NEW2 Wavemeter
10 s
1
10 s
OLD
NEW
Wavemeter1
time
frequency2
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Laser system
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Old New
New design fluctuates more in the short term.Little difference between the long term stability.
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Simple laser stabilization set-up
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Laser system
Fabry-Perot
cavity
Atomic signal
Red MOT
Fabry-Perot
cavity
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Pound-Drever-Hall (PDH) technique
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Require the laser linewidth < 7.5 kHz.
Noise broadens the linewidth to the MHz regime.
Uses Fabry-Perot cavity as a frequency reference.
Cavity peaks are spaced by the free spectral range :
Lc
FSR 2
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Pound-Drever-Hall (PDH) technique
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Phase modulator adds sidebands to the laser.
High-finesse Fabry-Perot cavity measures the time-varying frequency of the laser input.
An electronic feedback loop works to correct the frequency error and maintain constant optical power.
Laser
Phase modulato
r
FPD
Lock Box
Etalon4
PiezoCurrent
modulation
Theory: See E. Black., Am. J. Phys. 69 (1) 79 (2001)
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Pound-Drever-Hall (PDH) technique
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
4
FPD
PS
2
Slow feedback to
piezo
Fast feedback to
diode
Feedback to cavity piezo
Atomic signal
Laser
2
Lock Box
A crystal oscillator phase modulates the 689 nm beam at a frequency of 10 MHz.
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Pound-Drever-Hall (PDH) technique
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Laser locks to the central feature of the PDH error signal
Increasing the gradient of the error signal strengthens the lock and reduces the linewidth.
(a) (b) (c) (d)
Gradient depends on sideband power: carrier power ratio.
Gradient steepest when Ps = 0.42 Pc
Theory: See E. Black., Am. J. Phys. 69 (1) 79 (2001)
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Pound-Drever-Hall (PDH) summary
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Generate PDH signal
Gradient of error signal → strength of lock and laser linewidth
NEXT STEP: Finish high bandwidth servo
IMPROVEMENTS: Build high-finesse cavity
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Simple laser stabilization set-up
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Laser system
Fabry-Perot
cavity
Atomic signal
Red MOT
Atomic signal
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Locking to an atomic transition
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
CHALLENGE: Detecting the transition.
Two detection methods:
1. Electron Shelving
2. Fluorescence
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Electron shelving
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Excite atoms to the 3P1 and measure the rate at which these atoms decay out of the state.
Photon scattering rate is proportional to the linewidth of the transition.
1P1
3P1
1S0
λ = 689 nm
λ = 461 nm
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Electron shelving
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
1P1
3P1
1S0
λ = 461 nm
atomic beam
photodiode
The amount of scattered light is proportional to the
number of atoms initially in the 1S0 ground state.
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Electron shelving
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
1P1
3P1
1S0
λ = 689 nm
λ = 461 nm
atomic beam
photodiode
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Electron shelving: Experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
atomic beam
photodiode
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Electron shelving: Experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
atomic beam
photodiode
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Electron shelving: Experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
atomic beam
photodiode
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Electron shelving: Experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
≈ 32 MHz
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Electron shelving: Lifetime measurement
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Using a velocity of 500 ms-1
Lifetime of 3P1 is (23 ± 1) μs
Gradient: (8.9 ± 0.2) x 10-2 mm-1
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Electron shelving: Crossed beams
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
atomic beam
photodiode
FWHM crossed beams is ≈ 20 MHz.Linewidth has reduced by 1/3.
This is not narrow enough for the Fabry-Perot to lock to!
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Electron shelving: Summary
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Detected the transition indirectly via electron shelving.
Determined the lifetime of the 3P1 state.
And the lineshape?
Tried crossing the beams:
Did the linewidth reduce? Is this narrow enough for the laser to lock to?
Work in progress
Try a direct method of detection.
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Fluorescence: The experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Strontium has negligible vapour pressure at room temperature → heated to 900 K.
atomic beam
CCD camera takes spatially resolved images of the fluorescence.
Exposure length set to 65.5 ms.
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Fluorescence: The experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
(a) Slice along direction of laser beam → absorption and decay.
(b) Slice along direction of atomic
beam → transverse velocity distribution.
(b)(a)
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Fluorescence: The experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Gradient: (9.0 ± 0.3) x 10-2 mm-1
Using a velocity of 500 ms-1
Lifetime of 3P1 is (22.2 ± 0.7) μs
Other time resolved fluorescence detection: τ = (21.3 ± 0.5) μs See R Drozdowski., Phys. D. 41:125 (1997)
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Fluorescence: The experiment
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
BUT what about the absorption?
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Fluorescence: The model
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Solves optical bloch equations (OBEs) for a two level atom as a function of
distance.
Velocity distribution of atoms α Tk
mv
Bev 23
2
)(vf
Randomly selects a value of and .
If the value of is kept.
)(vf 'v
)'()( vfvf 'v
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Fluorescence: The model
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
x
Assuming the laser is on resonance the only other unknown in the OBEs is
the Rabi frequency.
Top hat pulse: Ed.
x
Gaussian pulse: 2
2)(2. waistwaistx
eEd
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Fluorescence: The model
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
0 .0 002 0 .0 004 0 .0 006 0 .00 08 0 .0 010 0 .00 12D istan cem0 .2
0 .4
0 .6
0 .8
1 .0
E xci ted po pu lat io n state 22
Top hat pulse Gaussian pulse
Velocity of 500 ms-1
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Fluorescence: The model
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
0 .00 1 0 .00 2 0 .0 03 0 .00 4 0 .00 5 0 .0 06D is tancem0 .1
0 .2
0 .3
0 .4
0 .5
0 .6
0 .7
E xcited pop u lat ion state 22
0 .001 0 .0 02 0 .003 0 .00 4 0 .00 5 0 .00 6D is tancem0 .2
0 .4
0 .6
E xcited po pu latio n state 22
2 x waist
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Fluorescence: Summary
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Detected the transition directly.
Determined the lifetime of the 3P1 state.
Written code to model absorption and decay.
Data and theory don’t quite agree.
NEXT: Try locking to this fluorescence signal.
Need to find source of problem.
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Summary
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
689 nm laser built and tested.
Need to finish PDH high bandwidth servo circuit.
Build high-finesse cavity.
Tested an indirect and direct method to detect the transition.
Measured lifetime of 3P1 state from both methods.
Try locking to fluorescence signal.
If this works….GREAT!
If it doesn’t work….try pump-probe spectroscopy
Red MOT → colder atoms
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Questions?
Progress towards laser cooling strontium atoms on the intercombination transition - May 2011
Thanks for listening Any questions?