controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis...

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Page 1: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

激发能相关的能级密度参数和重核衰变性质

叶 巍

(东南大学物理系 南京 )

Page 2: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

内容

◆ 问题背景

◆ 理论模型

◆ 计算结果和结论

Page 3: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

能级密度的重要性

● controlling the statistical decay of excited nuclei

● an crucial input for nucleosynthesis calculations (r-process), reactor science, etc.

Page 4: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Fermi-gas level-density expression

3/22

* *FG rot2

exp 2 aUa(E , J) 2J 1 , U E E (J)

2I 12 U

a

level-density parameter

It is employed in most statistical-model calculations

Page 5: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

The level density parameter a is parametrized as:

d( ) [1 )) W / U]a U a (1-exp(-U/ E

d

U :W ::

a smoothed level-density parameter thermal energy

shell correction to the liquid-drop mass 18-20 MeV

E

Page 6: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

1. Evaporation process: evaporation spectra

a

R.J.Charity, PRC82,014610(2010), and many other works

To fit energy spectra of evaporated particles, is large at low E* and small at higher E*, suggesting that must be dependent on E*

aa

Page 7: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

2. Fission process: cross sections, particle yields

Critical factors that strongly influence the decay

mechanism of heavy nuclei at high energy

include:

A, E*, J, a(U) [af /an], , etc.

Page 8: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Experimental observation of enhanced emission of light particles prior to fission (with respect to predictions from standard statistical models) with increasing excitation energy in fusion-fission reactions. This is due to dissipation effects.

Page 9: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Theoretical Model

Page 10: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

dq 1 dS(q,E*) T(t)

dt M dq M

The Langevin equation reads

q is the dimensionless fission coordinate and is definedas half of the distance between the center of mass of the future fission fragments divided by the radius of the compound nucleus. T is temperature, M is inertia parameter and is friction strength

(t) is a time-dependent stochastic variable which satisfies < (t) >=0 and < (t) (t’)> = 2δ(t-t’)

Page 11: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

The driving force of the Langevin equation is calculated from the entropy:

E* is the total internal energy of the system, V(q) is potential energy.

deformation-dependent level density parameter

a(q) = a1A + a2 A2/3Bs(q)

where Bs(q) is the dimensionless surface area (for a sphereBs= 1). It is used to calculate af /an.

s(q,E*) 2 a(q)[E* V(q)]

Page 12: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

● Evaporation residue cross section ER

Previous works on the role of the parameter af /an in the decay modes of thermal nuclei

B.Lott, et al. PRC 01, adjusting af /an to fit residue cross section data based on a statistical model

Page 13: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

af /an changes with fissility

W.Ye, PRC81 (2010) 011603(R)

Page 14: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

relativistic heavy-ion collisions vs. fusion reactions CN: (high E*,low L) vs. (low E*,high L)

W.Ye, PRC83 (2011) 044611

Page 15: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

● spin distribution of evaporation residue

cross sections ER(L)

Page 16: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

W.Ye, NPA853 (2011) 61

Page 17: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

● prescission particle yields

Page 18: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

role of spin: af /an (L)

Reactions systems

16O+181Ta 197Tl vs. 3,4He+197Au 200,201Tl

Page 19: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Scaling analysis of fission probability of systems 200Tl (right figure) and 201Tl (left figure) based on the standard statistical model

These figures are taken from L.G.Moretto et al., PRL75, 4186 (1995)and Th. Rubehn et al., PRC54, 3062 (1996)

Page 20: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

16O+181Ta 197Tl

W.Ye, PRC84 (2011) 034617

Page 21: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Recent work on excitation-energy dependent af /an(E*) and its effects on the decay of hot nuclei

suggested probes: excitation energy at scission

E* = E*sc + V(q) + Ecoll + Eevap (tsc)

Ecoll is the kinetic energy of the collective degrees

of freedom, and Eevap(t) is the energy carried

away by all evaporated particles by the scission

time tsc

Page 22: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

picture of fission process

Page 23: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

Choose spallation reactions induced by

high energy protons

Models: QMD + SM, L.Ou, Z.X.Li, X.Z.Wu, etc.

BUU + SM, G.C.Yong, W.Zuo

INCL + SM , Belgium

Page 24: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

main characteristics:

● the thermal excitation energy of the produced excited nuclei in spallation can reach 1 GeV

● significantly reduce side effects from compression, deformation and high spins. These distortions complicate the description of de-excitation process of excited nuclear systems

Page 25: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

W.Ye, PRC85 (2012) 011601(R)

Page 26: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc
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Page 29: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

● The sensitivity of E*sc to nuclear friction depends on the af /an (E*).

● Experimentally, to probe information of af /an (E*), populating heavy systems with spallation reactions can significantly lower side effects associated with angular momentum, deformation, etc.

● Applications to spallation-induced reactions and the decay of superheavy nuclei.

Conclusions

Thanks for your attentions

Page 30: controlling the statistical decay of excited nuclei an crucial input for nucleosynthesis calculations (r-process), reactor science, etc

W.Ye, High Energy Phys. Nucl. Phys. 26 (2000) 52

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