chapter 6: present day ozone distribution and trends relevant to climate change a. gaudel, o. r....

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Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper, G. Ancellet, J. Cuesta, G. Dufour, F. Ebojie, G. Huang, S. S. Kulawik, B. Latter, T. Leblanc, J. Liu, X. Liu, J. Neu, H. Petetin, I. Petropavlovskikh, H. Tanimoto, D. Tarasick, V. Thouret, C. Wespes, H. Worden, C. Vigouroux, J. Ziemke TOAR Workshop 1.03, Beijing, January 25 th 2016

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Chapter 6: Present day ozone distribution and trends relevant to climate change Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate 1.2 Description of the relevant metrics Section 2 – Description of data sets Section 3 – Present day distribution of ozone Section 4 – Trends Section 5 – Discussions and Conclusions

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Page 1: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

A. Gaudel, O. R. Cooper, G. Ancellet, J. Cuesta, G. Dufour, F. Ebojie, G. Huang, S. S. Kulawik, B. Latter, T. Leblanc, J. Liu, X. Liu, J. Neu, H. Petetin, I. Petropavlovskikh, H. Tanimoto, D. Tarasick, V. Thouret, C. Wespes, H. Worden, C. Vigouroux, J. Ziemke

TOAR Workshop 1.03, Beijing, January 25th 2016

Page 2: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction

Section 2 – Description of data sets

Section 3 – Present day distribution of ozone

Section 4 – Trends

Section 5 – Discussions and Conclusions

Page 3: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets

Section 3 – Present day distribution of ozone

Section 4 – Trends

Section 5 – Discussions and Conclusions

Page 4: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 1 – Introduction

1.1 Present day distribution and trends of ozone metrics relevant to climate Summary of what is already available in the peer-reviewed literature

1.2 Description of the relevant metrics Coordinate with Chapter 3. Must conform to the list of metrics approved by the TOAR

Steering Committee on July 31, 2015 and available on the TOAR website: http://www.igacproject.org/TOAR

Page 5: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets2.1 Satellite 2.2 FTIR and Umkehr2.3 IAGOS, Ozonesondes, TOST, lidar2.4 Regionally representative surface sites

Section 3 – Present day distribution of ozone

Section 4 – Trends

Section 5 – Discussions and Conclusions

Page 6: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets2.1 Satellite 2.2 FTIR and Umkehr2.3 IAGOS, Ozonesondes, TOST, lidar2.4 Regionally representative surface sites

Section 3 – Present day distribution of ozone

Section 4 – Trends

Section 5 – Discussions and Conclusions

Overlap with Chapter 2 = Same as in Chapter 2 with much less details

Page 7: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets2.1 Satellite 2.2 FTIR and Umkehr2.3 IAGOS, Ozonesondes, TOST, lidar2.4 Regionally representative surface sites

Section 3 – Present day distribution of ozone

Section 4 – Trends

Section 5 – Discussions and Conclusions

Overlap with Chapter 2, 3 and 4 = Different criteria, question of homogenization

Page 8: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 2 – Description of data sets

2.1 Satellite

OMI/MLS, SCIAMACHY, TES, IASI, IASI+GOME2, GOME, OMI

Unitsppbv, DU, Tg

MetricsMonthly mean

Key figuresGlobal map (5°x5°)Time series for latitude bandsRegional map

Relation used to convert DU to ppbvO3 (ppbv) = 1.25 x 1013.25 x TCO (DU) / (Ps – Pt ) (Ziemke et al., 2001)O3 (ppbv) = 1270 x TCO (DU) / (Ps – Pt )

Page 9: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 2 – Description of data sets

2.2 FTIR and Umkehr

Unitsppbv, DU

MetricsSeasonal mean

Key figuresTime series site by siteGlobal map

FTIR8 sites between 80N and 80S with 20yrs of datacolumn surface-8kmSunny day

Umkehr5 sites between 65N and 45S with 20yrs of data3 layers: 1-column surface-250hPa

2-surface-500hPa3-500-250hPa

Page 10: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 2 – Description of data sets

2.3 IAGOS, Ozonesondes, TOST, lidar

Unitsppbv, DU

MetricsMonthly meanAnnual meanSeasonal mean

Key figuresGlobal map upper troposphereGlobal map per altitude rangeTime series site by site

IAGOSFrankfurt/Munich North AmericaAsiaMiddle East

Ozonesondes12 sites with more than 20yrs of data without changing instrument

Lidar OHP, FranceTable Mountain, California, USA

TOSTGlobal tropospheric ozone with resolution: 5°x5°x1km

Page 11: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 2 – Description of data sets

2.4 Regionally representative surface sites

Rural sites - regionally representative and minimally impacted by local emissions

based on human population and nighttime lights

Page 12: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets2.1 Satellite 2.2 FTIR and Umkehr2.3 IAGOS, Ozonesondes, TOST, lidar2.4 Regionally representative surface sites

Section 3 – Present day distribution of ozone3.1 Surface sites 3.2 Free tropospheric mixing ratios 3.3 Tropospheric columns

Section 4 – Trends

Section 5 – Discussions and Conclusions

Page 13: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Surface Sites - Seasonal cycleSurface rural sites US 2006-2010 Summer (JJA)

3.1 Surface sites

Section 3 - Present day distribution of tropospheric ozone

Page 14: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

TOST - 8-10km in ppbv 2009-2012

DJF MAM

JJA SON

20 100

IAGOS - Upper troposphere (15-75 hPa below 2pvu) in ppbv 2009-2013

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.1 Global maps of the lower, mid- and upper troposphere

DJF MAM

JJA SON

0 200100

Page 15: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

TOST - 8-10km in ppbv 2009-2012

DJF MAM

JJA SON

20 100

IAGOS - Upper troposphere (15-75 hPa below 2pvu) in ppbv 2009-2013

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.1 Global maps of the lower, mid- and upper troposphere

DJF MAM

JJA SON

0 200100

Page 16: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

TOST - 8-10km in ppbv 2009-2012

DJF MAM

JJA SON

20 100

IAGOS - Upper troposphere (15-75 hPa below 2pvu) in ppbv 2009-2013

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.1 Global maps of the lower, mid- and upper troposphere

DJF MAM

JJA SON

0 200100

Page 17: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

4.5km in ppbv 2009-2012 – TOST

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.1 Global maps of the lower, mid- and upper troposphere

1.5km in ppbv 2009-2012 – TOST

Page 18: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

4.5km in ppbv 2009-2012 – TOST

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.1 Global maps of the lower, mid- and upper troposphere

1.5km in ppbv 2009-2012 – TOST

Page 19: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 3 - Present day distribution of tropospheric ozone

3.2 Free Troposphere mixing ratios3.2.2 Diurnal Variability

IAGOS – Frankfurt – Diurnal variability from the surface to the tropopause between Aug 1994 and Dec 2013

Audrey Gaudel
I have to get the last update of the plot
Page 20: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 3 - Present day distribution of tropospheric ozone 3.2 Free Troposphere mixing ratios

3.2.3 Regional distribution of lower tropospheric ozone

Surface-6km in DU 6-12km in DUIASI

DJF

MAM

JJA

SON

Over ChinaIn 2010

IASI+GOME2 Over EuropeIn August 2009

Surf-3km in ppbv 3-9km in ppbv

4 32 10 50

Page 21: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

DJF MAM

JJA SON

TOC in DU 2000s – TOST

Section 3 - Present day distribution of tropospheric ozone

3.3 Global distribution of tropospheric ozone column

TOC in DU 2009-2013 – OMI/MLSDJF MAM

JJA SON

5°x5°

0

60

0 60

5°x5°

Page 22: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

DJF MAM

JJA SON

TOC in DU 2000s – TOST

Section 3 - Present day distribution of tropospheric ozone

3.3 Global distribution of tropospheric ozone column

TOC in DU 2009-2013 – OMI/MLSDJF MAM

JJA SON

5°x5°

0

60

0 60

5°x5°

Page 23: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

DJF MAM

JJA SON

TOC in DU 2000s – TOST

Section 3 - Present day distribution of tropospheric ozone

3.3 Global distribution of tropospheric ozone column

TOC in DU 2009-2013 – OMI/MLSDJF MAM

JJA SON

5°x5°

0

60

0 60

5°x5°

Page 24: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 3 - Present day distribution of tropospheric ozone

3.3 Global distribution of tropospheric ozone column

0 10060

in ppbv

Page 25: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Chapter 6: Present day ozone distribution and trends relevant to climate change

Section 1 – Introduction 1.1 Present day distribution and trends of ozone metrics relevant to climate1.2 Description of the relevant metrics

Section 2 – Description of data sets2.1 Satellite 2.2 FTIR and Umkehr2.3 IAGOS, Ozonesondes, TOST, lidar2.4 Regionally representative surface sites

Section 3 – Present day distribution of ozone3.1 Surface sites 3.2 Free tropospheric mixing ratios 3.3 Tropospheric columns

Section 4 – Trends4.1 Surface sites 4.2 Free tropospheric mixing ratios4.3 Tropospheric columns

Section 5 – Discussions and Conclusions

Page 26: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

Trends between 1990-1999 and ending between 2000-2010 Surface below 1km Surface above 1km lower troposphere from ozonesondes lower troposphere from aircraft

4.1 Surface sites

Page 27: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

Trends between 1990-1999 and ending between 2000-2010 Surface below 1km Surface above 1km lower troposphere from ozonesondes lower troposphere from aircraft

4.1 Surface sites

Page 28: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.2 Free troposphereGreen triangle = Mountain sitesMountain sites

DJF MAM

SONJJA

Page 29: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.2 Free troposphereMountain sites - Median

DJF MAM

SONJJA

Green triangle = Mountain sites

Page 30: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.2 Free troposphere

Sonde/MOZAIC/SurfaceMOZAIC/IAGOS over Frankfurt

Page 31: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

TOST (ppbv) – 4.5 km

TOST (ppbv) – 1.5 km

4.2 Free troposphere

Page 32: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

5°x5° deg

4.3 Tropospheric column

Page 33: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column

OMI/MLS TOC 2005-2015 5°x5°Annual mean

White dots indicate grid cells with statistically significant trends

Page 34: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

5x5 deg

DJF MAM

4.3 Tropospheric column

OMI/MLS TOC 2005-2015 5°x5°

Page 35: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

JJA SON

4.3 Tropospheric column

OMI/MLS TOC 2005-2015 5°x5°

Page 36: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column

OMI/MLS - Tg

Page 37: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Mean Value Deseasonalized % Anomalies

Anomaly = 100 * (xmonth(lat) – time mean [xmonth(lat)])/time mean

Tropics andN. mid-lat reachhighest % anomaly2010-2011

Section 4 - Global trends of tropospheric ozone 4.3 Tropospheric column

Page 38: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column

IASI Column Average VMR surface-400 hPa IASI Column Average VMR (surface-400 hPa) Anomaly

Page 39: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column

GOME/OMI - ppbv GOME-1/GOME-2A - VMR

Page 40: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column FTIR surface-8km in DUDJF MAM

SONJJA

Page 41: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric column FTIR surface-8km in DUDJF MAM

SONJJA

Significant positive trends Lauder in boreal springIzana in boreal summer

Page 42: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric columnDJF MAM

SONJJA

Umkehr surface-250hPa in DU

Page 43: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Section 4 - Global trends of tropospheric ozone

4.3 Tropospheric columnDJF MAM

SONJJA

Umkehr surface-250hPa in DU

Significant positive trends Fairbanks in boreal spring

Significant negative trends OHP and Perth in boreal spring and summer

Page 44: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Summary

High ozone values over East Asia, India, East Mediterranean in MAM/JJA Increase of ozone over Asia Global increase of ozone according to surface sites and OMI/MLS Decrease of ozone according to TES-IASI and some Umkehr stations

Page 45: Chapter 6: Present day ozone distribution and trends relevant to climate change A. Gaudel, O. R. Cooper,…

Coordination/overlap with other chapter

Chapter 2: description of data setsChapter 7: metrics used to evaluate modelsChapter 2, 4, 5: Criteria for the regional representativeness of surface sites