The Fukushima Daiichi Nuclear Plant

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Remediation Program For Japan


An Assisted Remediation Emergency PlanThe Fukushima Daiichi nuclear plantSir Daniel BilbruckBison Resource Development GroupP.O. Box 18223, Boulder, Colorado 803081.303. 468.5237

The Fukushima Daiichi nuclear plant site and its surroundings are being monitored by a variety of U.S. aircraft, including:

U-2 spy planes. The U-2s, flying out of Okinawa, have "radiation suites" that can take readings at various altitudes.Global Hawk Drone. The Global Hawk remote-controlled plane, now on its second run, has multispectral imaging capabilities, including thermal infrared and synthetic aperture radar. Kyodo News Service quoted Japanese government sources as saying that the Global Hawk was taking images of the inside of the reactor buildings.

WC-135 Constant Phoenix aircraft. One radiation-sniffing WC-135, basically a converted Boeing 707 jet, is on its way from Offutt Air Force Base in Nebraska to the area around Japan, where it will take atmospheric readings.

Intelligence experts are saying that the United States has a network of ground-level stations around the world that monitor radiation and can backtrack to calculate how much has been dispersed from a specific site.




5As of 10 P.M. local time on Thursday, the JAIF listed the following status of the six Fukushima Daiichi reactors:

Buildings around reactor Nos. 1, 3 and 4 were "severely damaged"; the building housing reactor No. 2 was "slightly damaged"; Cooling was not working for reactor Nos. 1, or 3; Water levels were covering more than half of the fuel in reactor No. 2; reactor Nos. 1 and 3 water levels were covering only about half of the fuel. Structural integrity of the spent fuel pools was unknown for reactor Nos. 1 and 2; Reactor Nos. 3 and 4 had low water levels; pool temperature was continuing to rise for reactor Nos. 5 and 6.

The spent fuel pools are of significant concern, Marvin Resnikoff, a radioactive waste management consultant, said in a Wednesday press briefing organized by the nonprofit organization Physicians for Social Responsibility. Resnikoff noted that the pools at each reactor are thought to have contained the following amounts of spent fuel, according to The Mainichi Daily News:

Reactor No. 1 fuel pool: 50 tons of nuclear fuel Reactor No. 2 fuel pool: 81 tons Reactor No. 3 fuel pool: 88 tons Reactor No. 4 fuel pool: 135 tons Reactor No. 5 fuel pool: 142 tons Reactor No. 6 fuel pool: 151 tons Also, a separate ground-level fuel pool contains 1,097 tons of fuel; and some 70 tons of nuclear materials are kept on the grounds in dry storage.

The reactor cores themselves contain less than 100 tons of fuel, Resnikoff noted.

How Much Spent Nuclear Fuel Does the Fukushima Daiichi Facility Hold?As Japan attempts to cool overheating nuclear fuel with seawater, experts worry that the damaged spent-fuel pools pose the greatest threat

6Promoting Nuclear Fuel

Cycle spent nuclear fuel contains unused fissionable uranium and newly produced plutonium. These substances can be collected, reprocessed, and reused as new fuel, to achieve effective utilization of energy resources.

This process of recycling uranium resources is referred to as the nuclear fuel cycle. As a country that relies heavily on imports for most its energy needs, Japan is actively pursuing the establishment of the nuclear fuel cycle as a means for securing stable, long-term supplies of energy resources through the effective utilization of uranium, and for ensuring the proper treatment and disposal of radioactive waste.

Plutonium-thermal Power Generation

In plutonium-thermal ("plu-thermal") power generation, plutonium is removed from spent fuel and mixed with uranium to produce MOX* fuels for use in existing nuclear power plants. This effective utilization of limited uranium resources is expected to contribute significantly to securing stable energy supply in the future.

To promote the introduction of plutonium-thermal power generation, electric power companies in Japan are making various efforts to obtain broad public acceptance of this new power generation method. At TEPCO, wthey have loaded MOX fuel into Unit 3 at the Fukushima Daiichi Nuclear Power Station in August 2010, and was steadily working their way toward the implementation of plutonium-thermal power generation.

MOXMixed oxide composed of uranium and plutonium

AP WWII Survivors of the atomic bomb attack of Nagasaki walk through the destruction as fire rages in the background,7The schematic diagram above shows the GE Mark I Boiling Water Reactor reacter building structure, the Fukushima Dai-ichi Unit 1

8Numbers 1, 2, and 3 are all boiling water reactors, made by General Electric in the early- to mid-1970s. A boiling water reactor, or BWR, is the second-most-common reactor type in the world.

A BWR contains thousands of thin, straw-like tubes 12 feet in length, known as fuel rods, that in the case of Fukushima are made of a zirconium alloy. Inside those fuel rods is sealed the actual fuel, little ceramic pellets of uranium oxide. The fuel rods are bundled together in the core of the reactor. During a nuclear fission chain reaction, the tubes heat up to extremely high temperatures, and the way to keep them safe turns out to also be the way to extract useful energy from them. The rods are kept submerged in demineralized water, which serves as a coolant. The water is kept in a pressurized containment vessel, so it has a boiling point of around 550 F. Even at such a high boiling point, the burning hot fuel rods produce large amounts of steam, which is actually what we want from this whole complicated arrangementthe high-pressure steam is used to turn the turbines on dynamos, producing electricity.

Boiling Water Reactor Schematic: 1. Reactor pressure vessel (RPV) 2. Nuclear fuel element 3. Control rods 4. Circulation pumps 5. Engine control rods 6. Steam 7. Feed water 8. High pressure turbine (HPT) 9. Low pressure turbine 10. Generator 11. Exciter 12. Condenser 13. Coolant 14. Pre-heater 15. Feed water pump 16. Cold water pump 17. Concrete enclosure 18. Mains connection


10Construction of the Fukushima nuclear power plants

The plants at Fukushima are Boiling Water Reactors (BWR for short). A BWR produces electricity by boiling water, and spinning a a turbine with that steam. The nuclear fuel heats water, the water boils and creates steam, the steam then drives turbines that create the electricity, and the steam is then cooled and condensed back to water, and the water returns to be heated by the nuclear fuel. The reactor operates at about 285 C.

The nuclear fuel is uranium oxide. Uranium oxide is a ceramic with a very high melting point of about 2800 C. The fuel is manufactured in pellets (cylinders that are about 1 cm tall and 1 com in diameter). These pellets are then put into a long tube made of Zircaloy (an alloy of zirconium) with a failure temperature of 1200 C (caused by the auto-catalytic oxidation of water), and sealed tight. This tube is called a fuel rod. These fuel rods are then put together to form assemblies, of which several hundred make up the reactor core.

The solid fuel pellet (a ceramic oxide matrix) is the first barrier that retains many of the radioactive fission products produced by the fission process. The Zircaloy casing is the second barrier to release that separates the radioactive fuel from the rest of the reactor.

The core is then placed in the pressure vessel. The pressure vessel is a thick steel vessel that operates at a pressure of about 7 MPa (~1000 psi), and is designed to withstand the high pressures that may occur during an accident. The pressure vessel is the third barrier to radioactive material release.

The entire primary loop of the nuclear reactor the pressure vessel, pipes, and pumps that contain the coolant (water) are housed in the containment structure. This structure is the fourth barrier to radioactive material release. The containment structure is a hermetically (air tight) sealed, very thick structure made of steel and concrete. This structure is designed, built and tested for one single purpose: To contain, indefinitely, a complete core meltdown. To aid in this purpose, a large, thick concrete structure is poured around the containment structure and is referred to as the secondary containment.

Both the main containment structure and the secondary containment structure are housed in the reactor building. The reactor building is an outer shell that is supposed to keep the weather out, but nothing in. (this is the part that was damaged in the explosions, but more to that later).

11Fundamentals of nuclear reactions

The uranium fuel generates heat by neutron-induced nuclear fission. Uranium atoms are split into lighter atoms (aka fission products). This process generates heat and more neutrons (one of the particles that forms an atom). When one of these neutrons hits another uranium atom, that atom can split, generating more neutrons and so on. That is called the nuclear chain reaction. During normal, full-power operation, the neutron population in a core is stable (remains the same) and the reactor is in a critical state.

It is worth mentioning at this point that the nuclear fuel in a reactor can never cause a nuclear explosion like a nuclear bomb. At Chernobyl, the explosion was caused by excessive pressure buildup, hydrogen explosion and rupture of all structures, propelling molten core material into the environment. Note that Chernobyl did not have a containment structure as a barrier to the environment. Why that did not and will not happen in Japan, is discussed further below.

In order to control the nuclear chain reaction, the reactor operators use control rods. The control rods are made of boron which absorbs neutrons. During normal operation in a BWR, the control rods are used to maintain the chain reaction at a critical state. The control rods are also used to shut the reactor down from 100% power to about 7% power (residual or decay heat).

The residual heat is caused from the radioactive decay of fission products. Radioactive decay is the process by which the fission products stabilize themselves by emitting energy in the form of small particles (alpha, beta, gamma, neutron, etc.). There is a multitude of fission products that are produced in a reactor, including cesium and iodine. This residual heat decreases over time after the reactor is shutdown, and must be removed by cooling systems to prevent the fuel rod from overheating and failing as a barrier to radioactive release. Maintaining enough cooling to remove the decay heat in the reactor is the main challenge in the affected reactors in Japan right now.

It is important to note that many of these fission products decay (produce heat) extremely quickly, and become harmless by the time you spell R-A-D-I-O-N-U-C-L-I-D-E. Others decay more slowly, like some cesium, iodine, strontium, and argon all of which is in these reactors.12

13 Bison Resource Development Group Remediation Plan

Remediation process that is being proposed for The Fukushima Daiichi nuclear plant:

Bison Resource Development Group will use high pressure flow through cementing pipe and fittings that are secured together with spin on/off Weco type fittings used to secure the pipe strings together. From the manifold system several strings of pipe will be laid out to all of the reactors at one time through hole/window/doorway and or through already established fittings such as the water coolant system.

Only one egress will be required on to and into the contaminated areas. All the trucks will be tied to one operating system computer that controls the flow from all the pumpers. The mixture of products will blended right at the trucks and then pumped from an environmentally safe distance. utilizing various product mixtures as required to solve various situations that may arise.

Generators, water, water storage and pumps, cement storage tanks, clay tanks and hemp storage for the remediation will be established next to the staging area for the pump trucks. There will have to be pipe racks set up with smaller cranes put in place to move pipes as they arrive for assembly.

A robot would be used to research, verify and visualize the remediation process and for the safety of the remediation crews.

Four 150 foot extended boom cranes will be used for lifting and placing of pipe sections. The booms of the cranes will have video cameras to show and verify the exact locations where the pipe is being placed. All camera and project management will be operated through a command center vehicle that will be environmentally safe.

There will be a decon center established at a safe distance out of the established contaminated perimeter along with a portable camp for remediation crews.

A complete remediation plan will be developed if this proposal is accepted as this is only a preliminary operational proposal. The Microwave and Laser program are classified programs and will only be released at the decision making point in time by officials that approve the remediation plan. This is a need-to-know process.

14At Bison Resource Development Group (BRDG), we pledge to support our clients by providing safe and knowledgeable staff at fair prices. We will treat our employees, associates, sub-contractors, and suppliers honestly through the establishment of equitable relationships BRDG is committed to distinctive quality and unparalleled customer service in all aspects of our business. There are no magic formulas. Our success is guaranteed by creative, productive employees who are empowered to make suggestions while thinking "outside the box". Every job is essential to fulfilling our mission to "provide distinctive quality and unparalleled customer service" everyday to more people who "trust and respect" us. The primary goal at BRDG is to live our vision statement and be an industry leader. We achieve this through dedicated hard work and commitment from every employee. It is the desire of BRDG's management, from top to bottom, to have every employee succeed in their job, and assist in achieving our goals. At BRDG, we strive to recognize the contributions of all employees!

Accidents Do Happen Whether Manmade or Natural15

Partial Suggested Equipment And Chemicals To Be Used For This Project.

New material traps radioactive Cesium ions via "Venus flytrap" mechanism. Like a Venus flytrap, a newly discovered chemical material is a picky eaterit won't snap its jaws shut for just anything. Instead of flies, however, its favorite food is radioactive nuclear waste.

Mercouri Kanatzidis, a scientist at the U.S. Department of Energy's (DOE) Argonne National Laboratory, and Nan Ding, a chemist at Northwestern University, have crafted a sulfide framework that can trap radioactive cesium ions. This mechanism has the potential to help speed clean-up at power plants and contaminated sites.

Above left: the metal sulfide framework's default conformation leaves a pore open to attract positive ions from the surroundings. Above right: With a Cesium ion inside, the framework changes to trap the ion.

16ENCAPSULATION OF HAZARDOUS WASTE MATERIALS Document Type and Number: WIPO Patent Application WO/1998/054107 Kind Code:A1 Abstract:A method of encapsulating hazardous waste materials including heavy metals such as arsenic, mercury, nickel and chromium residues, as well as radioactive materials. The method involves adding the hazardous waste material to a settable composition, forming a slurry, and allowing the slurry to set to encapsulate the waste material. The settable composition is a powdered flowable cement composition containing calcium carbonate and a caustic magnesium oxide. Tests conducted on the encapsulated material indicate that virtually none of the hazardous waste material is leached out of the set composition which has a concrete-like appearance.Radioactive Monazite

Tests were conducted using a powdered sample of the mineral monazite. Monazite is a monoclinic phosphate of the rare earth elements containing the cerium groups (Ce, La, Y, Th) PO4, as well as some uranium and thorium. Monazite is relatively abundant in beach sands, and is one of the principal sources of rare earth minerals and thorium. Thorium is used as a radioactive source in scientific instruments. Rare earth compounds are used in various manufacturing processes, including the manufacturing of glass and certain metals.

Analysis of the monazite material employed in the tests found that it contained 246 Becquerels per gram (Bq/gm) of thorium-232 and 28 Bq/gm of uranium-238. The half life of the thorium contained in the monazite is approximately 4.5 billion years (4.5 x 109). The monazite particle size can be from dust (approx. 0.lem) up to particles of approximately 1.Omm, ideally. The lead tailings, caustic magnesium oxide and calcium carbonate were all pre-ground to approximately 110pm, ie. 90% passed through a 150pm sieve.

EXAMPLE 9 300 grams of monazite, of radioactivity 246 becquerels per gram thorium and 28.1 becquerels per gram uranium, 400 grams of caustic magnesium oxide and a mixture of 480 grams of lead tailings (ex Mt. Isa) and 320 grams calcium carbonate were thoroughly dry mixed with 100 grams of aluminium sulphate and 25 grams of citric acid. To this was added 300 mLs of water to form a thick rapidly setting paste. The thickness of the total mixture could be adjusted by the addition of water to form a mouldable composition. The total mixture was poured into moulds and allowed to set. The radioactivity of the encapsulated monazite mixture was measured to be 44.60+0.20 becquerels per gram thorium and 5.06 + 0.21 becquerels per gram uranium.

17A leach rate analysis (TCLP test) was carried out at 14 days and 28 days to determine the leachable uranium and thorium. At 14 days the leachable uranium was less than 0.05 micrograms per litre and the leachable thorium was 0.25 micrograms per litre. At 28 days the leachable uranium was 0.05 micrograms per litre and the leachable thorium was 0.45-0.50 micrograms per litre. Gamma spectroscopy was carried out on the TCLP solutions to determine the levels of radioactive uranium and thorium at 14 and 28 days. At 14 days the leachable uranium radioactivity was below detectable levels or equivalent to


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