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Hindawi Publishing Corporation Physics Research International Volume 2012, Article ID 648758, 2 pages doi:10.1155/2012/648758 Editorial Nonlinear Optics of Nanostructures Vladimir I. Gavrilenko, 1 Tatiana V. Murzina, 2 and Goro Mizutani 3 1 Department of Physics, Center for Materials Research, Norfolk State University, Norfolk, VA 23504, USA 2 Department of Physics, Moscow State University, Moscow 119991, Russia 3 Japan Advanced Institute of Science and Technology, School of Materials Science, 1-1 Asahidai, Ishikawa, Nomi 923-1292, Japan Correspondence should be addressed to Vladimir I. Gavrilenko, [email protected] Received 31 October 2012; Accepted 31 October 2012 Copyright © 2012 Vladimir I. Gavrilenko et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. The optical properties of nanostructures are fascinating and useful for a variety of applications. Nanotechnologies are poised to revolutionize medicine, manufacturing, energy production, and other fundamental features of everyday life in the 21st century. The unique nonlinear optical properties of nanoscale materials are size dependent; they do not naturally occur in larger bulk materials. The selected collection of papers included in this special issue demon- strates that nonlinear optics of the bulk contrasts markedly with the current state of knowledge about the optics of surfaces and interfaces in nanomaterials. It is challenging to understand optical properties of dierent complex materials (aggregated molecular and polymer systems, crystalline and noncrystalline solids) at the microscopic scale. One of the major objectives of nanoscience is a detailed understanding of the physics and chemistry behind the inter- action between objects (surfaces, particles, and individual molecules) at the nanoscale. Questions need to be answered regarding how nanoparticles can be stabilized, and in what media, how nanoparticles interact and influence each other and solid surfaces, and what proportions in a hybrid system make a critical dierence. How can these characteristics be realistically predicted and extracted from nonlinear optics? The papers of this special issue address the following topics: (i) experimental technique of nonlinear optics in nano- materials; (ii) theory of nonlinear optical response from surfaces and nanostructures; (iii) modeling and simulation of nonlinear optical func- tions in nanomaterials; (iv) nonlinear optics of surfaces and interfaces; sur- face steps and imperfections; low-dimensional sys- tems, quantum wells, and nanowires; nanoplasmonic structures and metamaterials; chiral nanostruc- tures; nanostructured photonics crystals; micro- and nanocavities, ring cavities; excitons in nanoparticles; self-assembled monolayers; biophotonic crystals; (v) electrical- and magnetic-field-induced nonlinear optics in surfaces and nanostructures; (vi) nonlinear magnetooptics of nanostructures and mag- netophotonic crystals; (vii) Terra-Herz generation in nanoparticles; (viii) ultrafast nonlinear spectroscopy of nanoparticles. Second harmonic generation (SHG) data from Si(001)/ SiO 2 heterostructures and multiquantum well systems are reviewed by T. V. Murzina et al. The SHG response from these samples comes from the thin interface layers containing information about specifics of the microscopic structures on Si(001)-SiO 2 interface. Transient atomic vibration of Cu(111) covered with alkali metals is studied using ultrafast time-domain SHG technique by K. Watanabe and Y. Matsumoto. They discovered that the initial phases of the oscillating component of SHG intensity after the excitation pulse reflects the origin of the relevant electronic excitation at the metal-metal interface. A nonlinear optical microscope developed to produce three-dimensional images of second harmonic generation from polar surfaces is described by H. Yokota et al. This approach represents activity in the development of next generation nonlinear optical diagnostics of solid surfaces and interfaces.

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Page 1: Editorial NonlinearOpticsofNanostructuresdownloads.hindawi.com/archive/2012/648758.pdf · useful for a variety of applications. Nanotechnologies are poised to revolutionize medicine,

Hindawi Publishing CorporationPhysics Research InternationalVolume 2012, Article ID 648758, 2 pagesdoi:10.1155/2012/648758

Editorial

Nonlinear Optics of Nanostructures

Vladimir I. Gavrilenko,1 Tatiana V. Murzina,2 and Goro Mizutani3

1 Department of Physics, Center for Materials Research, Norfolk State University, Norfolk, VA 23504, USA2 Department of Physics, Moscow State University, Moscow 119991, Russia3 Japan Advanced Institute of Science and Technology, School of Materials Science, 1-1 Asahidai, Ishikawa, Nomi 923-1292, Japan

Correspondence should be addressed to Vladimir I. Gavrilenko, [email protected]

Received 31 October 2012; Accepted 31 October 2012

Copyright © 2012 Vladimir I. Gavrilenko et al. This is an open access article distributed under the Creative Commons AttributionLicense, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properlycited.

The optical properties of nanostructures are fascinating anduseful for a variety of applications. Nanotechnologies arepoised to revolutionize medicine, manufacturing, energyproduction, and other fundamental features of everydaylife in the 21st century. The unique nonlinear opticalproperties of nanoscale materials are size dependent; theydo not naturally occur in larger bulk materials. The selectedcollection of papers included in this special issue demon-strates that nonlinear optics of the bulk contrasts markedlywith the current state of knowledge about the optics ofsurfaces and interfaces in nanomaterials. It is challenging tounderstand optical properties of different complex materials(aggregated molecular and polymer systems, crystalline andnoncrystalline solids) at the microscopic scale.

One of the major objectives of nanoscience is a detailedunderstanding of the physics and chemistry behind the inter-action between objects (surfaces, particles, and individualmolecules) at the nanoscale. Questions need to be answeredregarding how nanoparticles can be stabilized, and in whatmedia, how nanoparticles interact and influence each otherand solid surfaces, and what proportions in a hybrid systemmake a critical difference. How can these characteristics berealistically predicted and extracted from nonlinear optics?The papers of this special issue address the following topics:

(i) experimental technique of nonlinear optics in nano-materials;

(ii) theory of nonlinear optical response from surfacesand nanostructures;

(iii) modeling and simulation of nonlinear optical func-tions in nanomaterials;

(iv) nonlinear optics of surfaces and interfaces; sur-face steps and imperfections; low-dimensional sys-tems, quantum wells, and nanowires; nanoplasmonicstructures and metamaterials; chiral nanostruc-tures; nanostructured photonics crystals; micro- andnanocavities, ring cavities; excitons in nanoparticles;self-assembled monolayers; biophotonic crystals;

(v) electrical- and magnetic-field-induced nonlinearoptics in surfaces and nanostructures;

(vi) nonlinear magnetooptics of nanostructures and mag-netophotonic crystals;

(vii) Terra-Herz generation in nanoparticles;

(viii) ultrafast nonlinear spectroscopy of nanoparticles.

Second harmonic generation (SHG) data from Si(001)/SiO2 heterostructures and multiquantum well systems arereviewed by T. V. Murzina et al. The SHG response fromthese samples comes from the thin interface layers containinginformation about specifics of the microscopic structures onSi(001)-SiO2 interface.

Transient atomic vibration of Cu(111) covered with alkalimetals is studied using ultrafast time-domain SHG techniqueby K. Watanabe and Y. Matsumoto. They discovered that theinitial phases of the oscillating component of SHG intensityafter the excitation pulse reflects the origin of the relevantelectronic excitation at the metal-metal interface.

A nonlinear optical microscope developed to producethree-dimensional images of second harmonic generationfrom polar surfaces is described by H. Yokota et al. Thisapproach represents activity in the development of nextgeneration nonlinear optical diagnostics of solid surfaces andinterfaces.

Page 2: Editorial NonlinearOpticsofNanostructuresdownloads.hindawi.com/archive/2012/648758.pdf · useful for a variety of applications. Nanotechnologies are poised to revolutionize medicine,

2 Physics Research International

The theoretical paper by Zh. Kudyshev et al. is focusedon generalized analytical solution for nonlinear wave prop-agation in waveguide couplers. Quite a general case ofthe system is considered characterized by linear refractiveindexes with opposite signs, nozero phase mismatch betweenthe channels, and arbitrary nonlinear coefficients.

SHG generation from the Pt-nanowire arrays fabricatedon MgO(110) templates is reviewed by Y. Ogata and G.Mizutani. A contribution of roughness has been discussed ina context of the nanowire array radiation sensitivity.

All contributions to this issue contain analysis of trendsand suggestions towards a rapid development of the nonlin-ear optical diagnostics of nanostructures.

Vladimir I. GavrilenkoTatiana V. Murzina

Goro Mizutani

Page 3: Editorial NonlinearOpticsofNanostructuresdownloads.hindawi.com/archive/2012/648758.pdf · useful for a variety of applications. Nanotechnologies are poised to revolutionize medicine,

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