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LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and Relocation by J.T. Maki and J.E. Meyer Energy Laboratory Report No: MIT-EL 78-038 October, 1978

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Page 1: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

LWR FUEL PERFORMANCE ANALYSISFuel Cracking and Relocation

byJ.T. Maki and J.E. Meyer

Energy Laboratory Report No: MIT-EL 78-038

October, 1978

Page 2: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 3: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

LWR FUEL PERFORMANCE ANALYSIS

Fuel Cracking and Relocation

by

J.T. Maki and J.E. Meyer

Energy Laboratoryand

Department of Nuclear Engineering

Massachusetts Institute of TechnologyCambridge, Massachusetts 02139

Final Report for Research Project

sponsored by

Northeast Utilities Service Co.Yankee Atomic Electric Co.

under theMIT Energy Laboratory Electric Utility Program

Energy Laboratory Report No. MIT-EL 78-038

October, 1978

Page 4: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
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i

TABLE OF CONTENTS

Topic Page

List of Figures iii

SUMMARY I

1. INTRODUCTION 3

1.1 Objective 31.2 Cracking Scenario 31.3 Crack Patterns 31.4 Major Thermal Effects of Cracking 41.5 Effects of Cracking on Fission Gas Release 4

1.6 Major Mechanical Effects of Cracking 51.7 Crack Healing 6

2. THERMAL CALCULATIONS NOT DEPENDENT ON CRACKING 72.1 Outline of Computer Calculations 72.2 Cladding Temperature Profile 72.3 Cladding Thermal Strain 92.4 Cladding Stored Heat 102.5 Fuel Thermal Strain 112.6 Fuel Stored Heat 112.7 Fuel Rod Equivalent Temperature 12

3. THERMAL CALCULATIONS FOR UNCRACKED FUEL PELLETS 153.1 Pellet Surface Temperature and Gap Conductance 153.2 Pellet Temperature Profile 15

4. THERMAL CALCULATIONS FOR CRACKED FUEL PELLETS 194.1 Pellet Surface Temperature and Gap Conductance 194.2 Pellet Temperature Profile 20

5. ILLUSTRATIVE EXAMPLE 25

5.1 Fuel Pellet Surface Temperature 255.2 Fuel Pellet Centerline Temperature 275.3 Fuel Rod Equivalent Temperature 295.4 Fractional Radius for Grain Growth 295.5 Gap Closure 325.6 Pellet - Clad Contact 32

6. EXPERIMENTAL EVALUATION 37

7. CONCLUSIONS 39

7.1 Relocation Into Gap 39

7.2 Reduced Fuel Thermal Conductivity 397.3 Fuel Rod Equivalent Temperature 397.4 Crack Healing 40

Page 6: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

ii

Topic

APPENDIX A

APPENDIX B

APPENDIX C

APPENDIX D

APPENDIX E

APPENDIX F

Additional Figures from Fuel Pellet ThermalCalculations

Material PropertiesB.1 Fuel Thermal ConductivityB.2 Fuel Thermal StrainB.3 Fuel Specific Heat CapacityB.4 Enthalpy Change for FuelB.5 Cladding Thermal ConductivityB.6 Cladding Thermal StrainB.7 Cladding Specific Heat and EnthalpyB.8 Thermal Conductivity of Fill Gas

Input ParametersC.1 General Design ParametersC.2 Outside Cladding Temperature

Halden Fuel Rod Parameters

Computer Program Listing

Table of Symbols

REFERENCES

Page

41

53

53

59

59

62

64

64

66

71

73

73

73

87

89

107

111

Page 7: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

iii

LIST OF FIGURES

Fig. 2-1 Flow chart for comparative study computerprogram.

Fig. 4-1 Comparison of circumferential pellet-cladcontact models.

Fig. 5-1 Comparison of cracked/uncracked fuel pelletsurface temperature (cold radial gap width =95 m).

Fig. 5-2 Comparison of cracked/uncracked fuel pelletcenterline temperature (cold radial gapwidth = 95 pm).

Fig. 5-3 Comparison of cracked/uncracked fuel rodequivalent temperature (cold radial gapwidth = 95 um).

Fig. 5-4 Comparison of cracked/uncracked fuel pelletfractional radius for the onset of graingrowth (cold radial gap width = 95 m).

Fig. 5-5 Comparison of cracked/uncracked fuel gapclosure (cold radial gap width = 95 m).

Fig. 5-6 Circumferential pellet-cladding contactbehavior for cracked fuel pellets.

Fig. 6-1 Comparison of computational models toHalden experimental fuel rod data (experi-mental data from Ref. 11).

Fig. A-1 Comparison of cracked/uncracked fuel pelletsurface temperature (cold radial gapwidth = 75 m).

Fig. A-2 Comparison of cracked/uncracked fuel pelletsurface temperature (cold radial gapwidth = 115 m).

Fig. A-3 Comparison of cracked/uncracked fuel pelletcenterline temperature (cold radial gapwidth = 75 m).

Fig. A-4 Comparison of cracked/uncracked fuel pelletcenterline temperature (cold radial gapwidth = 115 m).

Fig. A-5 Comparison of cracked/uncracked fuel rodequivalent temperature (cold radial gapwidth = 75 m).

Page 8: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

iv

Fig. A-6 Comparison of cracked/uncracked fuel rodequivalent temperature (cold radial gapwidth = 115 m).

Fig. A-7 Comparison of cracked/uncracked fuel pelletfractional radius for the onset of graingrowth (cold radial gap width = 75 pm).

Fig. A-8 Comparison of cracked/uncracked fuel pelletfractional radius for the onset of graingrowth (cold radial gap width = 115 pm).

Fig. A-9 Comparison of cracked/uncracked fuel gapclosure (cold radial gap width = 75 pm.

Fig. A-10 Comparison of cracked/uncracked fuel gapclosure (cold radial gap width = 115 m).

Fig. B-1 Comparison of EPRI and MATPRO UO2 thermalconducitivity.

Fig. B-2 Comparison of EPRI and MATPRO porosity factors.

Fig. B-3 Comparison of EPRI and MATPRO conductivityintegrals.

Fig. B-4 MATPRO's version of thermal strain foruranium dioxide.

Fig. B-5 MATPRO's version of specific heat capacityfor uranium dioxide.

Fig. B-6 Enthalpy change correlation for uranium dioxide.

Fig. B-7 Comparison of MATPRO and CENPD thermalconductivity for Zircaloy-4.

Fig. B-8 MATPRO's version of thermal strain forZircaloy-4.

Fig. B-9 MATPRO's version of specific heat capacityfor Zircaloy-4.

Fig. B-10 Enthalpy change correlation for Zircaloy-4.

Fig. B-ll MATPRO's version of thermal conductivityfor helium.

Fig. C-1 Correlation for the enthalpy change ofwater at 15 MPa pressure.

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v

Fig. C-2 Behavior of H 0 coolant at a system

pressure of 1 MPa.

Fig. C-3 Behavior of nominal fuel rod at 100% corepower.

Fig. C-4 Behavior of hot fuel rod at 100% core power

Fig. C-5 Comparison of nominal fuel rod outsidecladding temperature to modeled outsidecladding temperature correlation.

Fig. C-6 Comparison of hot fuel rod outside claddingtemperature to modeled outside claddingtemperature correlation.

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SUMMARY

It is expected that virtually all fuel pellets in a pressurized

water reactor (PWR) are cracked during power operation. This report

provides quantitative estimates of the thermal effects of cracking for

a case of interest (relatively new fuel in the Maine Yankee Reactor).

The method to account for cracking has been previously developed by

others.

Results show that it is important to account for cracking. The

equivalent temperature that represents heat stored in a fuel rod oper-

ating at 40 kW/m is 892°C for the cracked pellet versus 1016°C for a

no-crack calculation, a decrease of 124 K.

Methods used in this study were designed to isolate cracking as a

single effect for a representative case. The method used for obtaining

fuel rod outside surface temperature as a function of linear heat gen-

eration rate for this representative case is felt to be especially

suited for use in this and other isolated effect studies.

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1. INTRODUCTION

1.1 Objective

During normal power changes in light water reactors, thermal

stresses within the fuel rod cause the uranium dioxide fuel pellets

to crack. Associated with cracking is relocation, defined as the

geometry changes of the fuel pellet by displacement of the cracked

pieces. Pellet cracking and relocation has several important mech-

anical and thermal consequences. This report primarily gives a quan-

titative comparison of those thermal effects for cracked and uncracked

fuel pellets at the beginning of life. Even though all ceramic fuel

pellets crack, calculations for uncracked pellets permit making esi-

mates of the cracking contribution to fuel behavior. The estimates

can also be used to indicate the nature of errors in fuel rod modeling

codes in which the cracking/relocation effects are neglected.

1.2 Cracking Scenario

During the first rise to power, a temperature gradient within the

fuel rod causes the center of the pellet to expand more than the cooler

periphery. Thermo-elastic deformation proceeds until the fracture

stress of the pellet is exceeded. For typical light water reactors,

the fracture stress of the fuel is reached at a linear heat generation

rate of about 5 kW/m. Once the fracture stress is exceeded, sudden

jumping of the pellet pieces occurs upon cracking (Ref. 1). With in-

creasing power, further relocation results from thermo-elastic deform-

ation of each cracked pellet piece. If cladding contact is made, the

crack void in the bulk of the fuel is under compressive forces and

accommodates some fraction of the pellet thermal expansion. After the

crack void is consumed, radial expansion is approximately equal to the

free thermal expansion of the pellet.

1.3 Crack Patterns

Photomacrographs display distinctive crack patterns that seem

different for fast than for thermal reactor fuel (Refs. 2 and 3). After

cooldown, fast reactor fuel exhibits radial cracking from the central

void to the periphery. Light water power reactor fuel displays an

Page 14: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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irregular crack pattern. It is apparent, therefore, that findings

concerning cracking from fast reactor research may not be applicable

for light water power reactor cases (see also Sec. 1.7).

1.4 Major Thermal Effects of Cracking

Due to nonperfect radial cracking, the fuel to cladding gap width

will be circumferentially nonuniform. The gap width may vary between

that calculated for a non-cracked operating fuel rod and essentially

zero. Relocation of the pellet pieces into the gap causes improved

heat transfer between fuel and cladding. The effective fuel to cladding

gap conductance corresponds to a value reflecting both contact and open

gap conductance. However, cracking also causes fuel to fuel gaps to

open within the fuel pellet. Some of these gaps are oriented so as to

degrade heat conduction, counteracting at least some of the effect of

improved heat transfer at the pellet surface. Estimates of the magni-

tude of change resulting from both these effects are given later in

this report.

1.5 Effects of Cracking on FissiOn Gas Release

One possible mode of fission gas release concerns gases formed

in the columnar grain growth region of the pellet. Such gases diffuse

to the center of the pellet and are contained under pressure by the

plastic central region. When the fuel is cooled, thermal stresses

crack the pellet and the gas is released (Ref. 4). Another postulated

mechanism is that gas is released from all free surfaces of the fuel

pellet. When pellet cracking occurs, the free surface area increases

by an order of magnitude. Thus, pellet cracking apparently playsa sig-

nificant role in fission gas release (Ref. 5). At least at the time of

preparation of the MATPRO Version 09 report, the state-of-the-art was

represented by quoting an Argonne National Laboratory quarterly report

and indicating that the effects of fuel cracking on gas release are not

well documented (Ref. 6, p. 146). Such effects will be omitted from

the remainder of this report as well.

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1.6 Major Mechanical Effects of Cracking

There have been a number of fuel rod failures by clad cracking

during plant up-power maneuvers. It is thought that physical features,

which characterize such failures, include:

- as the power level is increased, the thermal expansionof the fuel pellet is larger than the expansion of theclad;

- if the fuel/clad gap is nearly closed at the start ofthe maneuver, then contact forces between pellet andclad can develop as the power is increased (pellet-cladmechanical interaction, PCMI);

- fission products from the pellet (such as iodine and/orcesium), possibly freshly released, are available forchemical attack on the clad (pellet-clad chemicalinteraction, PCCI);

- the combined effect of clad stresses from PCMI and localcorrosive action from PCCI can lead to clad failure fromstress corrosion cracking (SCC); and

- SSC failures require the action of both a corrosive en-vironment and a sufficiently high stress for a suf-ficiently long period of time.

If the reactor is brought to power very slowly, it is thought

that PCMI forces are reduced. This action is called "conditioning"

the fuel. Existing fuel vendor conditioning recommendations can man-

date power ascensions as long as one or two days (rather than few hour

startups that could otherwise be employed). High costs of power to

replace that lost during the long startups and load dispatching plant

readiness considerations emphasize the importance of eliminating over-

conservatisms in the conditioning recommendations.

Fuel cracking and relocation can influence the SCC situation in

several ways. Edges of broken pieces which contact the clad can pro-

vide locations for highly concentrated PCMI forces to act (and perhaps

also to break protective clad oxide layers). The cracks themselves

may act as routes by which fission products can reach the clad. Finally,

the broken pieces of the fuel may not fit together easily during the

pellet compaction caused by the PCMI forces. But the compaction could

be accomplished by smaller PCMI forces if very local creep deformations

of the fuel occur. Thus the time dependent compaction of cracked and

Page 16: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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relocated fuel could play a role in fuel pellet conditioning. Time de-

pendent compaction information is not now available. It has also been

omitted from the present study.

1.7 Crack Healing

During steady state reactor operation, healing of cracks may

occur simultaneously with grain growth if the pellet exceeds 1400°C

(approximately the onset of equiaxed grain growth) (Refs. 7,8,9 and 10).

Typical light water reactor fuel rarely exceeds this temperature and

thus, healing essentially does not occur. Fast reactor fuel often

exceeds 17000 C (the onset of columnar grain growth) whereby extensive

healing occurs. Healing and columnar grain formations contribute to

the crack pattern differences noted in Sec. 1.3.

Healing is used to describe a re-establishment of solid materialwhere previously a cracked surface existed. The local creep de-formation of Sec. 1.6, on the other hand, could occur with achange in shape which does not affect the existence of thecracked surface.

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2. THERMAL CALCULATIONS NOT DEPENDENT ON CRACKING

The computational procedures used in the comparative study of

cracked/uncracked fuel pellets are presented in this and the next two

chapters. This chapter deals with thermal calculations needed for both

cracked and uncracked fuel pellets.

2.1 Outline of Computer Calculations

Before describing the cracked and uncracked fuel model calcula-

tions in detail, an overview of the computational method is presented.

Serving as a general outline for this and the following two chapters,

Figure 2-1 presents a simplified flow chart of the computer program

developed for this study.

The computer program is initialized by reading in the input data

whereby the cladding temperature profile, thermal strain, and stored

heat are computed. Not evident by the diagram is that a branch exists

after the cladding stored heat calculation is made. Each model

(cracked/uncracked) has its own computational procedure for the fuel

pellet temperature profile calculations and fuel stored heat calcula-

tion. Regardless of model, however, an iterative process for computing

the fuel pellet temperature profile is utilized. An initial guess of

the gap width (the cold gap width) is made whereby the pellet tempera-

tures are calculated, followed by the fuel thermal strain calculation

which gives the new hot gap width. The above procedure is repeated

until the hot gap converges within 0.05 pm where the iterative process

is stopped. Following this, each model undergoes the same fuel rod

equivalent temperature calculation.

2.2 Cladding Temperature Profile

Beginning with the steady-state heat conduction equation

-V(k VT) = q"' (2-1)c

where q' = rate of heat deposition per unit volume;

k = cladding thermal conductivity; and

T = temperature,

a relation for the cladding temperature profile may be derived.

Page 18: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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heat

<ii

Flow chart for comparative study computer program.

Calculate fuelrod equivalenttemperature

Print out

res ults

Figure 2-1.

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If internal heat deposition in the clad is neglected, Eq. (2-1)

may be manipulated to give

T,-q' r

k dT = n() (2-2)c 27r rT

where To = outside cladding temperature;

r = outside radius of cladding;

T = temperature at radius r;

and q' = linear heat generation rate (LHGR) of the fuel rod.

With a relation for the thermal conductivity of Zircaloy-4 given

in Appendix B, the left side of Eq. (2-2) is evaluated to yield a

second order expression in temperature. Solving the quadratic equa-

tion gives

T(r) = -1.015x105 { 1.3959x10 - [1.9485x10

+ 1.9704x10-5(1.3959x10-2T + 4.9261x10-6T 2o o

1+ n( } (2-3)27r r

where

T(r) = temperature of cladding at radius r in C;

To = outside cladding temperature in C;

and

q' = LHGR in kW/m.

2.3 Cladding Thermal Strain

The average cladding thermal strain is calculated from the

equation

c 2 r2 Jo (ST) r dr (2-4)r - r1

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where c = average cladding thermal strain;

(ET) = cladding thermal strain at radius r (given inc Appendix B);

rl = hot inside cladding radius;

and r0 = hot outside cladding radius.

To perform the above integration, the trapezoidal rule is em-

ployed, using twenty five equally spaced mesh intervals of size M

where

r° - r1M = 25 (2-5)

The calculation of the average thermal strain requires hot dimensions

which are determined by

rhot r cold( + Ec (2-6)

Since the hot dimensions and the average thermal strain are dependent

upon one another, an iterative approach is taken in which the hot inside

cladding radius converges within 0.5 pm.

2.4 Cladding Stored Heat

The cladding stored heat is defined by the equation

SH = A H p 2wr dr (2-7)

Note that either cold dimensions and cold density or hot dimensions

and hot local density should be employed in this calculation. How-ever, the temperature profiles utilized in the computation are basedupon hot dimensions. Therefore hot dimensions are combined, forsimplicity, with cold density in Eqs. (2-7) and (2-9). It is feltthat only slight error arises from this practice.

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where SH = cladding stored heat;c

= density of Zircaloy-4 = 6550 kg/m

and AH = enthalpy change of cladding at radius r (givenin Appendix B).

Utilizing the trapezoidal method with 25 trapezoids, an explicit solu-

tion to Eq. (2-7) is obtained. The value for the stored heat is used

in the equivalent fuel rod temperature calculation.

2.5 Fuel Thermal Strain

The average fuel thermal strain calculation is similar to that for

the cladding thermal strain. For the fuel pellet

r2-f 2 2f 2 (T) f r dr (2-8)

r2 o

where of = average fuel thermal strain;

(T) f = fuel thermal strain at radius r (givenin Appendix B);

and r2 = hot fuel pellet radius.

Fifty equally spaced mesh intervals are employed in the trapezoidal

method to solve the above integral. The fuel thermal strain is de-

termined for each iteration of the fuel temperature profile calcula-

tion until hot gap width convergence is reached.

2.6 Fuel Stored Heat

The fuel stored heat calculation is also similar to that for the

cladding. For the fuel

r2SHf = AHf DPf 27r dr (2-9)

*See footnote accompanying Eq. (2-7).

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where SHf = fuel stored heat;

D = fractional theoretical density

p = fuel density = 10 980 kg/m3f

r2 = hot fuel pellet radius

and AHf = enthalpy change of fuel at radius r (givenin Appendix B).

Again, fifty trapezoids are used to numerically solve this integral.

2.7 Fuel Rod Equivalent Temperature

The actual stored heat of a fuel rod may be equated to the stored

heat if the rod were at some constant temperature. That constant

temperature may then be defined as the fuel rod equivalent temperature

Teq. In physical terms, Teq is the temperature that would be reached

by the fuel rod if all internal heating and external cooling were in-

stantaneously stopped. In mathematical terms

SHf + SH = (SHf) + (SHc)eq (2-10)

At constant temperature, the stored heat equations become

(SHf) = DPf AHf(Teq) rr2 (2-11)

(SH ) P AH (T ) (ro - r) (2-12)c)eq c c eq 1

It should be noted that the stored heat from the fill gas has been

deleted from consideration because it is insignificant compared to

that of the fuel and cladding. Rearranging Eq. (2-10),

f(Tq) = (SHf)eq + (SHc) -q SHf (2-13)

where T = fuel rod equivalent temperature, as yet unknown.eq

The root of Eq. (2-13), T , may be found by using Newton's method of

slope intercept. The slope intercept is determined by

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f(T )T = T - s (2-14)

s f'(Ts)

where TI = slope intercept temperature;

T = temperature where the slope is evaluated;

f(Ts) = value of the function f at T ;

f'(Ts) = the derivative of the function f, evaluated

at T;

and where the derivative of the function f is

f'(T) = D pf (C (T)) rr2 + p (C (T))c (r2 r (2-15)Ip f c p c o 1

where (C ) = constant pressure specific heat capacity of UO2 (givenin Appendix B)

and (C ) = constant pressure specific heat capacity of the claddingpn c (given in Appendix B).

Beginning with an initial guess for T (fuel pellet surface temperature),

TI is calculated by Eq. (2-14) and replaces T for another calculation.

Through this successive iteration, the fuel rod equivalent temperature

is determined when TI converges upon itself within 0.05°C where

eq I

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3. THERMAL CALCULATIONS FOR UNCRACKED FUEL PELLETS

This chapter contains the computational methods used for un-

cracked UO2 pellets employed in the comparative thermal effects study.

3.1 Pellet Surface Temperature and Gap Conductance

Solving the steady-state heat conduction equation for the gap

yields an equation for the pellet surface temperature

T2 T1+ 27rr h (3-1)2g

where T2 = pellet surface temperature

T1 = inside cladding temperature

q' = LHGR

r2 = hot fuel pellet radius

and h = gap conductance.

The gap conductance is determined by

kh = --- (3-2)g 6+6'

where k = thermal conductivity of fill gas (100% helium given ing Appendix B);

6 = hot radial gap width;

and 6' = root mean square cladding-fuel surface roughness.

3.2 Pellet Temperature Profile

The fuel temperature profile (based on constant volumetric heat

deposition rate) is calculated from the following equation

T T2 1 I

J kdT 12 A kdT + 1 X r )2 (3-3)

o

T

where f kdT = conductivity integral for 95% theoreticalo density fuel (given in Appendix B);

PF = porosity factor (given in Appendix B);

and T = temperature at radius r.

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The temperature of the fuel pellet at radius r may be determined

by equating the value of the conductivity integral (a function of r)

to its corresponding temperature. This is accomplished by fitting

second order equations to the conductivity integral. The pellet tem-

perature profile is then computed from equations of the form:

T(r) = A + Bx + Cx2 (3-4)

where x = fT kdT in kW/m

and A, B, C = constants.

The constants A, B, and C are presented in Table 3-1. The ac-

curacy of the above fit to the conductivity integral for 250 < T < 28000C

is ±+0.40C. This error is deemed insignificant compared to the overall

assumptions made in the study.

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Table 3-1

Constants for Temperature of Conductivity Integral Equation (Eq. 3-4)

Range A

T < 5850C(x < 3.441)

26.68

B

72.42

'C

26.08

585 < T < 1000°C

(3.441 < x < 4.814)

1000 < T < 1405°C

(4.814 < x < 5.866)

1405 < T < 18000 C

(5.866 < x < 6.783)

1800 < T < 22050 C

(6.783 < x < 7.723)

T > 22050C(x > 7.723)

126.7

40.26

-630.9

-1750.15

12.82

46.48

274.13

604.12

35.01

31.75

12.43

-11.91

-2589.9 822.27 -26.08

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4. THERMAL CALCULATIONS FOR CRACKED FUEL PELLETS

This chapter deals with the computational methods used for

cracked pellet thermal effects.

4.1 Pellet Surface Temperature and Gap Conductance

As in Section 3, the pellet surface temperature may be deter-

mined by

T2 = T1 + 2rrh (4-1)2g

However, the gap conductance for a cracked fuel pellet takes the

form (Ref. 11)

h = (l-F)h + F h (4-2)g 0 c

.k

where h = zero contact pressure conductance = g

h = contact conductance = -g .c 6'

k = thermal conductivity of fill gas (given in Appendix B);

and F = fraction of pellet circumference lying against the cladding.

Two models for the fraction of circumferential cracked pellet

contact were investigated. The Kjaerheim & Rolstad model (Ref. 12)

may be expressed as

F = 0.3 + 0.7[0.2](5 0 6/r2) (4-3)

where 6 = hot radial gap width in mm;

and r2 = hot fuel pellet radius in mm.

The FRAP-S model is given below for fuels with burnups less

than 0.6 MWd/kgU (Ref. 11).

1006 4 -1F = 0.3 + [100() + 1.429] (44)

r 2

and for burnups greater than 0.6 MWd/kgU

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F = 0.3 + [A(00) B + 1.429] 1 (4-5)r2

where A = 100-98 Fb;

B = 4-0.5 Fb;

Fb = 14 (x-0.6)4 + 1]-1

and x = burnup in MWd/kgU.

It should be noted that the burnup factor Fb, and thus, the

fraction of pellet-clad contact, F, reaches an asymptotic limit near

10 MWd/kgU burnup.

Figure 4-1 presents the Kjaerheim & Rolstad model and the FRAP-S

model for burnups under 0.6 MWd/kgU and for 10 MWD/kgU. Only at

larger ratios of 6/r2 does the Kjaerheim & Rolstad model predict a

larger fraction of pellet contact than the FRAP-S model (regardless

of burnup). With increasing burnup, the FRAP-S model predicts a larger

fraction of pellet contact for all ratios of 6/r2. Due to the accumu-

lation of gaseous fission products at the grain boundaries in the fuel,

the fuel pellet tends to crack more and thus causes greater contact

with the cladding.

Noting that the FRAP-S model is more conservative in the usual

operating range of 6/r2 than the Kjaerheim & Rolstad model, and that

the FRAP-S model is capable of including burnup considerations, the

FRAP-S model was chosen for incorporation into the study.

4.2 Pellet Temperature Profile

The cracked fuel pellet temperature profile is calculated from

the steady state heat conduction equation

- V(kVT) = q'" (4-6)

which can be put into the form

-q'r=T - (4-7)

dr 2 (47)27r2 k

Page 31: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-21-

c -'0 O

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a

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Page 32: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-22-

Using a finite difference method

dT T(rn) - T(rn-Ar)dT _ n fl (4-8)

dr Ar

Eq. (4-7) is rearranged to

q'r Ar

Tn+ = T + (4-9)

27rr2 (kf)n

where Tn = fuel pellet temperature at radius r ;

n = index with range 2 < n < 52;

Ar = r2/50 = radial increment;

q' = LHGR;

and (kf)n = U02 thermal conductivity at radius r .

Beginning at the surface of the pellet, the temperature at the

first radial increment is computed using a temperature T2 obtained from

gap calculations. Equation (4-9) is then used successively to step

toward the center of the pellet and obtain the temperature profile of

the fuel.

The cracked pellet temperature profile is calculated in 50 radial

increments. Comparison of uncracked pellet centerline temperatures cal-

culated from the conductivity integral and from the finite difference

equation (also using 50 radial increments) displayed a maximum deviation

of 0.1°C. From these calculations it can be assumed that 50 increments

would produce sufficient accuracy for the cracked pellet temperature

calculations.

To account for the reduction in heat transfer due to cracks in the

fuel, an effective U02 thermal conductivity is employed in Eq. (4-9).

The effective UO2 thermal conductivity is (Ref. 12)

-3 -2k = kf[ - 3.175x0 + 1] (4-10)e kk+

r2(0.077 - + 0.015)kf

Page 33: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-23-

where kf - U02 thermal conductivity (given in Appendix B);

k = fill gas conductivity (given in Appendix B);

6 = hot radial gap width in m;

and r2 = hot fuel pellet radius in mm.

Page 34: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 35: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-25-

5. ILLUSTRATIVE EXAMPLE

This chapter presents the results of the computer calculations

for cracked/uncracked fuel pellets with a nominal cold radial gap width

of 95 m. This and other dimensions are based on the nominal fuel rod

dimensions for the Maine Yankee reactor (see also Appendix C). Calcu-

lations were also made for initial radial gap widths of 75 and 115 pm

and are presented in Appendix A. The 75 and 115 m radial gap widths

are estimates which correspond to the extreme tolerances expected in

the determination of the nominal gap width (Ref. 13).

Note that the calculations of this chapter have been performed

for linear heat generation rates (LHGR) between zero and 60 kW/m. The

local peak LHGR for Maine Yankee is 35.8 kW/m. In addition, occurrences

such as columnar grain growth and central hole formation occur when

temperatures rise above '1700°C. Therefore, portions of the plots

above approximately 40 kW/m should be regarded as mathematical extrap-

olations from the lower LHGR results. These portions are included for

the purposes of illustrating how the calculations behave, but may be

significantly in error because of the neglect of some significant high

temperature phenomena.

5.1 Fuel Pellet Surface Temperature

Figure 5-1 shows the fuel surface temperature as a function of

LHGR for a cracked and uncracked pellet. The uncracked pellet consis-

tently shows a higher temperature than the cracked pellet with a maxi-

mum difference of about 210°C at 40 kW/m. This effect is due to the

fact that the cracked pellet relocates into the gap, resulting in im-

proved gap conductance and a lower fuel surface temperature.

The uncracked fuel surface temperature decreases with increasing

LHGR above 45 kW/m. Beyond this LHGR, the pellet core becomes hotter

where thermal strains expand the pellet into the gap and improved gap

conductance results in a lower surface temperature. Within 60 kW/m,

the cracked fuel pellet does not exhibit this effect.

The surface temperature for uncracked fuel displays a concave

downward function of LHGR, while the cracked pellet displays a nearly

linear function. For both cases, a kink exists at 25 kW/m in the

Page 36: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

to0

)

04- 0

I . 3

Hi o HOl

c V Cmo 0 0b U) n~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~c-(Do) mQiVnaaWL

-26-

Page 37: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-27-

surface temperature plot. This kink corresponds to the LHGR at which

the outside cladding temperature changes from an increasing function of

LHGR to a constant temperature at the onset of nucleate boiling (see

Appendix C for further details on the determination of the outside

cladding temperatures).

The general shape of the surface temperature curves remainsun-

changed with different gap sizes. However, with increasing initial

gap size, the uncracked pellet surface temperature increases at all

linear heat generation rates. The differences between the cracked/

uncracked pellet surface temperaturesalso increases with increasing

cold gap size. The maximum difference occurs at higher temperatures

for larger cold gap widths. Remaining within 1°C of themselves, the

surface temperature of the cracked pellets is unaffected by cold gap

sizes up to linear heat generation rates of 40 kW/m. The largest

calculated difference is 6.5°C (at 60 kW/m for the two extreme cold

gap widths).

5.2 Fuel Pellet Centerline Temperature

Figure 5.2 shows the fuel centerline temperature as a function

of LHGR for a cracked and an uncracked pellet. For all linear heat

generation rates, the cracked pellet exhibits a lower centerline tem-

perature. With increasing LHGR, the difference in temperature between

the cracked and uncracked pellets increases. At 30 kW/m this dif-

ference is only 20°C, while at 60 kW/m the difference increases to

about 130°C.

With increasing cold gap size, the centerline temperature for

uncracked and cracked pellets increases for all linear heat generation

rates. Only for the larger cold radial gap width of 115 pm does the

cracked pellet centerline temperature exceed that of the uncracked

pellet. That is, from 10 kW/m up to 45 kW/m the cracked pellet center-

line temperature is higher than that for the uncracked pellet with a

maximum difference of about 40°C at 24 kW/m. Beyond 45 kW/m, the

uncracked pellet temperature is higher with a centerline difference

of about 60°C at 60 kW/m.

Page 38: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-28-

o 80 00 0

(Do) a tun~za

0so

B

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Page 39: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-29-

5.3 Fuel Rod Equivalent Temperature

The fuel rod equivalent temperature as a function of LHGR for

cracked/uncracked pellets is presented in Fig. 5-3. For all linear

heat generation rates, the uncracked pellet displays a higher equiva-

lent temperature. At 30 kW/m, the difference is 104°C, at 60 kW/m the

equivalent temperature difference increases to 170°C.

As the cold gap size increases, the equivalent fuel rod tempera-

ture increases for both the uncracked/cracked cases. The relative

difference between the equivalent temperatures for the two cases is

unaffected by the cold gap size at each LHGR.

5.4 Fractional Radius for Grain Growth

A temperature for equiaxed grain growth, 1400°C, and a tempera-

ture for columnar grain growth, 17000C, were arbitrarily chosen. How-

ever, these temperatures are within the range of those determined by

other investigators (Ref. 14). In addition, a fixed temperature for

grain growth in U02 is a gross assumption in itself because grain

growth is a function of burnup, fuel stoichiometry, and duration of

irradiation. The 1400°C and 1700°C grain growth temperatures do serve

to indicate the extent of microstructural change (including crack

healing) regions, however.

Crack healing occurs simultaneously with grain growth. At the

lower pellet temperatures (within a grain growth regime), the time at

a steady state operating temperature may not be long enough to allow

for the diffusionally controlled grain growth and healing processes

to occur. However, higher fuel temperatures (as found in fast reactor

fuel) do allow equiaxed grain growth, columnar grain growth, and heal-

ing to occur quite extensively during normal reactor operating cycles.

Figure 5-4 presents the fractional radii for grain growth in

cracked and uncracked fuel pellets. For this consideration, a frac-

tional radius of 1.0 is defined as the surface of the fuel pellet.

Consistent with the higher temperature profile for the uncracked pellet,

grain growth occurs throughout more of the uncracked pellet than for

the cracked pellet at all linear heat generation rates. Crack healing

may be expected to begin at the pellet center at about 30 kW/m. At

40 kW/m, about 21% of the cracked pellet is within the grain growth/

heaing regime, while at 60 kW/m, 41% of the pellet is in this range.

Page 40: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-30-

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Page 42: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-32-

With increasing cold gap size, a lower LHGR is required to

initiate grain growth, and more of the pellet is within the grain

growth area at each LHGR. This is consistent with the higher tempera-

ture profiles for larger initial gap pellets.

Only at the larger cold radial gap width of 115 m does the

cracked pellet initiate grain growth at a lower LHGR than the uncracked

pellet. This effect reflects the fact that the cracked pellet has a

higher central temperature profile over the lower range of linear heat

generation rates than the uncracked pellet.

5.5 Gap Closure

Figure 5-5 displays the percentage of gap closure for uncracked

and cracked fuel pellets. The gap width considered here is an undis-

turbed gap, where the fuel pellet is treated as uniformly circular and

free from pellet piece relocation. Regardless of the cold gap size,

the uncracked pellet achieved greater gap closure than the cracked

pellet for all linear heat generation rates. Even though the cracked

pellet relocates into the gap, the improved heat transfer results in a

lower average pellet temperature and lower thermal strain. Thus, from

reduced thermal expansion, the cracked pellet has a larger undisturbed

hot gap width than the uncracked pellet at all linear heat generation

rates.

For both cracked and uncracked cases, the percentage of gap closure

decreases with increasing cold gap size at each LHGR. Even though the

larger cold gap pellets have higher temperature profiles, and larger

absolute changes in pellet size, thermal expansion alone cannot pro-

portionally close up the original gap as that of a smaller cold gap pellet.

5.6 Pellet - Clad Contact

The uncracked pellet model assumes a perfectly circular pellet.

Thus, only with 100% gap closure, where the gap width equals the pellet-

cladding surface roughness, does pellet-clad contact exist. Up to

60 kW/m, pellet to cladding contact was not reached under the conditions

employed in this report for uncracked pellets.

Figure 5-6 presents the calculated circumferential pellet-cladding

contact for cracked pellets. With increasing LHGR, the fraction of

contact increases. This is to be expected since the amount of contact

Page 43: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-33-

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Page 44: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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Page 45: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-35-

is a function of the hot gap width. With higher linear heat generation

rates, the hot gap becomes smaller which results in more contact. Also,

with larger cold gap pellets, the hot gap width is larger which results

in less pellet-clad contact at each LHGR.

Page 46: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 47: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-37-

6. EXPERIMENTAL EVALUATION

Beginning of life experimental fuel performance data was obtained

from an instrumented fuel assembly irradiated at the Halden Heavy Boil-

ing Water Reactor (Ref. 11). The fuel rods in this assembly are typical

of pressurized light water reactor design in dimensions and materials

(see Appendix D). Utilizing the models described in this report, cal-

culated pellet centerline temperatures are compared to the Halden ex-

perimental data in Fig. 6-1.

The comparisons indicate that, for these experiments, only slight

differences exist between the uncracked (non-relocation affected gap

conductance, solid pellet thermal conductivity) and cracked (relocation

affected gap conductance, cracked pellet thermal conductivity) model

predictions. Both models produce reasonable pellet centerline tempera-

tures for the third and fourth power cycles. However, when pellet piece

relocation is considered in the gap conductance and a solid pellet

thermal conductivity is assumed, the model drastically underestimates

the centerline temperature for all power cycles. This indicates that a

model incorporating pellet piece relocation in the gap conductance must

also consider the crack induced heat transfer barriers within the fuel

pellet to obtain reasonable results.

As displayed in Fig. 6-1, experimental evidence indicates that

thermal stabilization of a fuel rod is obtained approximately after the

third power cycle (Refs. 2 and 11). This asymtopic effect may result

because the internal thermal stresses which cause the major amount of

pellet cracking are essentially relieved during the heatup-cooldown

phases of cycling, and because further pellet piece relocation is in-

hibited by pellet-clad contact interference. Even though the model

utilized in this study for cracked pellet-clad contact does not ex-

plicitly incorporate cycling effects, the model correlates quite well

to fuel rods thermally conditioned by power cycling.

Extrapolating a best fit curve through the third and fourth power

ramp experimental data points, an estimated difference of 50°C exists

between the cracked pellet model prediction and the experimentally de-

termined centerline temperature at 40 kW/m. Assuming the same propor-

tional difference in the Maine Yankee calculations, a 550C discrepancy

would result between the cracked pellet model and actual beginning of life

pellet centerline temperature at 40 kW/m, with the calculated temperatures

being higher.

Page 48: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-38-

10 20 30

LINEAR HEAT GENERATION RATE (kW/m)

Figure 6-1. Comparison of computational models to Halden experimental

fuel rod data (experimental data from ref. 11).

2000

1600

Oo

frIER

A:pr;

r4

1200

800

400

o 40

Page 49: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-39-

7. CONCLUSIONS

This chapter presents the conclusions from this study based upon

Maine Yankee light water reactor fuel under steady-state, beginning of

life operation.

7.1 Relocation Into Gap

Once the fuel pellet cracks, a fraction of the fuel pieces lie

against the cladding. This contact results in better heat transfer

conditions than for an assumed uncracked pellet which has not relocated

into the gap. When compared to an uncracked pellet under the same

operating conditions, the cracked fuel pellet exhibits a lower surface

temperature. This difference may be as much as 210°C at 40 kW/m.

7.2 Reduced Fuel Thermal Conductivity

Some of the cracks within the fuel pellets form heat barriers

and degrade overall heat transfer conditions. To account for this heat

transfer degradation, an effective fuel thermal conductivity is used

which essentially serves to reduce the normal U02 thermal conductivity.

Generally, the adverse thermal effects of internal cracks are countered

by the crack induced relocations into the gap. Only for large cold gap

widths does the cracked pellet centerline temperature exceed that of

the uncracked pellet. At 35 kW/m with an initial radial gap size of

115 m, the cracked fuel centerline temperature exceeds that of an un-

cracked pellet by about 400C. Regardless of initial gap size, the ef-

fects of internal cracks are diminished by the relocation improved gap

conductance. Thus, cracked pellets always display a cooler outer tem-

perature distribution resulting in a lower average thermal strain, less

undisturbed gap closure, and less stored heat than for an uncracked

fuel pellet.

7.3 Fuel Rod Equivalent Temperature

Due to the cooler outer temperature profile which results in less

stored heat, the cracked fuel pellet always exhibits a lower fuel rod

equivalent temperature than the uncracked pellet. At any particular

LHGR, the difference between the equivalent temperatures for cracked/

uncracked pellets is approximately the same for any initial gap width.

Page 50: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-40-

During a LOCA, the cladding and the fuel will equilibrate to

roughly the same temperature since the heat transfer to coolant is

poor and the heat deposition rate is low. The lower equivalent tem-

perature indicates less severe LOCA conditions. Thus, the stored heat

of an uncracked pellet at 30 kW/m will produce the same equivalent

temperature as a cracked pellet at 37.5 kW/m.

7.4 Crack Healing

Significant crack healing is expected when extensive grain growth

has occurred. Only at 35 kW/m does 10% of a fuel pellet with a nominal

initial gap width reach into the grain growth regime (fuel temperature

greater than 1400°C). Under normal reactor operating conditions, LWR

fuel pellets seldom exceed this LHGR. Thus, extensive crack healing

is not expected in typical light water reactor fuel.

Page 51: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-41-

APPENDIX A

ADDITIONAL FIGURES FROM FUEL PELLET THERMAL CALCULATIONS

This appendixpresents the figures for cracked/uncracked fuel

pellet thermal effects at initial radial gap widths of 75 and 115 m.

These two gap widths were chosen as the extreme tolerances for the

determination of the nominal cold gap width. The figure captions

should be self-explanatory, but if further explanation is required,

refer to Chapter 5.

Page 52: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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Page 54: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

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Page 62: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 63: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-53-

APPENDIX B

MATERIAL PROPERTIES

This appendS presents the material properties for uranium dioxide,

Zircaloy-4, and helium used in this study. In some cases, a comparison

between two relations for a particular property, and a discussion con-

cerning the choice of a relation incorporated into the work will be

given.

B.1 Fuel Thermal Conductivity

Two relations for the thermal conductivity of uranium dioxide were

investigated. The thermal conductivity used by EPRI is (Ref. 15)

kf = PF [402.4+T + 6.12x10 (T+273) (B-1)

PF 1.1316(1-P)PF = (B-2)l+P+10P

where kf = U02 thermal conductivity in W/mK

PF = porosity factor, normalized to 95% theoreticallydense fuel (dimensionless);

P = fractional porosity of fuel (dimensionless);

and T = temperature in C.

MATPRO's version of the UO2 thermal conductivity correlation for

0°C < T < 16500 C is (Ref. 6)

kf = PF 464+T + 1.216x102 exp(l.867xlO-3T) (B-3)f 464+T~~~~~~for 1650 < T < 28400 C

Page 64: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-54-

kf = PF [1.91 + 1.216x10- 2 exp(1.867x1 T)] (B-4)

PF = - (2.58-5.8x10 -4T) (1-D) (B-5)PF -4 (B-5-

1 - (2.58-5.8x10-4 T) (0.05)

where kf = UO2 thermal conductivity in W/m'K;

PF = porosity factor, normalized to 95% theoreticallydense fuel (dimensionless);

D = %T.D./100 (dimensionless);

and T = temperature in C.

The above correlations for 95% T.D. fuel are plotted in Fig. B-1.

Both relationships give essentially the same thermal conductivity over

the temperature range of primary concern, 3000 C to 20000C. Above this

range, the MATPRO version increases more sharply than the EPRI corre-

lation, thus resulting in a 4.5% difference at 20000 C and increasing

to a 29% difference at the melting point (2800°C).

Figure B-2 presents the porosity factors from EPRI and MATPRO at

500°C and 2000°C. At low temperatures, small differences exist between

the two porosity factors. With increasing temperatures, the difference

increases. For fuel near 95% T.D., both porosity factors equate quite

well for all operating temperatures.

Using the two thermal conductivities, the following conductivity

integrals were derived for 95% T.D. fuel with an arbitrarily choosen

reference temperature of 0°C. From EPRI:

T

kf dT = 3.824 n 1 + 40 + 1.53x10 1 4 (T+273)4

-5- 8.5x10 (B-6)

Page 65: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-55-

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Page 66: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-56-

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Page 67: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-57-

T

where f kf dT = conductivity integral in kW/m;

0o

and T = temperature in C.

From MATPRO for 0°C < T < 1650°C

T

f 464] 6.513x10o

exp(l.867x10-3T) - 6.513x10- 3 (B-7)

for 16500 C < T < 2840°C

T

fkf dT = 1.91x10-T + 6.513x10-3

exp(l.867x10-3T) + 2.974 (B-8)

T

where k dT = conductivity integral in kW/m;

o

and T = temperature in C.

The values of the above integrals are plotted in Fig. B-3. Over

most of the fuel operating temperature range, the difference between

the two conductivity integrals is approximately constant. This dif-

ference will result in a discrepancy of about 500C for a fuel center-

line temperature calculation.

Due to itsgreater simplicity and ease of mathematical manipulation,

it was decided to use the EPRI version of the UO2 thermal conductivity

in this study. Furthermore, since most fuel operating temperatures are

below 2000°C, minute differences would result from cracked pellet

Page 68: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-58-

I I -I I I I I I I

I I I ,I - I I I .

N ao e- '3 u'v (- m N *4

(//M) lP

00

uoN.

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Page 69: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-59-

temperature profile calculations if the MATPRO thermal conductivity

were used. If only 95% T.D. fuel were to be considered for uncracked

pellet calculations (where the porosity factor is normalized to one),

then the MATPRO correlation would have been used. However, to ensure

greater flexibility, incorporation of the porosity factor was deemed

necessary. Integration of the complete MATPRO relation (with its

temperature dependent porosity factor) would have resulted in an ex-

ceedingly burdensome equation. Also, a different reference temperature

for the conductivity integral (i.e., 2000C) would reduce the calculated

pellet centerline temperature differences. Thus, for consistency in

the comparative study of cracked and uncracked pellets, the EPRI U02

thermal conductivity correlation was employed.

B.2 Fuel Thermal Strain

A relation used for uranium dioxide thermal strain was taken from

MATPRO and is presented below

cT = -4.972x10- 2 + 7.107x10 4T

+ 2.581x10 -7T2 + 1.14x10l T3 (B-9)

where ST = UO2 thermal strain in %

and T = temperature in C.

Figure B-4 displays this correlation in graphical form. The

root of the thermal strain equation lies at about 65°C.

B.3 Fuel Specific Heat Capacity

For use in stored heat and equivalent fuel rod temperature calcu-

lations, a correlation for uranium dioxide specific heat capacity was

taken from MATPRO. The following equation is also plotted in Fig. B-5.

Page 70: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-60-

~4- ~ ~ K n N( KUI r4l SH MIY&LbS 'tywuawi a r e

,4H

CH

0

o 4

IQHEd l 0Ed 0

0H

.1

Page 71: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-61-

0 0 0 0O0 o coO gX) 1'70 4H N

(xs/r) LLIDYvJYD IS DIAIDSdS

.iH

qa§

I .C'

. 4,a

o

o0

.4

IQAIa,a

Page 72: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-62-

535 28585.005 exp( T )

T

2 535 285 2

T

-8+ 2.432 x 10 T

1.6591x106 -18971+ 2 exp T )T

(B-10)

where C = U 2 specific heat capacity in MJ/kg-K

and T = temperature in K.

B.4 Enthalpy Change for Fuel

The enthalpy change for U02 may be derived from the following

equation

T

AHf(T) =

Tref

C dTP

(B-ll)

Using the MATPRO specific heat capacity, U02 enthalpy is calculated

below for a reference temperature of 250 C.

AHf(T) .158803 + 1.216x10-8T2

535 285)-exp( T- )-l

+ 87.455 exp(- 18971) - 3.2705x10- 2

T

AH(T) = U02 enthalpy in MJ/kg

T = temperature in K.

(B-12)

Figure B-6 presents the UO2 enthalpy change in graphical form.

p

where

and

Page 73: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-63-

0 0

(9/rw) IDNYHD xdrEvHma

U

U

0

Ido

0.-4CH

0

0

I

4)

.1

0

Page 74: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-64-

B.5 Cladding Thermal Conductivity

Taken from MATPRO and CENPD-218 (Ref. 16), two correlations for

the thermal conductivity of Zircaloy-4 were investigated. MATPRO's

version takes the form

k = 7.51 + 2.09x10-2 T - 1.45x10-5 T + 7.67x10 T (B-13)c

where k = Zircaloy-4 thermal conductivity in W/m.k

and T = temperature in K.

The relation from CENPD-218 is

k = 13.959 + 9.8522x10l T (B-14)c

where k = Zircaloy-4 thermal conductivity in W/m.k

and T = temperature in C.

The above two conductivities are presented in Fig. B-7. At 3000C the

MATPRO conductivity differs by 4.4% from that of CENPD. With increas-

ing temperature, this difference decreases, where at 500C, the dif-

ference is only 1.8%.

To allow for a simple and explicit cladding temperature profile

relation, the CENPD thermal conductivity was chosen. The use of the

MATPRO thermal conductivity is expected to produce similar results for

inside cladding temperature calculations. However, the complexity of

the MATPRO relation does not lend itself towards a direct computation

of the cladding temperature profile; this made its application unwarranted.

B.6 Cladding Thermal Strain

The correlation used for the cladding thermal strain was taken

from MATPRO. For 27 < T < 800°C, the thermal strain relation is

ET = -2.373x10-2 + 6.721xlO-4T (B-15)

Page 75: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-65-

00co

40

0,q

0 a0.

0o a0

00*--I0c 'o go

B 4

3a

. F

QN CO 4CNl w -I

(X. /A) LIAIM1nOD IYWdL

Page 76: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-66-

where ¢T = Zircaloy-4 thermal strain in %

T = temperature in C.

The above correlation is presented in Fig. B-8. The root of the

thermal strain equation lies at about 350C.

B.7 Cladding Specific Heat and Enthalpy

From data points supplied by MATPRO, the following equations were

derived from linear interpolation for specific heat capacity and

enthalpy of Zircaloy-4. These equations may be expressed as

(C )p c

AH (T)C

where CP

= A + BT

= C + DT +

(B-16)

ET2 (B-17)

= specific heat capacity of Zircaloy-4 in J/kgK;

AH(T) = enthalpy change of Zircaloy-4 in MJ/kg;

T = temperature in C;

and A,B,C,D,E = constant.

The values of A, B, C, D, and E are given in Table B-1. The specific

heat of the cladding is plotted in Fig. B-9, and the enthalpy change

is presented in Fig. B-10.

and

Page 77: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-67-

I I I I I I I I I I

f- ..... I .. I . I _ I .0o; O

MIYUIS A'IDVO14H: IU( d

00No -1

"-I ;d

U tq

0r.oH r4I -I

o

_ __

Page 78: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-68-

o 0o o( ) I

(x.2/r) ;mIayo3 A DIdlodS

0-4

0

0o N8 tq0

qI0

d

< M

I0 0

H

0C'

of

00

Page 79: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-69-

.4. N0r c0(t3/vr) SDMYHD X&IYHJM¶

0

o

IsV 1

a C4.0EH

0-:A

Pim

V.A

a

<6

ED4

O0C

Page 80: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-70-

Table B-1

Constants Used in Specific Heat and EnthalpyEquations for Zircaloy-4 (Eqs. B-16 and B-17)

A B C D

25<T<1270C

126<T<367°C

367<T<8170C

817<T<820 0°C

820<T<840°C

840<T<8600C

860<T<880°C

880<T<9000C

900<T<920°C

920<T<975 0°C

T>9750C

275

287

295

-34200

- 3110

- 460

- 3860

- 3550

2890

7690

356

.21

.121

.0978

42.3

4.4

1.25

5.2

4.85

-2.3

-7.53

0.0

-7.67x103

-9.23x10-3

14.1

1.33

.222

1.68

1.55

-1.35

-3.56

1.72x10-2

2.87x10

-42.95x10

-3.42x102

-3-3.11xlO- 3

-4.6x104

-3.86x10-3

-3.55x10-3

2.89x103

7.69x10-3

3.56x10- 4

6.04x10-8

4.89x10-8

2.12x10

2.2x10- 6

6.25x10-7

2.6x106

2.42x10 6

-1.15x106

-3.76x106

0.0

Range E

Page 81: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-71-

B.8 Thermal Conductivity of Fill Gas

A relation for the thermal conductivity of helium was also taken

from MATPRO. The correlation is

-3 0.668k = 3.366 x 10 (T) (B-18)g

where k = heliunthermal conductivity in W/m.K

and T = temperature in K.

The above equation is plotted in Fig. B-ll.

Page 82: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-72-

O 4 C

N)3 /0A OD 0(M N/M) IIAIMflUOD AceZHJ

i

0)

§

o ,io

I !o0 0

x

1fM ma

4)

q-I

N

Page 83: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-73-

APPENDIX C

INPUT PARAMETERS

The input parameters were supplied by Yankee Atomic Electric Company

from base case design and operating data. The data is characteristic

of Maine Yankee PWR fuel. However, the conclusions from this study

are applicable to other light water reactor fuel.

C.1 General Design Parameters

The following is a list of design features of the MaineYankee

fuel incorporated into this study. In addition, the tolerances on the

initial radial gap have been estimated for this study to be ±20 pm

(similar to LWBR, Ref. 13, Table 4.2.1-1). Therefore, the nominal and

the extreme tolerances are included in the calculations. The diameter

of the fuel pellet remained unchanged, whereby the cladding dimensions

were altered (at constant thickness) to allow for the differing cold

gap widths.

Parameter Value

Fuel Density 95% T.D.

Fill Gas 100% Helium

Cladding Material Zircaloy-4

Fuel-Cladding SurfaceRoughness (arithmetic mean) 1.5 pm

Fuel Pellet Radius 4.782 mm

Cladding Thickness 711 m (Nominal)

Cladding Outside Radius 5.568 mm 5.588 mm 5.608 mm

Cladding Inside Radius 4.857 mm 4.877 mm 4.897 mm

Cold Radial Gap Width 75 pm 95 pm 115 pm

C.2 Outside Cladding Temperature

The following data from Yankee Atomic Electric Company is used in

developing an input model for the cladding surface temperature as a function

of linear heat generation rate.

Page 84: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-74-

Parameter

Active Fuel Length

Core Average LHGR

Average LHGR for Peak Rod(average x 1.45)

Axial Peaking Factor(peak/average)

Peak LHGR for Peak Rod(28.64x1. 25)

System Pressure

Fuel Rod Pitch

Coolant Passage EquivalentDiameter

Coolant Velocity

Coolant Inlet Temperature

Coolant Average Temperature

Value

3.472 m

19.75 kW/m

28.64 kW/m

1.25

35.8 kW/m

15.5 MPa

14.73 mm

13.55 mm

4.63 m/sec.

282°C

304°C

Other parameters consistent with the core average temperature at

100% core power are derived below. From enthalpy data which is presented

in Fig. C-1, the specific heat capacity of the coolant may be deter-

mined (Ref. 17). (All thermodynamic data presented in this Appendix is

for water at a pressure of 15 MPa. The error associated with this de-

parture from the system pressure of 15.5 MPa is expected to be insig-

nificant.) Instead of evaluating the specific heat directly at the

core average temperature of 304°C, it was decided to make the calcula-

tion at the inlet and outlet bulk temperatures. At 100% core power,

the temperature rise from the inlet to the core average is equal to

the rise from the core average to the bulk outlet temperature for a

nominal channel. Thus,

AH

(C) = wpw AT (C-l)

where AHw = H20 enthalpy rise

= (1.4905 - 1.241) MJ/kg = 0.249.5 NJ/kg;

AT = H20 temperature rise

= (326 - 282)°C = 440C;

Page 85: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

i00o

00 i

Ittt1-% , +1

oC) aa

I q

-0

04

00

3-b

CH9

It

D H

i

C3,0

qa&OU

C4U 0£ . . ..

(t2/rw) asNiHr XAdIc&

-75-

T-

Page 86: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-76-

and (Cp) H20 specific heat = 5.67x10 3 MJ/kg-K.

The coolant mass flow rate is also derived for nominal conditions.

Here,

q' Icore

m A (C-2)w

where q' = core average LHGR = 19.75 kW/mcore

Q2 = active fuel rod length = 3.472 m;

AH = H20 enthalpy rise = 0.2495 MJ/kg;w

and m = coolant mass flow rate = 0.275 kg/sec.

Using the Dittus-Boelter equation with Maine Yankee and published

thermodynamic data, the bulk-cladding heat transfer coefficient may be

calculated (Refs. 17,18). Rearranging the Dittus-Boelter equation

h= 0.6 08 (Cp)w0h = 0.023K (Vp ) 0.4 (C-3)0.2 ( w ()

e

for H20 at 3000C, 15 MPa pressure

where k = H20 thermal conductivity = 0.559 W/m..K;w 2

De = equivalent coolant passage diameter = 13.55 mm;

V = coolant velocity = 4.63 m/sec;

pw = H20 density = 726.2 kg/m 3;

and (v)w = H20 viscosity = 9.17 x 10- 5 kg/m-s results in

h = bulk-cladding heat transfer coefficient = 33.2 kW/m --K.

The bulk temperature rise across a coolant channel may be ex-

pressed as

ATb = (C) (C-4)p w

Page 87: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-77-

q' = average LHGR of a fuel rod in the coolant channel

the other parameters as defined above.

ATb = bulk coolant temperature rise = (2.23 kW/) q' (C-5)

The following convention is used for the various linear heat generation

rates

%C Pq, = 35.80 kw/m ~l00

qominal = 24.69 kW/m ( Pnominal,max 100

q' =q' /1.25max

(C-6)

(C-7)

(C-8)

where %C.P. = percent core power.

Using Eqs. (C-4) through (C-8), Fig. C-2 displays the coolant behavior

as a function of core power with a constant inlet temperature of 282°C

and a saturation temperature of 344.80 C.

Correlations for bulk temperature and outside cladding temperature

as a function of axial position are given below

Tb = Tbb b-inlet

+ ATb [1+ sin( ex) sin( ex)

where

and

Thus,

(C-9)

Page 88: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-78-

0 0 0'0o( ) gaa N a

o0'-4

-4t

'90

iU)'-4 0o 0)

aa0 0o I 0

0o t4 0u c

1z I

oTo

IVO +-

0m0Of *r-~N

00)

.1.Cg0I0

arx.

rz.

Page 89: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-79-

q' max ( f)T =T + cos (C-10)To Tb + 2wr h (C-10)

o ex

where z = axial position (z = 0 at core midplane);

£ = active fuel length;

= extrapolated zero flux fuel length;ex

h = bulk-cladding heat transfer coefficient;

Tb = bulk coolant temperature;

Tbinle t = inlet bulk temperature;

ATb = bulk temperature use across channel;

and T = cladding outside temperature.

Assuming an axial cosine power distribution and an axial power

peaking factor of 1.25, the extrapolated zero flux fuel rod length

may be determined by trial and error from the equation

1/2

qax cos ( ) dz

q' -Z/2 ex

* - Q/2

f dz

which results in

2 = 4.82 m.ex

With this value and others previously given, the bulk and outside

cladding temperature profiles reduce to

Page 90: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-80-

sin (Q) 1Tb Tbinlet + 1 ATb 1 + ex (C-12)

and T = T + 0.628 q' Cos( (C-13)o b max

ex

where q' = maximum LHGR of the fuel rod in kW/m.max

For conditions when the coolant is undergoing nucleate boiling,

the outside cladding temperature is determined by the Jens and Lottes

correlation (Ref. 19). For the Maine Yankee Parameters, this relation

reduces to

(To)& L 344.8 + 0.845 [qma cos( Z)] 0.25 (C-14)ex

where q = maximum LHGR in kW/mmax

and (T )J&L = outside cladding temperature in °C.

Figures C-3 and C-4 show the bulk and outside cladding axial

temperature distribution at 100% core power for a nominal fuel rod and

a hot fuel rod. At 100% core power, the nominal rod does not undergo

nucleate boiling while the hot fuel rod does.

For various core powers, Figs. C-5 and C-6 display the cladding

outside temperature as a function of linear heat generation rate for a

nominal and hot fuel rod. Superimposed on each figure is the corre-

lation used in the study for the cladding outside temperature. Even

though based upon an arbitrary choice, this correlation closely re-

flects the actual operating conditions. In mathematical terms, the

outside cladding temperature correlation is

Page 91: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-81-

I I I . I I I I I I

to

c a

0

N T C4

.. L .. I .. . I 0

(Do) a y

o0CN

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Z0H

; ¢H

PS

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P4

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C

rz4

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_ __ · __ __ ·

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Page 92: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-82-

I I I I I I I I I

cn

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D E:

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_

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Page 93: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-83-

0 0 0(.o,,)mmlvnn

0'%0

0

4°EDo SZ to

S 0

=,R

Page 94: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-84-

O 0 0:Et~ - _I om ' C C-4

(3o) Mmlyax;'

0

0o

§ o.-% p 4w IO

,'% E* q B Ze o

H

H 0a .e

1 0o U. #

o

Z '

0o ai' :

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Page 95: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-85-

T = 282 + 2.6 q'T

T = 347so

for 0 q' < 25 kW/m

for q' > 25 kW/m

T = outside cladding temperature in °Co

q' = LHGR in kW/m.

where

and

(C-15)

Page 96: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 97: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-87-

APPENDIX D

HALDEN FUEL ROD PARAMETERS

This appendix presents the Halden Boiling Water Reactor experi-

mental fuel rod and operating parameters discussed in Chapter 6 (Ref. 20).

These parameters also represent the fuel rod conditions inputted to

the calculational models.

Parameter

Fuel assembly

Fuel rod

Core active length

Axial power peaking factor

Coolant

System pressure

Coolant inlet temperature

Coolant saturation temperature

Fill gas

Fill gas pressure

Cladding

Fuel

% T.D.

Cladding outside diameter

Cladding inside diameter

Fuel pellet diameter

Cold radial gap width

Burnup

Value

IFA-226

AA

1.7 m

1.2 to 1.7

D20

3.45 MPa

237°C

240°C

Helium

10.1 kPa

Zircaloy-4

90.5% UO2, 9.5% PuO2

92.1

10.69 mm

9.51 mm

9.30 mm

105 pm

0 - 0.1 MWd/kg U

An outside cladding temperature has again been represented as a

two line straight function of linear heat generation rate. Using the

Jens-Lottes equation for nucleate boiling (as in Appendix C), the

following representation seems reasonable:

Page 98: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-88-

T = 240 + 0.6 q'

T = 255o

for 0 < q' < 25 kW/m

(D-1)

for q' > 25 kW/m

T = outside cladding temperature in °Co

q' = LHGR in kW/m.

where

and

Page 99: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-89-

APPENDIX E

COMPUTER PROGRAM LISTING

A sample listing of input parameters is presented in Table E-1.

Not a complete tabulation, this table merely presents an example of

the form for inputting data to initialize the computer program. The

variable names are explained below.

xmodel = the model designation, 1 being the uncracked model,2 being the cracked model

den = fractional theoretical density of the fuel

tco = outside cladding temperature in °C

q = linear heat generation rate in kW/m

gapc = cold radial gap width in pm

radco = outside cold clad radius in mm

radci = inside cold clad radius in mm

radfc = cold fuel pellet radius in mm

Table E-2 displays the computer output for one set of input data.

The input parameters are listed first which identifies the calculation.

These are followed by the parameters computed by the program.

Following Table E-2 is the listing of the Fortran computer pro-

gram used in this study. For a flow chart of this program see

Chapter 2.

Page 100: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-90-

ii . , s4 ni - 4 .: i _. 4 4 4 4 r4 _i 4 4i 4' 4 -4 4 4. 4

m mco m W C o c c 0 o O m 3 3 3 C3 -

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en NNNNNNN 0 C' O O- . 0.'

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in m n 3

N N N N N N N N N N N N r N 1 0 0 ON 101- C- 10% Dc 0c 0- 0% 0I 0% a -M 0% *I 0

NNNNNNNNNNNNNNNNNNN a a ( 0 0 * a * *4I 4 4T 4T 4T 4 4T 4 4 4T 4 4T 4 4 4 4 4 IT 4

00000004 40 0 o.40n 4 40

00 0 '0 '0*, 44

in in in

03 0 0 a 0 3 0 030 3 0000000000040 0 0 0 4 0 4 0 4 0 4.0 4

in in 101 m 3 1) in in in in

00000000000000000000000000oooooo o ooooo00* 0 * 0 c * 0 0 0 * 0 0 0 0 0 0 0 O0 0 0

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0000000000000000000000o 0 0 0 * * * * * * 4 4 4 4 4 4 * * *.. * + * 0n io O iO O n f O nl O O n OO0 - V4 %S _t4 V4 . t NY N m m M M f a a tm i 0 0 0 "a

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00 0 O0 0 C O O0 C O- 0 -- O- OO O0 O0 O0 0 0 0

1

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Eq00 0000 00000000000000000- 4,k 4 4 4 4 4 4 4 4 _ N 4 4 4 4 4 4 4 4 4 4

WI CM1 W CM W CM WI CMt WI Cii WI Cii WI CM WI ~C~ W r ( N C ii Wf· · I~ Ci W Cii W

a

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Page 101: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-91-

model 1 traditional model 2 cracked this is

fractional densit 0.9500

outside clad tem - 347,00 c

linear heat eneration rate = 40.00 kw er

cold aP width = 95.00 um

outside cold clad radius = 5.588 nmm

inside cold clad radius = 4.877 mr,

cold Pellet radius = 4781 mm

inside clad temrP 396,15 c

fuel surface tem = 419.54 c

fuel centerline temp = 1749.62 c

hot fuel radius 4+829 mm

hot aP width = 58.890 um

Percent Pellet contact 30.449

fractional radius for eeuiaxed rain growth

fractional radius for columnar rain Srowth =

fuel rod euivalent temperature = 891+86 c

2.0

0.o 456752

0. 164658

Sample output from comparative study computer program.

'

m

Table E-2.

Page 102: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-92-

i

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-II

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Page 116: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 117: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-107-

APPENDIX F

TABLE OF SYMBOLS

DefiningSymbol Quantity Units Equation

T temperature °c,K

r radius m

6 radial gap width m

6' root mean square cladding-fuelsurface roughness m

%T.D. percent theoretically dense U02 none

D fractional theoretical dense U02 none

P fractional porosity of fuel pellet none

PF UO2 porosity factor (B-2)(normalized to 95% T.D.) none (B-5)

k thermal conductivity W/m.K

k effective UO2 thermal conductivity W/m-K (4-10)e 2

M mesh interval m (2-5)

ET thermal strain none

ET average thermal strain none (2-4)(2-8)

x fuel burnup MWd/kgU

Fb burnup factor none (4-5)

F fraction of circumferentialcracked pellet to claddingcontact none (4-5)

h zero contact pressure gap 2conductance W/m *K (4-2)

h contact gap conductance W/m .K (4-2)c

Page 118: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-108-

h gap conductance W/m *K (4-2)

g (3-2)

p density kg/m3

C constant pressure specificheat capacity J/kg.K

AH enthalpy change J/kg

SH stored heat J/m (2-7)(2-9)

(SH) constant temperature J/m (2-11)eq stored heat (2-12)

f(T) equivalent fuel rod J/m (2-13)temperature function

f'(T) derivative of the function f(T)with respect to temperature J/m.K (2-15)

T equivalent fuel rodeq temperature °C (2-10)

%C.P. percent core power none

q"' rate of heat depositionper unit volume W/m3

q'(LHGR) linear heat generation rate W/m

D equivalent coolant passagediameter m

z fuel rod axial position m

Z active fuel rod length m

e extrapolated zero fluxfuel rod length m

v coolant velocity along fuel rods m/s

(P)w core average H20 viscosity kg/m sw

m core average coolant massflow rate kg/s (C-2)

h bulk coolant to cladding 2heat transfer coefficient W/m *K (C-3)

Page 119: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-109-

ATb bulk coolant temperature riseacross fuel channel (C (C-4)

Tb bulk coolant temperaturealong fuel rod °C (C-9)

(T ) outside cladding temperaturefor the onset of nucleate boiling °C (C-14)

Subscripts

w H20

g fill gas

c cladding

f fuel

o outside cladding

1 inside cladding

2 fuel pellet surface

52 fuel pellet centerline

n radial increment index

Page 120: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …
Page 121: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-111-

REFERENCES

1. M. Ishida and L. Hosokawa, "Light Water Reactor Fuel Rod ModelingStudy at Hitachi, Ltd.", oral presentation at an EPRI sponsoredmeeting on Fuel Rod Modeling, April 1977.

2. K.P. Galbraith, "Pellet-to-Cladding Gap Closure from PelletCracking", XN-73-17, August 1973.

3. N. Fuhrman, V. Pasupathi, D.B. Scott, S.M. Temple, S.R. Pati andT.E. Hollowell, "Evaluation of Fuel Performance in Maine YankeeCore I, Task C", EPRI NP-218, November 1976.

4. T.B. Bailey and M.D. Freshley, "Internal Gas Pressure Behavior inMixed-Oxide Fuel Rods During Irradiation", Nucl. Appl. Tech. 9,233-241(1970).

5. R.M. Carroll, "Fission-Product Release from UO2", Nucl. Safety 4,35-42(1962).

6. P.E. MacDonald and L.B. Thompson, "MATPRO: Version 09, A Handbookof Materials Properties for Use in the Analysis of Light WaterReactor Fuel Rod Behavior", TREE-NUREG-1005, December 1976.

7. A.S. Bain, "Cracking and Bulk Movement in Irradiated Uranium OxideFuel Elements", AECL-1827, September 1963.

8. J.B. Ainscough and F. Rigby, "Measurements of Crack SinteringRates in UO2 Pellets", J. Nucl. Matl. 47, 246-250(1973).

9. J.T.A. Roberts and B.J. Wrona, "Crack Healing in U02", J. Am.Ceramic Soc. 56, 297-299(1973).

10. W.S. Lovejoy and S.K. Evans, "A Crack Healing Correlation Pre-dicting Recovery of Fracture Strength in LMFBR Fuel", Trans. Am.Nucl. Soc. 23, 174-176(1976).

11. P.E. MacDonald and J.M. Broughton, "Cracked Pellet Gap ConductanceModel: Comparison of FRAP-S Calculations with Measured FuelCenterline Temperatures", CONF-750360-2, March 1975.

12. P.E. MacDonald and J. Weisman, "Effect of Pellet Cracking onLight Water Reactor Fuel Temperature", Nucl. Tech. 31, 357-366(1976).

13. Shippingport Atomic Power Station Preliminary Safety AnalysisReport for Light Water Breeder Reactor, 1976.

14. O.R. Olander, "Fundamental Aspects of Nuclear Reactor FuelElements", p. 133, ERDA, 1976.

Page 122: LWR FUEL PERFORMANCE ANALYSIS Fuel Cracking and …

-112-

15. H.B. Meieran and E.L. Westermann, "Summary of Phase II of the EPRILWR Fuel Rod Modeling Code Evaluations Project Using the CYGRO-3,LIFE-THERMAL-1 and FIGRO Computer Programs", ODAI-RP0397-2,RP-397-2, March 1976.

16. M.G. Andrews, H.R. Freeburn, and S.R. Pati, "Light Water ReactorFuel Rod Modeling Code Evaluation, Phase II, Topical Report",CENPD-218, April 1976.

17. J.H. Keenan, F.G. Keyes, P.G. Hill and J.G. Moore, "Steam Tables,Thermodynamic Properties of Water Including Vapor, Liquid, andSolid Phases", John Wiley and Sons, New York, 1969.

18. M.M. El-Wakil, "Nuclear Heat Transport", p. 243, InternationalTextbook Co., New York, 1971.

19. J.R. Lamarsh, "Introduction to Nuclear Engineering", p. 346,Addison-Wesley Publishing Co., 1975.

20. E.T. Laats, P.E. MacDonald and W.J. Quapp, "USNRC-OECD HaldenProject Fuel Behavior Test Program: Experiment Data Report forTest Assemblies IFA-226 and IFA-239", ANCR-1270, December, 1975.