progress on deuteron-induced activation cross section evaluation

18
FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vie nna 1 Marilena Avrigeanu Progress on Deuteron-Induced Activation Cross Section Evaluation Marilena Avrigeanu 1 , Wolfram von Oertzen 2 , Robin Forrest 3 , Aura Obreja 1 , Faustin Roman 1 , Vlad Avrigeanu 1 (1) EURATOM-MEdC Fusion Association, "Horia Hulubei" National Institute for Physics and Nuclear Engineering, P.O. Box MG-6, Bucharest, Romania (2) Freie Universitat Berlin, Fachbereich Physik, 14195 Berlin, and Hahn- Meitner-Institut, 14109 Berlin, Germany (3) EURATOM-UKAEA Fusion Association, Culham Science Centre, Abingdon OX14 3DB, UK PN2_IDEI_149/2007 [ http://proiecte.nipne.ro/pn2/ ] [ http://www.cncsis.ro/ ] FENDL-3 1st Research Co-ordination Meeting NDS/IAEA, Vienna, 2-5 December 2008 http://tandem.nipne.ro/~vavrig/ , http://fp6.cordis.lu/fp6/partners /RCN 49105

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PN2_IDEI_149/2007 [ http://proiecte.nipne.ro/pn2/ ] [ http://www.cncsis.ro/ ]. FENDL-3 1st Research Co-ordination Meeting NDS/IAEA, Vienna, 2-5 December 2008. Progress on Deuteron-Induced Activation Cross Section Evaluation. - PowerPoint PPT Presentation

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Page 1: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 1 Marilena Avrigeanu

Progress on Deuteron-Induced Activation Cross Section Evaluation

Marilena Avrigeanu1, Wolfram von Oertzen2, Robin Forrest3, Aura Obreja1, Faustin Roman1, Vlad Avrigeanu1

(1) EURATOM-MEdC Fusion Association, "Horia Hulubei" National Institute for Physics and Nuclear Engineering, P.O. Box MG-6, Bucharest, Romania(2) Freie Universitat Berlin, Fachbereich Physik, 14195 Berlin, and Hahn-Meitner-Institut, 14109 Berlin, Germany(3) EURATOM-UKAEA Fusion Association, Culham Science Centre, Abingdon OX14 3DB, UK

PN2_IDEI_149/2007 [ http://proiecte.nipne.ro/pn2/ ] [ http://www.cncsis.ro/ ]

FENDL-3 1st Research Co-ordination Meeting NDS/IAEA, Vienna, 2-5 December 2008

http://tandem.nipne.ro/~vavrig/, http://fp6.cordis.lu/fp6/partners/RCN 49105

Page 2: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 2 Marilena Avrigeanu

IFMIF Data Needs

[U. Fischer, ND2007 & "Nuclear Data Libraries for Advanced Systems: Fusion Devices“,

TM, Nov 2007, IAEA, Vienna]

• Activation/transmutation data

• General purpose neutron data library – Urgent need for qualified IFMIF reference data library– IEAF/EAF (n, p, d), to be further developed, improved and validated– Cross section measurements required for

• neutrons (E >20 MeV): Cr, Co, V, W, Ta, Pb, Bi, Au, Mn• deuterons (E < 40 MeV): Cu, Al, Nb, • protons (E < 12 MeV): Cu, Al, Nb, Ta, W, Au, Pb

– Validation experiments, to be extended/continued

• Reliable gas production cross-section data (H, He)

• Dosimetry data file to be developed for E > 20 MeV (IRDF)

Page 3: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 3 Marilena Avrigeanu

• Optical Potential - key ingredient of cross-sections calculations

• NO GLOBAL OPTICAL POTENTIAL (OP) for d + Nucleus (A<27) (basis of TW5-TTMI-004-D5)

• COMPARATIVE ANALYSIS of global OMPs for d + 27Al, 63,65Cu, 54,56,58Fe, 93Nb:Lohr-Haeberli (1974): A~40-209, E=8-13 MeVPerey-Perey (1963,1976): A~40-208, E=12-25 MeVDaehnick et al. (1980): A~27-238, E=11.8-90 MeVBojowald et al. (1988): 27Al, 89Y, 120Sn, and 208Pb at Ed=58.7 and 85 MeV

• None of these global OMP describes data at E<15 MeV

• Semi-microscopic OMP by using realistic nucleon-nucleon interaction

• Average of the local OMP parameters for d+27Al,54,56Fe,63,65Cu,93Nb: Phenomenological OMP → cross-sections calculations

• Analysis of deuteron breakup mechanism: Contribution of breakup to the reaction and activation cross sections• Direct Reactions contribution considered through stripping mechanism

• Activation cross sections calculations for d+27Al interaction

INTRODUCTION

Page 4: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 4 Marilena Avrigeanu

27Al + d : most recent phenomenological potentials

10-1

100

9.8 MeV

10-1

100

9 MeV

0 30 60 90 120 150 180

10-2

10-1

100

101

c.m.

[deg]

58.7 MeV

10-1

100

Daehnick+ (1980) Haixia+ (2006) Han+ (2006)

7 MeV

100

d/

dR

uth

erf

ord

5 MeV

27Al(d,d0)

10-1

100

11 MeV

0 30 60 90 120 150 180

10-1

100

c.m.

[deg]

11.4 MeV

10-1

100

11.8 MeV

10-2

10-1

100

12.8 MeV

10-1

100

d/

dR

uth

erf

ord

13 MeV

10-1

100

15 MeV

10-2

10-1

100

52 MeV

0 30 60 90 120 150 180

100

102

11.8 MeV

d/

d

[m

b/s

r]

0 30 60 90 120 150 180

100

102

104

d/

d

[m

b/s

r]

c.m.

[deg]

15.8 MeV

0 10 20 30 40 50 60100

102

104

c.m.

[deg] d/

d

[m

b/s

r]

63 MeV

Page 5: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 5 Marilena Avrigeanu

M. Avrigeanu et al., Phys. Rev. C62 (2000) 017001

M. Avrigeanu et al., Nucl. Phys. A693 (2001) 616

M. Avrigeanu et al. Eur. Phys. J. A12 (2001) 399

M. Avrigeanu et al., Int. J. of Mod. Phys. E, 11 (2002) 249

M. Avrigeanu et al., Nucl. Phys. A723 (2003) 104

M. Avrigeanu et al., Nucl. Phys. A 759 (2005) 327

M. Avrigeanu et al, Nucl. Phys. A 764 (2006) 246

M. Avrigeanu et al., Phys. Rev. C62 (2000) 017001

M. Avrigeanu et al., Nucl. Phys. A693 (2001) 616

M. Avrigeanu et al. Eur. Phys. J. A12 (2001) 399

M. Avrigeanu et al., Int. J. of Mod. Phys. E, 11 (2002) 249

M. Avrigeanu et al., Nucl. Phys. A723 (2003) 104

M. Avrigeanu et al., Nucl. Phys. A 759 (2005) 327

M. Avrigeanu et al, Nucl. Phys. A 764 (2006) 246

OPTICAL MODEL : prime tool for all cross section calculations Phenomenological OMP global parameter sets: codes default

Microscopic OPs: reduced uncertainties

SCAT 2000 [O. Bersillon] - pure elastic scattering OP analysis

DFOLD [M. Avrigeanu] - double folding method(nucleons, d, 4,6,8He + 4-124A-target nuclei)

FRESCO - 2.3 [I.J. Thompson]- Coupled Reaction Channel

TALYS - 1.0 [A. Koning, S. Hilaire, M. Duijvestijn] - OMP:ECIS’97; EXCITON; Hauser-Feshbach

STAPRE - H95 (updated) [V.Avrigeanu, M.Avrigeanu] - OMP:SCAT2000; GDH / EXCITON; Hauser-Feshbach

Nuclear Model Calculations

Page 6: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 6 Marilena Avrigeanu

U(E,R)= dr1 dr2 1(r1) 2(r2) veff(ρ,E,s=R+r1-r2)

1,2 - density distributions of projectile (1) and target (2) veff(,E,r) = F()g(E)v(r)

F() = C[1+e-] (DDM3Y) C[1-] (BDM3Y)

g(E) = 1-0.002E/A (Reid NN interaction)

1-0.003E/A (Paris NN interaction)

v(r) - effective NN-interaction: isoscalar and isovector components of direct and exchange parts of M3Y interaction ( g-matrix using Reid/Paris NN potential )

Microscopic Real Optical Potential

Page 7: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 7 Marilena Avrigeanu

DME-leading term (Negele-Vautherin'72) (R,R+s)=(R+s/2)Ĵ 1[kF(R+s/2)s] Campi-Bouyssy'78 for average relative momentum, kF=kav kav(r)=5/(3(r))[(r)-(1/4)2(r)]1/2

Kinetic-Energy Density (: MTF-Krivine-Treiner'79) ()=(r)5/3 + ()2/ The frozen-density approximation (Satchler'79, Khoa'94) F()=F[1(r1+s/2)+2(r2-s/2)].

Approximations

Page 8: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 8 Marilena Avrigeanu

Density distributions & NN-interactions

0 2 4 6 80

20

40

60

80

r [fm]

11 MeV

0

20

40

60

80

9 MeV

0

20

40

60

80 Paris-Negele-Machleidt'01 Paris-Negele-Abbott Reid-Negele-Abbott

7 MeV

0

20

40

60

80 27Al(d,d0)27Al

5 MeV-UD

F(r

) [

Me

V]

0 2 4 6 810-5

10-3

10-1

Negele (1970)

r [fm]

27Al

(r)

[f

m-3 ]

(c)

0.1

0.2

0.3

0.4 2H u

(r)/

r [

fm-3

/2]

Machleidt (CD-Bonn) Machleidt (1989-Paris)

(a)

0 2 4 610-6

10-4

10-2

100

charge density (Abbott) Machleidt-CD-Bonn Machleidt-Paris

2H

(r)

[f

m-3]

(b)

Page 9: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 9 Marilena Avrigeanu

1

Strzalkowski+ (1962)

9.8 MeV

1

9 MeV

1

Al-Quraishi+ (2000)Schwandt+ (1968)

7 MeV

1

Lohr-Haeberli Daehnick+ This work: microscopic

5 MeV27Al(d,d

0)

(a)

1

11 MeV

0.1

1

/

Ru

the

rfo

rd

11.4 MeV

1Igo+ (1961)

11.8 MeV

1

12.8 MeV

1

Lohr+ (1974)

13 MeV

0 30 60 90 120 150 180

0.1

1

c.m.

(deg)

Joly+ (1963)

15 MeV

1

9.8 MeV

1

9 MeV

0 30 60 90 120 150 1800.01

10

c.m.

(deg)

58.7 MeV(d)

1

7 MeV

1

Haixia+TALYS-1.0This work: phenomenologic

5 MeV 27Al(d,d0)

1

11 MeV

0.1

1

11.4 MeV

1

11.8 MeV

0.1

1

12.8 MeV

1

13 MeV

0.1

1

15 MeV

1

52 MeV

10

20

-W

(M

eV

)

WD local

WD average(b)

WV local

WV average

0 10 20 30 40 50 60

-10

0

10

-U

(M

eV

)

V

D

Ed (MeV)

(c)

0 10 20 30 40 50 600

400

800

1200

R (m

b)

Haixia+ TALYS-1.0 ACSELAM this work

d + 27Al

Ed (MeV)

(e)

Mayo+ (1965)Dubat+ (1974)

1

Strzalkowski+ (1962)

9.8 MeV

1

9 MeV

1

Al-Quraishi+ (2000)Schwandt+ (1968)

7 MeV

1

Lohr-Haeberli Daehnick+ This work: microscopic

5 MeV27Al(d,d

0)

(a)

1

11 MeV

0.1

1

/

Ru

the

rfo

rd

11.4 MeV

1Igo+ (1961)

11.8 MeV

1

12.8 MeV

1

Lohr+ (1974)

13 MeV

0 30 60 90 120 150 180

0.1

1

c.m.

(deg)

Joly+ (1963)

15 MeV

1

9.8 MeV

1

9 MeV

0 30 60 90 120 150 1800.01

10

c.m.

(deg)

58.7 MeV(d)

1

7 MeV

1

Haixia+TALYS-1.0This work: phenomenologic

5 MeV 27Al(d,d0)

1

11 MeV

0.1

1

11.4 MeV

1

11.8 MeV

0.1

1

12.8 MeV

1

13 MeV

0.1

1

15 MeV

1

52 MeV

10

20

-W

(M

eV

)

WD local

WD average(b)

WV local

WV average

0 10 20 30 40 50 60

-10

0

10

-U

(M

eV

)

V

D

Ed (MeV)

(c)

0 10 20 30 40 50 600

400

800

1200

R (m

b)

Haixia+ TALYS-1.0 ACSELAM this work

d + 27Al

Ed (MeV)

(e)

Mayo+ (1965)Dubat+ (1974)

1

Strzalkowski+ (1962)

9.8 MeV

1

9 MeV

1

Al-Quraishi+ (2000)Schwandt+ (1968)

7 MeV

1

Lohr-Haeberli Daehnick+ This work: microscopic

5 MeV27Al(d,d

0)

(a)

1

11 MeV

0.1

1

/

Ru

the

rfo

rd

11.4 MeV

1Igo+ (1961)

11.8 MeV

1

12.8 MeV

1

Lohr+ (1974)

13 MeV

0 30 60 90 120 150 180

0.1

1

c.m.

(deg)

Joly+ (1963)

15 MeV

1

9.8 MeV

1

9 MeV

0 30 60 90 120 150 1800.01

10

c.m.

(deg)

58.7 MeV(d)

1

7 MeV

1

Haixia+TALYS-1.0This work: phenomenologic

5 MeV 27Al(d,d0)

1

11 MeV

0.1

1

11.4 MeV

1

11.8 MeV

0.1

1

12.8 MeV

1

13 MeV

0.1

1

15 MeV

1

52 MeV

10

20

-W

(M

eV

)

WD local

WD average(b)

WV local

WV average

0 10 20 30 40 50 60

-10

0

10

-U

(M

eV

)

V

D

Ed (MeV)

(c)

0 10 20 30 40 50 600

400

800

1200

R (m

b)

Haixia+ TALYS-1.0 ACSELAM this work

d + 27Al

Ed (MeV)

(e)

Mayo+ (1965)Dubat+ (1974)

1

Strzalkowski+ (1962)

9.8 MeV

1

9 MeV

1

Al-Quraishi+ (2000)Schwandt+ (1968)

7 MeV

1

Lohr-Haeberli Daehnick+ This work: microscopic

5 MeV27Al(d,d

0)

(a)

1

11 MeV

0.1

1

/

Ru

the

rfo

rd

11.4 MeV

1Igo+ (1961)

11.8 MeV

1

12.8 MeV

1

Lohr+ (1974)

13 MeV

0 30 60 90 120 150 180

0.1

1

c.m.

(deg)

Joly+ (1963)

15 MeV

1

9.8 MeV

1

9 MeV

0 30 60 90 120 150 1800.01

10

c.m.

(deg)

58.7 MeV(d)

1

7 MeV

1

Haixia+TALYS-1.0This work: phenomenologic

5 MeV 27Al(d,d0)

1

11 MeV

0.1

1

11.4 MeV

1

11.8 MeV

0.1

1

12.8 MeV

1

13 MeV

0.1

1

15 MeV

1

52 MeV

10

20

-W

(M

eV

)

WD local

WD average(b)

WV local

WV average

0 10 20 30 40 50 60

-10

0

10

-U

(M

eV

)

V

D

Ed (MeV)

(c)

0 10 20 30 40 50 600

400

800

1200

R (m

b)

Haixia+ TALYS-1.0 ACSELAM this work

d + 27Al

Ed (MeV)

(e)

Mayo+ (1965)Dubat+ (1974)

DF-real & phenomenological imaginary/s.o. potentials Phenomenological OMP

Page 10: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 10 Marilena Avrigeanu

d breakup

1 (a) fpTBU= 0.087 – 0.0066 Z + 0.00163 Z A1/3 + 0.0017 A1/3E – 2E-6 ZE2

1 (b) fELBU= 0.031 – 0.0028 Z + 0.00051 Z A1/3 + 0.0005 A1/3E – 1E-6 ZE2

elastic 27Al + d 27Al + n+ p

inelastic (27Al + n) + p (28Al*) + p 27Mg + p + p (2p ch. of 29Si* )

24Na + α + p (pα ch. of 29Si* ) inelastic (27Al + p) + n (28Si*) +n 27Si + n + n (2n ch. of 29Si* )

Empirical breakup enhancement fBU from (d,p) & (d,n) systematics

Page 11: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 11 Marilena Avrigeanu

Stripping contribution (FRESCO-code; 18 levels of 28Si)

0 30 60 90 120 150

1E-10

1E-9

1E-8

1E-7

1E-6

1E-5

1E-4

1E-3

0.01

0.1

1

Bohne+ (1969)

c.m.

(deg)

d/d

(mb/s

r)

g.s., 0+

27Al(d,n)28Si

Ed=6 MeV

1.779, 2+x102

x104

4.618, 4+

6.276, 3+

x106

x108

7.799, 3+

0 30 60 90 120 150

1E-10

1E-9

1E-8

1E-7

1E-6

1E-5

1E-4

1E-3

0.01

0.1

1

c.m.

(deg)

DR PE+CN DR+PE+CN

7.930, 2+

x103

8.543,6+ + 8.587,3+

x105

9.319, 3+

Bohne+ (1969)

x107

9.379,2+ + 9.41,5+

x109

10.379, 3+

Page 12: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 12 Marilena Avrigeanu

Stripping contribution (FRESCO-code; 35 levels of 28Al)

0 10 20 30 40 50

1E-11

1E-9

1E-7

1E-5

1E-3

0.1

10

0 30 60 90 120 150

1E-18

1E-16

1E-14

1E-12

1E-10

1E-8

1E-6

1E-4

0.01

1

100

Chen+ (1972)

c.m.

(deg)

d/d

(mb/s

r)

g.s., 3+

27Al(d,p)28AlE

d=6 MeV

0.031, 2+

x102

x104

1.014, 3+

2.138, 2+x106

x108

2.272, 4+

x1010

2.656, 4+

3.465, 4-

x1012

x1014

3.591, 3-

4.904, 2-

x1016

5.135, 3-

x1018

0 20 40 60 80 100

1E-28

1E-26

1E-24

1E-22

1E-20

1E-18

1E-16

1E-14

1E-12

1E-10

1E-8

1E-6

1E-4

0.01

1

c.m.

(deg)

g.s.

Ed=12 MeV

x103

0.031

x106

1.014

Carola+ (1971)

x109

2.138

x1012

2.272

x1015

2.656

x1018

3.465

x1021

3.591

4.765, 2-

4.904

x1024

x1027

DR PE+CN DR+PE+CN

c.m.

(deg)

g.s. + 0.031

1.014

x104

Maher+(1972)

Ed=23 MeV

x105

2.138x106

2.272

2.656

x107

x109

3.465x1010

3.591

4.033, 5-

x1011

4.315, 1+

x1013

g.s. + 0.031

Page 13: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 13 Marilena Avrigeanu

Breakup & DR

27Al + d (27Al + n) + p

(T) (B)

(27Al + p) + n

peak centroid: Ex = Ax/Ad*(Einc – 1.44ZdZT/(1.5AT1/3 + Rd) + 1.44ZxZB/(1.5AT

1/3 + Rd)

FWHM: = 0.3 (Einc + 15 MeV ) (1 – AT/1500) [Kalbach, 2007]

0 20 40 600.0

0.2

0.4

0.6

Ed (MeV)

(EB+BFDR) / R

EB+BF /R

DR /R

/

React

ion

d + 27Al(a)

0 5 10 15 20 25 300

5

10

15

Ed (MeV)

Ex

(MeV

) Ep

En

27Al(d,n+p)

(b)

Breakup energies for n & p

Page 14: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 14 Marilena Avrigeanu

BREAKUP contribution to the SECOND particle emission

σBF(p) vs Ed σBF

(p) vs Ed σBF(n) vs Ed

27Al(n,p)27Mg vs En 27Al(n,α)24Na vs En

27Al(p,n)27Si vs Ep

27Al(n,p)27Mg vs Ed 27Al(n,α)24Na vs Ed

27Al(p,n)27Si vs Ed

[via BF] [via BF] [via BF]

0 5 10 15 20 25 30

0.1

1

10

100

(

mb)

Wilson+ (1976)Bem+ (2007)

27Al(d,2p)27Mg

BF add-on BF add (smooth)

0.002*(p)BF

(a)

(p)BF

27Al(n,p)27

Mg

0 20 40 60

0.01

0.1

1

10

10027Al(d,p)24Na

(p)BF

27

Al(n,)24

Na

BF add-on BF add (smooth)

0.001*(p)BF

(b)

0 5 10 15 20 25 301

10

100

E (MeV)

27Al(d,2n)27Si Wilson+ (1976)

(n)BF

27Al(p,n)27Si BF add-on BF add (smooth)(c)

Page 15: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 15 Marilena Avrigeanu

d + 27Al: Activation cross-sections

5 10 15 20 250

5

10

15

20

25

(

mb)

Wilson+ (1976)Bem+ (2007) TALYS-1.0 ACSELAM BF+PE+CN BF STAPRE-H

(PE+CN)

27Al(d,2p)27Mg

(c)

0 5 10 15 20 250

100

200

300

400

500

TALYS-1.0 ACSELAM DR+PE+CN FRESCO (DR) STAPRE-H

(PE+CN)

27Al(d,p)28Al (a)

Wilson+(1976)Bem+ (2007)

10 20 30 40 50 600

20

40

60

80

Ed [MeV]

27Al(d,p)24NaMartens+ ('70)Watson+ ('73)Wilson+ ('76)Zarubin+ ('79)Weinreich+('80)Michel+ ('82)Tao Zhen+ ('87)Zhao Wen+ ('95)Takacs+ (2001)Hagiwara+(2004)Nakao+ (2006)Bem+ (2007)

TALYS-1.0ACSELAM

(f)

BF+PE+CN PE+CN BF

10 15 20 250

20

40

60

8027Al(d,2n)27Si

TALYS-1.0 ACSELAM BF+PE+CN BF STAPRE-H

(PE+CN)

(d)

Wilson+ (1976)

0 5 10 15 20 250

200

400

600

800

TALYS-1.0 ACSELAM DR+PE+CN FRESCO (DR) STAPRE-H

(PE+CN)

27Al(d,n)28Si(b)

0 5 10 15 20 250

50

100

150

200

250

TALYS-1.0 ACSELAM STAPRE-H

(PE+CN)

27Al(d,)25Mg Al-Quraishi+(2000): (d,x)

(e)

Page 16: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 16 Marilena Avrigeanu

Activation cross sections for d + 63,65Cu [ former approach ]

0.1

1

10

100

Fulmer+ (1970)-natCu NPI-Prague (2007)

TALYS EMPIRE

63Cu(d,3n)62Zn[0+ 9.3H]

0

100

200

300

400

[

mb

]

Okamura+ (1971) Gilly+ (1963) NPI-Prague (2007)

TALYS EMPIRE

63Cu(d,p)64Cu [1+ 12.8H]

0

100

200

300

400

Okamura+ (1971) Gilly+ (1963) NPI-Prague (2007)

TALYS EMPIRE

63Cu(d,2n)63Zn[3/2- 38.4M]

0 20 40 600

1

2

3

4

5

6

7

8

9

Ed [MeV]

Baron+ (1963) NPI-Prague (2007)

TALYS EMPIRE

65Cu(d,2p)65Ni[5/2- 2.6H]

0 20 40 600

200

400

600

800

Ed [MeV]

Okamura+ (1971)

Fulmer+ (1970) natCu Gilly+ (1963)

TALYS EMPIRE

65Cu(d,p)66Cu [1+ 5.1M]

0 5 10 15 20 25 300

300

600

900

1200

Ed [Mev]

Okamura+ (1971)

Fulmer+ (1970)) natCu Pement+ (1966) NPI-Prague (2007)

TALYS EMPIRE

65Cu(d,2n)65Zn[5/2- 245D]

Page 17: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 17 Marilena Avrigeanu

CONCLUSIONS Starting point: available (d,d) and R data for d+27Al,54,56,58,natFe,63,65,natCu,93Nb

poor description by global OMP parameter sets

Semi-microscopic OMP analysisUDF: ρd (charge) & ρAl (charge) & M3Y Paris-NNWD & VSO phenomenological

improved agreement with data adding the dispersion corrections

Phenomenological OMP analysis for 27Al agreement with all available measured data good description of (d,d) data vs. TALYS default OMPs improved description of (d,d) data vs. global OMPs

Completion of d+27Al activation cross sections Deuteron break-up mechanism contribution taken into account DR mechanism considered trough n & p stripping contributions Comparison of STAPRE-H / TALYS-1 activation cross sections

NEED to UPDATE the d-activation libraries

Page 18: Progress on Deuteron-Induced Activation Cross Section Evaluation

FENDL-3 1st Research Co-ordination Meeting, 2-5 December 2008, IAEA, Vienna 18 Marilena Avrigeanu

Thank you