nuclear reaction models for systematic analysis of fast neutron induced (n,p) reaction cross...
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NUCLEAR REACTION MODELS FOR SYSTEMATIC ANALYSIS OF FAST NEUTRON INDUCED
(n,p) REACTION CROSS SECTIONS
M.Odsuren, J.Badamsambuu, G.Khuukhenkhuu
Nuclear Research Center, National University of Mongolia, Ulaanbaatar, Mongolia
MOTIVATION
Investigation of fast neutron induced charged particle emission reactions is important:
1. Fundamental nuclear physics study: – The study of nuclear reactions mechanisms – Nuclear structure
2. Fission and fusion reactors technology:– Radiation damage – Residual radioactivity – Hydrogen and helium gas production
Systematical analysis of neutron cross sections is of interest: 1. To evaluate of neutron cross sections2. To estimate of authenticity for experimental data
Statistical Model: J.M.Blatt, V.F.Weisskopf, Theoretical Nuclear Physics, John Wiley and Sons, New York, (1952)
Compound Mechanism: N.Bohr, Nature, v.137 (1936), p.344
Pre-equilibrium Mechanism: J.Griffin, Phys.Rev.Lett. vol.17, 1966, p.478 Exciton Model
Direct Reaction Mechanism: J.R.Oppenheimer, M.Philips. Phys.Rev., v.48, Plane Wave Born Approximation N6, 1935, p.500
V.N. Levkovsky, Sov.J.Nucl.Phys. 18, N4, 1973, p.705 Empirical formula (n,p) and (n,) at En=14-15 MeV
Here: C=0.73 and, K=33 are fitting parameters.
A
ZNK
eArCpn
23/12
0 )1(),(
G.Khuukhenkhuu, JINR preprint. E3-93-205, Dubna, 1993
A
ZNK
comnp eRC
12)(
pVAA
ZC
4/33/1
121exp
4K
Here:
R, Z, N and A - radius, proton, neutron and mass numbers of target nuclei
- Wavelength of incident neutrons divided by 2Vp - Coulomb potential for protons
- Thermodynamic temperature of nuclei
and =i-f - Сonstants of Weizsacker’s formula.
G.Khuukhenkhuu, G.Unenbat, M.Odsuren et al. JINR Preprint, E3-2007-25,Dubna, 2007, -12p.
(1)
– Statistical Model:
– Exciton Model:
3
3
0
22
6
)(
)(2)(3.68
nn
pnpnpnr
prenp
BE
VQE
AK
MER
)( nr E3
0 MeV 400KpM
nE nB
npQ
dirnp
prenp
comnp
totnp
n
np2
0
dir
np E
Q1RC
Where 0C can be determined as best fitting the experimental data parameter.
Theoretical total (n,p) cross section:
(2)
(3)
G.Khuukhenkhuu, G.Unenbat, M.Odsuren et al.JINR Preprint, E3-2007-26, Dubna, 2007, -5p.
Where:
-Neutron induced reaction total cross section
- Mass of proton
and - Kinetic and binding energy of neutron
- Reaction energy
G.Khuukhenkhuu, G.Unenbat, M.Odsuren et al.JINR Preprint, E3-2007-27, Dubna, 2007, -7p
– Plane Wave Born Approximation:
SYSTEMATICS OF THE (n,p) REACTION CROSS SECTIONS
En (MeV) K C
6 75.2 17.5
8 62.8 11.9
10 52.1 6.80
13 38.8 2.74
14.5 37.3 2.43
16 33.5 1.42
18 22.4 0.39
20 17.9 0.25
En=20 MeV
C = 0.25K=17.9
1.E-03
1.E-02
1.E-01
1.E+00
0.02 0.06 0.10 0.14 0.18 0.22(N-Z+1)/A
n
p/
(R+l
)2
En=14.5 MeV
C = 2.43K=37.3
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0.02 0.06 0.10 0.14 0.18 0.22
N-Z+1/A
np
/(R
+l )
2
En=6 MeV
C = 17.5K=75.2
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0.02 0.06 0.10 0.14(N-Z+1)/A
np/ (
R+l )
2
Statistical model (n,p) cross sections and experimental data:
COMPARISON OF EXPERIMENTAL AND THEORETICAL (n,p) CROSS SECTIONS
En=6 MeV
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
1.E+04
0.02 0.06 0.10 0.14(N-Z+1)/A
np(m
b)
Experiment
Compound
En=20MeV
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.02 0.06 0.10 0.14 0.18 0.22
(N-Z+1)/A
np (m
b)
Experiment
Compound
En=14.5 MeV
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
1.E+04
0.02 0.06 0.10 0.14 0.18 0.22N-Z+1/A
(m
b)
Experiment
Compound
A
1ZNK
2com
np eRC
)(
Exciton model (n,p) cross sections and experimental data:
En=14.5 MeV
1.E-03
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.00 0.05 0.10 0.15 0.20 0.25
(N-Z+1)/A
n
p (m
b)
Experiment
Pre-equilibrium
En=6 MeV
1.E-03
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.02 0.06 0.10 0.14(N-Z+1)/A
np (
mb
)
Experiment
Pre-equilibrium
En=20MeV
1.E+00
1.E+01
1.E+02
1.E+03
0.02 0.06 0.10 0.14 0.18 0.22
(N-Z+1)/A
n
p(b
m)
Experiment
Pre-equilibrium
3
nn
3pnpn
0
pnr
2
2
6pre
npBE
VQE
AK
M2ER368
)(
)()(.
PWBA (n,p) cross sections and experimental data:
En=14.5 MeV
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.00 0.05 0.10 0.15 0.20 0.25
(N-Z+1)/A
np
(mb)
Experiment
Direct
En=6 MeV
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.02 0.06 0.10 0.14(N-Z+1)/A
np(m
b)
Experiment
Direct
En=20MeV
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
0.02 0.06 0.10 0.14 0.18 0.22
(N-Z+1)/A
np (m
b)
Experiment
Direct
n
np2
0
dir
np E
Q1RC
The total (n,p) cross sectiondirnp
prenp
comnp
totnp
The theoretical total (n,p) cross sections are satisfactorily in agreement with experimental values for En=6, 14.5 and 20 MeV. Also, in the case of En=8, 10, 13, 16 and 18 MeV neutrons we have almost the same results.
En=14.5 MeV
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
1.E+04
0.00 0.05 0.10 0.15 0.20 0.25
(N-Z+1)/A
np
(mb)
Experiment
Comp+Pre+Dir
En=6 MeV
1.E-02
1.E-01
1.E+00
1.E+01
1.E+02
1.E+03
1.E+04
0.02 0.06 0.10 0.14(N-Z+1)/A
np( m
b)
Experiment
Comp+Pre+Dir
n
np20
dirnp E
Q1RC
3
3
0
22
6
)(
)(2)(3.68
nn
pnpnpnr
prenp
BE
VQE
AK
MER
A
ZNKcom
np eRC1
2)(
En=20MeV
1.E+00
1.E+01
1.E+02
1.E+03
1.E+04
0.02 0.06 0.10 0.14 0.18 0.22
(N-Z+1)/A
n
p (m
b)
Experiment
Com+Pre+Dir
CONCLUSION
1. Using the statistical model, exciton model and PWBA are deduced formulae for the fast neutron induced (n,p) reaction cross sections.
2. The formulae were used for systematical analysis of fast neutron induced (n,p) reaction cross sections.
3. It was shown that the theoretical and experimental total (n,p) cross sections for En=6-20 MeV are satisfactorily in agreement.
NUCLEAR RESEARCH CENTERTOTAL REFLECTION X-RAY SPECTROMETER
lg
10010ysensitivit
KeV95at
eV180resolution
.