magnetotransport in multi-weyl semimetals: a kinetic

26
Prepared for submission to JHEP Magnetotransport in multi-Weyl semimetals: A kinetic theory approach Renato M. A. Dantas, Francisco Peña-Benitez, Bitan Roy, Piotr Surówka Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Str. 38, 01187 Dresden, Germany E-mail: [email protected], [email protected], [email protected], [email protected] Abstract: We study the longitudinal magnetotransport in three-dimensional multi-Weyl semimetals, constituted by a pair of (anti)-monopole of arbitrary integer charge (n), with n =1, 2 and 3 in a crystalline environment. For any n> 1, even though the distribution of the underlying Berry curvature is anisotropic, the corresponding intrinsic component of the longitudinal magnetoconductivity (LMC), bearing the signature of the chiral anomaly, is insensitive to the direction of the external magnetic field (B) and increases as B 2 , at least when it is sufficiently weak (the semi-classical regime). In addition, the LMC scales as n 3 with the monopole charge. We demonstrate these outcomes for two distinct scenarios, namely when inter-particle collisions in the Weyl medium are effectively described by (a) a single and (b) two (corresponding to inter- and intra-valley) scattering times. While in the former situation the contribution to LMC from chiral anomaly is inseparable from the non-anomalous ones, these two contributions are characterized by different time scales in the later construction. Specifically for sufficiently large inter-valley scattering time the LMC is dominated by the anomalous contribution, arising from the chiral anomaly. The predicted scaling of LMC and the signature of chiral anomaly can be observed in recently proposed candidate materials, accommodating multi-Weyl semimetals in various solid state compounds. Keywords: Multi-Weyl semimetal, Chiral anomaly, Longitudinal magnetotransport ArXiv ePrint: 1802.07733 arXiv:1802.07733v2 [cond-mat.mes-hall] 28 Nov 2018

Upload: others

Post on 27-Jun-2022

6 views

Category:

Documents


0 download

TRANSCRIPT

Page 1: Magnetotransport in multi-Weyl semimetals: A kinetic

Prepared for submission to JHEP

Magnetotransport in multi-Weyl semimetals: Akinetic theory approach

Renato M. A. Dantas, Francisco Peña-Benitez, Bitan Roy, Piotr Surówka

Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Str. 38, 01187 Dresden, Germany

E-mail: [email protected], [email protected], [email protected],[email protected]

Abstract: We study the longitudinal magnetotransport in three-dimensional multi-Weylsemimetals, constituted by a pair of (anti)-monopole of arbitrary integer charge (n), withn = 1, 2 and 3 in a crystalline environment. For any n > 1, even though the distributionof the underlying Berry curvature is anisotropic, the corresponding intrinsic component ofthe longitudinal magnetoconductivity (LMC), bearing the signature of the chiral anomaly,is insensitive to the direction of the external magnetic field (B) and increases as B2, atleast when it is sufficiently weak (the semi-classical regime). In addition, the LMC scales asn3 with the monopole charge. We demonstrate these outcomes for two distinct scenarios,namely when inter-particle collisions in the Weyl medium are effectively described by (a)a single and (b) two (corresponding to inter- and intra-valley) scattering times. Whilein the former situation the contribution to LMC from chiral anomaly is inseparable fromthe non-anomalous ones, these two contributions are characterized by different time scalesin the later construction. Specifically for sufficiently large inter-valley scattering time theLMC is dominated by the anomalous contribution, arising from the chiral anomaly. Thepredicted scaling of LMC and the signature of chiral anomaly can be observed in recentlyproposed candidate materials, accommodating multi-Weyl semimetals in various solid statecompounds.

Keywords: Multi-Weyl semimetal, Chiral anomaly, Longitudinal magnetotransport

ArXiv ePrint: 1802.07733

arX

iv:1

802.

0773

3v2

[co

nd-m

at.m

es-h

all]

28

Nov

201

8

Page 2: Magnetotransport in multi-Weyl semimetals: A kinetic

Contents

1 Introduction 1

2 Berry curvature and topology of a multi-Weyl semimetal 4

3 Kinetic Theory 63.1 Collisions with single effective relaxation time 73.2 Collisions with inter-valley and intra-valley relaxation times 9

4 Magnetotransport in the multi-Weyl system 114.1 LMC with single effective relaxation time 114.2 LMC with two relaxation times 14

5 Conclusions and Discussions 14

A Computation of Berry Curvature 15

B Calculation of magnetoconductance with two relaxation times 16

C Computation of magnetoconductivity 18C.1 Multi-Weyl semimetal 19C.2 Power Series Expansion 20

1 Introduction

Quantum phenomena can have macroscopic manifestations, such as the anomaly-inducedtransport in systems, constituted by linearly dispersing massless Weyl fermions in threedimensions. The most celebrated ones are the chiral magnetic and chiral vortical effects [1–5], both being intimately related with quantum anomalies [6, 7]. The non-dissipative currentdescribing these phenomena is given by

J = σB B + σω ω, (1.1)

where B and ω are magnetic and vorticity fields, respectively. Here, σB and σω respectivelycorresponds to the chiral magnetic and chiral vortical conductity.

At the classical level, massless left- and right-handed Weyl spinors separately exhibitchiral symmetries and independent rotations of the phase can be performed for each species.By contrast, at the quantum level at most one of these rotations can be preserved (leav-ing the path-integral action invariant), a phenomenon known as quantum anomaly. Inparticular, the electromagnetic gauge invariance requires U(1)e = U(1)L + U(1)R to be

– 1 –

Page 3: Magnetotransport in multi-Weyl semimetals: A kinetic

Figure 1. Quasiparticle spectra in a multi-Weyl system along various high-symmetry directionsin the close vicinity of Weyl nodes, characterized by an integer monopole charge n. Note thatdispersion always scales linearly with pz (see panel A) for any n. But, in the px − py plane theenergy scales as E ∼ |p⊥| for n = 1 (see panel B), E ∼ |p⊥|2 for n = 2 (see panel C) and E ∼ |p⊥|3

for n = 3 (see panel D), where p⊥ =√p2x + p2y. A rotational symmetry is always present in the

px − py plane. Here, momentum p = (px, py, pz) is measured from the Weyl node. Note that forn > 1 the system looses the Lorentz covariance.

preserved, while its chiral counterpart U(1)5 = U(1)L − U(1)R suffers an anomalous viola-tion [8, 9]. In three spatial dimensions there may be two different sources to the anomalousnon-conservation of the chiral charge. The first one, the so-called pure gauge anomaly, ispresent when parallel electric and magnetic field are switched on in the system [10, 11].The second one is called mixed gauge-gravitational anomaly and violates the conservationof chiral charge when the system is placed on a curved background [12]. Even though sig-natures of these anomalies can be found in transport, for concreteness we only consider theimprint of pure gauge anomaly in multi-Weyl systems 1. In the high-energy physics such aneffect is expected to be present in the quark-gluon plasma, experimentally created in heavy-ion collisions (see Ref. [16] and references therein). Furthermore, chiral anomaly leaves itssignature in condensed matter systems, accommodating emergent Weyl quasiparticles atlow-energies [17]. Due to a no-go theorem [18], Weyl fermions are always realized in pairs

1For a detailed description of the effect of the mixed-gauge gravitational anomaly on transport coefficientssee Refs. [7, 13, 14]. For an experimental signature of such an anomaly in a Weyl semimetal consult Ref. [15].

– 2 –

Page 4: Magnetotransport in multi-Weyl semimetals: A kinetic

(except on the surface of a time-reversal invariant four-dimensional topological insulators)and each copy can be classified according to its chirality : left or right. On the other hand,it has been shown that chiral magnetic effect vanishes in Weyl semimetals at equilibrium(for a detailed discussion see [19–21]). Therefore, nonequilibrium signatures need to beexplored in order to measure the effects of anomalies in Weyl materials.

Any non-orthogonal arrangement of the electric E and magnetic B fields (such thatE · B 6= 0) causes a violation of the conservation of chiral charge. But, for the sake ofconcreteness, we restrict ourselves to the situation where the external electric and mag-netic fields are always parallel to each other. We show that the system then becomesmore conductive with an increasing magnetic field, an effect often refered as negative lon-gitudinal magnetoresistance (LMR), a hallmark signature of the Adler-Jackiw-Bell chiralanomaly [22]. Such an observation should be contrasted with the situation in a normalmetal, without any Berry curvature, where magnetoresistence is typically positive.

In the language of condensed matter physics, the Weyl nodes, where Kramers non-degenerate valence and conduction bands touch each other, act as source and sink of AbelianBerry flux or curvature. Typically, Weyl points with different chiralities are separated inthe momentum space. Otherwise, such defects in the reciprocal space can be characterizedwith an integer monopole number that in turn also defines the topological invariant ofthe system (see Appendix A). In fact the Berry flux and quantum anomalies are directlyconnected [23], as we demonstrate here for multi-Weyl semimetals (see Ref. [24]).

So far, both theoretical [3, 25–35] and experimental [36–40] focus have largely beencentered around simple Weyl systems, possessing pairs of (anti-)monopole with unit charge(n = 1). However, various condensed matter systems endow an unprecedented opportunityto explore the territory of multi-Weyl semimetals, characterized by pairs of (anti)-monopoleof arbitrary integer charge n [41–44]. The quasiparticle dispersion for any n > 1 possessesa natural anisotropy, as displayed in Fig. 1. But, underlying discrete rotational symmetryin a lattice imposes a strict restriction on the available monopole charge in real materi-als, namely |n| ≤ 3 [44]. Thus far most of the known examples of Weyl materials haven = 1 [17, 45, 46]. Nevertheless, Weyl points with n = 2 (known as double-Weyl nodes)can in principle be found in HgCr2Se4 [41, 42] and SrSi2 [43], and A(MoX)3 (with A=Rb,Tl; X=Te) can accommodate Weyl points with n = 3 (known as triple-Weyl nodes) [47].We also note that charge-neutral BdG-Weyl quasiparticles with n = 2 can also be foundin superconducting states of 3He-A [48], URu2Si2 [49], UPt3 [50], SrPtAs [51], YPtBi [52],for example. Therefore, unveiling the imprint of chiral anomaly in general Weyl semimet-als, besides its genuine fundamental importance, is also experimentally pertinent. In thisarticle we study longitudinal magnetotrasport (LMT) in multi-Weyl semimetals, in thesemi-classical regime. More specifically, resorting to the kinetic theory we compute thetotal out of equilibrium longitudinal magnetoconductivity (LMC) in the parameter regimeT

√B µ, where T is the temperature and µ is the chemical potential, measured from

the Weyl nodes. Note that semiclassical theory of transport is applicable in a parameterregime where quantum corrections can be neglected. In our analysis T µ, and hence thechemical potential or Fermi momentum sets the infrared cutoff in the system. The semi-classical theory is then applicable when

√B µ. By contrast, if T µ then semiclassical

– 3 –

Page 5: Magnetotransport in multi-Weyl semimetals: A kinetic

appraoch is valid when√B T [53]. Manifestation of chiral anomaly in thermal transport

for neutral BdG-Weyl quasiparticles is, however, left as a subject for a future investigation.Kinetic theory can capture the longitudinal magnetotransport in the weak magnetic

field limit when ωcτ 1, where ωc is the cyclotron frequency and τ is the average relax-ation time, dominantly arising from elastic scattering due to impurities. In the analysisof longitudinal magnetotransport, which necessarily involves charge pump from the left tothe right chiral Weyl point, the relaxation time (τ) is set by backscattering. In this regimethe Landau levels are not sharply formed (justifying the approach based on kinetic theory)and the path between two successive collision is approximately a straight line. Therefore,in the semi-classical (or weak magnetic field) regime, τ is independent (effectively) of themagnetic field strength and we treat it as a phenomenological input in our analysis fromoutset. By contrast, in the strong magnetic field limit, the path between two successivecollision gets sufficiently curved, such that τ ≡ τ(B) in addition to (ωc/µ 1), and theanalysis of magnetotransport demands a quantum mechanical analysis [54]. We here focusonly on the former situation.

We now provide a brief synopsis of our main findings. We here investigate the LMCin a mutli-Weyl system within the framework of semi-classical theory by considering twopossible scenarios, when (a) relaxation of both regular and axial charge is controlled by onlyone effective time scale in the system (see Sec. 3.1), and (b) there exists two scattering timesin the system (see Sec. 3.2), arising from the inter-valley (τinter) and intra-valley (τintra)processes, for example. While τinter is responsible for the relaxation of the axial charge, theintra-valley scattering ensures the isotropy of the distribution function. Irrespective of thesedetails, we show that LMC (σjj) always increases as σjj ∼ B2 for any value of n as wellas for any choice of j = x, y, z, which can possibly be observed in experiments. Moreover,σjj scales as n3 with the monopole charge (see Sec. 4). However, with a single relaxationtime in the system, the contribution of chiral anomaly to LMC cannot be separated fromthe non-anomalous ones (see Sec. 4.1). Such a separation arises quite naturally in thepresence of two scattering times in the medium. In particular, we explicitly demonstratethat when the inter-valley scattering time is sufficiently longer than in intra-valley one (i.e.τinter τintra), the postive LMC is dominated by the anomalous contribution, bearing thesignature of the chiral anomaly (see Sec. 4.2).

The rest of the paper is organized as follows. In the next section we introduce thelow-energy model for a multi-Weyl semimetal and compute the Berry curvature. In Sec. 3,we discuss the general formalism of kinetic theory in the context of Weyl semimetals. Sec. 4is devoted to the longitudinal magnetotransport in a multi-Weyl metal. The concludingremarks and a discussion on related issues are presented in Sec. 5. Additional technicaldetails are relegated to the Appendices.

2 Berry curvature and topology of a multi-Weyl semimetal

We begin the discussion by computing the Berry curvature and the associated integertopological invariant of a multi-Weyl semimetal, featuring Weyl nodes with arbitrary integer

– 4 –

Page 6: Magnetotransport in multi-Weyl semimetals: A kinetic

monopole charge n. The low-energy Hamiltonian of a multi-Weyl semimetal is given by [41,42, 44, 55, 56]

Hn (p) = αnpn⊥ [cos (nφp)σx + sin (nφp)σy] + vpzσz ≡ εp (np · σ) , (2.1)

where φp = tan−1 (py/px), p⊥ =√p2x + p2

y, np = (αnpn⊥ cos (nφp) , αnp

n⊥ sin (nφp) , vpz)ε

−1p ,

and the set of Pauli matrices σ = (σx, σy, σz) operate on the (pseudo-)spin indices. Mo-mentum p is measured from the Weyl node. The energy dispersion in the close proximityto a Weyl node is given by ±εp, where ± respectively corresponds to the conduction andvalence bands, and

εp =√α2np

2n⊥ + v2p2

z. (2.2)

The quasiparticle spectra in a multi-Weyl semimetal along various high symmetry directionsare shown in Fig. 1. Due to the doubling theorem Weyl nodes always appear in pairs [18],which we refer here as valley degrees of freedom.The components of the Berry curvature close to a Weyl node are defined as

Ω±p a = ±1

4εabcnp ·

(∂np

∂pb× ∂np

∂pc

), (2.3)

for the conduction (Ω+p ) and valence (Ω−p ) bands. For concreteness, we now focus on the

conduction band and for brevity take Ω+p → Ωp. For a multi-Weyl semimetal we then find

Ω(s)p =

s

2

nvα2n

ε3pp

2(n−1)⊥ (px, py, npz) , (2.4)

with s = ± corresponds to two valley. Notice that upon integrating the Berry curvatureover a closed surface Σ, we find the integer topological invariant of a multi-Weyl semimetal

s n =1

∮Σ

Ω(s)p · dS, (2.5)

where dS is the differential area vector (see Appendix A for details). Therefore, the integertopological invariant of a Weyl node measures the amount of Berry flux enclosed by a unitarea surface, and the Weyl nodes act as source and sink of Abelian Berry curvature ofstrength n.

At this point it is worth pausing to appreciate the dimensionality of various physicalquantities in the natural units, in which we set ~ = c = kB = 1. Here the Fermi velocity(vF ) plays the role of the velocity of light (c). In units of energy, the electric charge hasdimension zero, while electric and magnetic fields have dimensions two, v is dimensionlessand αn has dimension 1−n 2. At last, the central quantity of this study, the conductivity,has dimension one, as guaranteed by the gauge invariance.

2While the Fermi velocity vF and α1 are dimensionless in the natural unit, αn for n ≥ 2 bears thedimension of (energy)1−n, such that αnk

n⊥ has the dimension of energy. Note that α1 and α2 are respectively

the Fermi velocity and the inverse mass of gapless Weyl excitations in the xy-plane However, there is nostandard nomenclature for αn with n > 2.

– 5 –

Page 7: Magnetotransport in multi-Weyl semimetals: A kinetic

3 Kinetic Theory

Kinetic theory is a semiclassical framework, which we employ for the rest of our analysis.We assume the following hierarchy of scales T

√B µ, where T is temperature, B is

the magnetic field and µ is the chemical potential, measured from the band-touching point.In this regime, one can ignore the Landau quantization and use Boltzmann kinetic equation

∂tf(s) +∇xf

(s) · x(s) +∇pf(s) · p(s) = C[f (s)], (3.1)

which describes the evolution of the particle distribution function f (s) in the phase space,where s is the valley index and C

[f (s)

]denotes the collision integral. The effective semi-

classical dynamics of Weyl quasiparticles is modified by the Berry curvature in momentumspace, which leads to the following equations of motion

x(s) = vp + p(s) ×Ω(s)p , p(s) = eE + ex(s) ×B, (3.2)

where vp = ∇pεp is the group velocity [57]. A comment about the energy dispersion (εp) isdue at this stage. In this article we take εp to be the dispersion relation obtained from theeffective Hamiltonian [see Eq. (2.2)]. Wave-packet construction reveals that a correctionproportional to the inner product of the wave-packet orbital magnetization and the magneticfield should be added to the standard energy dispersion εp [58]. In particular for n = 1

Weyl semi-metals, Lorentz invariance requires εp → εp ∓ 12p2

p ·B [75, 76]. However, sucha correction can lead to an undesired consequence: group velocity becomes bigger than theFermi velocity vf [59], as vf plays the role of the velocity of light in our construction. Onthe other hand, in [35] the LMC was studied for Weyl semi-metals in the context of kinetictheory concluding that such a modification in the dispersion relation only changes the LMCquantitatively, without altering its overall B2 dependence. Therefore, considering the issueswith the group velocity and the conclusions of [35], we neglect this correction in the presentarticle and leave its imprint on LMC as a subject for a future investigation.

The challenge to solve Eq. (3.1) arises from the complex form of the collision term,which captures the interactions between particles. Nevertheless, significant progress can bemade by employing the so-called relaxation time approximation, which encodes the fact thatthe system returns to equilibrium via scattering events among its constituent particles andimpurities [63]. This process is controlled by a phenomenological parameter which can beinterpreted as the average time between two successive collisions. The nature of collisionsshould follow as a physical input and different choices correspond to different physical out-comes. Specifically, we here analyse two different collision integrals and the correspondingphysical scenarios in two subsequent sections. Most importantly we assume that in thesemiclassical limit the average scattering times can be considered to be independent of themagnetic field strength for the following reason: in the weak field limit, the radius of thecyclotron orbit is so large that the path between to successive collisions can be approxi-mated as a straight line, and concomitantly B-independent. We also assume the relaxationtime to be independent of the angles.

– 6 –

Page 8: Magnetotransport in multi-Weyl semimetals: A kinetic

3.1 Collisions with single effective relaxation time

Our first choice of the collision term assumes the existence of a single relaxation time(τ). The collision integral then takes the following form

C1[f (s)] = −δf(s)

τ, (3.3)

where δf (s) = f (s) − f0, and f0 the equilibrium Fermi-Dirac distribution function. Thistype of collision integral was recently used in Refs. [60–62]. The above collision integral hasto be taken with care as it assumes that impurity scattering relaxes both regular and axialcharge densities [63]. Therefore we assume the equilibrium state is given by fixed electronand vanishing axial chemical potentials. Such a scenario is common for open systems, anexample given by electronic systems in the presence of charged impurities. However, wehere do not derive the above collision integral from any microscopic model, rather treat itas a phenomenological input in the kinetic theory formalism. To show this explicitly wecalculate the semiclassical expressions for the chiral currents (J(s)). First we invert thesemiclassical equations of motion and obtain [64–66]

x(s) =(

1 + eB ·Ω(s)p

)−1 [vp + eE×Ω

(s)p + e

(vp ·Ω(s)

p

)B], (3.4)

p(s) =(

1 + eB ·Ω(s)p

)−1 [eE + evp ×B + e2 (E ·B) Ω

(s)p

]. (3.5)

The presence of the Berry curvature modifies the phase space volume element by the factor(1 + eB ·Ω(s)

p ), which satisfies the Liouville equation [66]

∂t(1+eB·Ω(s)p )+∇x ·

[(1 + eB ·Ω(s)

p )x(s)]+∇p ·

[(1 + eB ·Ω(s)

p )p(s)]

= 2πsn e2E·B δ3(p) .

(3.6)Combining the last expression with the Boltzmann equation [Eq. (3.1)] we arrive at thefollowing continuity equation

∂tρ(s) +∇ · J(s) =

s e3 n

4π2E ·B− δρ(s)

τ, (3.7)

where the charge (ρ) and current (J) densities are respectively defined as

ρ(s) = e

∫d3p

(2π)3

(1 + eB ·Ω(s)

p

)f (s), J(s) = e

∫d3p

(2π)3

(1 + eB ·Ω(s)

p

)xf (s) . (3.8)

Notice that Eq. (3.7) already discerns the connection between the Berry curvature andchiral anomaly, and will imply relaxation of both electromagnetic and axial charges.

Our goal here is to study the system in a homogeneous and stationary state3. Therefore,linearising the Boltzmann equation we obtain

δf (s) = − τ

1 + eB ·Ω(s)p

[(eE + e2 (E ·B) Ω

(s)p

)· vp

] ∂f0

∂εp= −τeE · x(s) ∂f0

∂εp, (3.9)

3Notice that in order to achieve a steady state, axial charge needs to be relaxed by the presence ofimpurities, otherwise the parallel electric and magnetic fields would pump charges indefinitely into thesystem and the LMC would be infinite.

– 7 –

Page 9: Magnetotransport in multi-Weyl semimetals: A kinetic

to the leading order. The out-of-equilibrium distribution function is proportional to thework done by the electric field between successive collisions. The injected energy is used bythe system in two different mechanisms:• Transport of charge. The first term in Eq. (3.9) is proportional to the work done

by the electric field to move the electrons along a trajectory with effective velocity vp.• Creation of charges via the anomaly. Eq. (3.7) suggests that the second term

in Eq. (3.9) is proportional to the induced charge, δρ ∼ nτE ·B.Hence we can split the out-of-equilibrium distribution function as δf (s) = δf

(s)O + δf

(s)A ,

where

δf(s)O = − eτ(E · vp)

1 + eB ·Ω(s)p

∂f0

∂εp, δf

(s)A = −e

2τ(Ω(s)p · vp)

1 + eB ·Ω(s)p

∂f0

∂εp(E ·B) . (3.10)

Now the current operator can be decomposed as J(s) = JO(s) + JAH

(s) + JCM(s) [66],

where JO(s), JAH

(s) and JCM(s) denotes the Ohmic, anomalous Hall and out-of-equilibrium

chiral magnetic currents, respectively. For simplicity we will assume the multi-Weyl metalis made of two valleys, therefore the specific form of each component reads

JO = e∑s=±

∫d3p

(2π)3vp δf

(s), (3.11)

JAH = e2E×∑s=±

∫d3p

(2π)3Ω

(s)p δf (s), (3.12)

JCM = e2B∑s=±

∫d3p

(2π)3

(vp ·Ω(s)

p

)δf (s) . (3.13)

As we are interested in computing the LMC, and the anomalous Hall current is alwaystransverse to the electric field, we ignore it from now on. Note that each component of thecurrent receives two sub-contributions, which can be appreciated by expressing them as

JO = e∑s=±

∫d3p

(2π)3vp

4π2eδρ(s)

sn

(vp ·Ω(s)

p

)1 + eB ·Ω(s)

p

+eτ(E · vp)

1 + eB ·Ω(s)p

(−∂f0

∂εp

)(3.14)

JCM = e2 B∑s=±

∫d3p

(2π)3

4π2eδρ(s)

sn

(vp ·Ω(s)

p

)2

1 + eB ·Ω(s)p

+eτ(E · vp)

(vp ·Ω(s)

p

)1 + eB ·Ω(s)

p

(−∂f0

∂εp

).

The first term is proportional to an imbalance of charge, which causes a net currentalong the direction of the group velocity or the external magnetic field. The second contri-bution is related to the energy needed to transport the particles with an effective velocitygiven by vp. Nonetheless, we would like to emphasize that even though we identify ananomalous contribution in the current with this collision integral [see Eq. (3.3)], it is notpossible to disentangle it from the non-anomalous one, due to the presence of a singleeffective scattering time τ . However, if we introduce two different scattering times in the

– 8 –

Page 10: Magnetotransport in multi-Weyl semimetals: A kinetic

µ

p

L R

p

inter intraintra

Figure 2. A schematic representation of two scattering processes in a simple Weyl metal, pos-sessing linear dispersion along all three direction. Respectively the forward (intravalley) and back(intervalley) scattering processes are shown by turquoise and blue arrows. The chemical potential(µ) is measured from the band touching point. This construction is also applicable for arbitrarymonopole charge n. Here L and R respectively denotes the Weyl node with left and right chirality.

collision integrals, which can arise from inter- and intra-valley scattering processes, then it isconceivable to isolate the anomalous contributions from the non-anomalous one, specificallywhen τinter τintra, which we discuss in the next section.

3.2 Collisions with inter-valley and intra-valley relaxation times

In this subsection we introduce a different collision integral that corresponds to thesituation in which there exist two relaxation times. The collision with impurities can eitherchange the chirality of the particle or keep it intact. The former process is captured by theso-called inter-valley relaxation time and the latter one by the intra-valley relaxation time(see Fig. 2). The inter-valley scattering changes the relative number of particles betweentwo valleys, and is responsible for the “charge-pump" between them. It involves a largemomentum transfer and is assumed to be dominated by elastic scattering of particles fromimpurities. In particular, Gaussian impurities can be a microscopic source of such an inter-valley scattering, while Coulomb impurities, at least in the weak field limit, give rise toforward or intra-valley scattering. Formally we may write the collision term as [35]

C2[f (s)] =f (s) − f (s)

τintra+f (s) − f (s)

τinter≡ f (s) − f (s)

τ∗+ Λ(s), (3.15)

– 9 –

Page 11: Magnetotransport in multi-Weyl semimetals: A kinetic

where τ∗ = τinterτintra/ (τinter + τintra), s = −s,

f (s) =⟨(

1 + eB ·Ω(s)p

)f (s)

⟩, Λ(s) =

f (s) − f (s)

τinter.

The angular brackets stand for a generalized average over the angles (θ and φ)

〈. . .〉 =Γ(1

2 + 1n)

2π3/2 Γ( 1n)

∫dφdθ (sin θ)2/n−1 . . . , (3.16)

introduced in the new coordinate system

px =

(εp

sin θ

α

)1/n

cosφ, py =

(εp

sin θ

α

)1/n

sinφ, pz = εpcos θ

v, (3.17)

compatible with the symmetry of the problem.After introducing this average the phase space volume integral reads∫

d3p

(2π)3. . . =

2π3/2 Γ( 1n)

nvΓ(12 + 1

n)

∫ (εpαn

)2/n dεp(2π)3

〈. . .〉 . (3.18)

Given this new collision integral the continuity equation can be written as follows

∂tρ(s) +∇ · J(s) =

s e3 n

4π2E ·B− s

2

ρ5

τinter. (3.19)

From the above equation, after writing the corresponding electromagnetic and axial conti-nuity equations, it can be seen how τinter relaxes only the axial charge ρ5 = (ρ(+)−ρ(−))/2.

By solving the kinetic equation we obtain the following leading order solution for thedistribution function

f (s) = f (s) + τ∗(

Λ(s) − p(s) · v ∂εpf0

), (3.20)

where Λ(s) can be obtained by averaging the product of the phase space measure with thekinetic equation (see Appendix B for the detailed computations), leading to

Λ(s) = se2 (E ·B)n2v( εα

)−2/n Γ(12 + 1

n)

π1/2 Γ( 1n)∂εpf0. (3.21)

Finally, the expression for the vector current (considering only a pair of nodes) reads as

J = e2τinterB

∫d3p

(2π)3

(vp ·Ω(+)

p

)Λ(−) − 2e2τ∗B

∫d3p

(2π)3

(vp ·Ω(+)

p

)Λ(−)

+ eτ∗∑s=±

∫d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (−p(s) · vp ∂εpf0

). (3.22)

The first term in the above expression for the current corresponds to the LMC computedin Refs. [25, 67, 68] for n = 1 Weyl semimetals, which becomes the dominant once we takeτinter τintra. The rest of the contributions are associated to the effective relaxation timeτ∗. Notice that the second line coincides with Eqs. (3.14) after setting τ → τ∗. Now weproceed to the computation of LMC with the above two collision integrals.

– 10 –

Page 12: Magnetotransport in multi-Weyl semimetals: A kinetic

4 Magnetotransport in the multi-Weyl system

Previous studies reporting a positive LMC in a simple Weyl semimetal (with n = 1),solely computed the contribution which has a simple connection to the chiral magneticeffect. Here we show that even in the general case with higher monopole charge (withn > 1), the LMC is possitive for both collision integrals. Otherwise, the LMC (σjj) can becomputed from the following definition

σjj =∑s=±

∂Js

∂Ej· j, (4.1)

where j is the unit vector in the jth direction. The electric and magnetic fields are assumedto have the following form E = Ej and B = Bj. We here present the analysis for twodifferent physical scenarios corresponding to the collision integrals [see Eq. (3.3) and (3.15)].

4.1 LMC with single effective relaxation time

A single relaxation time does not distinguish between the processes relaxing the axialand vector currents. As a result LMC receives contributions from both chiral magnetic andOhmic processes. For convenience we split the total conductivity as follows

σjj = 2σ(1)jj;τ + σ

(2)jj;τ + σ

(3)jj;τ , (4.2)

where various components (σ(k)jj ) in the above equation are given by the following integral

expressions

σ(1)jj;τ = τe3B

∑s=±

∫d3p

(2π)3

(vp)j(Ω(s)p · vp)

1 + eB ·Ω(s)p

(−∂f0

∂εp

), (4.3)

σ(2)jj;τ = τe4B2

∑s=±

∫d3p

(2π)3

(Ω(s)p · vp)2

1 + eB ·Ω(s)p

(−∂f0

∂εp

), (4.4)

σ(3)jj;τ = τe2

∑s=±

∫d3p

(2π)3

(vp)2j

1 + eB ·Ω(s)p

(−∂f0

∂εp

). (4.5)

Next we compute the components of σjj for various choices of j (for concreteness we choosej = x, y, z) for arbitrary n (monopole charge of the Weyl node). A generalization of thesimple Weyl-node metal involves a momentum space merging of n simple Weyl points withthe same chirality at a specific point in the momentum space. This situation is qualitativelysimilar to the ones in two-dimensional bilayer (for n = 2) and trilayer (for n = 3) graphene,where respectively the bi-quadratic and bi-cubic touching of the valence and conductionbands can be considered as merging of two and three momentum space vortices. As aresult a defect in the form of double- and triple-vortex is realized in these two systems,respectively [69]. The low energy dispersion can then be characterized by multi-Weyl nodeswith linear dispersion only along one high symmetry direction and nth polynomial dispersion

– 11 –

Page 13: Magnetotransport in multi-Weyl semimetals: A kinetic

along the remaining two directions. For concreteness, the linear dispersion is chosen to bealong the z-direction. We seek to understand how such spectral anisotropy manifest inLMC and, in particular, how does it affect the response from anomalies. In what follows wethus compute the LMC along the z direction and perpendicular to it (in the x− y plane).First we consider the situation where E = Ez and B = Bz. Following the steps highlightedabove (see Appendices C.1 and C.2 for details) we find the various components of LMC[defined in Eqs. (4.3)-(4.5)] to be

σ(1)zz;τ = f1(n) σn0 , σ(2)

zz;τ = f2(n) σn0 , σ(3)zz;τ = f3(n) σnM + f4(n) σn0 , (4.6)

where

f1(n) = −n3Γ

[2− 1

n

]16π3/2Γ

[72 −

1n

] , f2(n) =n3Γ

[2− 1

n

]8π3/2Γ

[52 −

1n

] ,f3(n) =

Γ[1 + 1

n

]4π3/2Γ

[32 + 1

n

] , f4(n) =3n3Γ

[2− 1

n

]32π3/2Γ

[92 −

1n

] , (4.7)

and

σn0 = v

(αnµ

)2/n

τe4B2, σnM = v

(αnµ

)−2/n

τe2 (4.8)

bear the dimensionality of conductivity for any value of n, and respectively they capturethe magnetoductivity and metallic conductivity. The scaling of the functions fj(n)s areshown in Fig. 3(a). In the above expression we kept the terms only up to the order B2.Therefore, the total LMC along the z direction in a multi-Weyl system is given by

σzz = [2f1(n) + f2(n) + f4(n)]σn0 + f3(n)σnM ≡ F (n)σn0 + f3(n)σnM . (4.9)

The scaling of the function F (n) is shown in Fig. 3(b) (blue curve). Finally we alignthe electric and magnetic fields along the x direction. Following the exact same steps weimmediately find

σ(1)xx;τ = f5(n)σn0 , σ(2)

xx;τ = σ(2)zz;τ , σ(3)

xx;τ =τe2nµ2

6π2v+ f6(n)σn0 , (4.10)

where

f5(n) = −n3Γ

[3− 1

n

]16π3/2Γ

[72 −

1n

] , f6(n) =3n3Γ

[4− 1

n

]64π3/2Γ

[92 −

1n

] . (4.11)

Scaling of f5(n) and f6(n) with n is shown in Fig. 3(a) . Hence, the total LMC along thex direction in a multi-Weyl system is given by

σxx = [2f5(n) + f2(n) + f6(n)]σn0 +τe2nµ2

6π2v≡ G(n)σn0 +

τe2nµ2

6π2v. (4.12)

The scaling of the function G(n) is shown in Fig. 3(b) (green curve). Due to an in-planerotational symmetry, σ(i)

xx = σ(i)yy , implying σxx = σyy.

We now discuss the results. Notice that the contribution to the LMC solely arising fromσ

(2)jj;τ , is independent of the choice of j = x, y, z. Such a behaviour unveils the underling

– 12 –

Page 14: Magnetotransport in multi-Weyl semimetals: A kinetic

1 2 3 4 5-0.6

-0.3

0

0.3

0.6

1

2

3

4

5

6

(a)

1 2 3 4 50

0.4

0.8

1.2

F

G

(b)

Figure 3. Scaling of the functions (a) fj(n)s for j = 1, · · · , 6, defined in Eqs. (4.7) and (4.11) and(b) F (n) and G(n), respectively appearing in Eqs. (4.9) and (4.12), with the monopole’s charge n,for n ∈ [1, 5].

topological protection of the chiral anomaly on LMC. However, the rest of the contributionsto the LMC, namely σ(1)

jj;τ and σ(3)jj;τ scales differently along various high symmetry directions.

This should be contrasted with the linear n dependence of the equilibrium chiral magneticconductivity. As a result the total LMC σjj despite being always positive, is directiondependent [compare Eq. (4.9) and Eq. (4.12)]. We also note that for weak enough magneticfield the leading contribution to LMC goes as B2, irrespective of the direction. Otherwise,σjj scales as n3 with the monopole charge of the Weyl nodes.

We would like to make a final remark regarding the positive LMC. This observable isbelieved to be a direct indication of the underling chiral anomaly. However, to the bestof our knowledge there is no solid proof of that statement (directly connecting negativeLMR arising from the Berry curvature with the quantum chiral anomaly computed fromthe triangle diagrams)4 [71–73]. Nonetheless, upon splitting the LMC of the multi-Weylsemimetal in terms of the out-of-equilibrium chiral magnetic and the Ohmic5 conductivities(see Eq. (3.14))

σCMzz =n3Γ

[3− 1

n

]16π3/2Γ

[72 −

1n

]σn0 , σOzz = −n3Γ

(3− 1

n

)32π3/2Γ

(92 −

1n

)σn0 , (4.13)

σCMxx =n2 (3n− 1) Γ

[2− 1

n

]32π3/2Γ

[72 −

1n

] σn0 , σOxx = −(5n− 1)n2Γ

(3− 1

n

)128π3/2Γ

(92 −

1n

) σn0 , (4.14)

we observe that the dominant LMC for arbitrary n is the one related to the chiral magneticconductivity. This supports the idea of a direct relation between positive LMC and thechiral anomaly. in the next section we show that in presence of two distinct time scales itpossible to demonstrate a one-to-one correspondence between LMC and the chiral anomalywhen τinter τintra.

4In Ref. [70] a positive LMC is discused in a context without Weyl nodes.5For comparative reasons we ignore the Drude part in the Ohmic conductivity.

– 13 –

Page 15: Magnetotransport in multi-Weyl semimetals: A kinetic

4.2 LMC with two relaxation times

We now present the expression for magnetotransport when both intervalley and in-travalley scattering times are taken into account. This corresponds to the collision term,shown in Eq. (3.15). In this case the computation reduces to the evaluation of only the firstline of Eq. (3.22) [see Appendix B for details], since the second line identically matcheswith the expression for LMC for the single relaxation time collision integral after changingτ → τ∗. Therefore the LMC for the actual case can be written down as follows

σjj = τintere4n3vΓ(1

2 + 1n)

4π5/2Γ( 1n)

µ

)2/n

B2 (4.15)

− τ∗e4n3vΓ(1

2 + 1n)

2π5/2Γ( 1n)

µ

)2/n

B2 + 2σ(1)jj;τ∗ + σ

(2)jj;τ∗ + σ

(3)jj;τ∗ ,

where σ(1)τ∗ , σ

(2)τ∗ , σ

(3)τ∗ are given by Eqs. (4.6)-(4.11). In this case we see that when τ∗

τinter, corresponding to τinter τintra, we obtain the generalization of the LMC of Ref. [25]for the multi-Weyl case. In this limit, the LMC is purely governed by the chiral anomaly,which is direction independent and thus topological in nature.

5 Conclusions and Discussions

To summarize, we here present a comprehensive analysis of LMC in a three-dimensionalmulti-Weyl semimetal in the semi-classical regime, which can be accessed in experimentsfor sufficiently weak magnetic field, such that ωcτ 1 (thus no Landau quantization).The distribution of the underlying Berry curvature in the momentum space is isotropiconly when n = 1, for which the dispersion of Weyl fermions scales linearly with all threecomponents of momentum. By contrast, due to a natural anisotropy in the Weyl dispersionfor n > 1 [see Fig. 1], the system looses Lorentz covariance and the Berry curvature is nolonger uniformly distributed [see Sec. 2]. In this work we investigate the imprint of the(anisotropic) Berry curvature on LMC in multi-Weyl system.

Throughout we assume the electric and magnetic fields to be parallel to each other.Specifically, we considered two different types of collision integrals corresponding to twodifferent physical scenarios: (a) When both regular and axial charge are relaxed by a singleeffective scattering time (τ) [see Sec. 3.1], and (b) in the presence of both inter-valley andintra-valley scattering processes, respectively characterized by τinter and τintra [see Sec. 3.2and Fig. 2]. In the latter construction only τinter causes the relaxation of the axial charge.

Within the framework of single scattering time approximation, we show that the con-tribution to LMC arising from the chiral anomaly gets mixed with the non-anomalous ones,and they cannot be separated [see Sec. 4.1]. By contrast, these two contributions are sep-arated when we invoke two different time-scales in the collision integrals in the form ofinter-valley (τinter) and intra-valley (τintra) scattering times [see Sec. 4.2]. In particular,when τinter τintra the dominant contribution to LMC arises from chiral anomaly [see

– 14 –

Page 16: Magnetotransport in multi-Weyl semimetals: A kinetic

Eq. (4.15)] and proportional to the inter-valley scattering time τinter. However, irrespectiveof these details we show that the LMC always increases as σjj ∼ B2 for j = x, y, z, andscales as n3 with the monopole charge. While in the single scattering time approximationthe amplitude of σjj is always direction dependent, LMC becomes direction independentin the presence of two scattering times, but only when τinter τintra. In this regime LMCsolely arises from the chiral anomaly, and its direction independence reveals its topologicalorigin. In brief, our work strongly suggests an one-to-one correspondence among the un-derlying Berry curvature of the Weyl medium, the chiral anomaly and the positive LMCin a multi-Weyl system. The proposed topologically robust LMC can be observed in Weylsystems at weak magnetic fields, if back-scattering dominates over the forward one (yield-ing τinter τintra), which can be realized when concentration of Gaussian impurities issufficiently larger than that for Coulomb impurities. We also note that for sufficiently weakmagnetic field the weak anti-localization effect leads to a negative LMC [74]. The interplayof chiral anomaly and weak anti-localization effects and the crossover behaviour betweenthem remains an unresolved issue at this moment.

Finally, we wish to draw a comparison between our conclusions regarding the LMC in amulti-Weyl system in the weak field and the one obtained in a quantum limit (ωcτ 1) [77],when Landau levels are sharply formed (strong magnetic field regime). In the strong fieldlimit it has been demonstrated that positive LMC scales linearly with the monopole charge(n) and magnetic field (B), as long as it is applied along the z direction (separating two Weylnodes). The linear-dependence of positive LMC on n comes from the fact that the zerothLandau level in a multi-Weyl semimetal possesses an exact and topologically protected n-fold degeneracy [78]. In a simple Weyl semimetal (n = 1) such a linear dependence on theB-field is insensitive to its direction. However, for n = 2 and 3 as one tilts the field awayfrom the z direction the LMC (still positive) starts to develop a non-linear dependence onthe B-field, and most likely scales as B2 when the field is aligned in the x−y plane. Such astark distinct crossover behaviour of LMT from semi-classical to quantum regime (accessedby systematically increasing the strength of the magnetic field or strength of impurityscattering) along various direction of a multi-Weyl system is extremely fascinating, whichcan also be observed in real materials by tilting the magnetic field away from high symmetrydirections.

Acknowledgments

B. R. is thankful to Nordita for hospitality. P. S. is supported by the Deutsche Forschungs-gemeinschaft via the Leibniz Programme. We thank Dam Thanh Son for discussions.

A Computation of Berry Curvature

In this appendix we elaborate on the computation of the integer topological invariantof generalized Weyl semimetals. To proceed with the analysis we exploit the azimuthalsymmetry of the system for n > 1. First, we express the Berry curvature in cylindrical

– 15 –

Page 17: Magnetotransport in multi-Weyl semimetals: A kinetic

A = (0, 0, Pz)

B = (0, 0,−Pz)

C = (P⊥, 0,−Pz)

A

B

O

C

Figure 4. Illustration of the chosen surface for the computation of flux of the Berry curvature ina multi-Weyl semimetal (see Appendix A). The Weyl monopole is placed at O.

coordinates according to

Ωp =nα2

nvp2n−1⊥

2(α2np

2n⊥ + v2p2

z)3/2

(ep⊥ + npzp−1⊥ epz). (A.1)

Then, choosing the surface Σ to be a cylinder centred around the monopole (see Fig. 4),we obtain

∮Σ

Ωp · dS =

∫ΣS

Ωp · dSS +

∫ΣT

Ωp · dST +

∫ΣB

Ωp · dSB

=

∫ Pz

−Pz

πnα2nvP

2n⊥[

α2nP

2n⊥ + v2p2

z

]3/2dpz + 2

∫ P⊥

0

πn2α2nvp

2n−1⊥ Pz

[α2np

2n + v2P 2z ]3/2

dp⊥ = 2πn. (A.2)

Note that ΣS , ΣT and ΣB respectively represents the side (S), top (T ) and bottom (B)surfaces of the cylinder.

B Calculation of magnetoconductance with two relaxation times

In this Appendix, we display details of the computation of LMC in the presence of twoscattering time in the collision integral [see Eq. (3.15)]. We begin with the kinetic equation

∂tf(s) + x(s) · ∂xf (s) + p(s) · ∂pf (s) =

f (s) − f (s)

τ∗+f (s) − f (s)

τinter(B.1)

≡ f (s) − f (s)

τ∗+ Λ(s), (B.2)

– 16 –

Page 18: Magnetotransport in multi-Weyl semimetals: A kinetic

where f (s) =⟨(

1 + eB ·Ω(s))f (s)

⟩. The angular brackets stand for a generalized average

over the angles, to be specified below.Given the symmetry of the system, we work with the coordinate system in which the

radial component corresponds to the energy dispersion relation

εp =√α2(p2

x + p2y)n + v2p2

z, (B.3)

defined by

px =

(εp

sin θ

α

)1/n

cosφ, py =

(εp

sin θ

α

)1/n

sinφ, pz = εpcos θ

v. (B.4)

In this coordinate system, the group velocity and the Berry curvature take the simple form

vp =1

h1εp, Ωp =

n2vα2

2ε2

(ε sin θ

α

)2(n−1)/n

h1εp, (B.5)

where h1 =

√cos2 θv2

+ 1n2ε2p

(εp sin θα

)2/n. Finally, the above mentioned average of a quantity

g over the angles is defined as follows

〈g〉 =Γ(1

2 + 1n)

2π3/2 Γ( 1n)

∫dφdθ (sin θ)2/n−1 g. (B.6)

To compute the explicit form of Λ(s) for static and homogeneous solutions we angle-average the kinetic equation after multiplying it by the phase space measure, yielding

⟨(1 + eB ·Ω(s)

p

)p(s) · ∂pf (s)

⟩=

⟨(1 + eB ·Ω(s)

p

)( f (s) − f (s)

τ∗+ Λ(s)

)⟩. (B.7)

Since⟨(

1 + eB ·Ω(s)p

)⟩= 1, we find

Λ(s) =⟨(

1 + eB ·Ω(s)p

)p(s) · ∂pf (s)

⟩. (B.8)

Using the equations of motion, we obtain the following simplified expression for Λ(s) withinthe linear response

Λ(s) =⟨(eE · v + e2 (E ·B) Ω

(s)p · vp

)⟩∂εpf0

= se2 (E ·B)n2v( εα

)−2/n Γ(12 + 1

n)

π1/2 Γ( 1n)∂εpf0, (B.9)

where f0 =[1 + eβ(εp−µ)

]−1, and µ is the equilibrium chemical potential. The solution ofthe kinetic equation (in linear response) is given by

f (s) = f (s) + τ∗(

Λ(s) − p(s) · vp ∂εpf0

). (B.10)

– 17 –

Page 19: Magnetotransport in multi-Weyl semimetals: A kinetic

The current is defined as 6

J(s) = e

∫d3p

(2π)3

(1 + eB ·Ω(s)

p

)x(s)f (s) (B.11)

= e

∫d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B]f (s)

+ eτ∗∫

d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (

Λ(s) − p(s) · vp ∂εpf0

)= e

∫d3p

(2π)3

[e(vp ·Ω(s)

p

)B] (f (s) + τ∗Λ(s)

)+ eτ∗

∫d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (−p(s) · vp ∂εpf0

). (B.12)

For a pair of nodes the vector current can be computed yielding

J = e∑s=±

∫d3p

(2π)3

(1 + eB ·Ω(s)

p

)x(s)f (s)

= e

∫d3p

(2π)3e (vp ·Ωp) B

[sf (s) + sf (s) + τ∗

(sΛ(s) + sΛ(s)

)]+ eτ∗

∑s=±

∫d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (−p(s) · vp ∂εpf0

)= e

∫d3p

(2π)3e (vp ·Ωp) B

[τinterΛ

(−) − 2τ∗Λ(−)]

+ eτ∗∑s=±

∫d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (−p(s) · vp ∂εpf0

). (B.13)

Note that

eτinter

∫d3p

(2π)3[e (vp ·Ωp) B] Λ(−) =

e4τintern3vΓ(1

2 + 1n)

4π5/2Γ( 1n)

µ

)2/n

(E ·B) B, (B.14)

eτ∗∫

d3p

(2π)3

[vp + e

(vp ·Ω(s)

p

)B] (−p(s) · vp ∂εpf0

)= Jb, (B.15)

where Jb has the same structure than the vector current computed for C1

[f (s)

]but it is

now proportional to τ∗. Therefore, the total LMC (in the presence of two scattering times)for a pair of Weyl nodes is given by Eq. (4.15).

C Computation of magnetoconductivity

We now present some essential details of the computation of LMC for multi-Weylsemimetal (with n > 1) that appear in both single and two relaxation time approximations,namely σ(k)

jj,τ for k = 1, 2, 3 and j = x, y, z. Finally, we also justify the power series expansionin powers of B for the calculation of the LMC.

6Note that we here ignore the term responsible for the Hall current.

– 18 –

Page 20: Magnetotransport in multi-Weyl semimetals: A kinetic

C.1 Multi-Weyl semimetal

The aim of this section is to illustrate how we obtain the results quoted in Eqs. (4.6)-(4.12). We present the full computation for one of the terms, as the remaining ones can beevaluated in a similar way. Let us focus on σ(1)

zz,τ which can be written as

σ(1)zz,τ =

τe3B

(2π)2

∑s=±

s

∫ ∞0

dp⊥

∫ ∞−∞

dpz(n2α2

nv3)p2n+1⊥ pz δ(µ−

√α2np

2n⊥ + v2p2

z)

2p2⊥(α2

np2n⊥ + v2p2

z)3/2 + vn2α2

n(seB)p2n⊥ pz

.

Now we perform the variable substitution pz → pz/v and p⊥ → p⊥α−1/nn , yielding

σ(1)zz,τ =

τe3B

(2π)2

∑s=±

s

∫ ∞0

dp⊥

∫ ∞−∞

dpz(n2α

−2/nn v)p2n+1

⊥ pz δ(µ−√p2n⊥ + p2

z)

2α−2/nn p2

⊥(p2n⊥ + p2

z)3/2 + n2(seB)p2n

⊥ pz.

Next, we take p⊥ = p1/n⊥ . For brevity we drop the tildes and find

σ(1)zz,τ =

τe3B

(2π)2

∑s=±

s

∫ ∞0

dp⊥

∫ ∞−∞

dpz(nα

−2/nn v)p⊥pz δ(µ−

√p2⊥ + p2

z)

2α−2/nn (p2

⊥ + p2z)

3/2 + n2(seB)p2(n−1)/n⊥ pz

.

At last, performing the transformation p⊥ = R sin θ and pz = R cos θ, we obtain

σ(1)zz,τ =

τe3B(nα−2/nn v)

(2π)2

∑s=±

s

∫ π

0dθ

∫ ∞0

dRR3 sin θ cos θ δ(µ−R)

2α−2/nn R3 + (seB)n2(R cos θ)(R sin θ)2(n−1)/n

=τe3B(nv)

2(2π)2

∑s=±

s

∫ π

0dθ

sin θ cos θ

1 + ( seB2µ2

)n2α2/nn cos θ(µ sin θ)2(n−1)/n

. (C.1)

The previous coordinates transformations amount to going from the Cartesian coordinatesto the ones introduced in Eq. (B.4). Performing the same steps, it is straight forward toshow that

σ(2)zz,τ =

τe4B2(n3α2/nn v)

4(2π)2µ2

∑s=±

∫ π

0dθ

sin θ(µ sin θ)2(n−1)/n

1 +(seB2µ2

)n2α

2/nn cos θ(µ sin θ)2(n−1)/n

,

σ(3)zz,τ =

τe2vµ

(2π)2nα2/nn

∑s=±

∫ π

0dθ

cos2 θ(µ sin θ)2/n−1

1 +(seB2µ2

)n2α

2/nn cos θ(µ sin θ)2(n−1)/n

,

σ(1)xx,τ =

τe3B(n2α1/nn )

2(2π)3µ2

∑s=±

s

∫ 2π

0dφ

∫ π

0dθ

(µ sin θ)3−1/n cosφ

1 +(seB2µ3

)nvα

1/nn (µ sin θ)2−1/n cosφ

,

σ(2)xx,τ =

τe4B2(n3α2/nn v)

4(2π)3µ3

∑s=±

∫ 2π

0dφ

∫ π

0dθ

(µ sin θ)3−2/n

1 +(seB2µ3

)nvα

1/nn (µ sin θ)2−1/n cosφ

,

σ(3)xx,τ =

τe2nµ2

(2π)3v

∑s=±

∫ 2π

0dφ

∫ π

0dθ

sin3 θ cos2 φ

1 +(seB2µ3

)nvα

1/nn (µ sin θ)2−1/n cosφ

. (C.2)

To compute these integrals, next we need to perform a series expansion of the integrandsin powers of eB/2µ2 (see Appendix C.2).

– 19 –

Page 21: Magnetotransport in multi-Weyl semimetals: A kinetic

C.2 Power Series Expansion

0 2 4 6 8 100

5

10

15

20

ρ(n)

Figure 5. Scaling of ρ(n) [defined in Eq. (C.7)] with the monopole number n of generalized Weylfermions.

We seek to perform the integrals from Eqs. (C.1) and (C.2). As before, let us focuson σ(1)

zz,τ . To compute σ(1)zz,τ , we make use of the power series expansion

1

1 + ε=∞∑i=0

(−1)iεi, (C.3)

which allows us to write

σ(1)zz,τ =

τe3B(nv)

2(2π)2

∑s=±

s

∫ π

0dθ

∞∑i=0

sin θ cos θ(−1)i[(

seB

2µ2

)n2α2/n

n cos θ(µ sin θ)2(n−1)/n

]i.

(C.4)

To proceed further we need to interchange the integral with the sum sign. A sufficientcondition is

∑n

∫dx|fn(x)| < ∞, or equivalently,

∫dx∑

n |fn(x)| < ∞. Let us prove theformer condition. First of all, note that

∫ π

0dθ

∣∣∣∣∣∣(−1)i

[(eB

2

)n2

(αnµ

)2/n

cos θ(sin θ)2(n−1)/n

]isin θ cos θ

∣∣∣∣∣∣=

(eB)in2i(αnn

)2i/nΓ[1 + i

2

]Γ[1 + i− i

n

]2iΓ

[2 + i

(32 −

1n

)] . (C.5)

Next we compute the ratio

r = limi→∞

∣∣∣∣ai+1

ai

∣∣∣∣ = limi→∞

∣∣∣∣ eB2µ2

∣∣∣∣∣∣∣∣∣ α2/n

n

µ2/n−2

∣∣∣∣∣∣∣∣∣∣ n2Γ

[3+i

2

]Γ[2 + i− 1+i

n

]Γ[2 + i

(32 −

1n

)]2Γ[1 + i

2

]Γ[1 + i− i

n

]Γ[2 + (1 + i)

(32 −

1n

)]∣∣∣∣∣

– 20 –

Page 22: Magnetotransport in multi-Weyl semimetals: A kinetic

=

∣∣∣∣ eB2µ2

∣∣∣∣∣∣∣∣∣ α2/n

n

µ2/n−2

∣∣∣∣∣ limi→∞

ρi(n). (C.6)

Specifically, for integer n bigger or equal to 1, we have

ρ(n) = limi→∞

ρi(n) = n(n− 1)(n−1)/n

(3n

2− 1

)1/n( n

3n− 2

)3/2

. (C.7)

We can now study ρ(n) as a function of n (see Fig. 5). For the series to converge r < 1.With no loss of generality, we can assume αn/µ to be a positive finite number. Thus, for

finite n, we can always find the regime where∣∣∣ eB2µ2

∣∣∣ < (∣∣∣ α2/nn

µ2/n−2

∣∣∣ ρ(n))−1

, making the seriesconvergent.

It can be shown for all the other terms that we can choose eB/2µ2 to be small inorder for the series to be convergent. Therefore, we can compute the desired integrals byexpanding the integrands in powers of eB/2µ2. Keeping only the terms up to quadraticorder in the magnetic field, we arrive at the results quoted in Eqs. (4.6)-(4.12).

References

[1] A. Vilenkin, Macroscopic parity-violating effects: Neutrino fluxes from rotating black holesand in rotating thermal radiation, Phys. Rev. D 20 (1979) 1807.

[2] A. Vilenkin, Equilibrium parity-violating current in a magnetic field, Phys. Rev. D 22 (1980)3080.

[3] K. Fukushima, D. E. Kharzeev and H. J. Warringa, Chiral magnetic effect, Phys. Rev. D 78(2008) 074033.

[4] J. Erdmenger, M. Haack, M. Kaminski and A. Yarom, Fluid dynamics of R-charged blackholes, JHEP 01 (2009) 055, [0809.2488].

[5] N. Banerjee, J. Bhattacharya, S. Bhattacharyya, S. Dutta, R. Loganayagam and P. Surówka,Hydrodynamics from charged black branes, JHEP 01 (2011) 094, [0809.2596].

[6] D. T. Son and P. Surówka, Hydrodynamics with Triangle Anomalies, Phys. Rev. Lett. 103(2009) 191601, [0906.5044].

[7] K. Landsteiner, E. Megias and F. Pena-Benitez, Gravitational Anomaly and Transport, Phys.Rev. Lett. 107 (2011) 021601, [1103.5006].

[8] R. A. Bertlmann, Anomalies in Quantum Field Theory. International Series of Monographson Physics. Clarendon Press, 2001.

[9] K. Fujikawa and H. Suzuki, Path Integrals and Quantum Anomalies. International Series ofMonographs on Physics. Clarendon Press, 2004.

[10] S. L. Adler, Axial-vector vertex in spinor electrodynamics, Phys. Rev. 177 (1969) 2426.

[11] J. S. Bell and R. Jackiw, A PCAC puzzle: π0 → γ γ in the sigma model, Nuovo Cim. A60(1969) 47.

[12] R. Delbourgo and A. Salam, The gravitational correction to PCAC, Physics Letters B 40(1972) 381.

– 21 –

Page 23: Magnetotransport in multi-Weyl semimetals: A kinetic

[13] A. Lucas, R. A. Davison and S. Sachdev, Hydrodynamic theory of thermoelectric transportand negative magnetoresistance in Weyl semimetals, Proc. Nat. Acad. Sci. 113 (2016) 9463,[1604.08598].

[14] K. Landsteiner, Y. Liu and Y.-W. Sun, Odd viscosity in the quantum critical region of aholographic Weyl semimetal, Phys. Rev. Lett. 117 (2016) 081604, [1604.01346].

[15] J. Gooth et al., Experimental signatures of the mixed axial-gravitational anomaly in the Weylsemimetal NbP, Nature 547 (2017) 324, [1703.10682].

[16] J. Liao, Chiral Magnetic Effect in Heavy Ion Collisions, Nucl. Phys. A956 (2016) 99,[1601.00381].

[17] N. P. Armitage, E. J. Mele and A. Vishwanath, Weyl and dirac semimetals inthree-dimensional solids, Rev. Mod. Phys. 90 (2018) 015001.

[18] H. B. Nielsen and M. Ninomiya, No Go Theorem for Regularizing Chiral Fermions, Phys.Lett. 105B (1981) 219.

[19] K. Landsteiner, Anomalous transport of Weyl fermions in Weyl semimetals, Phys. Rev. B89(2014) 075124, [1306.4932].

[20] G. Basar, D. E. Kharzeev and H.-U. Yee, Triangle anomaly in Weyl semimetals, Phys. Rev.B89 (2014) 035142, [1305.6338].

[21] M. M. Vazifeh and M. Franz, Electromagnetic response of weyl semimetals, Phys. Rev. Lett.111 (Jul, 2013) 027201.

[22] H. Nielsen and M. Ninomiya, The adler-bell-jackiw anomaly and weyl fermions in a crystal,Physics Letters B 130 (1983) 389.

[23] D. T. Son and N. Yamamoto, Berry Curvature, Triangle Anomalies, and the Chiral MagneticEffect in Fermi Liquids, Phys. Rev. Lett. 109 (2012) 181602, [1203.2697].

[24] T. Hayata, Y. Kikuchi and Y. Tanizaki, Topological properties of the chiral magnetic effect inmulti-weyl semimetals, Phys. Rev. B 96 (Aug, 2017) 085112.

[25] D. T. Son and B. Z. Spivak, Chiral anomaly and classical negative magnetoresistance of weylmetals, Phys. Rev. B 88 (2013) 104412.

[26] T. Osada, Negative interlayer magnetoresistance and zero-mode landau level in multilayerdirac electron systems, Journal of the Physical Society of Japan 77 (2008) 084711.

[27] A. G. Grushin, Consequences of a condensed matter realization of Lorentz-violating QED inWeyl semi-metals, Phys. Rev. D 86 (2012) 045001.

[28] V. Aji, Adler-bell-jackiw anomaly in weyl semimetals: Application to pyrochlore iridates,Phys. Rev. B 85 (2012) 241101.

[29] A. A. Zyuzin and A. A. Burkov, Topological response in weyl semimetals and the chiralanomaly, Phys. Rev. B 86 (2012) 115133.

[30] P. Goswami and S. Tewari, Axionic field theory of (3 + 1)-dimensional weyl semimetals,Phys. Rev. B 88 (2013) 245107.

[31] M. M. Vazifeh and M. Franz, Electromagnetic response of weyl semimetals, Phys. Rev. Lett.111 (2013) 027201.

[32] E. V. Gorbar, V. A. Miransky and I. A. Shovkovy, Chiral anomaly, dimensional reduction,and magnetoresistivity of weyl and dirac semimetals, Phys. Rev. B 89 (2014) 085126.

– 22 –

Page 24: Magnetotransport in multi-Weyl semimetals: A kinetic

[33] D. A. Pesin, E. G. Mishchenko and A. Levchenko, Density of states and magnetotransport inweyl semimetals with long-range disorder, Phys. Rev. B 92 (2015) 174202.

[34] A. Jimenez-Alba, K. Landsteiner, Y. Liu and Y.-W. Sun, Anomalous magnetoconductivityand relaxation times in holography, JHEP 07 (2015) 117.

[35] V. A. Zyuzin, Magnetotransport of weyl semimetals due to the chiral anomaly, Phys. Rev. B95 (2017) 245128.

[36] X. Huang, L. Zhao, Y. Long, P. Wang, D. Chen, Z. Yang et al., Observation of thechiral-anomaly-induced negative magnetoresistance in 3d weyl semimetal taas, Phys. Rev. X5 (2015) 031023.

[37] Y.-Y. Wang, Q.-H. Yu, P.-J. Guo, K. Liu and T.-L. Xia, Resistivity plateau and extremelylarge magnetoresistance in NbAs2 and TaAs2, Phys. Rev. B 94 (2016) 041103.

[38] G. Zheng, J. Lu, X. Zhu, W. Ning, Y. Han, H. Zhang et al., Transport evidence for thethree-dimensional dirac semimetal phase in ZrTe5, Phys. Rev. B 93 (2016) 115414.

[39] C.-L. Zhang, S.-Y. Xu, I. Belopolski, Z. Yuan, Z. Lin, B. Tong et al., Signatures of theAdler–Bell–Jackiw chiral anomaly in a Weyl fermion semimetal, Nature Communications 7(2016) 10735.

[40] Q. Li, D. E. Kharzeev, C. Zhang, Y. Huang, I. Pletikosić, A. V. Fedorov et al., Chiralmagnetic effect in ZrTe5, Nature Physics 12 (02, 2016) 550.

[41] G. Xu, H. Weng, Z. Wang, X. Dai and Z. Fang, Chern semimetal and the quantizedanomalous hall effect in HgCr2Se4, Phys. Rev. Lett. 107 (2011) 186806.

[42] C. Fang, M. J. Gilbert, X. Dai and B. A. Bernevig, Multi-weyl topological semimetalsstabilized by point group symmetry, Phys. Rev. Lett. 108 (2012) 266802.

[43] S.-M. Huang, S.-Y. Xu, I. Belopolski, C.-C. Lee, G. Chang, T.-R. Chang et al., New type ofweyl semimetal with quadratic double weyl fermions, Proc. Nat. Acad. Sci. 113 (2016) 1180,[http://www.pnas.org/content/113/5/1180.full.pdf].

[44] B.-J. Yang and N. Nagaosa, Classification of stable three-dimensional dirac semimetals withnontrivial topology, Nature Communications 5 (2014) 4898.

[45] M. Z. Hasan, S.-Y. Xu, I. Belopolski and S.-M. Huang, Discovery of weyl fermion semimetalsand topological fermi arc states, Annual Review of Condensed Matter Physics 8 (2017) 289,[https://doi.org/10.1146/annurev-conmatphys-031016-025225].

[46] B. Yan and C. Felser, Topological materials: Weyl semimetals, Annual Review of CondensedMatter Physics 8 (2017) 337,[https://doi.org/10.1146/annurev-conmatphys-031016-025458].

[47] Q. Liu and A. Zunger, Predicted realization of cubic dirac fermion in quasi-one-dimensionaltransition-metal monochalcogenides, Phys. Rev. X 7 (2017) 021019.

[48] G. E. Volovik, The Universe in a Helium Droplet. International Series of Monographs onPhysics. Clarendon Press, 2003.

[49] P. Goswami and L. Balicas, Topological properties of possible Weyl superconducting states ofURu2Si2, ArXiv e-prints (2013) , [1312.3632].

[50] P. Goswami and A. H. Nevidomskyy, Topological weyl superconductor to diffusive thermalhall metal crossover in the B phase of UPt3, Phys. Rev. B 92 (2015) 214504.

– 23 –

Page 25: Magnetotransport in multi-Weyl semimetals: A kinetic

[51] M. H. Fischer, T. Neupert, C. Platt, A. P. Schnyder, W. Hanke, J. Goryo et al., Chirald-wave superconductivity in SrPtAs, Phys. Rev. B 89 (2014) 020509.

[52] B. Roy, S. A. A. Ghorashi, M. S. Foster and A. H. Nevidomskyy, Topologicalsuperconductivity of spin-3/2 carriers in a three-dimensional doped Luttinger semimetal,ArXiv e-prints (2017) , [1708.07825].

[53] M. Stephanov, H.-U. Yee and Y. Yin, Collective modes of chiral kinetic theory in a magneticfield, Phys. Rev. D 91 (Jun, 2015) 125014.

[54] P. N. Argyres and E. N. Adams, Longitudinal magnetoresistance in the quantum limit, Phys.Rev. 104 (1956) 900.

[55] S. Bera, J. D. Sau and B. Roy, Dirty weyl semimetals: Stability, phase transition, andquantum criticality, Phys. Rev. B 93 (2016) 201302.

[56] B. Roy, P. Goswami and V. Juričić, Interacting weyl fermions: Phases, phase transitions,and global phase diagram, Phys. Rev. B 95 (2017) 201102.

[57] G. Sundaram and Q. Niu, Wave-packet dynamics in slowly perturbed crystals: Gradientcorrections and berry-phase effects, Phys. Rev. B 59 (1999) 14915.

[58] D. Xiao, M.-C. Chang and Q. Niu, Berry phase effects on electronic properties, Rev. Mod.Phys. 82 (Jul, 2010) 1959–2007.

[59] E. V. Gorbar, I. A. Shovkovy, S. Vilchinskii, I. Rudenok, A. Boyarsky and O. Ruchayskiy,Anomalous maxwell equations for inhomogeneous chiral plasma, Phys. Rev. D 93 (May,2016) 105028.

[60] E. V. Gorbar, D. O. Rybalka and I. A. Shovkovy, Second-order dissipative hydrodynamics forplasma with chiral asymmetry and vorticity, Phys. Rev. D95 (2017) 096010, [1702.07791].

[61] Y. Hidaka, S. Pu and D.-L. Yang, Nonlinear Responses of Chiral Fluids from Kinetic Theory,Phys. Rev. D97 (2018) 016004, [1710.00278].

[62] D. O. Rybalka, E. V. Gorbar and I. A. Shovkovy, Hydrodynamic modes in magnetized chiralplasma with vorticity, 1807.07608.

[63] R. Soto, Kinetic Theory and Transport Phenomena. Oxford Master Series in Physics. OxfordUniversity Press, 2016.

[64] C. Duval, Z. Horvath, P. A. Horvathy, L. Martina and P. Stichel, Berry phase correction toelectron density in solids and ’exotic’ dynamics, Mod. Phys. Lett. B20 (2006) 373,[cond-mat/0506051].

[65] R. Loganayagam and P. Surówka, Anomaly/Transport in an Ideal Weyl gas, JHEP 04 (2012)097.

[66] M. A. Stephanov and Y. Yin, Chiral kinetic theory, Phys. Rev. Lett. 109 (2012) 162001.

[67] B. Z. Spivak and A. V. Andreev, Magnetotransport phenomena related to the chiral anomalyin weyl semimetals, Phys. Rev. B 93 (2016) 085107.

[68] A. A. Burkov, Chiral anomaly and diffusive magnetotransport in weyl metals, Phys. Rev.Lett. 113 (2014) 247203.

[69] A. H. Castro Neto, F. Guinea, N. M. R. Peres, K. S. Novoselov and A. K. Geim, Theelectronic properties of graphene, Rev. Mod. Phys. 81 (Jan, 2009) 109–162.

– 24 –

Page 26: Magnetotransport in multi-Weyl semimetals: A kinetic

[70] X. Dai, Z. Z. Du and H.-Z. Lu, Negative magnetoresistance without chiral anomaly intopological insulators, Phys. Rev. Lett. 119 (2017) 166601.

[71] K. Fujikawa, Quantum anomaly and geometric phase: Their basic differences, Phys. Rev. D73 (2006) 025017.

[72] N. Mueller and R. Venugopalan, Chiral anomaly, berry phase, and chiral kinetic theory fromworldlines in quantum field theory, Phys. Rev. D 97 (2018) 051901.

[73] K. Fujikawa, Characteristics of chiral anomaly in view of various applications, Phys. Rev. D97 (2018) 016018.

[74] G. Bergmann, Weak localization in thin films: a time-of-flight experiment with conductionelectrons, Physics Reports 107 (1984) 1.

[75] D. T. Son and N. Yamamoto, Kinetic theory with Berry curvature from quantum fieldtheories, Phys. Rev. D87 (2013) 085016, [1210.8158].

[76] J.-Y. Chen, D. T. Son, M. A. Stephanov, H.-U. Yee and Y. Yin, Lorentz Invariance in ChiralKinetic Theory, Phys. Rev. Lett. 113 (2014) 182302, [1404.5963].

[77] X. Li, B. Roy and S. Das Sarma, Weyl fermions with arbitrary monopoles in magnetic fields:Landau levels, longitudinal magnetotransport, and density-wave ordering, Phys. Rev. B 94(2016) 195144.

[78] B. Roy and J. D. Sau, Magnetic catalysis and axionic charge density wave in weylsemimetals, Phys. Rev. B 92 (2015) 125141.

– 25 –