a p m e q a 6s 6p p t pb - williams college

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AP RECISE M EASUREMENT OF THE E LECTRIC Q UADRUPOLE A MPLITUDE IN THE 6s 2 6p 23 P 0 3 P 2 T RANSITION IN P B E LI H OENIG ’17, D R .M ILINDA R UPASINGHE ,P ROF .T IKU M AJUMDER Work supported by NSF Grant 1404206 I NTRODUCTION Motivations Precise measurements and accurate theoretical models of atomic structure in Cs, Tl and Pb provide atomic-physics based tests of the Standard Model. Experimental measurement, E related to quantity predicted by SM, Q W , according to E = Q W C (N,Z ), where C (N,Z ) is atomic structure factor. The Goldilocks zone: tractable atomic structure and a large nu- clear mass. Current Precision of Experiment and Theory Recent advancements [Porsev et al., 2016] in Pb atomic theory re- vive element’s relevance in atomic physics tests of SM. Element Theory C (N,Z ) Experiment E Cs .27% [Porsev et al., 2009] 0.35% [C.S. Wood et al., 1997] Tl 2.5% [Kozlov et al., 2001] 1% [Vetter et al., 1995] Pb 4% [Porsev et al., 2016] 1.2% [Meekhof et al., 1995] Currently, few independent experimental measurements of Pb atomic structure to check new wavefunction calculations. Our measurements aim to guide the further refinement of this newly developed theory. C URRENT AND R ELEVANT W ORK Present Work Measure ratio of the Electric Quadrupole (E2) 6s 2 6p 23 P 0 3 P 2 to Mag- netic Dipole (M1) 3 P 0 3 P 1 transition amplitudes in 208 Pb. Previous Work in the Ma- jumder Lab In 1999, measurement of Tl E2/M1 amplitude ra- tio completed [Majumder, Tsai, 1999]. Measurement of E2/M1 = 0.239(4) agrees well with theory (E2/M1 = .237 [Safronova et al., 2005]) and obtained 1% accuracy. Mixed E2/M1 transition, 6s 2 6p 2 P 1/2 2 P 3/2 . Used a single laser, ana- lyzed a single spectrum to extract ratio; presently we must alternately record two separate spectra. 208 Pb Low Lying States 203 Tl Low Lying States E XPERIMENTAL S ETUP S IGNAL D ETECTION The Faraday rotation method detects changes to the overall polar- ization of the laser light. I (ν )= I o T (ν ) h 2φ m φ pb cos(ωt)+ 1 2 φ 2 m cos(2ωt)+ φ 2 pb + 1 2 φ 2 m i . Two oscillating terms whose ratio leads to pure rotation curve: 1f :2I o T (ν )φ m φ pb 2f : 1 2 I o T (ν )φ 2 m Apparatus is sensitive to rotations down to 1μrad. Polarimeter & Glan-Thompsan prism I NDUCING O PTICAL R OTATION Longitudinal magnetic field induces Zeeman split- ting amongst magnetic sub- levels. Differential phase shift and absorption for σ + and σ - polarized light. Difference of two disper- sion shapes leads to Fara- day lineshape. S PECTRA FOR 939 NM AND 1279 NM T RANSITIONS R ESULTS AND I NTERPRETATION Preliminary Result h2||E2||0i h1||M1||0i = .191(03)(10) Data Interpretation Ratio cancels n‘ leaves f (ν ) and hT i 2 : φ pb n‘ hT i 2 f (ν ). Experimental Faraday peak ratio depends on the line- shape parameters. Need reliable values for the Lorentzian and Gaus- sian widths. Height of convolved shape is scaled up by ten. h2|E2|0i h1|M1|0i = h F (ω 0 ) expmt,e F (ω 0 ) expmt,m * F peak,m F peak,e * ω 0,m ω 0,e * g l,m g l,e i 1/2 Ratio depends directly on: Observed spectral am- plitude, lineshape peak, Landé g-factors, laser fre- quencies. Reduced matrix element re- lated to observed ratio ac- cording to Wigner-Eckart theorem. Propagation of Lorentzian Width Error. h2||E2||0i h1||M1||0i = r 5 3 h2|E2|0i h1|M1|0i F UTURE W ORK Immediate Explore analysis methods. Lorentzian width accuracy particularly elusive. More data to be collected 207 Pb measurement (pres- ence of hyperfine struc- ture). In Coming Years Measure atomic polariz- abilities in nearby electric dipole transitions with the atomic beam unit. High vapor pressure of lead and single step transition, but small fractional thermal excitation.

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Page 1: A P M E Q A 6s 6p P T PB - Williams College

A PRECISE MEASUREMENT OF THE ELECTRIC QUADRUPOLE AMPLITUDE IN THE 6s26p2 3P0 → 3P2 TRANSITION IN PBELI HOENIG ’17, DR. MILINDA RUPASINGHE, PROF. TIKU MAJUMDER

Work supported by NSF Grant 1404206

INTRODUCTIONMotivations• Precise measurements and accurate theoretical models of atomic

structure in Cs, Tl and Pb provide atomic-physics based tests ofthe Standard Model.

• Experimental measurement, E related to quantity predicted bySM, QW, according to E = QW C(N,Z), where C(N,Z) is atomicstructure factor.

• The Goldilocks zone: tractable atomic structure and a large nu-clear mass.

Current Precision of Experiment and Theory• Recent advancements [Porsev et al., 2016] in Pb atomic theory re-

vive element’s relevance in atomic physics tests of SM.

Element Theory C(N,Z) Experiment ECs .27% [Porsev et al., 2009] 0.35% [C.S. Wood et al., 1997]Tl 2.5% [Kozlov et al., 2001] 1% [Vetter et al., 1995]Pb 4% [Porsev et al., 2016] 1.2% [Meekhof et al., 1995]

• Currently, few independent experimental measurements of Pbatomic structure to check new wavefunction calculations.

• Our measurements aim to guide the further refinement of thisnewly developed theory.

CURRENT AND RELEVANT WORKPresent Work

• Measure ratio of theElectric Quadrupole (E2)6s26p2 3P0 → 3P2 to Mag-netic Dipole (M1) 3P0 →3P1 transition amplitudesin 208Pb.

Previous Work in the Ma-jumder Lab• In 1999, measurement of

Tl E2/M1 amplitude ra-tio completed [Majumder,Tsai, 1999].

• Measurement of E2/M1 =0.239(4) agrees well withtheory (E2/M1 = .237[Safronova et al., 2005]) andobtained ∼ 1% accuracy.

• Mixed E2/M1 transition,6s26p 2P1/2 → 2P3/2.

• Used a single laser, ana-lyzed a single spectrum toextract ratio; presently wemust alternately record twoseparate spectra.

208Pb Low Lying States

203Tl Low Lying States

EXPERIMENTAL SETUP

SIGNAL DETECTION• The Faraday rotation method detects changes to the overall polar-

ization of the laser light.

I(ν) = IoT (ν)[2φmφpb cos(ωt) +

12φ

2m cos(2ωt) + φ2pb +

12φ

2m

].

• Two oscillating terms whose ratio leads to pure rotation curve:

1f : 2IoT (ν)φmφpb 2f :1

2IoT (ν)φ

2m

Apparatus is sensitive to rotationsdown to 1µrad.

Polarimeter & Glan-Thompsan prism

INDUCING OPTICAL ROTATION

• Longitudinal magneticfield induces Zeeman split-ting amongst magnetic sub-levels.

• Differential phase shift andabsorption for σ+ and σ−polarized light.

• Difference of two disper-sion shapes leads to Fara-day lineshape.

SPECTRA FOR 939 NM AND 1279 NM TRANSITIONS

RESULTS AND INTERPRETATIONPreliminary Result

〈2||E2||0〉〈1||M1||0〉

= .191(03)(10)

Data Interpretation

• Ratio cancels n` leavesf(ν) and 〈T 〉2:φpb ∝ n` 〈T 〉2 f(ν).

• Experimental Faraday peakratio depends on the line-shape parameters.

• Need reliable values forthe Lorentzian and Gaus-sian widths.

Height of convolved shape is scaledup by ten.

〈2|E2|0〉〈1|M1|0〉

=[ F (ω0)expmt,e

F (ω0)expmt,m∗Fpeak,m

Fpeak,e∗ ω0,m

ω0,e∗ gl,mgl,e

]1/2• Ratio depends directly

on: Observed spectral am-plitude, lineshape peak,Landé g-factors, laser fre-quencies.

• Reduced matrix element re-lated to observed ratio ac-cording to Wigner-Eckarttheorem. Propagation of Lorentzian Width

Error.

〈2||E2||0〉〈1||M1||0〉

=

√5

3

〈2|E2|0〉〈1|M1|0〉

FUTURE WORK

Immediate• Explore analysis methods.

Lorentzian width accuracyparticularly elusive.

• More data to be collected• 207Pb measurement (pres-

ence of hyperfine struc-ture).

In Coming Years• Measure atomic polariz-

abilities in nearby electricdipole transitions with theatomic beam unit.

• High vapor pressure of leadand single step transition,but small fractional thermalexcitation.