irradiation devices and testing materials assessment meetingirradiation devices and testing a....

22
Materials Assessment Meeting Karlsruhe, 5-8 June 2001 Irradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany Content: n n n Major European Irradiation Facilities n n n Long Term Strategy n n n IFMIF Project n n n Comparison of irradiation properties n n n Small Specimen Test Technology T hi s fi l e c o ntai n s a cu t out of t he t ot al pres e ntati on

Upload: others

Post on 24-Feb-2020

3 views

Category:

Documents


0 download

TRANSCRIPT

Page 1: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Materials Assessment MeetingKarlsruhe, 5-8 June 2001

Irradiation Devices and TestingA. Möslang

Forschungszentrum Karlsruhe FZK, Germany

Content:���� Major European Irradiation Facilities���� Long Term Strategy ���� IFMIF Project���� Comparison of irradiation properties���� Small Specimen Test Technology

This file contains a cutout

of the total presentation

Page 2: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

International Fusion Strategy

Materials Assessment Meeting, FZK, 5-8 June 2001

Construction RunupITER

DEMO

PROTO

RA-FM-Steels

Fission Reactors

IFMIF-CDE(staged Approach)

Operation

Design Construction Operation

Design

HighPerformanceMaterial

Data validationin Fusion Environm.

Ref

. Mat

eria

l 10

dpa

Fusi

on-F

issio

n C

orr.

Irrad

iatio

nFa

ciliti

esM

ater

ials

Dev

ices

Ref

. Mat

eria

l for

DEM

O (7

0 dp

a)

Hig

h Pe

rform

ance

Mat

eria

ls fo

rPR

OTO

(150

dpa

)

Data base developm.incl. Fiss.React.irrad.

Critical issuesTechnology DevelopmentFission Reactor Irradiation

Alternative MaterialsV-alloysSiC/SiC CompositesTi, Cr-alloys

KEP

0 10years20 30 40

EDA + Constr. Phase I(50 mA)

Phase II(125 mA)

Full Operation(2 x 125 mA)

Constr.

Page 3: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

International Fusion Strategy JET 2010 2020 2030

ITER

IFMIF

DEMO

Page 4: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Materials Assessment Meeting, FZK, 5-8 June 2001, A. Möslang

ΟΟΟΟ Existing irradiation facilities only partly fulfill the needs for materialsdevelopment for DEMO reactors (≈≈≈≈150 dpa):οοοο Fission reactors: large irradiation volumes, appropriate n-flux,

but n-spectrum not adequateοοοο Accelerators (e.g. p, He): appropriate dpa & gas production rates, favorable

conditions for in-situ tests, but small volumesΟΟΟΟ ITER testing is limited because fluence accumulation is restricted to ≤≤≤≤10 dpa

and the mode of operation is very different from DEMO(e.g. low temperature, strongly pulsed operation)

However, it is a valuable test bed for integral testing of components likeTBM’s in the low fluence regime.

There is presently no irradiation source that combinesοοοο fusion similar spectrumοοοο high fluence for accelerated materials testingοοοο sufficiently large test volume

Why do we need a dedicatedInternational Fusion Materials Irradiation Facility?

Page 5: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

International Fusion Materials Irradiation FacilityIFMIF

Mission:(i) Qualification of candidate materials up to about full

lifetime of anticipated use in a fusion DEMO reactor

(ii) Calibration and validation of datagenerated from fission reactors and particle accelerators

(iii) Identify possible new phenomena which might occur due to thehigh energy neutron exposure

Page 6: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

D-Li Stripping Neutron Source

Typical Reactions: 7Li(d,2n)7Be 6Li(d,n)7Be 6Li(n,T)4HeDeuterons: 32, 36, 40 MeV 2x 125 mA Beam footprint 5x20 cm2

High flux Medium flux Low fluxLiquid Li Jet (>20 dpa, 0.5 L) (20-1 dpa, 6 L) (<1 dpa, >8 L)

IonSource RFQ Drift Tube Linac

Test CellDeuteron Accelerator Region

Page 7: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Requirements for an Intense Neutron Source(IEA-Workshop in San Diego 1989)

1. Neutron flux/volume relation: Equivalent to 2MW/m2 in 10 L volume [1 MW/m2 ≅ 4.5x1017 n/m2s; E = 14 MeV, 3x10-7 dpa/s for Fe]

2. Neutron spectrum:- Should meet FW neutron spectrum as near as possible- Quantitative criteria are: Primary recoil spectrum (PKA)- Important transmutation reactions (He, H)

3. Neutron fluence accumulation: Demo-relevant fluence 150 dpaNRT in few years

4. Neutron flux gradient: ≤≤≤≤10%/cm5. Machine availability: 70%6. Time structure: Quasi continuous operation7. Good accessibility of irradiation volume for experiments & instrumentation

1 MWy/m2 ≅ 10 dpaNRT for Fe

Page 8: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

10-3 10-2 10-1 100 1010,0

0,2

0,4

0,6

0,8

1,0

no neutron moderator with W moderator with W+C moder. DEMO reactor

Frac

tion

of D

amag

e E

nerg

y pr

oduc

ed b

y P

KA

s

PKA Energy T, MeV

Charakterization of PKA spectra

DEMO-relevant PKA spectra can be perfectly adjusted with neutron moderators & reflectors

IFMIF High Flux Test Module

Point defects→ Creep→ Segregation

Cascades→ Hardening→ Embrittlement

Page 9: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Sensitivity of damage to PKA spectraComparison of different neutron sources

IFMIF (hatched area) meets perfectly the conditions of DEMO-reactor blankets

10-3 10-2 10-1 100 101 1020,0

0,2

0,4

0,6

0,8

1,0

IFMIF no moder. IFMIF with W IFMIF with W+C Fusion DEMO 14 MeV peak

Frac

tion

of D

amag

e E

nerg

y pr

oduc

ed b

y P

KA

s

PKA Energy T, MeV

HFRReactor

Spallation

56Fe

Page 10: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Helium and DPA Production

10-3 10-2 10-1 100 10110-3

10-2

10-1

100

101

102

*preliminary calculation(Filges, Haft)

ESS(Reflector position*)

ESS(Target position*)

DEMO 2.5 MW/m2

HFR

ORR

HFIR

IFMIF (MF)IFMIF (HF)

LAMPF

RTNS

He [a

ppm

/ w

eek]

Displacements [DPA / week]

Page 11: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Damage and Transmutation Calculations

3D MCNP-code calculations based on collided neutrons in Fe and detailed geometrical models

Irradiation parameter ITER* DEMO* IFMIFHFTM**

IFMIFMFTM***

Total neutron flux [n/(s cm2)] 4 x 1014 7.1 x 1014 4x1014 - 1015 3.8 x 1014

Hydrogen production [appm/FPY] 445 780 1000 - 2500 300Helium production [appm/FPY] 114 198 250 - 600 78Damage production [dpa/FPY] 10 19 20 - 55 9H/dpa ratio [appm/dpa] 44.5 41 35 - 50 33He/dpa ratio [appm/dpa] 11.4 10.4 9.5 - 12.5 9Nuclear heating [W/cm3] 10 22 30 - 55 9Wall load [MW/m2] 1.0 2.2 3 - 8 1

* Outboard blankets ** Dependent on the exact position inside the HFTM ***Presently improved

Page 12: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Damage and Transmutation Calculations

3D MCNP-code calculations based on collided neutrons in Fe and detailed geometrical models

Irradiation parameter ITER* DEMO* IFMIF** GDT-NSTotal neutron flux [n/(s cm2)] 4 x 1014 7.1 x 1014 4x1014 - 1015 5.8 x 1015

Hydrogen production [appm/FPY] 445 780 1000 - 2500 707Helium production [appm/FPY] 114 198 250 - 600 167Damage production [dpa/FPY] 10 19 20 - 55 14.4H/dpa ratio [appm/dpa] 44.5 41 35 - 50 49.1He/dpa ratio [appm/dpa] 11.4 10.4 9.5 - 12.5 11.6Nuclear heating [W/cm3] 10 22 30 - 55 18Wall load [MW/m2] 1.0 2.2 3 - 8 1.8

* Outboard blankets ** Dependent on the exact position inside the HFTM

• Correct scaling of H, He and dpa production in all facilities• IFMIF: Accelerated irradiation in

limited volume

02468

101214

Vanadium

Iron

appm

He/

dpa

ITER DEMO IFMIF

Page 13: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Comparison of different neutron spectra

10-3 10-2 10-1 100 101100

101

102

103

104

105

106

107

Neu

tron

Flux

[1010

n/(c

m2 s

)/MeV

]

Neutron Energy [MeV]

DEMO fusion reactor HFR Petten IFMIF HFTM IFMIF MFTM

Page 14: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Neutron spectra in high flux region

10-3 10-2 10-1 100 101100

101

102

103

104

105

106

107

CDA-Design (1996) KEP-Design (2001) DEMO fusion reactor

IFMIF High Flux Test ModuleN

eutro

n flu

x de

nsity

[1010

s-1 c

m-2M

eV-1]

Neutron energy [MeV]

Page 15: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Neutron spectra in medium flux region

10-3 10-2 10-1 100 101100

101

102

103

104

105

106

107

CDA-Design (1996) KEP-Design (2001) DEMO fusion reactor

IFMIF Medium Flux Test ModuleN

eutro

n flu

x de

nsity

[1010

s-1 c

m-2 M

eV-1]

Neutron energy [MeV]���� Neutron spectra improvement: Substantial progress has been achieved very recently���� High and medium flux volumes can be irradiated practically under DEMO reactor conditions

Page 16: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

PKA spectra

103 104 105 10610-8

10-7

10-6

10-5

10-4

10-3

10-2

IFMIF High Flux Test Module Fusion Demo Reactor(HCPB) Fast Reactor (Phenix) High Flux Fission Reactor (Petten)

dσ/d

T [b

arn/

eV]

PKA energy

56Fe

Page 17: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

VTA1VTA2

VIT

Central Shielding Plug

Beam Pipe

Lithium Target

Quench Tank

Shieldingbody

2.5m

1m

Baseline design concept: • Gas coolant systems for all test modules • Modular and highly flexible • Easy user access • Capacity for upgrades

Two-PartTest CellCover

Central Shielding Plug

VTA1

VTA2 VITShielding Body

BeamDirection

IFMIF Test Cell System

Page 18: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

IFMIF Model of Li-Target and Test Assemblies

Page 19: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

• 27 rigs, He-gas cooled• Individual rig temperatures (ohmic heating)• Tirr: 300 - 1000 °C• SSTT: - 7 specimen types - 400-700 specimen - significant volume reduction (20-125 times)

IrradiationCapsule

Rig Wall

Rig Vessel

Rib

FractureToughnessSpecimen

Dynamic/staticFracture ToughnessSpecimen

HeliumInlet

Push-pullFatigueSpecimen

Electrical Heater& Thermocouple

IFMIF High Flux Test Module

Page 20: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

DPA Distribution of High Flux Test Module

>40 dpa/fpy

>30 dpa/fpy

>20 dpa/fpy

FZK-IMF1-ED-AM

Page 21: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Proposed specimen geometry

Small Specimen Test Technology (SSTT)

✔ development not necessary

✔ development completed; YS, UTS and Ag independent on size; generation of material intrinsic properties.✔ development almost completed at FZK; generation of material intrinsic properties;

X experience under irradiation is required; potential for material intrinsic properties

X Properties strongly size & geometry dependent World wide efforts ongoing in US, JA, EU Modelling includes presently: - Master curve shift approachX - FEM modelling - Micro-toughness modelling

✔ X Charpy tests: KLST specimen has become quasi standard in IEA countries Frac. toughness tests: R&D efforts ongoing

Materials Assessment Meeting, FZK, 5-8 June 2001, A. Möslang

Page 22: Irradiation Devices and Testing Materials Assessment MeetingIrradiation Devices and Testing A. Möslang Forschungszentrum Karlsruhe FZK, Germany ... Embrittlement. Sensitivity of damage

Materials Assessment Meeting, FZK, 5-8 June 2001, A. Möslang

Conclusions IFIMIF1. The availability of a dedicated neutron source is indispensable for the qualification of

materials for design and safe operation of DEMO-type fusion reactors.

2. Why the accelerator based D-Li neutron source IFMIF?– Suitability: IFMIF meets all relevant user requirements

(in contrast to earlier concepts like FMIF or ESNIT)

– Feasibility: IFMIF is based on almost established technology and has practically no technological risk

– The developed reference design includes detailed RAM and safety analyses and is conceived for long-term operation with an annual availability of at least 70%

3. The IFMIF conceptual design is at a level of maturity that would readily justify, on atechnical basis, a positive decision towards an engineering phase.

4. SSTT is of outstanding importance for IFMIF

Irradiation devices and testing