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Time-modulation of electron-capture decay factordetected at GSI, Darmstadt

Byung Kyu Park

Department of PhysicsUniversity of California, Berkeley

Physics 250March 20, 2008

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 1 / 19

Outline

1 The Experiment

2 Hypotheses

3 Neutrino Oscillation

4 Prospects

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 2 / 19

The Facility

Gesellschaft für Schwerionenforschung, Darmstadt1

1http://www.gsi.de/Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 3 / 19

What they study

Decay schemes for neutral Pr-140 and Pm-142

Atomic charge state affects decay rates and branching ratio.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 4 / 19

Heavy-ion production and storage

For runs 1 and 2

Schematic layout of the facility with heavy-ion synchrotron SIS, thefragment separator FRS, and the storage-cooler ring ESR highlighted.2

2Yu. A. Litvinov et al., arXiv:nucl-ex/0509019Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 5 / 19

Heavy-ion production and storage

For runs 3 and 4

Revolution frequency of ions in storage is measured by Schottky massspectroscopy. This experiment is described in detail by Litvinov.3

3Yu. A. Litvinov et al., arXiv:0801.2079v1Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 6 / 19

Heavy-ion production and storage

Tabulated experimental parameters for all runs

run ion E(152Sm) L(9Be) #inj[MeV/u] [mg/cm2]

1 140Pr58+ 507.8 1032 4532 140Pr58+ 507.8 1032 8423 140Pr58+ 601.1 2513 58074 142Pm60+ 607.4 2513 7011

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 7 / 19

Weak decay

Example signal

electron-capture: 140Pr58+ →140 Ce58+ + νe + KE, ∆f ≈ 300 Hz

β+ decay: 142Pm60+ →142 Nd59+ + e+ + νe + KE, ∆f ≈ −150 kHz

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 8 / 19

Weak decay

Example signal

electron-capture: 140Pr58+ →140 Ce58+ + νe + KE, ∆f ≈ 300 Hz

β+ decay: 142Pm60+ →142 Nd59+ + e+ + νe + KE, ∆f ≈ −150 kHz

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 8 / 19

Experimental result

with 140Pr58+

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result

with 140Pr58+

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result

with 140Pr58+

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result

with 140Pr58+

Exponential decay with a modulation at a period of ≈ 7 s.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result

with 142Pm60+

Inset shows Fourier transform of the datashowing a peak at f = 0.14 Hz again.

Data with the sinusoidal fit for first 36seconds

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 10 / 19

Experimental result

Fit parameters

Fit parameters of 140Pr dataEq. N0λEC λ a ω χ2/DoF1 34.9(18) 0.00138(10) - - 107.2/732 35.4(18) 0.00147(10) 0.18(3) 0.89(1) 67.18/70

Fit parameters of 142Pm dataEq. N0λEC λ a ω χ2/DoF1 46.8(40) 0.0240(42) - - 63.77/382 46.0(39) 0.0224(41) 0.23(4) 0.89(3) 31.82/35

Null hypothesis of pure exponential decay is excluded to 99%confidence level based on χ2 tests.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 11 / 19

Hypotheses: (1) technical artifact?

Procommon period of 7 s for140Pr58+ and 142Pm60+.

Conapparatus sensitive to singleionPr and Pm ions coast ondifferent orbits in ESRuncertainty of decay time(≈ 1 s) less than observedperiod.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 12 / 19

Hypotheses: (1) technical artifact?

Procommon period of 7 s for140Pr58+ and 142Pm60+.

Conapparatus sensitive to singleionPr and Pm ions coast ondifferent orbits in ESRuncertainty of decay time(≈ 1 s) less than observedperiod.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 12 / 19

Hypotheses: (2) quantum beat of hyperfine states

Pro140Pr and 142Pm have nuclearspin I = 1.H-like ions probably producedin coherent superposition oftwo 1s hyperfine states withF = 1/2 and F = 3/2.Final state (daughter ion plusνe) has F = 1/2.EC-decay from F = 3/2 stateis not allowed.

ConThe well-known hyperfinesplitting in hydrogen is inmicrowave range(ν = ∆E/h = 1420 MHz), withperiod of,

T = h/∆E = 0.7 ns,

and T for 140Pr58+ is evensmaller by a factor of ≈ 105.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 13 / 19

Hypotheses: (2) quantum beat of hyperfine states

Pro140Pr and 142Pm have nuclearspin I = 1.H-like ions probably producedin coherent superposition oftwo 1s hyperfine states withF = 1/2 and F = 3/2.Final state (daughter ion plusνe) has F = 1/2.EC-decay from F = 3/2 stateis not allowed.

ConThe well-known hyperfinesplitting in hydrogen is inmicrowave range(ν = ∆E/h = 1420 MHz), withperiod of,

T = h/∆E = 0.7 ns,

and T for 140Pr58+ is evensmaller by a factor of ≈ 105.

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 13 / 19

Hypotheses: (3) neutrino oscillation

Suggestive kinematic considerationFor two mass eigenstates, m1 and m2,{

E1 + p21/2M = QEC

E2 + p22/2M = QEC

In approximation (E1 + E2)/2M � 1

∆E = E2 − E1 = (m22 −m2

1)/2M

From KamLAND data4, with M = 140 amu,

∆E ≈ 6× 10−16 eV, andT = h/E ≈ 7 s

4Phys. Rev. Lett. 94, 081801 (2005), ∆m2 ≈ 8× 10−5 eV2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation

Suggestive kinematic considerationFor two mass eigenstates, m1 and m2,{

E1 + p21/2M = QEC

E2 + p22/2M = QEC

In approximation (E1 + E2)/2M � 1

∆E = E2 − E1 = (m22 −m2

1)/2M

From KamLAND data4, with M = 140 amu,

∆E ≈ 6× 10−16 eV, andT = h/E ≈ 7 s

4Phys. Rev. Lett. 94, 081801 (2005), ∆m2 ≈ 8× 10−5 eV2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation

Suggestive kinematic considerationFor two mass eigenstates, m1 and m2,{

E1 + p21/2M = QEC

E2 + p22/2M = QEC

In approximation (E1 + E2)/2M � 1

∆E = E2 − E1 = (m22 −m2

1)/2M

From KamLAND data4, with M = 140 amu,

∆E ≈ 6× 10−16 eV, andT = h/E ≈ 7 s

4Phys. Rev. Lett. 94, 081801 (2005), ∆m2 ≈ 8× 10−5 eV2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation

Suggestive kinematic considerationFor two mass eigenstates, m1 and m2,{

E1 + p21/2M = QEC

E2 + p22/2M = QEC

In approximation (E1 + E2)/2M � 1

∆E = E2 − E1 = (m22 −m2

1)/2M

From KamLAND data4, with M = 140 amu,

∆E ≈ 6× 10−16 eV, andT = h/E ≈ 7 s

4Phys. Rev. Lett. 94, 081801 (2005), ∆m2 ≈ 8× 10−5 eV2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation

Suggestive kinematic considerationFor two mass eigenstates, m1 and m2,{

E1 + p21/2M = QEC

E2 + p22/2M = QEC

In approximation (E1 + E2)/2M � 1

∆E = E2 − E1 = (m22 −m2

1)/2M

From KamLAND data4, with M = 140 amu,

∆E ≈ 6× 10−16 eV, andT = h/E ≈ 7 s

4Phys. Rev. Lett. 94, 081801 (2005), ∆m2 ≈ 8× 10−5 eV2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Neutrino oscillation, a brief introduction

Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogywith a similar phenomenon in neutral kaons.5

flavor (e, µ, τ ) eigenstates: |να〉 =∑

i U∗αi |νi〉

mass (1, 2, 3) eigenstates: |νi〉 =∑

α Uαi |να〉

mixing matrix for two neutrinos: U =

(cos θ sin θ− sin θ cos θ

)

5http://en.wikipedia.org/wiki/Neutrino_oscillationByung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction

Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogywith a similar phenomenon in neutral kaons.5

flavor (e, µ, τ ) eigenstates: |να〉 =∑

i U∗αi |νi〉

mass (1, 2, 3) eigenstates: |νi〉 =∑

α Uαi |να〉

mixing matrix for two neutrinos: U =

(cos θ sin θ− sin θ cos θ

)

5http://en.wikipedia.org/wiki/Neutrino_oscillationByung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction

Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogywith a similar phenomenon in neutral kaons.5

flavor (e, µ, τ ) eigenstates: |να〉 =∑

i U∗αi |νi〉

mass (1, 2, 3) eigenstates: |νi〉 =∑

α Uαi |να〉

mixing matrix for two neutrinos: U =

(cos θ sin θ− sin θ cos θ

)

5http://en.wikipedia.org/wiki/Neutrino_oscillationByung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction

Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogywith a similar phenomenon in neutral kaons.5

flavor (e, µ, τ ) eigenstates: |να〉 =∑

i U∗αi |νi〉

mass (1, 2, 3) eigenstates: |νi〉 =∑

α Uαi |να〉

mixing matrix for two neutrinos: U =

(cos θ sin θ− sin θ cos θ

)

5http://en.wikipedia.org/wiki/Neutrino_oscillationByung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction

Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogywith a similar phenomenon in neutral kaons.5

flavor (e, µ, τ ) eigenstates: |να〉 =∑

i U∗αi |νi〉

mass (1, 2, 3) eigenstates: |νi〉 =∑

α Uαi |να〉

mixing matrix for two neutrinos: U =

(cos θ sin θ− sin θ cos θ

)

5http://en.wikipedia.org/wiki/Neutrino_oscillationByung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Decay amplitude, coherent or incoherent sum?

According to Ivanov et al.,6 decay amplitude is given by,

A(t) =∑

k=1,2,3

Ak (t) =∑

k

∫ t

0dτ〈If , νk |HW (τ)|Ii〉.

Giunti7 argues that A(t) is an incoherent sum over different channels,because,

|νe〉 =∑

k

U∗ek |νk 〉,

and in the time-dependent perturbation theory,

|νe(t)〉 =

∑j

|Aj(t)|2−1/2∑

k

Ak (t)|νk 〉.

6Ivanov et al. arXiv:0801.2121v1, Eq. 3, simplified7Giunti, arXiv:0801.4639v2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Decay amplitude, coherent or incoherent sum?

According to Ivanov et al.,6 decay amplitude is given by,

A(t) =∑

k=1,2,3

Ak (t) =∑

k

∫ t

0dτ〈If , νk |HW (τ)|Ii〉.

Giunti7 argues that A(t) is an incoherent sum over different channels,because,

|νe〉 =∑

k

U∗ek |νk 〉,

and in the time-dependent perturbation theory,

|νe(t)〉 =

∑j

|Aj(t)|2−1/2∑

k

Ak (t)|νk 〉.

6Ivanov et al. arXiv:0801.2121v1, Eq. 3, simplified7Giunti, arXiv:0801.4639v2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Decay amplitude, coherent or incoherent sum?

According to Ivanov et al.,6 decay amplitude is given by,

A(t) =∑

k=1,2,3

Ak (t) =∑

k

∫ t

0dτ〈If , νk |HW (τ)|Ii〉.

Giunti7 argues that A(t) is an incoherent sum over different channels,because,

|νe〉 =∑

k

U∗ek |νk 〉,

and in the time-dependent perturbation theory,

|νe(t)〉 =

∑j

|Aj(t)|2−1/2∑

k

Ak (t)|νk 〉.

6Ivanov et al. arXiv:0801.2121v1, Eq. 3, simplified7Giunti, arXiv:0801.4639v2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Analogy: double-slit interference

Lipkin8 asserts that coherence results from uncertainty relationship(localized ion, finite momentum uncertainty).

8Lipkin, arXiv:0801.1465v2Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference

Lipkin8 asserts that coherence results from uncertainty relationship(localized ion, finite momentum uncertainty).

8Lipkin, arXiv:0801.1465v2Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference

Lipkin8 asserts that coherence results from uncertainty relationship(localized ion, finite momentum uncertainty).

8Lipkin, arXiv:0801.1465v2Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference

Lipkin8 asserts that coherence results from uncertainty relationship(localized ion, finite momentum uncertainty).

8Lipkin, arXiv:0801.1465v2Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Prospects

Experimental verification“It is obvious that our findings must be corroborated by the studyof other two-body beta decays (EC and βb).”9

“A similar analysis can be applied to a K-capture experiment ...Here there are a number of initial states having different degreesof ionization. Interference can only occur between initial stateshaving the same degree of ionization. Otherwise the analysis isthe same.”10

New method for studying neutrino mixingIf the effect is real and realistic theoretical model can be set up,this is a new method to study neutrino oscillation without the needto directly detect neutrinos.

9Yu. A. Litvinov et al., arXiv:0801.2079v110Lipkin, arXiv:0801.1465v2Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 18 / 19

References

Litvinov, et al., “Observation of non-exponential orbital electroncapture decays of hydrogen-like 140Pr and 142Pm ions,”http://arxiv.org/abs/0801.2079v1

Ivanov, et al., “On the time-modulation of the K-shell electroncapture decay of H-like 140Pr58+ ions produced by neutrino-flavourmixing,” http://arxiv.org/abs/0801.2121v1Giunti, C., “Comment on the neutrino-mixing interpretation of theGSI time anomaly,” http://arxiv.org/abs/0801.4639v2(Note: this comment refers to arXiv:0801.1465v1.)Lipkin, H. J., “New method for studying neutrino mixing and massdifferences,” http://arxiv.org/abs/0801.1465v2

Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 19 / 19

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