nuclear data needs and capabilities for applications...
TRANSCRIPT
![Page 1: Nuclear Data Needs and Capabilities for Applications (NDNCA)bang.berkeley.edu/wp-content/uploads/LBNL_tornow.pdf · FELs: OK-4 (lin), OK-5 (circ) ... DE/E = 1.3% Vladimir Litvinenko](https://reader035.vdocuments.site/reader035/viewer/2022071021/5fd527f08ed3f475230d7c56/html5/thumbnails/1.jpg)
Nuclear Data Needs and Capabilities for Applications(NDNCA)
Triangle Universities Nuclear Laboratory Facilities Review
Werner TornowDuke University & TUNL
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2
TUNL: Accelerator Facilities1.2 GeV Storage Ring FELHigh Intensity Gamma Source (HIγS)
Eg = 1 – 100 MeVLinear and circular polarized photon beamsDelivering up to 103 γ/s/eV on target, HIgS is the most intense accelerator-driven γ-ray source in the world
World’s highest current proton beam for nuclear astrophysics research
Laboratory for Experimental Nuclear Astrophysics (LENA)
Tandem Laboratory: light-ion and pulsed neutron beams
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3
Tandem Lab
Accelerator and Source Features:TVmax = 10 MVParticles: light ions (p, d, 3He, 4He)Secondary beams: pulsed neutron beamsPolarized beams: p and d
Research examples:1. Few-nucleon dynamics: 2H(n,nnp)2. 2-nucleon transfer reactions
relevant to 0nbb, e.g., A(3He,n)3. Neutron multiplication: A(n,2ng)4. Detector Characterization (n scattering)5. Nuclear astrophysics6. Applications
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Concentrate on neutron physics capabilities
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Floor Plan of TUNL (Triangle Universities Nuclear Laboratory)
For neutron energies below En=0.6 MeV: 7Li(p,n)7BeFor neutron energies below En=4 MeV: 3H(p,n)3He
For neutron energies above En=4 MeV: 2H(d,n)3He
For neutron energies above En=14.5 MeV and below 35 MeV: 3H(d,n)4He
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DC or pulsed beam operation at 2.5 MHz (i.e., 400 ns between pulses) or factors of 2 in rep rate reduction
2H(d,n)3He; Q-value = + 3.27 MeV
� 2H(d,n)3He neutron source
� Id = (1-4) A, pulsed up to 1 A
� Deuterium gas pressure 1 - 8 atm
� Tunable energy from 4 to 20 MeV
� Flux on target (107 - 108) cm-2 s-1
� Energy spread dE/E = 0.02 to 0.15
NTOFTarget Room
ENGESpectrometer
Shielded Neutron SourceFN-Tandem 10 MVIon Sources
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Havar foil
D2
d
Ceramicinsulator
Aperture Suppressor
D2 gas inlet
High-pressureKr-86 sphere
Flange
n
Activation foils
(n,2n)
238U(n,2n)237U
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Activation and TOF Measurements at TUNL with PT Source
� 3H(p,n)3He neutron source
� Id = (1- 4) A, pulsed up to 1 A
� Tritiated titanium target (2 Ci)
� Tunable energy from 1 to 5 MeV
� Flux on target (105 - 106) cm-2 s-1
� Energy spread dE/E = 0.02 to 0.10
3H(p,n)3He; Q-value = - 0.763 MeV
Ion Sources FN-Tandem 10 MV Shielded Neutron Source
EngeSpectrometer
NTOFTargetRoom
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Havar foil
He
p,d
Ceramicinsulator
Aperture Suppressor
He gas inlet
FlangeTritiatedtitaniumlayer
Monitor foils
n 124Xe
Copperbacking Cd Cage
(n,g)
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3H(d,n)4He
108 n/(cm2s) at 14.1 to 14.8 MeV
Q=17.589 MeV
105 n/(cm2s) at 30 MeV
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DC or pulsed beam operation at 2.5 MHz (i.e., 400 ns between pulses) or factors of 2 in rep rate reduction
2H(d,n)3He; Q-value = + 3.27 MeV
� 2H(d,n)3He neutron source
� Id = (1-4) A, pulsed up to 1 A
� Deuteriumgas pressure 1 - 8 atm
� Tunable energy from 4 to 20 MeV
� Flux on target (107 - 108) cm-2 s-1
� Energy spread dE/E = 0.02 to 0.15
NTOFTarget Room
ENGESpectrometer
Shielded Neutron SourceFN-Tandem 10 MVIon Sources
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TUNL: 1 - 20 MeV mono-energetic neutrons
(n,n0) and (n,n’) ds/dW(q)
4 m detector
6 m detector
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FPY235U238U239Pu
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DC or pulsed beam operation at 2.5 MHz (i.e., 400 ns between pulses) or factors of 2 in rep rate reduction
2H(d,n)3He; Q-value = + 3.27 MeV
� 2H(d,n)3He neutron source
� Id = (1-4) A, pulsed up to 1 A
� Deuteriumcgas pressure 1 - 8 atm
� Tunable beam from 4 to 20 MeV
� Flux on target (107 - 108) cm-2 s-1
� Energy spread dE/E = 0.02 to 0.15
NTOFTarget Room
ENGESpectrometer
Shielded Neutron SourceFN-Tandem 10 MVIon Sources
![Page 15: Nuclear Data Needs and Capabilities for Applications (NDNCA)bang.berkeley.edu/wp-content/uploads/LBNL_tornow.pdf · FELs: OK-4 (lin), OK-5 (circ) ... DE/E = 1.3% Vladimir Litvinenko](https://reader035.vdocuments.site/reader035/viewer/2022071021/5fd527f08ed3f475230d7c56/html5/thumbnails/15.jpg)
Shielded Neutron Source: 2H(d,n)3He
~2x104n/(cm2s)
Neutron detectors
ds/dW(q)
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HPGe detectors
(n,n’g)
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NNSA Setup at TUNL
TUNL
� 4 Clovers + BGO
� 2 Planars + BGO
� 10 keV < Eg < 10 MeV
� 200 < qlab < 1600
� array = 1.4%@Eg = 1.33 MeV
Total cost of $1M
Excellent tool for precision neutron induced cross section measurements in the fast neutron energy region (4 En 18 MeV)
� g-g coincidence measurements
�Angular distribution measurements
� Lifetimes (by Doppler method)
Capabilities
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HIgS
High-Intensity g-ray Source
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160 MeV Linac pre-injector160 MeV – 1.2 GeV Booster injector240 MeV – 1.2 GeV Storage ringFELs: OK-4 (lin), OK-5 (circ)HIgS: two-bunch, 40 – 120 mA (typ)
HIgS (High-Intensity Gamma-ray Source): An electron-photon colliderEnergy (MeV): 1 – 100 MeV Laser: FEL, 1060 – 190 nm (1.17 – 6.53 eV)Total flux: 107– 3x1010g/s (max ~10 MeV)Spectral flux: 103g/s/eV (max ~10 MeV)Research: Nuclear physics,
National Security
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E
8
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How to produce g rays?
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HIgS: Intracavity Compton-Back Scattering
Example: Ee = 500 MeV Î g = 978lFEL = 400 nmħω = 3.11 eVEg = 11.9 MeV
Head-on collision: Eg ≈ 4γ2ħω
2500
1500
500
1950 2000 2050Eg (keV)
Inte
nsity Eg =2032 keV
DEg =26 keVDE/E = 1.3%
Vladimir Litvinenko
¾” dia.DE/E~3%
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Why do we have a booster synchrotron?
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160 MeV Linac pre-injector160 MeV – 1.2 GeV Booster injector240 MeV – 1.2 GeV Storage ringFELs: OK-4 (lin), OK-5 (circ)HIgS: two-bunch, 40 – 120 mA (typ)
HIgS (High-Intensity Gamma-ray Source): An electron-photon colliderEnergy (MeV): 1 – 100 MeV Laser: FEL, 1060 – 190 nm (1.17 – 6.53 eV)Total flux: 107– 3x1010g/s (max ~10 MeV)Spectral flux: 103g/s/eV (max ~10 MeV)Research: Nuclear physics,
National Security
![Page 27: Nuclear Data Needs and Capabilities for Applications (NDNCA)bang.berkeley.edu/wp-content/uploads/LBNL_tornow.pdf · FELs: OK-4 (lin), OK-5 (circ) ... DE/E = 1.3% Vladimir Litvinenko](https://reader035.vdocuments.site/reader035/viewer/2022071021/5fd527f08ed3f475230d7c56/html5/thumbnails/27.jpg)
How do we select our g-ray energy spread?
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HIgS: Intracavity Compton-Back Scattering
Example: Ee = 500 MeV Î g = 978lFEL = 400 nmħω = 3.11 eVEg = 11.9 MeV
Head-on collision: Eg ≈ 4γ2ħω
2500
1500
500
1950 2000 2050Eg (keV)
Inte
nsity Eg =2032 keV
DEg =26 keVDE/E = 1.3%
Vladimir LitvinenkoRep. rate 5.58 Mz: pulse every ~180 ns
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How do we change the g-ray energy?
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160 MeV Linac pre-injector160 MeV – 1.2 GeV Booster injector240 MeV – 1.2 GeV Storage ringFELs: OK-4 (lin), OK-5 (circ)HIgS: two-bunch, 40 – 120 mA (typ)
HIgS (High-Intensity Gamma-ray Source): An electron-photon colliderEnergy (MeV): 1 – 100 MeV Laser: FEL, 1060 – 190 nm (1.17 – 6.53 eV)Total flux: 107– 3x1010g/s (max ~10 MeV)Spectral flux: 103g/s/eV (max ~10 MeV)Research: Fundamental Nuclear Physics,
National Security
![Page 31: Nuclear Data Needs and Capabilities for Applications (NDNCA)bang.berkeley.edu/wp-content/uploads/LBNL_tornow.pdf · FELs: OK-4 (lin), OK-5 (circ) ... DE/E = 1.3% Vladimir Litvinenko](https://reader035.vdocuments.site/reader035/viewer/2022071021/5fd527f08ed3f475230d7c56/html5/thumbnails/31.jpg)
Gamma-ray Energy Tuning Range at HIgS
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E1 transition
M1 transition
mono-energetic,polarized and pencil-like beam
E
Asymmetry:
=-1 E1 transition=+1 M1 transition
Nuclear Resonance Fluorescence (NRF)(g,g) & (g,g’)
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2450 2500 2550 2600 2650
0
50
100
150
200
250
300
350
Runs 330, 334 (5 hr 21 min) - 240Pu @ 2.55 MeVHorizontal and Vertical RF Subtracted
2492
2578
2566
2547
25352523
2504Cou
nts
Energy (keV)
Horizontal Vertical
Ex
Energy (keV)Jπ1+/-
2+
0+
42.8
0.0
240Pu
240Pu: Determination of spin and parity
Nuclear Forensics
(g,n)
(g,f)
(g,g’)
NNSADNDO
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COSTS
Tandem: $ 200-250 per hour
HIgS: $ 950 per hour
PAC
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Backup
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37
Tandem: Enge split-pole spectrometer