generation iv nuclear energy systems

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Brookhaven Science Associates U.S. Department of Energy GENERATION IV NUCLEAR ENERGY SYSTEMS HOW THEY GOT HERE AND WHERE THEY ARE GOING GENERATION IV NUCLEAR ENERGY SYSTEMS GENERATION IV NUCLEAR ENERGY SYSTEMS HOW THEY GOT HERE AND WHERE THEY ARE GOING HOW THEY GOT HERE AND WHERE THEY ARE GOING David J. Diamond Brookhaven National Laboratory Energy Sciences and Technology Department Nuclear Energy and Infrastructure Systems Division Presented at the University of Tennessee April 30, 2003

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Page 1: GENERATION IV NUCLEAR ENERGY SYSTEMS

Brookhaven Science AssociatesU.S. Department of Energy

GENERATION IV NUCLEAR ENERGY SYSTEMSHOW THEY GOT HERE AND WHERE THEY ARE GOING

GENERATION IV NUCLEAR ENERGY SYSTEMSGENERATION IV NUCLEAR ENERGY SYSTEMSHOW THEY GOT HERE AND WHERE THEY ARE GOINGHOW THEY GOT HERE AND WHERE THEY ARE GOING

David J. DiamondBrookhaven National Laboratory

Energy Sciences and Technology DepartmentNuclear Energy and Infrastructure Systems Division

Presented at the University of TennesseeApril 30, 2003

Page 2: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 2

OUTLINE OF PRESENTATIONOUTLINE OF PRESENTATION

n Introduction to the Gen IV (long-term) Nuclear Energy Systems

n The Roadmap - how we got to the Gen IV concepts

n The Not-Gen IV Nuclear Energy Systemsaka the international near-term deployment concepts

n What do the Gen IV concepts look like; what are some of their R&D needs

Page 3: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 3

GENERATION IV NUCLEAR ENERGY SYSTEMSGENERATION IV NUCLEAR ENERGY SYSTEMS

Sodium Fast Reactor (SFR)

Gas-Cooled FastReactor (GFR)

Molten Salt Reactor(MSR)

Supercritical Water Reactor(SCWR)

Very High Temp.Gas Reactor (VHTR)

Lead-alloy Fast Reactor (LFR)

R&DApplicationsSizeFuel

CycleNeutron

Spectrum

Page 4: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 4

GENERATION IV NUCLEAR ENERGY SYSTEMSGENERATION IV NUCLEAR ENERGY SYSTEMS

ClosedFastSodium Fast Reactor (SFR)

ClosedFastGas-Cooled FastReactor (GFR)

ClosedThermalMolten Salt Reactor(MSR)

Open,Closed

Thermal,Fast

Supercritical Water Reactor(SCWR)

OpenThermalVery High Temp.Gas Reactor (VHTR)

ClosedFastLead-alloy Fast Reactor (LFR)

R&DApplicationsSizeFuel

CycleNeutron

Spectrum

Page 5: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 5

GENERATION IV NUCLEAR ENERGY SYSTEMSGENERATION IV NUCLEAR ENERGY SYSTEMS

Advanced Recycle

Electricity,Actinide Mgmt.

Med toLarge

ClosedFastSodium Fast Reactor (SFR)

Fuels, Materials,Safety

Electricity, Actinide Mgmt., Hydrogen

MedClosedFastGas-Cooled FastReactor (GFR)

Fuel, Fuel treatment,Materials, Safety and Reliability

Electricity, Actinide Mgmt., Hydrogen

LargeClosedThermalMolten Salt Reactor(MSR)

Materials, SafetyElectricityLargeOpen,Closed

Thermal,Fast

Supercritical Water Reactor(SCWR)

Fuels, Materials,H2 production

Electricity, Hydrogen,Process Heat

MedOpenThermalVery High Temp.Gas Reactor (VHTR)

Fuels, Materials compatibility

Electricity, Actinide Mgmt., Hydrogen

Small toLarge

ClosedFastLead-alloy Fast Reactor (LFR)

R&DApplicationsSizeFuel

CycleNeutron

Spectrum

Page 6: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 6

THE TECHNICAL ROADMAPTHE TECHNICAL ROADMAP

n Discusses the benefits, goals and challenges, and the importance of the fuel cycle

n Describes evaluation and selection process

n Introduces the six Generation IV systems chosen by the Generation IV International Forum

n Surveys system-specific R&D needs for all six systems

n Collects crosscutting R&D needs

n GIF countries will choose the systems they will work on

n Programs and projects will be founded on the R&D surveyed in theroadmap

n Information available at gif.inel.gov/roadmap/

Page 7: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 7

TECHNOLOGY GOALSTECHNOLOGY GOALS

n Sustainability1. Provide sustainable energy generation that meets clean air

objectives and promotes long-term availability of systems and effective fuel utilization for worldwide energy production

2. Minimize and manage their nuclear waste and notably reduce the long term stewardship burden, thereby improving protection for the public health and the environment

n Safety and reliability3. Operations will excel in safety and reliability

4. Will have a very low likelihood and degree of reactor core damage

5. Will eliminate the need for offsite emergency response

Page 8: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 8

TECHNOLOGY GOALSTECHNOLOGY GOALS

n Economics6. Will have a clear life-cycle cost advantage over other energy

sources

7. Will have a level of financial risk comparable to other energy projects

n Proliferation resistance and physical protection8. Will increase the assurance that they are a very unattractive and

the least desirable route for diversion or theft of weapons-usable materials, and provide increased physical protection against acts of terrorism

Page 9: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 9

INTERNATIONAL NEAR-TERM DEPLOYMENT (1/2)INTERNATIONAL NEAR-TERM DEPLOYMENT (1/2)n Deployment by 2015

n Industry involvement

n Improvement over current advanced LWR performance

n Advanced Boiling Water Reactors • ABWR-II• ESBWR• SWR-1000• HC-BWR

n Modular High-Temperature Gas-Cooled Reactors• GT-MHR• PBMR

Page 10: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 10

INTERNATIONAL NEAR-TERM DEPLOYMENT (2/2) INTERNATIONAL NEAR-TERM DEPLOYMENT (2/2)

n Advanced Pressure Tube Reactor• ACR-700

n Advanced Pressurized Water Reactors• AP-600• AP-1000• APR-1400• APWR+• EPR

n Integral Primary System Reactors• CAREM• IMR• IRIS• SMART

Page 11: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 11

GEN IV NUCLEAR ENERGY SYSTEMSGEN IV NUCLEAR ENERGY SYSTEMS

n Very High Temp. Gas Reactor (VHTR)

n Gas-Cooled Fast Reactor (GFR)

n Supercritical Water Reactor (SCWR)

n Sodium Fast Reactor (SFR)

n Lead-alloy Fast Reactor (LFR)

n Molten Salt Reactor (MSR)

Page 12: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 12

SEQUENCED DEVELOPMENT OF HIGH TEMPERATUREGAS COOLED NUCLEAR ENERGY SYSTEMSSEQUENCED DEVELOPMENT OF HIGH TEMPERATUREGAS COOLED NUCLEAR ENERGY SYSTEMS

PMRGFR

> 950°C for VHT heat process

Fast neutrons & integral fuel cycle for high sustainability

VHTR

Page 13: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 13

VHTR FOR HYDROGEN PRODUCTIONVHTR FOR HYDROGEN PRODUCTION

n Hydrogen demand is already large and growing rapidly• Heavy-oil refining consumes 5% of natural gas for hydrogen production

n Energy security and environmental quality motivate hydrogen as an alternative to oil as a transportation fuel

• Zero-emissions • Distributed energy opportunity

n Water is the preferred hydrogen “fuel”

• Electrolysis using off-peak power

• High-temperature electrolysis• High-temperature

thermochemical water splitting

Page 14: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 14

VERY HIGH TEMPERATURE REACTOR (VHTR)VERY HIGH TEMPERATURE REACTOR (VHTR)

Characteristics

• He coolant• 1000°C outlet temperature• Reactor coupled to H2production facility

• 600 MWth, nominally based on MHTGR

• Coated particle fuel, graphite block (or pebble?) core

Page 15: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 15

Reactor Cavity Cooling System

Reactor Pressure Vessel

Control Rod Drive Stand Pipes

Power Conversion System Vessel

Floors Typical

Generator

Refueling Floor

Shutdown Cooling System Piping

Cross Vessel (Contains Hot & Cold Duct)

35m(115ft)

32m(105ft)

46m(151ft)

GT-MHR REACTOR BUILDINGGT-MHR REACTOR BUILDING

Page 16: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 16

Control Rod Drive Assembly

Refueling Stand Pipe

Control Rod Guide tubes

Cold leg Core Coolant Upper Plenum

Central Reflector Graphite

Annular shaped Active Core

Outer Side Reflector Graphite

Core Exit Hot Gas Plenum

Graphite Core Support Columns

Reactor Vessel

Upper Plenum Shroud

Shutdown Cooling System Module Hot Duct

Insulation Module

Cross Vessel Nipple

Hot Duct Structural Element

Metallic Core Support Structure

Core Inlet Flow

Core Outlet Flow

Insulation Layer for Metallic Core Support Plate

Upper Core Restraint Structure

Control Rods

7m(23 ft)

23.7m(78ft)

2.2m(7ft)

8.2m(27ft) Dia Vessel Flange

Upper plenum -hot plume

mixing - “LOF”

Core -depressurized

cooldown

Flow between hotter/ cooler

channels - “LOF”

Lower plenum - hot

jet mixing

Natural convection and thermal radiation

Core flow -normal operation

GT-MHRGT-MHR

Page 17: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 17

CORE FLOW ISSUES DURING NORMAL OPERATIONCORE FLOW ISSUES DURING NORMAL OPERATION

n Calculation of the coolant channel temperatures during normal operation• Significant local variations in power occur across the core due the non-uniform

location of the reflectors, control rods, and burnable poison assemblies and due to the fuel loading

• Power variations are amplified in the hot channels due to the buoyancy resistance• Therefore the coolant temperatures can vary by more than + or - 200°C from the

average

n Calculation of the core lower plenum flow mixing and pressure drop• Hot jet mixing, complex 3-dimensional flow around the core supports, and the flow

acceleration near the hot duct need to be calculated

n Calculation of the hot duct coolant mixing and insulation effectiveness• Permeation of the hot gas into the insulation is a concern • The entrance conditions are somewhat uncertain, but the flow must be well mixed by

the time it reaches the turbine

Page 18: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 18

Thermal-hydraulic Issues

n Mixing of the gases during bypass events

n Flow distributions among the recuperators and recuperatorefficiency

n Hot streaks at the turbine inlet

Generator

Thrust Bearing

Turbine

High Pressure Compressor

Recouperator

Recouperator

Low Pressure Compressor

Precooler/ Intercooler

Cold Gas to Reactor

Hot Gas from Reactor

PCS Vessel

34m(112ft)

8.2m(27ft) Dia. Vessel Flange

POWER CONVERSION UNITPOWER CONVERSION UNIT

Page 19: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 19

THERMAL-HYDRAULIC ISSUES -ACCIDENT CONDITIONSTHERMAL-HYDRAULIC ISSUES -ACCIDENT CONDITIONS

n Rejection of the heat by natural convection and thermal radiation from the reactor pressure vessel outer wall to the passive cooling system

• Local effects around the hot duct need to be considered• Some separate effects proof testing may be needed

n Reliability, robustness, and effectiveness of the Reactor Cavity Cooling System

n Flow through the core during a loss of circulation accident• Up flow in the hot channels and down flow in the cool channels results in hot

plumes in the upper plenum• The hot and cold channel flow distribution and the upper plenum mixing are

uncertain• Low Reynolds number flow with turbulent, transitional, and/or laminar flow,

buoyancy effects, and gas property variations

n Core cool down during a LOCA

n Air or water ingress during a LOCA

Page 20: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 20

GAS-COOLED FAST REACTOR (GFR)GAS-COOLED FAST REACTOR (GFR)

Characteristics• He (or SC CO2) coolant, direct

cycle energy conversion• 850°C outlet temperature• 600 MWth/288 MWe• U-TRU ceramic fuel in coated

particle, dispersion, or homogeneous form

• Block, pebble, plate or pin core geometry

• Combined use of passive and active safety systems

• Closed fuel cycle system with full TRU recycle

• Direct Brayton cycle energy conversion

Page 21: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 21

ADVANTAGES OF GFRADVANTAGES OF GFR

n GFRs share the sustainability attributes of fast reactors• Effective fissioning of Pu and minor actinides• Ability to operate on wide range of fuel compositions (“dirty fuel”)• Capacity for breeding excess fissile material

n Advantages offered by use of He coolant • Ease of in-service inspection• Chemical inertness• Very small coolant void reactivity (<ßeff)• Potential for very high temperature and direct cycle conversion

n High temperature potential opens possibilities for new applications, including hydrogen production

Page 22: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 22

GFR R&D NEEDSGFR R&D NEEDSn Safety case difficult with low thermal inertia and poor heat transfer

properties of coolant

• Reliance on active and “semi-passive” systems for decay heat removal• Passive reactivity shutdown is also targeted

n High actinide-density fuels capable of withstanding high temperature and fast fluence

• Modified coated particle or dispersion type fuels, e.g.,– (U,TRU)C/SiC– (U,TRU)N/TiN

• Fuel pins with high-temperature cladding, e.g., infiltrated kernel particle

n Core structural materials for high temperature and fast-neutron fluenceconditions (ceramics, composites, refractory alloys)

Page 23: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 23

FUEL / CORE CONFIGURATIONSFUEL / CORE CONFIGURATIONS

n GFR• Metal or ceramic matrix (similar to prismatic)• Pin, plate types (ceramic, metallic)• Pebble/particle

C o m p o s i t e C e r a m i c sF u e l E l e m e n t C o r e L a y - o u t

C o r e V e s s e l

Page 24: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 24

SCWR: GENERAL CHARACTERISTICSSCWR: GENERAL CHARACTERISTICS

n LWR operating at higher pressure (>22.1 MPa) and temperature (280-550°C)• Operating conditions with fossil plant experience

n Higher thermal efficiency (44% vs. 33%)

n No change of phase• Larger enthalpy rise in core• Lower flow rate (~10% of BWR)• Lower pumping power (smaller pumps)

n Simplified direct cycle system• No recirculation• Smaller reactor pressure vessel/containment

n Thermal or fast spectrum possible• Fuel cycle flexibility

Improved Economics

Page 25: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 25

SCWR: OPTIMIZATION OF LWR TECHNOLOGY SCWR: OPTIMIZATION OF LWR TECHNOLOGY

Reactor

Turbine/Generator

Reactor

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Reactor

Turbine/Generator

Reactor

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Reactor

Turbine/Generator

Reactor

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

ReactorSteam-water separation system

Recirculation system

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Reactor

Steam generatorPressurizer

Turbine/Generator

Page 26: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 26

SCWR: EFFECT OF SIMPLIFICATIONSCWR: EFFECT OF SIMPLIFICATION

Page 27: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 27

Fuel assembly

SCWR NEUTRONIC DESIGNSCWR NEUTRONIC DESIGN

n Considerations with core design• Large change in density axially• Average coolant density higher than

in BWR• Downward flow in water rods• Other moderators (BeO, ZrH2)• Square or hexagonal geometry

Water rod

nSafety consideration•Rod ejection accident•Negative moderator reactivity coefficient

Page 28: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 28

BASIC DATA - HEAT TRANSFERBASIC DATA - HEAT TRANSFER

Heat-transfer data at prototypical SCWR conditions (i.e., supercritical water, complex bundle geometry, high heat flux) are needed.

Single-phase heat transfer: Data exist for either simple round tubes and/or surrogate fluids. Existing SCW heat-transfer database and correlations are inconsistent.

Existing correlations and models for SCW heat transfer exhibit large discrepancies and diverging trends

Page 29: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 29

CODES - NUMERICAL INSTABILITIESCODES - NUMERICAL INSTABILITIES

Large (albeit continuous) variation of the thermo-physical properties…

… may result in code execution failures.

Page 30: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 30

SODIUM-COOLED FAST REACTOR (SFR)SODIUM-COOLED FAST REACTOR (SFR)

Characteristics• Sodium coolant, 550°C Tout• 150 to 1500 MWe• Pool or loop plant configuration

• Intermediate heat transport system

• U-TRU oxide or metal-alloy fuel

• Hexagonal assemblies of fuel pins on triangular pitch

Page 31: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 31

SFR SAFETY R&D NEEDSSFR SAFETY R&D NEEDS

n Demonstration of passive safety design: providing assurance that the physical phenomena and related design features relied upon to achieve passive safety are adequately characterized

• Axial fuel expansion and radial core expansion– Experimental data plus deterministic models required for accurate core

representation (particularly, minor-actinide-bearing fuels)– Reduce uncertainties in T-H quantities by using more detailed models

- Multi-pin subassembly, full assembly-by-assembly, coupled neutronics-thermal-hydraulic calculation

- Accurate duct-wall and load pad temperatures required for calculating bending moments in each subassembly to characterize core restraint and expansion

- CFD tools for benchmark calculations or routine design calculations?

• Self-activated shutdown systems• Passive decay heat removal systems

– CFD models useful for resolution of complex natural circulation flow paths

Page 32: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 32

SFR SAFETY R&D NEEDS (CONT’D)SFR SAFETY R&D NEEDS (CONT’D)

n Accommodation of extremely low probability but higher consequence accident scenarios• Demonstrate that passive mechanisms exist to preclude recriticality in

a damaged reactor• Show that debris from fuel failure is coolable within the reactor vessel

n Implication for safety analysis tools• Requires analytical and experimental investigations of mechanisms

that will ensure passively safe response to bounding events that lead to fuel damage– e.g., out-of-pile experiments involving reactor materials are

recommended for metal fuels• Local feedback and material motion modeling required

Page 33: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 33

LEAD-COOLED FAST REACTOR (LFR)LEAD-COOLED FAST REACTOR (LFR)

Characteristics

• Pb or Pb/Bi coolant

• 550°C to 800°C outlet temperature

• Fast Spectrum

• Multi-TRU recycle

• 50–1200 MWe

• 15–30 year core life

Options• Long-life (10-30 yrs), factory-fabricated

battery (50-150 MWe) for smaller grids and developing countries

• Modular system rated at 300-400 MWe• Large monolithic plant at ~1,200 MWe• Long-term, Pb option is intended for

hydrogen generation – outlet temperature in the 750-800oC range

Page 34: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 34

CHARACTERISTICS OF LEAD ALLOY COOLANTCHARACTERISTICS OF LEAD ALLOY COOLANT

n Low Neutron Absorption and Slowing Down Power• Allow to open the lattice, increase coolant volume fraction absent a

neutronics penalty – pumping requirements also dictate open lattice• Facilitates natural circulation

n High Boiling Temperature at Atmospheric Pressure (~1700°C)• Unpressurized primary (precludes loss of coolant accident initiator)• Margins are available to employ passive safety – based on

thermo/structural feedbacks• Potential to raise core outlet temperature (~800°C suitable for H2

production and other process heat missions)n Non-vigorous reaction with air and water

• Potential to simplify heat transport circuits• Potential to simplify refueling approaches

Page 35: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 35

MOLTEN SALT REACTOR (MSR)MOLTEN SALT REACTOR (MSR)

HeatExchanger

Reactor

GraphiteModerator

SecondarySalt Pump

Off-gasSystem

PrimarySalt Pump

PurifiedSalt

ChemicalProcessing

Plant

Turbo-Generator

FreezePlug

Critically Safe, Passively Cooled Dump Tanks(Emergency Cooling and Shutdown)

Steam Generator

NaBF _NaFCoolant Salt

4

72LiF _Th

Fuel Salt

_BeF F _UF4 4

566Co

704Co

454Co

621Co

538 Co

Page 36: GENERATION IV NUCLEAR ENERGY SYSTEMS

Slide 36

MOLTEN SALT REACTOR (MSR)MOLTEN SALT REACTOR (MSR)

Characteristics• Molten fluoride salt fuel• 700–800°C outlet temperature• Intermediate heat transport

circuit• ~1000 MWe or larger• Low pressure (<0.5 MPa)• Graphite core structure

channels flow of actinide bearing fuel

Safety analysis issues• Modeling of nuclear, thermal,

& physio-chemical processes (e.g., FP and MA solubility, noble metal FP plate-out, …)

• Lack of established analysis capabilities

• Regulatory framework not defined