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IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JUNE 1995 539 Monolithic Multiple Colliding Pulse Mode-Locked Quantum-Well Lasers: Experiment and Theory Joaquim F. Martins-Filho, Student Member, IEEE, Eugene A. Avrutin, C. N. Ironside, and J. S. Roberts Abstract— We report here on a monolithic multisectioned quantum-well laser that operates as multiple colliding pulse mode-lockhg source. With thk type of operation several puises are present wittdn a laser simultaneously and it produces high-repetition rate pulse trains (up to 375 GHz) and pulse widths of around 1-3 ps, as deduced from linear correlation technique measurements. By changing the configuration of the sections 1, 2, 3, cm 4 pulse operation can be selected; frequency- and time-domairl theories have been developed to explain this type of behavior. I. INTRODUCTION s EMICONDIJCTOR lasers are compact and efficient sources of picosecond and subpicosecond pulses. Due to their small size, low pumping power requirement, low cost and robustness they are the most suitable laser device for integration in optical circuits for ultrafast photonic applica- tions, such as high-speed communication systems, ultrafast data processing, optical computing and opto-microwave- electronic interfacing. Among the different methods of short pulse generation in semiconductor lasers mode-locking is able to produce shorter pulses, with better spectral characteristics at higher repetition. rates [1]–[3]. The most common approaches to mode-lock semiconductor lasers are passive, active and hybrid mode-locking, in monolithic or external extended cavity configuration [11, [2]. Monolithic mode-locked semiconductor lasers devices offer the possibility of very low cost sources of ultrashort pulses which are compact, reliable, robust, efficient and can be mass-produced. The monolithic passive mode- locking scheme is attractive for achieving high-repetition rates, above 100 GHz since it does not require the injection of a high-frequency RF signal. This scheme can be very simply implemented by integrating a saturable absorber in the laser cavity [1]–[3]. The fast dynamics of the nonlinear behavior of the saturation and recovery of both absorber and gain sections of the laser is responsible for its ultrafast characteristics pl]–[6]. Portnoi et al. first observed mode-locking at 200 GHz, by using proton bombardment to form the saturable absorber section in the laser [7]. Chen et al. used a 250 pm long Manuscript received November 3, 1994 revised Jarmary 31, 1995. This work was supported by the EPSRC through Grant GIVH82471. One of the authors (J. F. Martins-Filho) was supported by CNPq (Brazilian Research Council). J. F. Martins-Filllo, E. A. Avmtirr, and C. N. Ironside are with the Department of Electronics and Electricrd Engineering, University of Glasgow, Glasgow G12 8LT UK. J. S. Roberts is with the Department of Electronics and Electrical Engi- neering, University of Sheffield, Sheffield S 1 3JD UK. IEEE Log Number 9411694. 4 - b L14 L14 L14 L14 (a) + (b) Fig. 1. Top view diagram (a) and longitudinal cross-section of the wavegnide (b) of the MCPM laser. In Fig. 2(b), the schematic electrical connections for forward and reverse biasing (for the case of having three absorbers in the cavity) are stso shown. monolithic passive colliding pulse mode-locked (CPM) laser to obtain 0.65 ps pulses at 350 GHz [8]. The CPM configuration consists of placing a saturable absorber section precisely in the middle of the laser cavity, which makes the laser generate two counter propagating pulses that collide in the absorber section [3], [8]. The saturable absorber section is implemented by simply applying a reverse bias to the central part of the split contact of the laser [8], [9]. More recently a growing interest has been apparent in the generation of ultrashort pulses at ultrahigh-repetition rates [10]-[13], reaching terahertz rates [14], [15]. Such high speed is achieved by inducing the laser to operate at harmonics of the fundamental inverse round-trip time of the cavity. Generation of harmonics of the repetition rate can be achieved in actively mode-locked lasers by suitable choice of the repetition frequency of the driving signal [2], [3]. In passive mode-locked lasers, several harmonics have been observed in a multistable behavior [16], [17], where the operating hatmonic is dependent on the gain section current [10], [14]–[17]. In this paper, we present the progress on generation of short pulses at high-repetition rates by multiple colliding pulse mode-locked (MCPM) quantum-well lasers. These devices are monolithic multi-sectioned passive mode-locked semiconduc- tor lasers that can generate short pulses at harmonics of the cavity round trip frequency, depending on the electrical bias applied to each of their sections. Fig. 1(a) shows the top 1077-260K/95$04.00 0 1995 IEEE

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  • IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JUNE 1995 539

    Monolithic Multiple Colliding Pulse Mode-LockedQuantum-Well Lasers: Experiment and TheoryJoaquim F. Martins-Filho, Student Member, IEEE, Eugene A. Avrutin, C. N. Ironside, and J. S. Roberts

    Abstract— We report here on a monolithic multisectionedquantum-well laser that operates as multiple colliding pulsemode-lockhg source. With thk type of operation several puisesare present wittdn a laser simultaneously and it produceshigh-repetition rate pulse trains (up to 375 GHz) and pulsewidths of around 1-3 ps, as deduced from linear correlationtechnique measurements. By changing the configuration of thesections 1, 2, 3, cm 4 pulse operation can be selected; frequency-and time-domairl theories have been developed to explain thistype of behavior.

    I. INTRODUCTION

    sEMICONDIJCTOR lasers are compact and efficientsources of picosecond and subpicosecond pulses. Dueto their small size, low pumping power requirement, low costand robustness they are the most suitable laser device forintegration in optical circuits for ultrafast photonic applica-

    tions, such as high-speed communication systems, ultrafast

    data processing, optical computing and opto-microwave-electronic interfacing. Among the different methods of shortpulse generation in semiconductor lasers mode-locking is ableto produce shorter pulses, with better spectral characteristics athigher repetition. rates [1]–[3]. The most common approachesto mode-lock semiconductor lasers are passive, active andhybrid mode-locking, in monolithic or external extended cavityconfiguration [11, [2]. Monolithic mode-locked semiconductorlasers devices offer the possibility of very low cost sources of

    ultrashort pulses which are compact, reliable, robust, efficientand can be mass-produced. The monolithic passive mode-locking scheme is attractive for achieving high-repetition

    rates, above 100 GHz since it does not require the injectionof a high-frequency RF signal. This scheme can be verysimply implemented by integrating a saturable absorber inthe laser cavity [1]–[3]. The fast dynamics of the nonlinearbehavior of the saturation and recovery of both absorberand gain sections of the laser is responsible for its ultrafast

    characteristics pl]–[6].Portnoi et al. first observed mode-locking at 200 GHz, by

    using proton bombardment to form the saturable absorbersection in the laser [7]. Chen et al. used a 250 pm long

    Manuscript received November 3, 1994 revised Jarmary 31, 1995. Thiswork was supported by the EPSRC through Grant GIVH82471. One of theauthors (J. F. Martins-Filho) was supported by CNPq (Brazilian ResearchCouncil).

    J. F. Martins-Filllo, E. A. Avmtirr, and C. N. Ironside are with theDepartment of Electronics and Electricrd Engineering, University of Glasgow,Glasgow G12 8LT UK.

    J. S. Roberts is with the Department of Electronics and Electrical Engi-neering, University of Sheffield, Sheffield S 1 3JD UK.

    IEEE Log Number 9411694.

    4 - b

    L14 L14 L14 L14

    (a)

    +

    (b)

    Fig. 1. Top view diagram (a) and longitudinal cross-section of the wavegnide(b) of the MCPM laser. In Fig. 2(b), the schematic electrical connections forforward and reverse biasing (for the case of having three absorbers in thecavity) are stso shown.

    monolithic passive colliding pulse mode-locked (CPM) laser toobtain 0.65 ps pulses at 350 GHz [8]. The CPM configurationconsists of placing a saturable absorber section precisely inthe middle of the laser cavity, which makes the laser generatetwo counter propagating pulses that collide in the absorber

    section [3], [8]. The saturable absorber section is implementedby simply applying a reverse bias to the central part of the

    split contact of the laser [8], [9].More recently a growing interest has been apparent in the

    generation of ultrashort pulses at ultrahigh-repetition rates[10]-[13], reaching terahertz rates [14], [15]. Such high speedis achieved by inducing the laser to operate at harmonicsof the fundamental inverse round-trip time of the cavity.Generation of harmonics of the repetition rate can be achievedin actively mode-locked lasers by suitable choice of therepetition frequency of the driving signal [2], [3]. In passivemode-locked lasers, several harmonics have been observed in amultistable behavior [16], [17], where the operating hatmonicis dependent on the gain section current [10], [14]–[17].

    In this paper, we present the progress on generation ofshort pulses at high-repetition rates by multiple colliding pulsemode-locked (MCPM) quantum-well lasers. These devices aremonolithic multi-sectioned passive mode-locked semiconduc-tor lasers that can generate short pulses at harmonics of thecavity round trip frequency, depending on the electrical biasapplied to each of their sections. Fig. 1(a) shows the top

    1077-260K/95$04.00 0 1995 IEEE

  • 540 IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JUNE. 1995

    metallic contact (NiCrlAu)

    Si02 injectionbl~cking layer U:pperc’ad%]r

    ,oJer:,ad&ng,ayel,

    r Iactive region (4 QW)metallic contact (Au/Ge/Au/Ni/Au)

    Fig. 2. Transversal cross section of the laser, showing waveguide andmaterial structure.

    840 860 880 900 9

    (a)

    view diagram of the MCPM laser and Fig. 1(b) shows itslongitudinal cross section with the electrical connections forforward and reverse biasing. The laser has a contiguouslyelectrically connected gain section and 3 separated sectionsplaced at every quarter of the cavity length. Each of the three

    sections (labeled a, b, and c on the diagram) is separatelyelectrically addressable and when reverse biased it behaves

    as a saturable absorber and when forward biased as a gain

    section. Therefore, by selectively biasing, one can choosethe number and position of saturable absorbers in the lasercavity, which causes the laser to have 1, 2, 3, or 4 pulsescirculating in the cavity, giving first to fourth harmonic of therepetition rate, respectively. In contrast to the lasers reportedin [10], [14]–[ 17] the multiple pulse operation (or harmonicsgeneration) here does not depend on the current applied to thegain section. To date our highest repetition has been achievedwith a 400-~m long MCPM laser, where we obtained l-pspulses at 375 GHz [18].

    Section II of this paper describes the fabrication of theMCPM lasers. Details of the quantum-well material and wave-guide structure are discussed. Special attention is given to thedesign and mechanisms of operation of the monolithicallyintegrated saturable absorber sections. Section III presentsthe experimental results on the different modes of operationof the MCPM laser, whereas Section IV is concerned withtheoretical models and results. Finally, in Section V, we give

    the conclusion of the paper.

    II. DEVICE FABRICATION

    The MCPM laser is fabricated on a GaA–AIGaAs4 quantum-well material grown by atmospheric pressuremetal organic vapour phase epitaxy (APMOVPE). Thesemiconductor material structure consists of 0.2 ~m heavilyp-doped (2x 1019 cm–3) GaAs cap layer followed by 1 ~m

    P-tYPe cmbon doped (2.2x1017 cm–3) AIO.qsGaO.sTAs uppercladding layer. The quantum-well structure consists of four 10nm GaAs wells spaced by 10 nm ~10,ZOGa0,80As barriers andthey are surrounded by two 0.1 flm Alo,20Gao,80As layers ina separate confinement structure. The lower cladding layer is

    formed by AIO,qsGaO.sTAs silicon n-doped (1.4x 1017 cm-3)layer 1.7 Urn thick.

    The laser waveguide structure used is a 3-~m wide, 0.6-~m high stripe loaded waveguide formed by SiCIA reactiveion etching and it is defined by photolithography and NiCrmasking prior to etching. A 200-nm thick Si02 layer is

    ?0

    840 860 880 900 920Wavelength (rim)

    (b)

    Fig. 3. Transmission of TE (a) and TM (b) polarized light through semicond-uctor waveguide as a function of wavelength for several different reversebias values (O, 1, 2, 3, and 4 V).

    deposited on the material to serve as a current injectionblocking layer and a contact window is open on the waveguide

    by HF chemical etching. Fig. 2 shows the transversal crosssection of the laser waveguide, as well as the layers of thematerial structure. Gain and absorber sections are definedby photolithography, top metallization (NiCr–Au) and lift-off,leaving 10-~m gaps between sections (see Fig. 1). Substratethinning, metallic contact deposition (Au–Ge–Au–Ni–Au) andlaser cleaving complete the fabrication process. The lasersare mounted and wire bonded for CW operation. No contact

    annealing is used since it deteriorates the adhesion of thebonding pads to the Si02 layer underneath it, making bondingvery difficult. The fabrication technique described above issimpler and of lower cost than the buried heterostmcture usedin previous publications [3], [10], [14] since it does not involveany regrowth process.

    In our devices, saturable absorption is obtained by applyinga negative bias between the absorber sections a, b, and c inFig. 1 and the ground contact. This, reverse biasing techniquehas been successfully employed by a number of authors[2], [3], [9]. An electric field is applied transversally to thequantum wells, which induces a shift of the semiconductorband edge, known as quantum confined Stark effect [19], [20].It is shown in Fig. 3 where we obtain the spectra of light

    transmission through the laser waveguide for different reversebias. To obtain those we coupled the output of a tuneableTi: sapphire laser into a quantum-well laser waveguide, whichwas fully reverse biased for better signal contrast. The outputintensity was measured using a photodiode and lock-in ampli-fier. Spectrum for TE and TM polarization of the Ti: sapphire

  • MARTINS-F3LH0etal,:MONOLITHICMULTIPLECOLLIDINGPULSEMODE-LOCKEDQUANTUM-WELLLASERS

    laser were obtained. Fig. 3 shows that one can introduce a

    controlled amount of absorption in the semiconductor laser

    cavity using the reverse bias technique. The optical intensity ofthe mode-lockedl pulses inside the laser cavity can be estimatedto be of the order of 1.6 MW/cm2. In this estimation weassume a laser emitting 1.2-ps pulses at 240-GHz repetitionrate, with 8-mW average power. We also assume an effective

    waveguide cros:s-sectional area of 3 x 1 ~m or 3.0 x 10–8 cm2and a facet reflectivity of 0.3. This intensity is high enoughto saturate the absorption of the absorber section by mostlyband filling effect [19], [20]. The applied reverse bias actsonce again, now sweeping out the generated carries from theabsorber sections, helping the recovery to the unsaturated state[2], [3], [9]. The saturation and recovery processes describedabove may not be the only ones present in ultrafast mode-locked lasers. Fi~ster nonlinear effects, necessary for achievinghigh-repetitions rates and short pulses, will be discussed in

    the subsequent sections.

    The electrical. isolation between gain and absorber sections

    is an important issue on the design and fabrication of mode-Iocked lasers. A poor isolation allows current leak from thegain to the absorber section, decreasing the efficiency of thereverse bias on the absorber. It also drains current from the

    gain section in the vicinity of the absorber section, making thelatter effectively wider. A short and efficient absorber sectionis important for its saturation and recovery characteristics. Weimprove the electrical isolation by removing the highly dopedGRAS cap layer from the gap regions between sections usinga selective dry etching technique [21], [22] that stops on the

    AlGaAs layer. By measuring the resistance between gain andabsorber sections when no bias is applied we obtain a dc elec-

    trical isolation clf 1.5 k Q. We observe that this technique givesabout 5070 improvement on the original isolation (withoutetching). Better isolation can be achieved by deeper etchinginto the upper cladding layer or by using wider gaps betweensections. The isolation also depends on the doping level andthickness of the cap and upper cladding layers and the figurespresented here are for our particular material structure.

    III. EXPERIMENTALRESULTS

    The characterization of the MCPM lasers is performed bymeasuring the time averaged optical spectra and the linearcross-correlation trace. The linear cross-correlation method fortime-domain measurement uses a Michelson interferometer toscan a pulse through itself and its neighbors in a train ofpulses, obtaining pulse width, repetition rate and coherencelength of the laser [23]. This technique detects the mixing

    signal between light from each arm of the interferometer ata low speed photodetector and it does not employ second

    harmonic generation. The mixing technique employing a lock-in amplifier and two choppers (one in each arm of theinterferometer) removes the dc level generated by the directdetection of light from each individual arm of the interfer-ometer. Therefore, only the interference signal is detected[23]. Although this technique has some limitations concerningpulse width measurement [11 ], [23], it is attractive for char-acterization of mode-locked semiconductor lasers since these

    (a)

    (c)

    (e)

    ($3)

    (i)

    (k)

    (m)

    (o)

    Correlation Spectramm-0.3 -0.15 0 0.15 0.3 850 870 890

    MI--L-I-40 -20 0 866 868 870 872

    LAJLIL?J!-& .20 0 867 869 8;1 8+3

    -40 -20 0 867 869 871 873

    M l-il.-l-40 -20 0 869 871 873 875

    -40 -20 0 871 8;3 8;5 8;7~~

    WI---4-J-40 -20 0 870 872 874 876

    ldA@uM

    541

    (b)

    (d)

    (f)

    (h)

    (i)

    (1)

    (n)

    (P)

    -15 .10 -5 0 872 874 876 878

    Delay (ps) Wavelength (am)

    Fig. 4. Linear correlation traces and optical spectraof a 600-~miong MCPMIa{er for different modes of operation: spontaneous emission (a) ‘and (b);single longitudinal mode operation (c) and (d); multimode (e) and (f); 1 pulsemode-locking (g) and (h); 2 pulse CPM operation (i) and (j); 3 pulse MCPM(k) and (1); 4 pulge MCPM (m) and (n); and 4 pulse MCPM operation of a400-pm long laser (o) and (p). Verticat axes represent inten8ity in arbitraryunits and they all stat from zero intensity level in linear scale.

    devices generally generate low optical powers, which makessecond harmonic generation (SHG) more difficult in practice.

    The limitation of the technique consist of its insensitivity tothe effect of frequency chirp on pulses [11], [23]. Therefore

    measurements of time-bandwidth product could be misleading.

    However, it is reasonable for these lasers because there hasbeen no evidence of significant chirping from CPM lasers

    and measurements have generally indicated transform limited

    pulses [3], [8]. A detailed study of pulse structure is out of

    the scope of this paper since it involves more sophisticatedmeasurement schemes than correlation methods. Nevertheless

    we are implementing the SHG autocorrelation technique in thenear future as an attempt to have more information about chirpin pulses. Fig. 4 shows the correlation and optical spectra ofa MCPM laser for its different modes of operation, includingsingle mode, multimode, 1, 2, 3, and 4 pulse mode-locking,

  • 542 lEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JOiW 1995

    and to be complete we also show the spontaneous emission of

    the laser. The total cavity length of the laser is 600 ~m andeach one of its 3 independent sections a, b, and c in Fig. 1is 30-~m long. The laser operates on CW regime and when

    every section is forward biased the threshold current is 30 mA.Fig. l(b) shows the electrical connections to bias the laser in

    the case of 4 pulse mode-locking. A current source is usedto bias the gain sections, whereas a voltage source appliesthe reverse bias to the absorber sections. A 50 !2 resistor isused to limit the current flowing from the absorber sectionspreventing damage.

    Fig. 4(a) and (b) show the cross-comelation and optical

    spectrum of the spontaneous emission of the laser when it

    is operating below threshold, at 25 mA. The laser emits in

    a very broad spectral range, with no observable longitudinalmodes. The only feature observed in the correlation traceis a short double-sided exponential peak at zero delay. Thefast exponential decay with delay from the zero point of theinterferometer indicates that the emission is highly incoherent,as expected from spontaneous emission. The typical fringesproduced in interferograms are not resolved here.

    When every section of the laser is forward biased and it

    operates at currents not far beyond threshold the laser emits in

    a single longitudinal mode. It is shown in Fig. 4(c) and (d) for

    60 mA pumping current. The side mode suppression is of about25 dB (not measurable from the Fig. 4(d)).. The correlationtrace is flat in the observed range of 45 ps. No decay can benoticed, indicating the laser has a long coherence length [24].

    The laser can also emit several longitudinal modes. Multi-mode (free-running, nonlocked) operation occurs for currentsvery close to threshold and also for high currents, abovethe single-mode operation region. Fig. 4(e) and (f) show thecorrelation and optical spectrum for multimode operation when

    35 mA is applied to the laser. Fig. 4(e) shows peaks at the

    fundamental repetition rate of the cavity (60 GHz), which

    correspond to 0.15 nm spacing between modes in Fig. 4(f).These peaks arise from beating of the several longitudinalmodes observed in the spectra. This mode beating effect meansthat, in time domain, the laser produces a sequence of spikesin the form of a pulse train [24], [25]. Therefore, there ishere an apparent ambiguity between multimode and mode-locked operation. The ambiguity is removed by analyzingthe coherence properties of the laser. The difference between

    mode-locking and multimode behavior is that with a mode-locked laser the modes add together coherently and that there isa strong phase relationship between pulses in the pulse stream[24]. In an ideal mode-locked case, where the phase of themodes are exactly the same, the coherence length of the laserwould be infinite. A laser is considered to be mode-locked ifits coherence time is much longer than the round-trip-time ofthe cavity, or photon lifetime—for the strucures studied thosetwo times are of the same order of magnitude. One can observein Fig. 4(e) a pronounced exponential decay on the amplitudeof the peaks, indicating that the laser has a short coherencelength, of about 20 ps (6 mm), which is very close to theround trip time (16.4 ps). This means that there is no constantphase relationship between modes and the sequence of spikesproduced by them is formed and shaped in a rather chaotic

    and noisy fashion, not having the high regularity in shape

    and amplitude typical of mode-locked pulses. This kind ofambiguity also exists in the nonlinear correlation methods [24],[26]. In the autocomelation by second harmonic generationtechnique peaks also appear for multimode operation ~d the

    ambiguity is solved by observing the contrast ratio (peak tobackground), which is 3:1 for ideal mode-locking and 3:2for multimode operation [24], [26].

    Mode-locking can be achieved by reverse biasing one ofthe three sections a, b, or c in Fig. 1. If section a is reversebiased, providing saturable absorption, while sections b and c

    are forward biased, providing gain, the MCPM laser has one

    saturable absorber in the cavity and in this case it mode-locks

    at the repetition rate corresponding to the cavity round triptime. For the 600 pm long laser it is 60 GHz, which is the

    first harmonic of the repetition rate. Since only one pulse ispresent in the cavity at a time we call this mode of operation1 pulse mode-locking. Fig. 4(g) and (h) show this type ofoperation when we apply –0.95 V to section a and 60 mA tothe rest of the laser. The average width of the correlation tracepulses is 3.2 ps, obtained by measuring the width of eachpulse shown in Fig. 4(g), apart from the one at zero delay,

    which is the auto-correlated pulse and contains less reliableinformation about pulse width [23]. Assuming in this case

    a hyperbolic secant pulse shape the deconvolution factor of1.56 is used to obtain the actual pulse width [26], which is2.1 ps FWHM. The same procedure will be applied to pulsewidth measurements thereafter. The longitudinal mode spacemeasured in Fig. 4(h) is 0.15 nm, which correspond to the 60GHz repetition rate obtained from Fig. 4(g). In contrast to thecase of multimode operation discussed before, the coherencetime of the laser observed in Fig. 4(g) is much longer thanin Fig. 4(e). The measurement of the coherence length is

    limited by the continuous scanning range of the interferometer,

    which is 15 mm (50 ps) in our setup. But we have made anoncontinuous scan measurement, up to pulses 10 round-tripsapart (150 ps), which showed no noticeable change in pattern.This long coherence time compared to the round-trip time(16.4 ps) and the photon lifetime (about 5 ps) is an indicationof mode-locking operation. Due to symmetry similar resultsare obtained by reverse biasing section c and forward biasingsections a and b.

    Two pulse CPM operation is obtained when the centralsection of the laser (section b in Fig. 1) is reverse biased

    whereas the others (sections a and c) are forward biasedby connecting them to the gain section. This configurationcorresponds to standard CPM operation of lasers, which hasone saturable absorber in the middle of the cavity [3], [8],[271. Fig. 4(i) and (j) show the cross-comelation and opticalspectra for 2 pulse CPM operation when 0.37 V reverse biasis applied to section b and 54 mA is applied to the rest of thelaser. It can be seen in Fig. 4(j) that three longitudinal modesare apparent and the mode spacing is 0.3 nm which is twicethe original cavity mode space (O.15 nm) and corresponds to apulse repetition rate of 120 GHz. From previous work [3], [27]it is clear that this is the standard behavior of a semiconductorCPM laser and it indicates that two pulses are circulating in thecavity and colliding in the saturable absorber. With only three

  • MARTINS-FILHO et al.: MONOLITHIC MULTIPLE COLLIDING PULSE MODE-LOCRED QUANTUM-WELL LASERS 543

    modes locked it is difficult to fit a typical envelope shape to the

    optical spectra and the pulse shape can be close to a quasi-

    sinusoidal shape. But for the sake of simplicity, we assumehere and thereafter a hyperbolic secant pulse shape as well,

    which is the most commonly found in the literature for this

    type of device [2], [3]. From Fig. 4(i) we obtain a deconvolved

    pulse width of 3 ps, at 120 GHz repetition rate.The Fig. 4(k:) and (1) are obtained when the sections a

    and c are reverse biased with 0.74 V. The section b andthe gain section are forward biased with 54 mA. In thisconfiguration the laser has two saturable absorbers in thecavity. It can be seen in Fig. 4(1) that in this case the separation

    of the longitudinal modes is 0.45 nm, which is three timesthe original cavity mode space, corresponding to 180 GHz.

    Fig. 4(k) gives 2 ps pulse width and 180 GHz, which is the

    third harmonic of the repetition rate. As an extension of thetwo-pulse CPM operation, this is explained by assuming thatthe laser is operating in a three-pulse regime, where threepulses are present in the cavity. lko pulses collide at every1/3 of the cavity length, while the other is 2/3 of the cavitylength distant from them, that is at the facet. Although thecollision points do not correspond to the exact position ofthe saturable absorbers, the pulses are wide enough (2 ps

    pulsewidth is 150 pm long inside the laser) to overlap in thesaturable absorber section. Therefore, the pulses still collide

    in the absorber sections.Four pulse MCPM operation is achieved when the three

    sections (a, b, and c) are reverse biased. As a result thelaser has three saturable absorbers in the cavity. Fig. 4(m)and (n) show the cross-correlation and optical spectrum for0.33 V reverse bias applied to the three sections, whereas thegain section is forward biased with 65 mA. The longitudinalmode separation is 0.6 nm which corresponds to a pulse

    repetition rate of 240 GHz, which is the fourth harmonic. The

    pulse width measured is 1.6 ps. This configuration has fourpulses circulating in the cavity and they collide exactly in thesaturable absorber sections. Two of them collide with othertwo pulses in sections a and c, and after moving a quarter ofthe cavity length two pulses collide in the section b, whilethe other two pulses are at each facet of the laser [11]. Froma shorter laser, 400-pm long with 15-~m saturable absorbersections, operating in four-pulse mode we obtained 1-ps pulsewidth at 375 CrHz repetition rate, as it is shown in Fig. 4(o)

    and (p).For the deviees studied here, we could not find any change

    of harmonics (multistability) when the current is varied (upto 90 mA) for each laser configuration. It indicates that,in contrast to }previous work [10], [14]–[17], the multipulseoperation discussed here is due to the number and position ofthe saturable absorbers in the cavity and not the current level.It will be further discussed in Section IV.

    We also obtained ranges of current and absorber bias inwhich the laser operates in four-pulse MCPM mode. It isshown in the light versus current curve of Fig. 5. The outputoptical power is measured as a function of the gain sectioncurrent for different absorber biasing conditions. One canclearly see the increase of the threshold current of the laseras the absorber bias is decreased from M V. It is due to

    the insertion of loss in the cavity, which comes from theincreasing absorption in the absorber sections as a function

    of the applied reverse bias (see Fig. 3). The dark lines on theL x I curves show where stable 4 pulse mode-locking (at 240GHz) is found. Up to 7 mW average power, corresponding to

    25-mW peak power can be achieved. The pulse energy is 0.03

    pJ. These values are very similar to the ones reported in theliterature for this type of device [2], [3]. We also observed therange of mode-locking in a gain current versus absorber biasgraph and it is shown in Fig. 6. In this graph, the absorberbias is set at zero gain section current and we measure thechange of the bias as the gain current is increased, which gives

    the dashed lines in Fig. 6. The Iasing threshold and the areasof CW, mode-locking or self-pulsation operation are shown.Again the dark lines on the curves indicate where stable four-

    pulse MCPM is found. We can notice two main features thatdiffer this range of mode-locking from the ones found in theliterature [3]. This range is rather small in current and reversebias, and it shows two distinct areas where four-pulse MCPMis observed. From Fig. 6 it is clear that there are two pointswhere mode-locking is found for each absorber bias curve withinitial values between –2.8 and –3.3 V. We believe that theexplanation for these features lies on the need of very fastabsorption and gain recovery in order to sustain mode-locking

    at 240 GHz (4.1 ps duty cycle). This fast dynamics would beachieved with the help of the light and heavy hole excitonicnon-linearities, which would give rise to the two distinctregions of mode-locking. The previously reported ranges ofmode-locking are for longer lasers, generating lower repetitionrates, at about 80 GHz [3]. They naturally have more relaxedrequirements on fast dynamics of gain and absorption, whichprovokes the widening and merging of the two regions into acontinuous one.

    We have obtained strong indications that the same laser

    device can also operate Q-switched. Using a fast photodetectorand a RF spectrum analyser we observed that the laser canself-pulsate at about a few gigahertz repetitions rate range,depending on the forward current applied to the gain sectionand the reverse bias applied to the absorber sections. The laseremits a broadened optical spectrum, typical of Q-switching [1].In the L x I curves shown in Fig. 5, Q-switching occurs atlower currents than mode-locking, for a given reverse bias.Fig. 6 shows the area where Q-switching (self-pulsation) isfound. A comprehensive study and characterization of the Q-

    switching operation of these devices is out of the scope of thispaper and it will be subject of future work.

    IV. THEORY

    The aim of this section is to study the origin of multiple-colliding-pulse mode locking and to assess the roles playedby the physics of gain and saturable absorber (SA) media andthe geometry of the laser in establishing this regime. First, weshall concentrate on determining conditions for the regime totake place. The usual way of doing this is to describe the lasingregime in terms of mode amplitudes and phases, that is, to usea frequency-domain approach [5], [28]–[30]. Here, we shallextend it to colliding-pulse configurations, including MCPM.

  • 544 IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO, 2, JUNE 1995

    Current (mA)

    Fig. 5. Laser output power versus gaiu section current (L x 1 curve) forthe MCPM laser operating in four-pulse mode for several absorber biasingconditions: all sections forward biased, O, –2,8, –3, –3.3, –3.5, and –4 V.The bias is set for zero current applied to the gain section of the laser. Therange of mode-locking at 240 GHz is shown in dark lines.

    /’k,,t~,.,,“\

    ?.g

    80 ~ ~,, \\*\\y i, \ ~~ “,,

    \

    ;, ‘!, \$ ‘.. $. .

    ~ 60 “i, “’”’.. “’..,. “$:.,,,.. “,$.%. .4

    “8o 40

    ‘... ‘.., ‘\ “: :;, ‘. ‘;..... .. !,, {,,, .,,‘,,

    $.> \, ‘, ‘1,‘,. %‘!, ,I /-iv.2v -4V I

    Lasing thresholdo 1 1 I i 1 1 4

    210 -1-2-3-4

    Absorber bias (V)

    Fig. 6. Variation of the absorber section bias with the gain section currentfor several initial values of the bias (–1, –2, –2.8, –3, –3.2, –3.3, –3.5and —4 V), which are set at zero current (shown with dashed lines). Thefirst kirrk in the curves indicates the lasing threshold. The second kink marksthe transition from self-pulsation to either CW or mode-locking operation.Mode-locking is indicated with dark lines.

    A. The Frequency-Domain Model

    We start with a system of coupled-mode equations forcomplex mode amplitudes. Systems of that kind were appliedto semiconductor lasers by Lau [5], [28]–[30] for the caseof standard AM mode locking and also by Shore and Yee[31] for the case of the so-called frequency-modulation modelocking, caused by gain nonlinearities in a single-section laser.Here, we use a system [32] which is an extension of boththese models. The derivation of the model will be publishedelsewhere [33] and is skipped here since the structure of theresulting equations is close to those presented in [5], [28]–[30]and fairly physically transparent

    (1)m

    Here, Ek = Eb(t) exp (zp~(t)) istude of the kth mode, E~ and ~k

    A

    the complex mode ampli-being the mode amplitude

    and phase, 17 is the confinement factor, Vg = Clqg thegroup velocity of light (q and rlg being the phase and groupTefTaCtiVeindiCeS, respectively). gk and ak stand fOr gain inthe gain section of the laser and the absorption coefficient inthe saturable absorber (5A) section at the spectral positionof the kth mode. They should be understood as the “slow”

    components of corresponding quantities which vary in time

    only on non-ultrafast timescale, i.e., slower than the round-triptime of the cavity, for instance due to relaxation oscillations or

    self-pulsing, but not to mode locking. fg and f~ are fractionsof the cavity length occupied by gain and 5A sections, aCis the cavity loss, Auk is the frequency detuning of themode from its spectral position in the passive cavity. The lastterm in (1) takes into account the interaction between modesseparated in frequency by m fundamental interrnodal intervalsAf2 = rv~/L. The strength of the interaction G is given bythe following expression

    ‘m=(7EkE’+m)

    In (2), the first factor is the component of the light intensity

    oscillating at the frequency mAfl due to beating between

    modes; the second factor is the response of the active mediumof the 5A section (the first term in the figure brackets) andof the gain section (the second term) to these light intensityoscillations. Ag = 8g/8N and A. = –aa/aN are gainand 5A cross sections (carrier density derivatives), ag and

    a. are the linewidth enhancement factors in correspondingsections. The necessary assumption in (2) is that, althoughmode number (i.e., frequency) dependence of the net mode

    gain fggk – faak – a= is important for mode competition andtherefore retained in (l), the values g and a separately may beconsidered weakly dependent on mode number (frequency).

    Similarly, the dispersion of ag and a. is neglected, hence nomode subscript is assigned in (2) to g, a, Ag, A., ag, and a..

    ‘Ea,g = (l/Ta,g + vgAa,g )~IE;I ‘1mstand for the effective recombination times in 5A and gainsections, including both spontaneouslnonradiative and stimu-lated recombination. The first term in each square bracketsof (2) is then the “slow” term describing the light-inducedoscillations of saturable absorption and gain due to oscillationsof the total camier density in the corresponding section.

    ‘g’a), is introduced to take intoThe second, “fast,” term s~account pulsations of saturable absorption and gain due topulsations of the deviation of the carrier energy distributionfrom quasiequilibrium [34], of the carrier temperature [35],[36] and, specifically for QW absorbers, of the degree ofexciton ionization [37]. All these mechanisms (nonlinearities)

    are essentially fast, with characteristic relaxation times onsubpicosecond scale, hence the expression “fast term.” We

  • MARTINS-FILHOa al.: MONOLITHIC M1.JUTIPLECOLLIDING PULSE MODE-LOCKED QUANTUM-WELL LASERS 545

    assume for simplicity that in both gain and SA sections oneof these nonlinearities dominates over the others; otherwiseone should sum over all mechanisms involved. Similarly tothe slow term, the fast term may then be written as

    ~(a,g) =~(a,g)

    1 – imAfh-~’g)

    where c(”’9) are the phenomenological absorption/gain sup-

    pression coefficients and ~~’g) are the nonlinearity relaxationtimes.

    All the values discussed so far are independent on thegeometry of the laser cavity. The onl way this geometry

    r“a) These quantitiesenters the model is via the quantities ~~ .are overlap factors characterizing the spatial overlap betweenthe two interacting modes and the net gain (gain and sat-urable absorption) pulsations that lead to this interaction. The

    expression for these factors is [32]

    $g)a) = ! d.z , (U~U;+m) COSg,a (?(2+0 ‘3)In (3), the integration is over the fraction of the laser lengthoccupied by the corresponding section, the zero of z isassumed in the center of the cavity, ‘Uk are the longitudinalmode profiles (wave functions) of the cavity. The cosinefactor in (3) may be understood as the spatial profile of thenet gain pulsations. This factor is the important difference

    between the expressions (3), derived from the first principles,

    and the less accurate expressions empirically introduced by

    previous authors [30]—not all the features discussed below

    are predicted by that earlier model. For more details on modeprofiles and overlap factors, see Appendix.

    B. Mode-Locking Condition

    The usual way of defining the condition for mode lockinganalytically is to consider a single-mode solution of (1) andstudy the stability of this solution with respect to the excitationof weak side modes. If the single-mode solution is unstablethen the mode locking is expected to occur. A formallydifferent, but equivalent procedure was also performed byHaus and Silberberg [37]. In [5] and [28]–[30], the side modesare taken as the modes nearest to the initially existing mainmode, i.e., one interval Afl apart from it. For our purposes,we must allow the side modes to be separated from the mainmode bym=l,2,3,4 . . . intervals Af2, and shall then checkthe mode locking condition for various m. If for some rangeof parameters this condition is satisfied for a certain m >1

    but not satisfied for m = 1, this will mean that the MCPMregime (presumably with m pulses coexisting in the cavity)is indeed realized within this parameter range. Following theusual procedure of the (instability analysis, we consider thesystem (1) with only three modes, that is, the main mode (k =O) and the side modes (k = +rn), taken into account. Thesingle-mode solution E. >0, E~m = Ois the trivial solution ofthe system. The range of parameters within which this solutionis unstable should be derived from an obvious condition

    (dln E~ dln E.~max — dt ‘ dt ) >0. (4)E+m=o

    A straightforward application of the condition (4) to the systemof coupled-mode equations in the general form of (1) leadsto an apparently unexpected conclusion that the condition(4) may be satisfied without a saturable absorber. Indeed, itis known (see e.g., [31], [34], [36]) that even without the

    SA, gain nonlinearities can still ensure multimode lasing. Butmultimode emission, generally speaking, is not the same as

    mode locking, at least as amplitude-modulation mode locking,

    i.e. generation of short pulses, as discussed in Section III.

    This presents a problem for the interpretation of (4) which,however, is clearly not specific to MCPM (the same problemobviously arises when trying to accurately define conditionsfor ordinary mode locking in monolithic-cavity laser diodes)and will therefore be addressed elsewhere [33]. Here, we shallrestrict ourselves to a simplified approach [28]–[30], ignoringthe contribution of the refractive index related terms in (2),i.e. setting Qg = a. = O;Im (E(a’g) ) = O, and also ignoring

    gairdabsorber nonlinearities hidden in g and a (which may

    lead to multimode emission due to spectral hole burning).Then, indeed, multimode emission is synonymous with modelocking and, after some trivial calculations, (1) and (4) yieldan approximate condition for this regime in the form

    ,ff)a

    [

    vgAarz ~ ~(a)

    1 + (mAW-x.)2+

    1 + (mAW-~))2 1[

    _ &(#)g “9A9 “ 7X9 +C(9)

    1 + (mAW-zg)2 1 + (mAfh-~))2 1(5a)

    where the coefficients have been assumed real (as is usuallythe case); and Am = ~g(go – g~) – j~(ao – am).

    For monolithic-cavity lasers with the cavity lengths of theorder of hundreds of micrometers and realistic stimulated life-times, one may usually assume mAf%-x 9,.>> 1. Also, given

    (9)Q) < ~.subpicosecond nonlinearity relaxation times, mAflr.lSo (5a) is simplified to

    ,ff)a[

    vgAa 1[ vgA~(mAti)2’rxa + ~(”) – ‘&)g (mA~)~T=g + ‘(g)1(5b)

    Relating the expressions (5) directly to experimentally ob-served current and voltage ranges for mode locking wouldrequire more microscopic studies into the physics of the activemedia, most importantly of the SA. For instance, as waspointed in Section III, the two separate sub-regions of modelocking in the experimental diagrams (Fig. 6) strongly suggest

    that two exciton peaks may be involved in the mode locking,which in terms of this model would mean strong changes inboth A. and e(”) with pumping conditions). Presently, thevalue e(a) is the least well-known parameter in the modeland may be used as a fitting parameter. For instance, let usconsider the two absorber-related terms in the first squarebrackets of (5b) (the terms responsible for more locking) andestimate which of them is likely to be the most important. WithA. = 10-15 cm2 (a usual value in the literature), 7Xa = 20

  • 546 IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JUNE 1995

    ps (of the order of the round-trip time), Af2 = 27r* 60 GHz

    (corresponding to the cavity length of the laser studied), andm = 1 the value of the absorption suppression coefficientrequired for the fast term to dominate over the slow termis estimated as Et”) = 10–17 cm3. This is a reasonablymodest value, often quoted for gain nonlinearity coefficients,and absorber nonlinearities are likely to be stronger [38].For more pronounced MCPM (m> 1) the requirement forc(a) to dominate becomes increasingly more liberal. One may

    therefore suggest that for mode locking of laser diodes withshort monolithic cavities, and particularly for MCPM, fast

    nonlinearities may be the dominating contribution in estab-

    lishing the condition for mode locking regime. This somewhatcontradicts the conclusion made in [37] that, although thefast component of the saturable absorption largely definesthe parameters of the mode locking pulses, the conditionfor the regime to take place is likely to be defined by theslow SA. However, one notices that a) the authors of [37]distinctly kept in mind lasers with extended cavities, withvalues of Afl 1–2 orders of magnitude smaller, which makes

    the conclusion of [37] much more likely to hold, and b) in

    [37], only one specific absorber nonlinearity was considered,

    namely excitonic ionization, for which the value c(a) is not a

    free parameter, but is known to be small. An estimate similarto that made above suggests that the gain term in (5b) may alsobe dominated by gain nonlinearities, rather then pulsations oftotal density. Then the most important m-dependent variablesin (5b), determining whether mode locking will be normal or

    (g,”) (the(multiple) colliding pulse, are the overlap factors (mmargin Agm of the net gain is approximately proportional tom2, but is likely to be not very significant for well-developed

    lasing). Since the factors ~g’”) scale the strength of interactionbetween modes, they should affect not only the limits ofthe regime but also the characteristics of the well-developedMCPM. Therefore, we find it instructive to study the overlapfactors in some detail.

    C. Overlap Factors: The Effect of Laser Geometry

    (9c)ca1culated for dif-Fig. 7 shows the overlap factors

  • MARTINS-FILHOetal.:Monolithic MULTIPLECOLLIDINGPULSEMODE-LOCKEDQUANTUM-WELLLASERS 547

    indeed, be the four-pulse configuration, which is observed

    experimentally. However, since ~g) at m = 1, 2, 3 are

    nonzero, some modes with smaller amplitudes may be excitedin between the main modes, therefore the four pulses within

    one period may be expected to have different amplitudes.This is also corroborated by experimental evidence (note an

    envelope modulation in the correlation function) and will be

    confirmed hereafter by time-domain calculations.For the case where we experimentally observed “normal”

    mode locking with one side absorber a quarter of the cavity

    length apart from the facet (Fig. 7(c)), the picture is quali-tatively the same as in Fi . 7(b), but the difference between

    f(’P) and other values of f;) is much smaller. What one mayexpect in this case is therefore a series of modes separated bythe fundamentid interval Afl, but with each fourth mode beingsomewhat larger in amplitude. In time domain, this means onestrong pulse per repetition period with small leading and/or

    trailing pulses a quarter of the round-trip period apart from the(g,a)

    main one. Note that the values of f~ in this case, which,

    unlike all other cases studied, is strongly asymmetric, should

    be treated as absolute values. The actual values for m = 1,

    3 are complex..

    Finally, the most difficult to explain is the case when twoside absorbers are biased (Fig. 7(d)). Experimentally, this isthe three-pulse case, which means that the largest overlap

    ‘G) However, if one assumes that thecoefficient should be (3 .SA is exactly confined to the area beneath the corresponding

    contact or even the area including the separating grooves, then

    the dominating value is still f$). To make the coefficient

    &f) the largest, one has to assume that the absorbers actually

    stretch strongly beyond the contacts, approaching the pointsIzl = L/6 (i.e., one third of the cavity length apart fromthe facets). This is corroborated by time-domain simulations;furthermore, one notices that in the experiments, this is thecase when the MCPM is least clearly rendered.

    The main advantage of describing MCPM with the use of

    ‘g’”) (3) is that these factors are definedthe overlap factors ~~

    almost entireZy by the geometrical positions and lengths of

    the gain and SA sections and are virtually independent of the

    parameters of the active medium such as Ag, A., E(g),E(a),which are often not very well known. We believe this makesthe predictions ,made in this section general and reliable.However, the results obtained so far may indirectly proveonly the fact that MCPM should indeed take place, but cannotpredict the parameters of the well-developed regime. So weproceed with some numerical simulations of the mode lockingdynamics. The easiest way to perform such simulations wouldbe to fully numerically solve the multimode system ( 1), which

    for this purpose should be completed with usual rate equations

    for the (“slow”) carrier densities in gain and SA sections. Onenotes, however, that the model ( l)–(3) is essentially a small-signal model and its applicability, at least for high intensities,needs further investigation. Also, in its present form the modeldoes not take into account the colliding pulse effect (interactionof counterpropagating pulses via self-induced gratings in theSA [3]), which maybe expected to be of some significance fora regime such as MCPM, where the pulses are indeed colliding

    in the SA. Therefore, in order to avoid these limitations and to

    double check the results obtained from the frequency-domainmodel, we use a distributed time-domain model for full-scalenumerical calculations.

    D. The Time-Domain Model

    The model we use is a variation of the model used in [13]

    and is similar in its main features to those of [39] and [40]. Thelight propagation in the cavity is described by a propagation

    equation of the form

    where ER,L are complex amplitudes of the field of the lightwave propagating to the right and to the left respectively. Theoperator O includes a digital filter simulating gain dispersion

    [39]

    /

    co

    ijE=g. AOg. E(t – r) exp (–Af2g . T) d~o

    where Aflg is the gain linewidth and g is the USUd gain

    value used in the previous subsection (for the values of .zcorresponding to the SA subsections, g is obviously chimgedto a). The list of parameters, together with the values used,

    is given in the Table I. The last term in (6) representsthe random noise source [39] and is essential for runningthe model. A self-induced grating (colliding-pulse effect) isincluded by the distributed reflection terms KE, which aretaken into account only in SA sections. The dynamic couplingcoefficients KLR, R~ are calculated from the equations

    . ~~~(,z) – ivgAaa(EfiE~) (7a)

    KRL = –K~R (7b)

    where D is the ambipolar diffusion coefficient, and J the lasingwavelength (in vacuum); the term proportional to D takes intoaccount smoothing out of the grating by carrier diffusion. Thelinewidth enhancement factor for the SA region has been takenas zero.

    At the facets, the usual reflection boundary conditions areimposed. The dynamics of the carrier density is described bylocal rate equations with photon density defined as the squaredabsolute value of the local field

    S =IER12 + IEL12:aN(z, t) _ J(z, t) N

    & – ed – w(z)– vg9(lER(~, t)[2

    + lEL(~,t)12) (8)

    where the recombination time TN(z) is defined differently forgain and SA sections.

  • 548 ISEEJOURNALOFSELECTEDTOPICSIN QUANTUMELECTRONICS,VOL.1,NO,2, JUNE1995

    TABLE ILASER DIODE PAMMETERSUSED IN COMPUTATIONS

    Parameter I Sllnbol I Value I unit

    electron lifetime (in Eain section) ITN[ 11BN Is

    cavity losses % I/zin(l/R) I/cm

    pumpingcurrentin gainsection Jtpumpmg current ,n saturable absorber (SA) section Ja o

    active layer dickn.ess d

    bimolccut~ recombination coefficient B 1.5.10’0 cm ‘Is

    spontaneous emission factorBq Iod

    nonradiative recombination time h SA sectirm % 0.1 m

    group velocity of light us o.75*lo10 Cm/s

    confinement factor r 0.1

    gti crosssection Ag zp,o-ls cm 2SA cross section Aa **@ cm 2

    effective transparency canier density, gain section Nog 1.2*10’8 cm 3

    effective transparency carrier density, SA section NoO 1.2*1018 cm 3

    gain saturation (nonlinearity) coefficient &’2 5.Io18 cm 3

    gain notdine.wity relaxation time MC4 0.5 P

    SA safumfion (nontinetity) coefficient G5*~o17 cm 3

    SA nonlinetity relaxation time G,(.) 0.5 v1

    imensay reflection coefficients (both sides) R 0.36

    Iinewidtb enhancement factor (gain section) I ct. I 2 Igti tinewidth Ang 2*1013 1/s

    laserca~ity length L 600 bm

    Finally, to introduce gain nonlinearities with finite relaxationtime, we use an additional equation of the type

    dg _go – g(l + Ws)

    dt = (9) ; 90(~) = 4(N – ~Og), (9)‘nl

    a similar equation being used for the SA section.

    E. Simulation Results

    Fig. 8 shows some examples of the simulated temporal pro-files of the MCPM regime for different geometries correspond-ing to those studied theoretically in the previous subsectionand experimentally in Section III.

    For the case of “classical” colliding pulse mode locking(Fig. 8(a)) one observes a well-developed train of pulses atthe repetition rate of 2/T(T = 2T/A~ = 2L/v9) being

    the fundamental repetition period) with some period doubling

    present. This agrees reasonably well with both the frequency-domain results (some of the overlap coefficients for oddnumber of mode intervals being nonzero) and the experimentalobservations (note the envelope modulation in the measuredcorrelation curve).

    Fig. 8(b) illustrates the case with all three absorbers in-volved. Four approximately evenly spaced (T/4 apart fromone another) pulses are clearly observed within each funda-mental repetition period, as expected from the experimentalresults. The amplitudes of the pulses within one repetition

    period are different, and very strongly depend on the parametervalues used. For instance, for shorter SA sections (20 ~minstead of 40 ~m as in the figure), the amplitude of one of thepulses becomes virtually zero. More accurate measurements

    25

    20151050

    0 10 20 30 40 50time, ps

    (a)

    25 ,201510500 10 20 30 40 ;0

    time, ps

    (b)

    z~50

    time, ps

    (c)

    15

    10

    5

    00 10 20 30 40 50

    time, ps

    (d)

    10

    5

    00 10 20 30 40 50

    time, ps

    (e)

    Fig. 8. Simulated pulse trains for the MCPM emission for two-pulse (a),four-pulse (b), one-pulse (c), and three-pulse (d)–(e) cases. For parametersof the laser see Table I. The laser geometries in Fig. 8(a)–(e) are as inFig. 7(a)-(e), respectively, the currents 1 = 4.7th (a), (c), 6Jth (b), (d), (e).

    could determine which of the two cases is closer to theexperimental observations.

    Fig. 8(c) shows the case of a single SA a quarter of thecavity length away from the facet. The pulse train in this casehas a period of T, with a smaller trailing pulse following aquarter of the period after each main pulse (seen as a shoulderdue to the gain dispersion and finite nonlinearity relaxationtime).

    Fig. 8(d) and (e) show the expected three-pulse case (two

    absorbers biased). Here, we are also able to simulate a streamof pulses separated in time by T/3, but to do so, as in thefrequency-dependent model, we have to shift the absorbers

  • MARTINS-FILHO et al.: MONOLITHIC MULTIPLE COLLIDING PULSEMODE-LOCKEDQUANTLJIWWELLLASERS 549

    from the positions fixed by the contact towards the moreeven spacing (L/3), as seen in Fig. 8(e). For the absorberscentered as grown (Fig. 8(d)) we still observe a leading pulseapproximately (not exactly) a third of the period ahead of themain one, which also gives two intermediate peaks within eachperiod of the correlation function, but can hwdly explain theexperiment quantitatively, since the leading pulse amplitudeis very weak.

    Pulse durations in most cases varied within the range of 1–3ps (broader structures in. Fig. 8(c) and (d) are apparently dueto overlap of consecutive pulses). Such durations are in reason-able agreement with the estimates made from the experimentalobservation; detailed comparison seems premature at this stageof studies due to both the limitations of the experimental

    technique and the large number of fitting parameters in thesimulations.

    Finally, we briefly discuss the behavior of the results when

    some of the pamrneters are changed. Variation of nonlinearity

    recovery times within the subpicosecond limits changed therelative amplitudes of multiple pulses but brought no qualita-

    tive changes. With very small nonlinearity coefficients in theSA section, when (5b) was not fulfilled, the simulated laserexhibited steady single-mode lasing, as expected. For somerange of pumping levels, the model predicted an apparentlychaotic slow envelope of the pulse train, not observed in theexperiment. We believe the discrepancies may be due to thefact that the characteristic parameters of the gain and SAsections may vary with current in realistic circumstances (forinstance, due lto imperfect electric isolation, the SA voltagedecreases by absolute value as the current increases, thusprobably decreasing the absorption suppression coefficient),which is not taken into account by the model. Taking intoaccount the dynamic gratings (colliding pulse effect) shortensthe pulses by approximately 10-20%, but otherwise is not verysignificant.

    V. DISCUSSIONSAND CONCLUSION

    The operaticm of a monolithic multisectioned semiconductorlaser has been described. The laser can be operated as eithersingle mode, multimode, self-pulsating (or Q-switched) andmode-locked in either 1, 2, 3, or 4 pulse operation. This deviceis a very versatile source of high repetition rated (up to 375GHz) ultrashort pulses (around 1–3 ps) of light. The variousmodes of operation of the device have been experimentallyinvestigated and we have found experimental indications ofthe presence of excitonic nonlinearities in its operation.

    The theoretical results from the frequency domain model

    strongly suggest that for short monolithic cavities, fast non-linearities play a major role in mode-locking operation andthat the device geometry is highly favorable to MCPMoperation. Numerical simulations with a time-domain modelwere performed, using saturation coefficients and fast recove~times estimated from the frequency domain model. Goodagreement between the models and the experimental results forMCPM operation was obtained, although there are still somefeatures which require further investigation for a completeunderstanding of the laser. In particular the nature of the very

    rapid recovery of the saturable absorber, which we postulatehere (the time-domain simulations use a recovery time ofaround 0.5 ps), has been observed in pump-probe experimentson reverse biased multiple quantum-well material [6], but hasnot been fully understood. Also, it is not absolutely clearwhy the three-pulse operation occurs given that the saturableabsorbers are not placed 1/3 along the laser cavity.

    The device is a monolithic semiconductor chip which can

    be mass produced; it is low-cost, robust, efficient, and reliable.These are crucial features if ultrashort pulses of light are tofind wide-spread application outwith the laboratory.

    APPENDIX

    LONGITUDINAL MODE PROFILES AND

    OVERLAP FACTORS OF THE CAVITY

    The coupled-wave (1) are obtained by distributing the lasing

    light in the cavity into longitudinal modes:

    E(z’,t) = ~ Ek(t)uk(?z) + Cc. (lo)

    The technique for such distribution for realistic lasers withopen cavities was proposed by Siegman [41] and developedby Hamel and Woerdman [42]; a simple generalization forthe case of lasers with intracavity absorbers was performed in

    [32] and [33] to derive (1) and (3). The wave functions of thecavity are defined as

    where ?.L~Rand u~L are left-and right traveling waves, qh is

    the complex mode vector

    (12)

    (k) =where, in steady state, Tg (h) _gk in gain sections and T. –‘ah in absorber sections, so that

    The normalization factor N is chosen so that

    /

    L/2

    dZUk(.Z)Uk * (z) = 1.–L/2

    (13)

    Substituting (11 )–( 13) into (3), one obtains, after some trivialthough cumbersome calculations, the explicit expressions for

    (9@) [33]the overlap factors cm

    (14)

  • 550

    where the sumation

    IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, VOL. 1, NO. 2, JUNE 1995

    is over all the appropriate (gain or

    absorber) segments and

    t-h=*{’XP(’:Z)-lI’XPE’L,)‘$’XP(-Z’PLP)l

    +’” ((’Z+WL’)-l27rm

    ‘Yl+ly-IJ

    [( 27rm.211–1

    . exp i—L

    + ~7,Lp,=1 )

    ((

    27rmz~+l1

    +~exp –L ))1}+~7,LP 100 GHz) by mode locking;’ IEEE J.Quantum Electron., vol. 26, pp. 250-261, 1990.A. V. Uskov, J. R. Karin, R. Nagarajao, J. E. Bowers, and J. Mgmk,“Ultrafast dynamics in waveguide satnrable absorbers” in IEEE 14thInt. Semiccmduct. Laser Corf, Maui, W, 1994, paper P18, pp. 117–1 18.E. L. Portnoi and A. V. Chelnokov, “Passive mode-locking in a shortcavitv diode laser,” in IEEE 12th Int. Semiconduct. Laser Conf. Davos.Swi~erland, 1990, pp. 14@141.

    .,

    Y. K. Chen, M. C. Wu, T. Tanbun-Ek, R. A. Logan, and M. A.Chin, “Subpicosecond monolithic colliding-pulse mod~-locked multiplequantum well lasers,” Appl. Phys. Lett., vol. 58, pp. 1253–1255, 1991.

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    Eugene A. Avrutin for“aphotographaad biography,see this issue, p. 460.

    C. N. Ironside was born in Aberdeen,Scotland, in1950. HISPh.D. work, at Heriot-WattUniversity,was on a type of tnneable infraredsemiconductorlaserthe Spin-flipRamarrLaserwhich used InSb asthe gain medium.

    Workin thk arealed on to a studyof the resonantnonlinea’ opticat propertiesof InSb subsequentlyemployedin opticaflybktable devices. He movedtoOxford University to work on time resolved spec-troscopy of solids which included opticat energytransferprocesses in solids and exciton dynamics.

    He developed some new time-resolved spectroscopy techniques in this areaand developed an interest in ultrashort pulses. Since 1984, he has been atGlasgow University working mainly on the generation and application ofultra-short pulses in integrated optics. His research interests now include,high-speed atl-optical switching in semiconductor waveguides, optoelectronicproperties of RTD’s and modelocked semiconductor lasers.

    tudinat ei.gemnodes of a laser; Phys. Rev. A, vol. 40, pp. 2785–2793, J. S. Roberts, photograph and biography not available at the time of1989.

    Research Council). His

    Joaquim F. Martins-Fllho (S’94), was born inRecife, Brazil,in 1966.He receivedthe B. SC. degreein electronic engineering from the UniversidadeFederal de Pemambuco (UFPE), Recife, in 1989, theM. SC. degree in applied physics from the same in-stitution in 1991 studying nonlinear optics in opticatfibers, and is currently completing the Ph.D. thesis atthe University of Glasgow, Scotland, investigatingulfrafast opticat pulse generation from mode-lockedsemiconductor lasers.

    His Ph.D. work is supported by CNPq (Brazilianresearch interests are in the area of optoelectronic

    device design and fabrication.