studies of emissions & atmospheric composition, clouds and climate coupling by regional surveys...

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Where-Houston, TX; Palmdale, CA What- Studied the North American Monsoon, smoke from fires, and South Eastern U.S. air chemistry-focusing on critical climatic processes, clouds, and chemical inputs to the atmosphere- as well as satellite validation. Who-scientists and aircrew from NASA, NOAA, NCAR, universities, and companies When-August - September 2013

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Page 1: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Where-Houston, TX; Palmdale, CA

What- Studied the North American Monsoon, smoke from fires, and South Eastern U.S. air chemistry-focusing on critical climatic processes, clouds, and chemical inputs to the atmosphere- as well as satellite validation.

Who-scientists and aircrew from NASA, NOAA, NCAR, universities, and companies

When-August -September 2013

Page 2: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

SEAC4RS used airborne and ground-based instruments

NASA’s DC-8 with 28 remote sensing and in-situ instruments to provide chemistry and cloud

measurements.

NASA’s ER-2 with 15 remote sensing

instruments and in situ instruments

SPEC Inc Learjet with 15 probes to study cloud properties

Balloon launches for water, ozone

Instruments for aerosols and air chemical composition

Page 3: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Where Did We Go?

Page 4: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Goal 1. To understand air chemistry in the Southeast U.S.

Broad range of data on isoprene, terpene and their products in a variety of thermal, NOx, urban, rural, cloud and aerosol environments

OMI H2CO August

MODIS AOTSeptember

MODIS AOT

August

OMI H2CO September

D. Jacob, J. Reid

Page 5: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Some preliminary SEAC4RS results on Southeast U.S. chemistry

• First vertical flux measurements from DC-8 of isoprene and its products.

• Isoprene inferred from satellite measurements of formaldehyde. SEAC4RS finds relationship depends on chemical regime and vertical mixing.

• Inconsistent ground and satellite observations imply free tropospheric layers of biogenic aerosols. SEAC4RS observed elevated layers of organic aerosols associated with biomass burning. SOA formation can be investigated.

Page 6: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Goal 2. Determine the evolution of gases and aerosols in deep convective outflow

and implications for UT/LS chemistry.

Many penetrations of clouds were made, as well as many profiles in the UT/LS

Alan Fried

Page 7: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Some preliminary SEAC4RS results on vertical transport

Tropospheric chemistry•Enhanced aerosols and organic gases observed around cloud tops•Detailed in situ observations of cloud properties together with radar and remote sensing data

Stratospheric chemistry•Stratospheric tracers provide data to constrain transport times and mechanisms for redistributing tracers through the lower and middle stratosphere on seasonal time scales•Enhanced water vapor layers above the tropopause suggesting convective input

Page 8: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Goal 3. Identify the influences of aerosols on meteorology and climate through the

atmospheric heat budget or microphysical changes in clouds

Bob Yokelson

SEAC4RS measured the properties of many types of aerosols, and their interactions with clouds

Page 9: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Some preliminary SEAC4RS results on aerosols

• Observations made in ~30 smoke plumes from forest fires and agricultural burning.

• Unprecedented data set including in situ data on heating rates, optical depths, single scattering albedos, composition, response to humidity, coating thickness, etc and remote sensing observations.

• Many data obtained in conjunction with AERONET and other ground sites

Page 10: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Goal 4. To serve as a calibration/validation test bed for future satellite instruments and

missions.MODIS smoke optical depths

SEAC4RS made many remote sensing observations of aerosols and clouds that were coincident with in situ observations

Page 11: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

Some preliminary SEAC4RS results on satellite validation and instrument development

• Several prototype instruments flown on ER-2 with successful measurements.

• Observations made in complex scenes, such as aerosols over clouds, and aerosols embedded in clouds

• AERONET validation studies conducted for absorbing aerosols

Page 12: Studies of Emissions & Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC 4 RS) Brian Toon Department of Atmospheric and Oceanic

SEAC4RS next steps• Preliminary data in archive April 2014.

• Final data in archive and released in October 2014.

• Investigators can collaborate with anyone, or release final data, in advance of October 2014